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Jinxu Pu

Publications and source records attributed to Jinxu Pu.

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Metamagnetism in UTe2: the roles of itinerancy and localization

The metamagnetic transition in UTe$_2$ plays a key role in stabilizing two enigmatic field-induced superconducting phases. One of these phases (SC2) is truncated by the transition, lying directly below it, while the other (SC3) sits predominantly above it and appears to be stabilized because of it. While numerous pulsed field studies have examined this transition, comparatively few steady field experiments have investigated it. Here we report a suite of measurements of metamgnetism in UTe$_2$, at ambient pressure by torque magnetometry and extraction magnetometry techniques, and of the magnetoconductance under pressure. Our steady field measurements resolve a complex sub-structure within the transition, with separate features that possess different temperature evolutions, pointing to distinct contributions from itinerant and localized moments. The itinerant contribution might relate to a possible spin-density wave state. We theoretically model the evolution of Kondo and RKKY interactions and propose that the SC2 state is stabilized under pressure due to the collapse of magnetic anisotropy, leading to an enhancement of longitudinal spin fluctuations along the hard $b$ axis, which are pair-forming in the $p$-wave channel.

cond-mat.str-el

Electrically-controllable superconducting memory effect in UTe2

If a computer could be assembled from superconducting components, the energy efficiency would far surpass that of conventional electronics. Historic research efforts towards this goal yielded pivotal breakthroughs in the development and discovery of scanning tunnelling microscopy and high temperature superconductivity. Although recent strides have been taken in advancing superconducting diode and switching technologies, harnessing read/writeable memory functionality in superconducting platforms has remained challenging. Here we show that bulk single crystal specimens of the triplet superconductor candidate uranium ditelluride (UTe$_2$) possess such properties. Upon applying a magnetic field to access an intermediate regime straddling two distinct superconducting phases, we find that direct current pulses can push the material in and out of a metastable state possessing an enhanced critical current $J_c$. This switching is controllable by the strength and duration of the stimuli, with the system `remembering' whether it is in the high or low $J_c$ state for extended periods. We interpret this to be due to competition between two distinct vortex species, which can be perturbatively pushed into a non-equilibrium high-disorder configuration with stronger pinning forces and thus higher $J_c$. Rather than requiring proximate magnetic or semiconducting interfaces, this memory functionality appears to be an intrinsic property of UTe$_2$ rooted in the superconducting order itself. Our findings underscore the rich complexity of quantum vortex matter, and demonstrate the viability of engineering a new class of superconducting memory elements with ultralow-power switching.

cond-mat.supr-con

Evidence of high-temperature exciton condensation in a two-dimensional semimetal

Electrons and holes can spontaneously form excitons and condense in a semimetal or semiconductor, as predicted decades ago. This type of Bose condensation can happen at much higher temperatures in comparison with dilute atomic gases. Two-dimensional (2D) materials with reduced Coulomb screening around the Fermi level are promising for realizing such a system. Here we report a change in the band structure accompanied by a phase transition at about 180 K in single-layer ZrTe2 based on angle-resolved photoemission spectroscopy (ARPES) measurements. Below the transition temperature, gap opening and development of an ultra-flat band top around the zone center are observed. This gap and the phase transition are rapidly suppressed with extra carrier densities introduced by adding more layers or dopants on the surface. The results suggest the formation of an excitonic insulating ground state in single-layer ZrTe2, and the findings are rationalized by first principles calculations and a self-consistent mean-field theory. Our study provides evidence for exciton condensation in a 2D semimetal and demonstrates strong dimensionality effects on the formation of intrinsic bound electron-hole pairs in solids.

cond-mat.mes-hall