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Jishan Liu

Publications and source records attributed to Jishan Liu.

21 records · Page 2Linked to original sources

Directed exfoliating and ordered stacking of transition-metal-dichalcogenides

Two-dimensional van der Waals crystals arise limitless scope for designing novel combinations of physical properties via controlling the stacking order or twist angle of individual layers. Lattice orientation between stacked monolayers is significant not only for the engineering symmetry breaking but also for the study of many-body quantum phases and band topology. So far the state-of-art exfoliation approaches focusing on achievements of quality, size, yield, and scalability while lacking sufficient information on lattice orientation. Consequently, interlayer alignment is usually determined by later experiments, such as second harmonic generation spectroscopy, which increased the number of trials and errors for a designed artificial ordering and hampered the efficiency of systematic study. Herein, we report a lattice orientation distinguishable exfoliation method via gold favor epitaxy along the specific atomic step edges, meanwhile, fulfill requirements of high-quality, large-size, and high-yield of monolayers. Hexagonal- and rhombohedral-stacking configurations of bilayer transition metal dichalcogenides are built directly at once result of foreseeing the lattice orientation. Optical spectroscopy, electron diffraction, and angle-resolved photoemission spectroscopy are used to study crystals quality, symmetric breaking, and band tuning, which supports the exfoliating mechanism we proposed. This strategy shows the ability for facilitates the development of ordering stacking especially for multilayers assembling in the future.

cond-mat.mtrl-sci↗

Emergence of new van Hove singularities in the charge density wave state of a topological kagome metal RbV3Sb5

Quantum materials with layered kagome structures have drawn considerable attention due to their unique lattice geometry, which gives rise to flat bands co-existing with Dirac-like dispersions. The interplay between strong Coulomb correlations and nontrivial band topology in these systems results in various exotic phenomena. Recently, vanadium-based materials with layered kagome structures are discovered to be topological metals, which exhibit charge density wave (CDW) properties, significant anomalous Hall effect, and unusual superconductivity at low temperatures. Here we exploit high-resolution angle-resolved photoemission spectroscopy to investigate the electronic structure evolution induced by the CDW transition in a vanadium-based kagome material RbV3Sb5. A remarkable band renormalization in the CDW state is observed, which is consistent with first principles calculations based on an inverse star-of-David superstructure. The CDW phase transition gives rise to a partial energy gap opening at the Fermi level, a shift in the band dispersion, and most importantly, the emergence of new van Hove singularities associated with large density of states, which are absent in the normal phase and may be related to superconductivity observed at lower temperatures. Our work would shed light on the microscopic mechanisms for the formation of the CDW and superconducting states in these topological kagome metals.

cond-mat.supr-con↗

Electron-plasmon interaction induced plasmonic-polaron band replication in epitaxial perovskite SrIrO$_3$ films

Electron-boson interaction is fundamental to a thorough understanding of various exotic properties emerging in many-body physics. In photoemission spectroscopy, photoelectron emission due to photon absorption would trigger diverse collective excitations in solids, including the emergence of phonons, magnons, electron-hole pairs, and plasmons, which naturally provides a reliable pathway to study electron-boson couplings. While fingerprints of electron-phonon/-magnon interactions in this state-of-the-art technique have been well investigated, much less is known about electron-plasmon coupling, and direct observation of the band renormalization solely due to electron-plasmon interactions is extremely challenging. Here by utilizing integrated oxide molecular-beam epitaxy and angle-resolved photoemission spectroscopy, we discover the long sought-after pure electron-plasmon coupling-induced low-lying plasmonic-polaron replica bands in epitaxial semimetallic SrIrO$_3$ films, in which the characteristic low carrier concentration and narrow bandwidth combine to provide a unique platform where the electron-plasmon interaction can be investigated kinematically in photoemission spectroscopy. This finding enriches the forms of electron band normalization on collective modes in solids and demonstrates that, to obtain a complete understanding of the quasiparticle dynamics in 5d electron systems, the electron-plasmon interaction should be considered on equal footing with the acknowledged electron-electron interaction and spin-orbit coupling.

cond-mat.str-el↗