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Jixi Zhang

Publications and source records attributed to Jixi Zhang.

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Spot Profile Analysis Low Energy Electron Diffraction of Plasma-Enhanced Chemical Vapor Deposition Grown Epitaxial Few-Layer Graphene on Sapphire

We demonstrate the use of high-resolution spot-profile analysis low-energy electron diffraction to determine the mean grain size of plasma-enhanced chemical vapor deposition grown few-layer graphene on sapphire (Al$_2$O$_3$). The diffraction patterns exhibit broadened graphene spots, pronounced diffuse scattering, and azimuthally extended features, indicating finite crystallite size and rotational disorder. By analyzing the finite-size broadening of the specular (00) spot with an Airy-type diffraction profile, we determine a mean grain diameter of 3.7$\,$nm for the as-grown graphene layer. Post-growth annealing under ultrahigh-vacuum conditions increases the mean grain size to about 5.7$\,$nm and 6.8$\,$nm, respectively. These results establish SPA-LEED as a sensitive reciprocal-space method for quantifying the structural coherence of directly grown graphene on insulating substrates.

cond-mat.mtrl-sci

Mid-infrared snapshot spectral imaging via nonlinear radial dispersion

Mid-infrared (MIR) spectral imaging provides chemically specific contrast through molecular vibrational fingerprints, yet snapshot acquisition remains severely limited by the lack of high-sensitivity detectors and efficient spectral encoding mechanisms. Here we introduce snapshot MIR spectral imaging based on intrinsic nonlinear radial dispersion, in which wavelength-dependent phase matching simultaneously enables frequency upconversion and spectral multiplexing. Different spectral components are mapped to distinct output angles within a 4$f$ imaging architecture, enabling single-shot spectral encoding without external dispersive elements. In combination with speckle illumination encoding, spectral information is compressed and recovered without additional coding components. Leveraging nonlinear upconversion to the visible, the approach achieves room-temperature MIR spectral imaging with sensitivity approaching 1 photon/pixel/pulse across a broad spectral range from 2.5 to 4.0 $\mu$m. This work transforms spectral encoding from an external optical function into an inherent property of the nonlinear imaging process, providing a general route to high-sensitivity snapshot MIR spectral imaging.

physics.optics

Mid-infrared Fourier ptychographic upconversion imaging

Frequency upconversion technique offers an appealing approach for sensitive mid-infrared (MIR) imaging at room temperature. However, the spatial resolution of the upconversion imager has been notoriously restricted by the limited transverse section of the involved nonlinear crystal at the Fourier plane. Here, we implement a wide-field and high-resolution MIR upconversion imaging system based on elliptical pumping and Fourier ptychography. Specifically, an elliptical pump beam is engineered to accommodate the narrow aperture of chirped-poling crystals, thus facilitating the acquisition of high spatial frequency components in the lateral direction. Such an elliptical passband in the Fourier space is then discretely rotated to generate a sequence of upconversion images, which allows computational recovery of a high-resolution object image through a combination of synthetic aperture and phase retrieval operations. Consequently, an enhanced spatial resolution of 39 $\mu$m is achieved within a field of view about 25 mm, which corresponds to a space-bandwidth product of 3.2$\times$10$^5$, over tenfold larger than previously demonstrated values. Moreover, the MIR upconversion imager can operate under a low-light illumination of 1 photon/pulse/pixel. Therefore, the presented paradigm of nonlinear Fourier ptychography paves the way toward high-throughput infrared imaging with massive resolvable elements and single-photon sensitivity, which would stimulate a variety of applications such as industry inspection and biomedical diagnosis.

physics.optics

Wide-field mid-infrared edge-enhanced upconversion imaging

Edge-enhanced imaging is critical for visualizing weakly absorbing and transparent objects. Extending this functionality into the mid-infrared (MIR) region enables chemical sensitivity and improved imaging performance for biomedical, material, and remote-sensing applications. Here, we present a wide-field MIR edge-enhanced upconversion imaging system that integrates vortex-pump complex-amplitude engineering with aperiodic quasi-phase matching. In contrast to the bright-field modality, the wide-field edge-enhanced operation shows sensitive dependence on the crystal position relative to the Fourier plane. The system achieves single-shot operation with a 25-mm field of view and 79-$\mu$m spatial resolution, yielding a record-high space-bandwidth product of $7.9 \times 10^4$. We show that this capability enables direct visualization of phase gradients in transparent optical elements and enhances structural contrast in biological specimens. The demonstrated architecture combines high sensitivity, spectral specificity, and robust edge detection, offering a promising route toward advanced MIR imaging in industrial inspection and biomedical diagnostics.

physics.optics

High-order mid-infrared nonlinear topological differentiator

High-order edge-enhanced imaging enables precise feature localization and effective background suppression, offering a powerful tool for real-time recognition and high-contrast visualization. Extending this capability to the mid-infrared (MIR) regime is particularly valuable for applications such as biomedical diagnostics, material inspection, and remote sensing, yet remains limited by inadequate spatial-frequency modulation fidelity and low detection sensitivity. Here, we demonstrate a high-sensitivity MIR upconversion differentiator operating at 3 $\mu$m, which achieves isotropic high-order edge enhancement by optically imprinting topological complex-amplitude patterns onto MIR Fourier components via nonlinear parametric interaction. Vortex transfer functions $t(k_r, \phi) \propto k_r^\ell e^{i\ell\phi}$ are precisely encoded on a phase-only spatial light modulator to enable tunable MIR differentiation from first- to fourth- order, with real-time switching at up to 60 Hz. Benefiting from a low-noise upconversion process and a single-photon-sensitive silicon camera, the system achieves high-contrast edge imaging under low-light conditions. Experimental results confirm accurate edge extraction and background suppression for both amplitude and phase objects, hence underscoring its potential for noninvasive diagnostics and label-free material analysis.

physics.optics