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Jiong Li

Publications and source records attributed to Jiong Li.

18 recordsLinked to original sources

Geometric Superconducting Diode Effect in an NbN Nanoring

Superconducting diodes, which exhibit nonreciprocal critical currents, are promising building blocks for low-power cryogenic electronics and superconducting circuits. Existing superconducting diode platforms commonly rely on Josephson junctions, multilayer heterostructures, ferromagnetic elements, gate-difined structures. Here, we demonstrate a geometrically induced superconducting diode effect realized in a structurally minimal, single-materials NbN nanoring, where inversion-symmetry breaking is introduced solely by the asymmetric geometry. The device exhibits pronounced and polarity-switchable critical-current nonreciprocity. Systematic magnetic-field and temperature-dependent measurements reveal that, at low fields, the applied magnetic field redistributes the critical current asymmetrically between opposite bias directions without significantly reducing the overall superconducting current-carrying capability. Moreover, the maximal nonreciprocity and diode efficiency exhibit distinct temperature dependence: the maximal diode efficiency follows the evolution of the energy gap, whereas the maximal nonreciprocity is more closely associated with the superfluid density. These results establish asymmetric superconducting nanorings as a minimal geometric platform for studying nonreciprocal superconducting transport and provide a simple design principle for future superconducting electronics.

cond-mat.supr-con

Quantum criticality from spectral collapse in the two-photon Rabi model

Spectral collapse in the two-photon quantum Rabi model (tpQRM) has long been regarded as incompatible with quantum criticality due to the absence of a vanishing excitation gap. We show that, in the anisotropic tpQRM, spectral collapse constitutes a genuine continuous quantum phase transition governed by a single soft mode. The excitation gap within the same parity closes as $\epsilon_{sp} \sim |g - g_c|^{z\nu}$ with $z\nu = 1/2$, placing the system in the same universality class as the standard QRM, while the gap between different parities reflects symmetry-induced level splitting rather than a critical excitation. This soft mode defines a unique energy scale that controls both equilibrium and nonequilibrium properties, including macroscopic observables, quantum Fisher information, and Kibble-Zurek dynamics. These results establish spectral collapse as an experimentally accessible realization of quantum criticality in a few-body system and demonstrate that universality is fully determined by the soft-mode structure rather than by microscopic details.

quant-ph

Nanoscale electrothermal-switch superconducting diode for electrically programmable superconducting circuits

Superconducting diodes enable dissipationless directional transport, yet achieving electrical tunability and scalability remains a major challenge for circuit-level integration. Here, we demonstrate an electrothermal-switch superconducting diode in which a gate-controlled nanoscale hotspot dynamically breaks inversion symmetry in a superconducting nanowire. This mechanism gives rise to two coexisting nonreciprocal transport regimes-one associated with a nonreciprocal superconducting-to-normal transition and the other with ratchet-like vortex dynamics-both originating from the same electrothermal-switch process. The diode exhibits efficiencies up to 42% and 60% for the two regimes, respectively, and can be electrically switched on, off, or reversed in polarity in situ by applying a small gate current. These capabilities enable programmable superconducting circuits that realize electrically reconfigurable full-wave and half-wave rectification. The lithography-compatible design, high performance, and gate-controlled functionality establish a scalable platform for programmable superconducting electronics and hybrid quantum systems.

cond-mat.supr-con

Vortex-driven superconducting diode effect in asymmetric multilayer heterostructures

The superconducting diode effect (SDE), characterized by nonreciprocal critical currents, has attracted growing attention due to its potential applications in quantum technologies and energy-efficient devices. In this work, we explore the microscopic mechanism of the SDE by simulating asymmetric multilayer heterostructures within time-dependent Ginzburg-Landau theory. We systematically vary the layer thickness, external magnetic field and stacking order in a trilayer structure composed of niobium, vanadium, and tantalum, which share a similar structure to that in the pioneering experimental work, to clarify the role of vortex dynamics. Our simulations reveal a pronounced SDE originating from the interplay of Lorentz forces and asymmetric vortex dynamics, which strongly depend on layer stacking order. Besides, by simply changing the stacking order of the constituent layers, the SDE can be entirely suppressed. These findings offer insights into the microscopic mechanisms of the SDE and provide a feasible approach for controlling and eliminating the SDE in practical superconducting devices.

cond-mat.supr-con

Dissipative phase transitions of the Dicke-Ising model

The dissipative phase transitions in the open transverse and longitudinal Dicke-Ising model (DIM), which incorporates nearest-neighbor Ising-type spin interactions into the Dicke framework, are investigated within a mean-field approach and further validated by detailed stability analysis. While the dissipative phase diagram of the transverse DIM is only slightly shifted upward compared with its ground-state counterpart, dissipation in the longitudinal DIM stabilizes bistable nonequilibrium steady states and induces first-order phase transitions that are absent in the ground-state phase diagram. This bistable phase is characterized by the coexistence of superradiant and antiferromagnetic orders, and it converts a ground-state triple point into a tetracritical point, at which the boundaries of the first- and second-order transitions intersect. Our results reveal that the interplay among spin interactions, light-matter coupling, and dissipation supports a diverse set of nonequilibrium phase transitions and provides broad tunability of the phase diagram. These findings offer a theoretical foundation for exploring nonequilibrium physics in realistic open solid-state quantum systems.

quant-ph

$\mathcal{PT}$-symmetric two-photon quantum Rabi models

We investigate two non-Hermitian two-photon quantum Rabi models (tpQRM) that exhibit $\mathcal{PT}$ symmetry: the biased tpQRM (btpQRM), in which the qubit bias is purely imaginary, and the dissipative tpQRM (dtpQRM), where the two-photon coupling is made imaginary to introduce dissipation. For both models, we derive exact solutions by employing Bogoliubov transformations. In the btpQRM, we identify spectral collapse at a critical coupling strength, with accompanying $\mathcal{PT}$ symmetry breaking that correlates with exceptional points (EPs) arising from coalescing eigenstates. We establish a direct correspondence between $\mathcal{PT}$-broken regions and the doubly degenerate points of the Hermitian tpQRM, and analyze the effects of qubit bias via an adiabatic approximation. In the dtpQRM, although no spectral collapse occurs, both EPs and Juddian-type degeneracies are present, with well-separated behaviors distinguished by parity conservation. Through biorthogonal fidelity susceptibility and c-product, we successfully identify and classify the nature of these two types of level crossings. Finally, we compare the dynamical evolution of both models, revealing fundamentally different pathways to steady states governed by their respective non-Hermitian spectral structures. Our results provide exact characterizations of $\mathcal{PT}$-symmetric non-Hermitian tpQRMs and may offer theoretical insights for future experimental realizations.

quant-ph

Critical Spectrum and Quantum Criticality in the Two-Photon Rabi-Stark Model

We investigate the spectral properties and quantum criticality of the two-photon Rabi-Stark model. Using the exact solution of this model, we rigorously derive a condition for complete spectral collapse, where all bound states vanish. In this case, the energy gap closes at a critical coupling, signaling a continuous quantum phase transition. The corresponding gap exponent differs from those in both the one-photon Rabi-Stark model and the quantum Rabi model, suggesting a distinct universality class. While in the general case, an infinite number of discrete bound states exist when spectral collapse occur and the energy gap remains open. By mapping to an inverse square potential well, these bound levels approach the threshold energy exponentially. Our results offer new insights into novel spectral phenomena in nonlinear quantum Rabi models, with potential implications for experimental realizations in circuit QED and trapped ion systems.

quant-ph

$3d$ flat bands and coupled $4f$ moments in the kagome-honeycomb permanent magnet Sm$_{2}$Co$_{17}$

Rare earth permanent magnets (REPMs) with both localized moments and itinerant conduction bands are not only important for fundamental research but also have significant technological applications. In particular, Sm$_{\rm 2}$Co$_{\rm 17}$ is a prototypical high-temperture REPM, where the Co atoms form a kagome-honeycomb stacked lattice. Here we report synthesis of epitaxial Sm$_{\rm 2}$Co$_{\rm 17}$ films using molecular beam epitaxy and measurements of their momentum-resolved electronic structure from \textit{in-situ} angle-resolved photoemission spectroscopy. Our results unveil two flat bands from Co $3d$ orbitals near the Fermi level ($E_F$), one at $\sim$\,--300\,meV and another right at $E_F$, which arise from orbital-selective destructive interference and strong electron correlations, respectively. In addition, our results reveal that Sm $4f$ states are far away from $E_F$ (hence mostly localized) and exhibit an anomalous temperature dependence, caused by the $3d$-$4f$ magnetic coupling. Our findings provide direct spectroscopic insights to understand the strong uniaxial ferromagnetism in Sm$_{\rm 2}$Co$_{\rm 17}$ (and REPMs alike). Our work also opens avenues to explore flat-band physics near $E_F$ and emergent phenomena in correlated kagome-honeycomb lattices.

cond-mat.str-el

Critical spectrum of the anisotropic two-photon quantum Rabi model

The anisotropic two-photon quantum Rabi model is studied using the Bogoliubov operator approach. The doubly degenerate exceptional states are identified through analytical methods. By adjusting the position of the last exceptional point belonging to two adjacent energy levels, we derive a condition for the absence of the discrete spectrum at the critical coupling where ``spectral collapse" occurs. In this special case, the spectrum becomes fully continuous above a threshold energy, with no bound states existing, whereas the ground state remains gapped in the general case. This also signals a quantum phase transition. More interestingly, we rigorously find that a finite number of bound states exist between two anisotropy dependent critical atomic frequencies, with infinitely many bound states beyond this frequency regime. In this manner, all issues in the two-photon quantum Rabi model are resolved.

quant-ph

Vacuum Rabi Splitting and Quantum Fisher Information of a Non-Hermitian Qubit in a Single-Mode Cavity

A natural extension of the non-Hermitian qubit is to place it in a single-mode cavity. This setup corresponds to the quantum Rabi model (QRM) with a purely imaginary bias on the qubit, exhibiting parity-time ($\mathcal{P}\mathcal{T}$) symmetry. In this work, we first solve the $\mathcal{P} \mathcal{T}$-symmetric QRM using the Bogoliubov operator approach. We derive the transcendental function responsible for the exact solution, which can also be used to precisely identify exceptional points. The adiabatic approximation previously used can be easily formulated within this approach by considering transitions between the same manifolds in the space of Bogoliubov operators. By further considering transitions between the nearest-neighboring manifolds, we can analytically obtain more accurate eigensolutions. Moreover, these simple corrections can capture the main features of the dynamics, where the adiabatic approximation fails. Furthermore, the rich characteristics of the vacuum Rabi splitting in the emission spectrum are predicted. The width of the peaks increases with the coupling strength and the imaginary biases, reflecting the nature of open quantum systems. Additionally, we identify a {quantum-criticality-enhanced} effect by calculating the quantum Fisher information. Near the exceptional points, the quantum Fisher information in the $\mathcal{P} \mathcal{T}$-symmetric QRM is significantly higher than that of the non-Hermitian qubit component. This may open a new avenue for enhancing quantum sensitivity in non-Hermitian systems by incorporating coupling with an additional degree of freedom, enabling more precise parameter estimation.

quant-ph

$\mathcal{PT}$-symmetric quantum Rabi model: Solutions and exceptional points

The $\mathcal{PT}$-symmetric non-Hermitian quantum Rabi model (QRM) with imaginary coupling is solved using the Bogoliubov operators approach. A transcendental function responsible for the exact solutions is derived, with its zeros yielding the regular spectrum. We find two types of intersections: One is the exceptional point (EP), which is widely studied in the non-Hermitian system; another one is due to doubly degenerate states caused by the conserved QRM parity, which is well-known in the Hermitian QRM. These intersections are identified through this transcendental function. EPs emerge between pairs of adjacent excited energy levels, shifting toward lower coupling strengths as energy levels increase. The fidelity susceptibility diverges to negative infinity at the EPs, consistent with recent findings in non-Hermitian systems, while it diverges to positive infinity at the doubly degenerate points. The EPs are further confirmed by the vanishing c-product in the biorthogonal basis. All eigenstates are characterized by conserved energy and QRM parity. We conclude that the non-Hermitian QRM is integrable, analogous to its Hermitian counterpart.

quant-ph

Curiosity-driven Exploration in Sparse-reward Multi-agent Reinforcement Learning

Sparsity of rewards while applying a deep reinforcement learning method negatively affects its sample-efficiency. A viable solution to deal with the sparsity of rewards is to learn via intrinsic motivation which advocates for adding an intrinsic reward to the reward function to encourage the agent to explore the environment and expand the sample space. Though intrinsic motivation methods are widely used to improve data-efficient learning in the reinforcement learning model, they also suffer from the so-called detachment problem. In this article, we discuss the limitations of intrinsic curiosity module in sparse-reward multi-agent reinforcement learning and propose a method called I-Go-Explore that combines the intrinsic curiosity module with the Go-Explore framework to alleviate the detachment problem.

cs.AI

A durable and efficient electrocatalyst for saline water splitting with current density exceeding 2000 mA cm -2

Water electrolysis is promising for industrial hydrogen production to achieve a sustainable and green hydrogen economy, but the high cost of the technology limits its market share. Developing efficient yet economic electrocatalysts is crucial to decrease the cost of electricity and electrolytic cell. Meanwhile, electrolysis in seawater electrolyte can further reduce feedstock cost. Here we synthesize a type of electrocatalyst where trace precious metals are strongly anchored on corrosion-resistive matrix. As an example, the produced Pt/Ni-Mo electrocatalyst only needs an overpotential of 113 mV to reach an ultrahigh current density of 2000 mA cm-2 in saline-alkaline electrolyte, standing as the best performance so far. It shows high activity and long durability in various electrolytes and under harsh conditions, including strong alkaline and simulated seawater electrolytes, and under elevated temperatures up to 80 degree Celsius). This electrocatalyst is produced on a large scale at low cost and shows good performance in a commercial membrane electrode assembly stack, demonstrating its feasibility for practical water electrolysis

physics.chem-ph

Stabilized Hydroxide Mediated Nickel-Based Electrocatalysts for High Current Density Hydrogen Evolution in Alkaline Media

Large scale production of hydrogen by electrochemical water splitting is considered as a promising technology to address critical energy challenges caused by the extensive use of fossil fuels. Although nonprecious nickel-based catalysts work well at low current densities, they need large overpotentials at high current densities that hinders their potential applications in practical industry. Here we report a hydroxide-mediated nickel based electrocatalyst for high current density hydrogen evolution, which delivers a current density of 1000 mA cm-2 at an overpotential of 98 mV. Combined X-ray absorption spectroscopy and high resolution X-ray photoelectron spectroscopy results show charge redistribution of nickel sites caused by Mo and surface FeOx clusters, which can stabilize the surface nickel hydroxide at high current densities for promoting water dissociation step. Such catalyst is synthesized at the metre scale and shows a current density of 500 mA cm-2 at 1.56 V in the overall water splitting, which demonstrate its potential for practical use. This work highlights a charge-engineering strategy for rational design of catalysts that work well at high current densities.

physics.chem-ph

Two-photon Rabi-Stark model

The analytically exact solutions to the two-photon Rabi-Stark model are given by using the Bogoliubov operators approach. Transcendental functions responsible for the exact solutions are derived. The zeros of the transcendental functions reproduce completely the regular spectra. The first-order quantum phase transitions are also detected by the pole structure of the derived transcendental functions, similar to the one-photon Rabi-Stark model, different from the two-photon Rabi model where the energy levels for the ground-state and the first excited state do not cross. The spectra collapse characteristics resemble those in two-photon Rabi model. Some low lying levels can split off from the collapse energy, different from the one-photon Rabi-Stark model in which all levels collapse.

quant-ph

An infinite family of knots whose hexagonal mosaic number is only realized in non-reduced projections

We give an infinite family of knots such that for any given $r \geq 3$, the family contains a knot which can be embedded on a hexagonal $r$-mosaic, but cannot fit on a hexagonal $r$-mosaic in an embedding that achieves its crossing number. This extends the rectangular mosaic result of Ludwig, Evans, and Paat. We also introduce a new tool for systematically finding all possible flypes for the diagram of any link thus making it easier to find all possible minimal crossing embeddings of prime, alternating knots.

math.GT

Electronic structure of LaFe1-xCoxAsO from first principle calculations

Based on the first-principles calculations, we have investigated the geometry, binding properties, density of states and band structures of the novel superconductor LaFe1-xCoxAsO and its parent compounds with the ZrCuSiAs structure. We demonstrate that La-O bond and TM-As (TM=Fe or Co) bond are both strongly covalent, while the LaO and TMAs layers have an almost ionic interaction through the Bader charge analysis. Partial substitution of iron with cobalt modify the Fermi level from a steep edge to a flat slope, which explains why in this system Co doping suppresses the spin density wave (SDW) transition.

cond-mat.supr-con