arXiv subjects
Publications and source records attributed to Joachim Ankerhold.
Josephson-photonics devices have emerged in the last years as versatile platforms to study light-charge interactions far from equilibrium and to create nonclassical radiation. Their potential to operate as nanoscale heat engines has also been discussed. The complementary mode of cooling is investigated here in the regimes of low and large photon occupancy, where nonlinearities are essential.
A Josephson junction embedded in a dissipative circuit can be externally driven to induce nonlinear dynamics of its phase. Classically, under sufficiently strong driving and weak damping, dynamic multi-stability emerges associated with dynamical bifurcations so that the often used modeling as a Duffing oscillator, which can exhibit bi-stability at the most, is insufficient. The present work analyzes in this regime corresponding quantum properties by mapping the problem onto a highly-nonlinear quasi-energy operator in a rotating frame. This allows us to identify in detail parameter regions where simplifications such as the Duffing approximation are valid, to explore classical-quantum correspondences, and to study how quantum fluctuations impact the effective junction parameters as well as the dynamics around higher amplitude classical fixed points.
The Josephson effect in scanning tunneling microscopy (STM) is an excellent tool to probe the properties of the superconducting order parameter on a local scale through the Ambegaokar-Baratoff (AB) relation. Using single atomic contacts created by means of atom manipulation, we demonstrate that in the extreme case of a single transport channel through the atomic junction modifications of the current-phase relation lead to significant deviations from the linear AB formula relating the critical current to the involved gap parameters. Using the full current-phase relation for arbitrary channel transmission, we model the Josephson effect in the dynamical Coulomb blockade regime because the charging energy of the junction capacitance cannot be neglected. We find excellent agreement with the experimental data. Projecting the current-phase relation onto the charge transfer operator shows that at high transmission multiple Cooper pair tunneling may occur. These deviations become non-negligible in Josephson-STM, for example, when scanning across single adatoms.
Within the emerging field of quantum thermodynamics the issues of heat transfer and heat rectification are basic ingredients for the understanding and design of heat engines or refrigerators at nanoscales. Here, a consistent and versatile approach for mesoscopic devices operating with continuous degrees of freedom is developed valid from low up to strong system-reservoir couplings and over the whole temperature range. It allows to cover weak to moderate nonlinearities and is applicable to various scenarios including the presence of disorder and external time-dependent fields. As a particular application coherent one-dimensional chains of anharmonic oscillators terminated by thermal reservoirs are analyzed with particular focus on rectification. The efficiency of the method opens a door to treat also rather long chains and extensions to higher dimensions and geometries.
Josephson junctions operated in the dynamical Coulomb blockade regime recently gained an significant amount of attention as central building block in concepts to demonstrate the non-Abelian character of Majorana fermions. Its physical properties are strongly affected by the intimate interplay of intrinsic quantum fluctuations and environmentally-induced quantum fluctuations each of which promoting different Cooper pair transport mechanisms at small voltages around zero. To shed light on the detailed transport mechanisms occurring in this type of junction, we performed voltage-biased measurements on the small-capacitance Josephson junction of a scanning tunneling microscope at milli-Kelvin temperatures. The low voltage-regime of experimental current-voltage characteristics can be modeled by the two complementary descriptions of phase coherent and incoherent Cooper pair transport, signaling the occurrence of qualitatively different transport mechanisms. This observation receives further support from analyzing the calculated Fano factor of the current noise as a probe for correlations in Cooper pair transport, following a theoretical proposal. Together our experimental observations and related data analysis provide a clear signature of coherent Cooper pair transport along with the absence of perfect charge quantized transport around zero voltage, as well as of incoherent Cooper pair transport towards higher voltages.
Charge and heat transfer through a nanoscale conductor is not only determined by the transmission properties of the electrons, but can also be strongly impacted by coupling to other degrees of freedom in the environment of the conductor. Here, we analyze the influence of the electromagnetic environment on a simple, yet significant thermoelectric property, the thermopower, in the simple transport scenario of single-charge transfer across a tunnel junction. Considering both thermal and out-of-equilibrium steady-state environments, we find that the thermopower can be strongly affected by the environmental state and can, in turn, act as a sensitive probe of environmental properties.
Heat transport in open quantum systems is particularly susceptible to the modeling of system-reservoir interactions. It thus requires to consistently treat the coupling between a quantum system and its environment. While perturbative approaches are successfully used in fields like quantum optics and quantum information, they reveal deficiencies, typically in the context of thermodynamics, when it is essential to respect additional criteria such as fluctuation-dissipation theorems. We use a non-perturbative approach for quantum dissipative dynamics based on a stochastic Liouville-von Neumann equation to provide a very general and extremely efficient formalism for heat currents and its correlations in open harmonic chains. Specific results are derived not only for first but also for second order moments which requires to account for both real and imaginary parts of bath-bath correlation functions. Spatiotemporal patterns are compared with weak coupling calculations. The regime of stronger system-reservoir couplings gives rise to an intimate interplay between reservoir fluctuations and heat transfer far from equilibrium.
We analyze the creation and emission of pairs of highly nonclassical microwave photons in a setup where a voltage-biased Josephson junction is connected in series to two electromagnetic oscillators. Tuning the external voltage such that the Josephson frequency equals the sum of the two mode frequencies, each tunneling Cooper pair creates one additional photon in both of the two oscillators. The time-resolved statistics of photon emission events from the two oscillators is investigated by means of single- and cross-oscillator variants of the second-order correlation function $g^{(2)}(τ)$ and the waiting-time distribution $w(τ)$. They provide insight into the strongly correlated quantum dynamics of the two oscillator subsystems and reveal a rich variety of quantum features of light including strong antibunching and the presence of negative values in the Wigner function.
When connecting a voltage-biased Josephson junction in series to several microwave cavities, a Cooper-pair current across the junction gives rise to a continuous emission of strongly correlated photons into the cavity modes. Tuning the bias voltage to the resonance where a single Cooper pair provides the energy to create an additional photon in each of the cavities, we demonstrate the entangling nature of these creation processes by simple witnesses in terms of experimentally accessible observables. To characterize the entanglement properties of the such created quantum states of light to the fullest possible extent, we then proceed to more elaborate entanglement criteria based on the knowledge of the full density matrix and provide a detailed study of bi- and multipartite entanglement. In particular, we illustrate how due to the relatively simple design of these circuits changes of experimental parameters allow one to access a wide variety of entangled states differing, e.g., in the number of entangled parties or the dimension of state space. Such devices, besides their promising potential to act as a highly versatile source of entangled quantum microwaves, may thus represent an excellent natural testbed for classification and quantification schemes developed in quantum information theory.
We have studied the temporal evolution of a quantum system subjected to strong dissipation at ultra-low temperatures where the system-bath interaction represents the leading energy scale. In this regime, theory predicts the time evolution of the system to follow a generalization of the classical Smoluchowski description, the quantum Smoluchowski equation, thus, exhibiting quantum Brownian motion characteristics. For this purpose, we have investigated the phase dynamics of a superconducting tunnel junction in the presence of high damping. We performed current-biased measurements on the small-capacitance Josephson junction of a scanning tunneling microscope placed in a low impedance environment at milli-Kelvin temperatures. We can describe our experimental findings by a quantum diffusion model with high accuracy in agreement with theoretical predications based on the quantum Smoluchowski equation. In this way we experimentally demonstrate that quantum systems subjected to strong dissipation follow quasi-classical dynamics with significant quantum effects as the leading corrections.
The non-Markovian dynamics of open quantum systems is still a challenging task, particularly in the non-perturbative regime at low temperatures. While the Stochastic Liouville-von Neumann equation (SLN) provides a formally exact tool to tackle this problem for both discrete and continuous degrees of freedom, its performance deteriorates for long times due to an inherently non-unitary propagator. Here we present a scheme which combines the SLN with projector operator techniques based on finite dephasing times, gaining substantial improvements in terms of memory storage and statistics. The approach allows for systematic convergence and is applicable in regions of parameter space where perturbative methods fail, up to the long time domain. Findings are applied to the coherent and incoherent quantum dynamics of two- and three-level systems. In the long time domain sequential and super-exchange transfer rates are extracted and compared to perturbative predictions.
When a mesoscopic conductor is coupled to a high-quality electromagnetic cavity the flow of charges and the flux of photons leaking out of the cavity can both depend strongly on the coupled quantum dynamics of the system. Using a voltage-biased Josephson junction as a model system, we demonstrate that there is a simple connection between the full counting statistics of the charges and the photons in the long time limit. We then reveal the intimate relation between the counting statistics and the nonlinear dynamics of the system, uncovering novel regimes of coherent charge and photon transport associated with bifurcations in the classical dynamics of the system.
The tunnel junction between tip and sample in a scanning tunneling microscope is an ideal platform to access the local density of states in the sample through the differential conductance. We show that the energy resolution that can be obtained is principally limited by the electromagnetic interaction of the tunneling electrons with the surrounding environmental impedance as well as the capacitative noise of the junction. The parameter tuning the sensitivity to the environmental impedance is the capacitance of the tunnel junction. The higher the junction capacitance, the less sensitive the tunnel junction to the environment resulting in better energy resolution. Modeling this effect within P(E)-theory, the P(E)-function describes the probability for a tunneling electron to exchange energy with the environment and can be regarded as the resolution function of the tunnel junction. We experimentally demonstrate this effect in a scanning tunneling microscope with a superconducting aluminum tip and a superconducting aluminum sample at a base temperature of 15mK, where it is most pronounced.
The interplay of the tunneling transfer of charges and the emission and absorption of light can be investigated in a setup, where a voltage-biased Josephson junction is connected in series with a microwave cavity. We focus here on the emission processes of photons and analyze the underlying time-dependent statistics using the second-order correlation function $g^{(2)}(τ)$ and the waiting-time distribution $w(τ)$. Both observables highlight the crossover from a coherent light source to a single-photon source. Due to the nonlinearity of the Josephson junction, tunneling Cooper pairs can create a great variety of non-classical states of light even at weak driving. Analytical results for the weak driving as well as the classical regime are complemented by a numerical treatment for the full nonlinear case. We also address the question of possible relations between $g^{(2)}(τ)$ and $w(τ)$ as well as the specific information which is provided by each of them.
Work, moments of work and heat flux are studied for the generic case of a strongly driven twolevel system immersed in a bosonic heat bath in domains of parameter space where perturbative treatments fail. This includes particularly the interplay between non-Markovian dynamics and moderate to strong external driving. Exact data are compared with predictions from weak coupling approaches. Further, the role of system-bath correlations in the initial thermal state and their impact on the heat flux are addressed. The relevance of these results for current experimental activities on solid state devices is discussed.
We analyze the quantum dynamics of two electromagnetic oscillators coupled in series to a voltage biased Josephson junction. When the applied voltage leads to a Josephson frequency across the junction which matches the sum of the two mode frequencies, tunneling Cooper pairs excite photons in both modes simultaneously leading to far-from-equilibrium states. These states display highly non-classical features including strong anti-bunching, violation of Cauchy-Schwartz inequalities, and number squeezing. The regimes of low and high photon occupancies allow for analytical results which are supported by a full numerical treatment. The impact of asymmetries between the two modes is explored, revealing a pronounced enhancement of number squeezing when the modes are damped at different rates.
In the dissipative quantum dynamics of a mesoscopic aggregate of excited two level systems (atoms) coupled to a single resonance mode of a cavity, two physical phenomena associated with superradiance appear. A pronounced emission peak on short time scales is related to the known superradiant burst of excited atoms cooperatively radiating into free space. It is followed by relaxation to a stationary state of the composite system such that for sufficiently large atom-field coupling a strongly correlated state emerges. The crossover to this state can be interpreted as the precursor of the transition from normal to superradiant phase in the thermodynamic limit of the Dicke Hamiltonian. Motivated by recent experimental activities, these features are investigated in detail for a mesoscopic number of atoms and a cavity embedded in a dissipative medium described by a damped Dicke model. We identify observables and characteristics of the quantum dynamics on shorter time scales which allow to clearly distinguish weakly correlated from strongly correlated Dicke physics.
The heat flow between a quantum system and its reservoir is analyzed when initially both are in a separable thermal state and asymptotically approach a correlated equilibrium. General findings are illustrated for specific systems and various classes of non-Markovian reservoirs. System-bath correlations are shown to be substantial at low temperatures even in the weak coupling regime. As a consequence, predictions of work and heat for actual experiments obtained within conventional perturbative approaches may often be questionable. Correlations induce characteristic imprints in heat capacities which opens a proposal to measure them in solid state devices.