arXiv subjects

Jisu Ryu

Publications and source records attributed to Jisu Ryu.

12 recordsLinked to original sources

arXiv2026

Optical Lineshape Models and the Generalized Einstein Relation between Absorption and Stimulated Emission

Recently, Ryu et al. generalized Einstein's three coefficients for absorption, stimulated emission, and spontaneous emission between two quantum levels to a set of four spectra between two broadened bands. The spectra obey generalized Einstein relationships at thermal equilibrium; Einstein's relations are obtained as an approximation for line spectra. Here, the generalized Einstein relation between absorption and stimulated emission dipole-strength spectra is applied to investigate optical lineshape models. Lineshapes for the Bloch model, the stochastic model, and the semi-classical Brownian oscillator model do not obey the generalized Einstein relation and therefore fail to satisfy detailed balance with Planck blackbody radiation. The quantum Brownian oscillator model treats a harmonic quantum vibration that is bi-linearly coupled to a thermal bath of quantum harmonic oscillators which generate damping and a random force. The two-state quantum Brownian oscillator lineshape model provides lineshapes for transitions between two displaced, but otherwise identical, harmonic potential energy surfaces on which the same quantum vibration is coupled to the same thermal bath of quantum harmonic oscillators. The absorption and stimulated emission lineshapes were calculated using the quantum Brownian oscillator model in under-damped, critically damped, and over-damped cases. The thermal and reorganization energy were each varied from much less to greater than the vibrational quantum of energy. All quantum Brownian oscillator lineshapes obey the generalized Einstein relation within the numerical precision of the calculation (14 to 30 digits), suggesting this lineshape model is compatible with detailed balance. The formula giving the electric-dipole transition cross-section in terms of these lineshapes is presented.

physics.chem-ph↗

arXiv2026

Generalized Einstein Relations between Absorption and Emission Spectra in the Electric-Dipole Approximation

Recently, Ryu et al. showed that two broadened bands connected by a set of four Einstein-coefficient spectra for stimulated and spontaneous single-photon transitions will obey detailed balance at equilibrium if the spectra satisfy generalized Einstein relations. Here, quantum mechanical expressions for Einstein-coefficient spectra are obtained in the electric-dipole approximation using an intramolecular Boltzmann distribution and the quantized field operators in isotropic, dispersive media of Nienhuis and Alkemade. These expressions suggest relationships between Einstein-coefficient spectra and dipole-strength spectra. The electrodynamic relationship between the spectral density for electromagnetic energy and the spectral density for the square of the electric field is developed and used to define dipole-strength spectra in terms of conditional transition probabilities per unit time. These rigorously relate dipole-strength spectra to Einstein-coefficient spectra, thus establishing quantum formulas for dipole-strength spectra and new generalized Einstein relations between dipole-strength spectra. For transitions between two bands, the dipole-strength spectra depend on a single total dipole strength but replace Einstein's degeneracy ratio and transition frequency with a change in standard chemical potential and a single underlying lineshape that is manifested differently in the four spectra. At equilibrium, the relations specify the Stokes' shift between forward and reverse transitions. The relationships between dipole-strength spectra, spontaneous emission spectral densities and stimulated transition cross sections depend on the refractive index, the dielectric constant, and the local field, but not on the derivative of the refractive index. The broadband relationships reduce to known relationships for narrow spectra inside materials and for line spectra in vacuum.

physics.chem-ph↗

arXiv2024

Generalized Einstein Relations between Absorption and Emission Spectra at Thermodynamic Equilibrium

We present Einstein coefficient spectra and a detailed-balance derivation of generalized Einstein relations between them that is based on the connection between spontaneous and stimulated emission. If two broadened levels or bands overlap in energy, transitions between them need not be purely absorptive or emissive. Consequently, spontaneous emission can occur in both transition directions, and four Einstein coefficient spectra replace the three Einstein coefficients for a line. At equilibrium, the four different spectra obey five pairwise relationships and one lineshape generates all four. These relationships are independent of molecular quantum statistics and predict the Stokes' shift between forward and reverse transitions required by equilibrium with blackbody radiation. For Boltzmann statistics, the relative strengths of forward and reverse transitions depend on the formal chemical potential difference between the initial and final bands, which becomes the standard chemical potential difference for ideal solutes. The formal chemical potential of a band replaces both the energy and degeneracy of a quantum level. Like the energies of quantum levels, the formal chemical potentials of bands obey the Rydberg-Ritz combination principle. Each stimulated Einstein coefficient spectrum gives a frequency-dependent transition cross section. Transition cross sections obey causality and a detailed-balance condition with spontaneous emission, but do not directly obey generalized Einstein relations. Even with an energetic width much less than the photon energy, an absorptive forward transition with an energetic width much greater than the thermal energy can have such an extreme Stokes' shift that its reverse transition cross section becomes predominantly absorptive rather than emissive.

physics.chem-ph↗

arXiv2022

PAC-Net: A Model Pruning Approach to Inductive Transfer Learning

Inductive transfer learning aims to learn from a small amount of training data for the target task by utilizing a pre-trained model from the source task. Most strategies that involve large-scale deep learning models adopt initialization with the pre-trained model and fine-tuning for the target task. However, when using over-parameterized models, we can often prune the model without sacrificing the accuracy of the source task. This motivates us to adopt model pruning for transfer learning with deep learning models. In this paper, we propose PAC-Net, a simple yet effective approach for transfer learning based on pruning. PAC-Net consists of three steps: Prune, Allocate, and Calibrate (PAC). The main idea behind these steps is to identify essential weights for the source task, fine-tune on the source task by updating the essential weights, and then calibrate on the target task by updating the remaining redundant weights. Under the various and extensive set of inductive transfer learning experiments, we show that our method achieves state-of-the-art performance by a large margin.

cs.LG↗

arXiv2021

A Novel Approach for Semiconductor Etching Process with Inductive Biases

The etching process is one of the most important processes in semiconductor manufacturing. We have introduced the state-of-the-art deep learning model to predict the etching profiles. However, the significant problems violating physics have been found through various techniques such as explainable artificial intelligence and representation of prediction uncertainty. To address this problem, this paper presents a novel approach to apply the inductive biases for etching process. We demonstrate that our approach fits the measurement faster than physical simulator while following the physical behavior. Our approach would bring a new opportunity for better etching process with higher accuracy and lower cost.

stat.ML↗

arXiv2013

Spin-Wave Propagation in the Presence of Interfacial Dzyaloshinskii-Moriya Interaction

In ferromagnetic thin films, broken inversion symmetry and spin-orbit coupling give rise to interfacial Dzyaloshinskii-Moriya interactions. Analytic expressions for spin-wave properties show that the interfacial Dzyaloshinskii-Moriya interaction leads to non-reciprocal spin-wave propagation, i.e. different properties for spin waves propagating in opposite directions. In favorable situations, it can increase the spin-wave attenuation length. Comparing measured spin wave properties in ferromagnet$|$normal metal bilayers and other artificial layered structures with these calculations can provide a useful characterization of the interfacial Dzyaloshinskii-Moriya interactions.

cond-mat.mtrl-sci↗

arXiv2013

Current-driven domain wall motion with spin Hall effect: Reduction of threshold current density

We theoretically study the current-driven domain wall motion in the presence of both the spin Hall effect and an extrinsic pinning potential. The spin Hall effect mainly affects the damping ratio of the domain wall precession in the pinning potential. When the pinning potential is not too strong, this results in a significant reduction of a threshold current density for the depinning of a domain wall with certain polarity. We also propose one way to distinguish the spin Hall effect induced spin-transfer torque from the one induced by the Rashba spin-orbit coupling experimentally.

cond-mat.mes-hall↗

arXiv2012

Current-induced motion of a transverse magnetic domain wall in the presence of spin Hall effect

We theoretically study the current-induced dynamics of a transverse magnetic domain wall in bi-layer nanowires consisting of a ferromagnet on top of a nonmagnet having strong spin-orbit coupling. Domain wall dynamics is characterized by two threshold current densities, $J_{th}^{WB}$ and $J_{th}^{REV}$, where $J_{th}^{WB}$ is a threshold for the chirality switching of the domain wall and $J_{th}^{REV}$ is another threshold for the reversed domain wall motion caused by spin Hall effect. Domain walls with a certain chirality may move opposite to the electron-flow direction with high speed in the current range $J_{th}^{REV} < J < J_{th}^{WB}$ for the system designed to satisfy the conditions $J_{th}^{WB} > J_{th}^{REV}$ and α> β, where αis the Gilbert damping constant and βis the nonadiabaticity of spin torque. Micromagnetic simulations confirm the validity of analytical results.

cond-mat.mes-hall↗

arXiv2012

Magnetization dynamics induced by in-plane currents in ultrathin magnetic nanostructures

Ultrathin magnetic systems have properties qualitatively different from their thicker counterparts, implying that different physics governs their properties. We demonstrate that various such properties can be explained naturally by the Rashba spin-orbit coupling in ultrathin magnetic systems. This work will be valuable for the development of next generation spintronic devices based on ultrathin magnetic systems.

cond-mat.mes-hall↗

arXiv2011

Magnetic domain wall motion in a nanowire: depinning and creep

The domain wall motion in a magnetic nanowire is examined theoretically in the regime where the domain wall driving force is weak and its competition against disorders is assisted by thermal agitations. Two types of driving forces are considered; magnetic field and current. While the field induces the domain wall motion through the Zeeman energy, the current induces the domain wall motion by generating the spin transfer torque, of which effects in this regime remain controversial. The spin transfer torque has two mutually orthogonal vector components, the adiabatic spin transfer torque and the nonadiabatic spin transfer torque. We investigate separate effects of the two components on the domain wall depinning rate in one-dimensional systems and on the domain wall creep velocity in two-dimensional systems, both below the Walker breakdown threshold. In addition to the leading order contribution coming from the field and/or the nonadiabatic spin transfer torque, we find that the adiabatic spin transfer torque generates corrections, which can be of relevance for an unambiguous analysis of experimental results. For instance, it is demonstrated that the neglect of the corrections in experimental analysis may lead to incorrect evaluation of the nonadiabaticity parameter. Effects of the Rashba spin-orbit coupling on the domain wall motion are also analyzed.

cond-mat.mes-hall↗

arXiv2010

Universality between current- and field-driven domain wall dynamics in ferromagnetic nanowires

Spin-polarized electric current exerts torque on local magnetic spins, resulting in magnetic domain-wall (DW) motion in ferromagnetic nanowires. Such current-driven DW motion opens great opportunities toward next-generation magnetic devices controlled by current instead of magnetic field. However, the nature of the current-driven DW motion--considered qualitatively different from magnetic-field-driven DW motion--remains yet unclear mainly due to the painfully high operation current densities J_OP, which introduce uncontrollable experimental artefacts with serious Joule heating. It is also crucial to reduce J_OP for practical device operation. By use of metallic Pt/Co/Pt nanowires with perpendicular magnetic anisotropy, here we demonstrate DW motion at current densities down to the range of 10^9 A/m^2--two orders smaller than existing reports. Surprisingly the current-driven motion exhibits a scaling behaviour identical to the field-driven motion and thus, belongs to the same universality class despite their qualitative differences. Moreover all DW motions driven by either current or field (or by both) collapse onto a single curve, signalling the unification of the two driving mechanisms. The unified law manifests non-vanishing current efficiency at low current densities down to the practical level, applicable to emerging magnetic nanodevices.

cond-mat.mtrl-sci↗

arXiv2010

Roles of adiabatic and nonadiabatic spin transfer torques on magnetic domain wall motion

Electric current exerts torques-so-called spin transfer torques (STTs)-on magnetic domain walls (DWs), resulting in DW motion. At low current densities, the STTs should compete against disorders in ferromagnetic nanowires but the nature of the competition remains poorly understood. By achieving two-dimensional contour maps of DW speed with respect to current density and magnetic field, here we visualize unambiguously distinct roles of the two STTs-adiabatic and nonadiabatic-in scaling behaviour of DW dynamics arising from the competition. The contour maps are in excellent agreement with predictions of a generalized scaling theory, and all experimental data collapse onto a single curve. This result indicates that the adiabatic STT becomes dominant for large current densities, whereas the nonadiabatic STT-playing the same role as a magnetic field-subsists at low current densities required to make emerging magnetic nanodevices practical.

cond-mat.mtrl-sci↗