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Jizheng Wu

Publications and source records attributed to Jizheng Wu.

3 recordsLinked to original sources

Realization and manipulation of spiral charge density waves in a two-dimensional metal

Nearly degenerate charge-density-wave (CDW) states play a central role in the competition among collective phenomena. In real materials, however, these states are often intertwined by disorder, hindering their disentanglement and control. Here we show that strain can lift this near-degeneracy and spatially separate distinct CDW states in NbSe2. Using van der Waals (vdW) interactions, we stabilize a micron-scale strain network that produces spatially inhomogeneous strain fields. Within this landscape, the intrinsic 3 * 3 CDW superlattice of pristine NbSe2 transforms into an isolated unidirectional 4 * 1 order under 1D-confined compression, and into a 2 * 2 order under biaxial tension. The 4 * 1 CDW has a multiband origin and exhibits markedly enhanced thermal stability, persisting up to 70 K. At strain-network nodes, it further develops into chiral spiral textures, which can be melted by voltage pulses. These results establish strain as a powerful approach to disentangle, stabilize and manipulate competing electronic orders.

cond-mat.mes-hall↗

Enhancement of Ising superconductivity in monolayer NbSe$_2$ via surface fluorination

Recently discovered Ising superconductors have garnered considerable interest due to their anomalously large in-plane upper critical fields ($B_{c2}$). However, the requisite strong spin-orbital coupling in the Ising pairing mechanism generally renders these superconductors heavy-element dominant with notably low superconducting transition temperatures ($T_c$). Here, based on the Migdal-Eliashberg theory and the mean-field Bogoliubov-de Gennes Hamiltonian, we demonstrate a significant enhancement of Ising superconductivity in monolayer NbSe$_2$ through surface fluorination, as evidenced by concomitant improvements in $T_c$ and $B_{c2}$. This enhancement arises from three predominant factors. Firstly, fluorine atoms symmetrically and stably adhere to both sides of the monolayer NbSe$_2$, thereby maintaining the out-of-plane mirror symmetry and locking carrier spins out-of-plane. Secondly, fluorination suppresses the charge density wave in monolayer NbSe$_2$ and induces a van Hove singularity in the vicinity of the Fermi level, leading to a marked increase in the number of carriers and, consequently, strengthening the electron-phonon coupling (EPC). Lastly, the appearance of fluorine-related, low-frequency phonon modes further augments the EPC. Our findings suggest a promising avenue to elevate $T_c$ in two-dimensional Ising superconductors without compromising their Ising pairing.

cond-mat.supr-con↗

Quantifying proximity-induced superconductivity from first-principles calculations

Proximity induced superconductivity with a clean interface has attracted much attention in recent years. We discuss how the commonly-employed electron tunneling approximation can be hybridized with first-principles calculation to achieve a quantitative characterization starting from the microscopic atomic structure. By using the graphene-Zn heterostructure as an example, we compare this approximated treatment to the full \textit{ab inito} anisotropic Eliashberg formalism. Based on the calculation results, we discuss how superconductivity is affected by the interfacial environment.

cond-mat.supr-con↗