arXiv subjects

Joel N. Ullom

Publications and source records attributed to Joel N. Ullom.

At least 55 records · Page 3Linked to original sources

arXiv2020

Improved Plutonium and Americium Photon Branching Ratios from Microcalorimeter Gamma Spectroscopy

Photon branching ratios are critical input data for activities such as nuclear materials protection and accounting because they allow material compositions to be extracted from measurements of gamma-ray intensities. Uncertainties in these branching ratios are often a limiting source of uncertainty in composition determination. Here, we use high statistics, high resolution (~60-70eV full-width-at-half-maximum at 100 keV) gamma-ray spectra acquired using microcalorimeter sensors to substantially reduce the uncertainties for 11 plutonium (238Pu,239Pu,241Pu) and 241Am branching ratios important for material control and accountability and nuclear forensics in the energy range of 125 keV to 208 keV. We show a reduction in uncertainty of over a factor of three for one branching ratio and a factor of 2{3 for four branching ratios.

nucl-ex↗

arXiv2020

Microwave multiplexing on the Keck Array

We describe an on-sky demonstration of a microwave-multiplexing readout system in one of the receivers of the Keck Array, a polarimetry experiment observing the cosmic microwave background at the South Pole. During the austral summer of 2018-2019, we replaced the time-division multiplexing readout system with microwave-multiplexing components including superconducting microwave resonators coupled to radio-frequency superconducting quantum interference devices at the sub-Kelvin focal plane, coaxial-cable plumbing and amplification between room temperature and the cold stages, and a SLAC Microresonator Radio Frequency system for the warm electronics. In the range 5-6 GHz, a single coaxial cable reads out 528 channels. The readout system is coupled to transition-edge sensors, which are in turn coupled to 150-GHz slot-dipole phased-array antennas. Observations began in April 2019, and we report here on an initial characterization of the system performance.

astro-ph.IM↗

arXiv2019

Demonstration of 220/280 GHz Multichroic Feedhorn-Coupled TES Polarimeter

We describe the design and measurement of feedhorn-coupled, transition-edge sensor (TES) polarimeters with two passbands centered at 220 GHz and 280 GHz, intended for observations of the cosmic microwave background. Each pixel couples polarized light in two linear polarizations by use of a planar orthomode transducer and senses power via four TES bolometers, one for each band in each linear polarization. Previous designs of this detector architecture incorporated passbands from 27 GHz to 220 GHz; we now demonstrate this technology at frequencies up to 315 GHz. Observational passbands are defined with an on-chip diplexer, and Fourier-transform-spectrometer measurements are in excellent agreement with simulations. We find coupling from feedhorn to TES bolometer using a cryogenic, temperature-controlled thermal source. We determine the optical efficiency of our device is $η$ = 77%$\pm$6% (75%$\pm$5%) for 220 (280) GHz, relative to the designed passband shapes. Lastly, we compare two power-termination schemes commonly used in wide-bandwidth millimeter-wave polarimeters and find equal performance in terms of optical efficiency and passband shape.

astro-ph.IM↗

arXiv2019

Tuning Excited State Electron Transfer in Fe Tetracyano-Polypyridyl Complexes

We have investigated photoinduced intramolecular electron transfer dynamics following metal-to-ligand charge-transfer (MLCT) excitation of [Fe(CN)$_4$(2,2'-bipyridine)]$^{2-}$ (1), [Fe(CN)$_4$(2,3-bis(2-pyridyl)pyrazine)]$^{2-}$ (2) and [Fe(CN)$_4$(2,2'-bipyrimidine)]$^{2-}$ (3) complexes in various solvents with static and time-resolved UV-visible absorption spectroscopy and Fe 2p3d resonant inelastic X-ray scattering. We observe $^3$MLCT lifetimes from 180 fs to 67 ps over a wide range of MLCT energies in different solvents by utilizing the strong solvatochromism of the complexes. Intramolecular electron transfer lifetimes governing $^3$MLCT relaxation increase monotonically and (super)exponentially as the $^3$MLCT energy is decreased in 1 and 2 by changing the solvent. This behavior can be described with non-adiabatic classical Marcus electron transfer dynamics along the indirect $^3$MLCT->$^3$MC pathway, where the $^3$MC is the lowest energy metal-centered (MC) excited state. In contrast, the $^3$MLCT lifetime in 3 changes non-monotonically and exhibits a maximum. This qualitatively different behaviour results from direct electron transfer from the $^3$MLCT to the electronic ground state (GS). This pathway involves nuclear tunnelling for the high-frequency polypyridyl skeleton mode ($\hbarω$ = 1530 cm$^{-1}$), which is more displaced for 3 than for either 1 or 2, therefore making the direct pathway significantly more efficient in 3. To our knowledge, this is the first observation of an efficient $^3$MLCT->GS relaxation pathway in an Fe polypyridyl complex. Our study suggests that further extending the MLCT state lifetime requires (1) lowering the $^3$MLCT state energy with respect to the $^3$MC state and (2) suppressing the intramolecular distortion of the electron-accepting ligand in the $^3$MLCT excited state to suppress the rate of direct $^3$MLCT->GS electron transfer.

physics.chem-ph↗

arXiv2019

A Model for Excess Johnson Noise in Superconducting Transition-edge Sensors

Transition-Edge Sensors (TESs) are two-dimensional superconducting films used to detect energy or power. TESs are voltage biased in the resistive transition where the film resistance is both finite and a strong function of temperature. Electrical noise is observed in TESs that exceeds the predictions of existing noise theories. In this manuscript, we describe a model for the unexplained excess noise based on the dynamic resistance of the TES and noise mixed down from frequencies around the Josephson oscillations. We derive an expression for the power spectral density of this noise and show that its predictions match measured data.

cond-mat.supr-con↗

arXiv2019

Testing general relativity with accretion onto compact objects

The X-ray emission of neutron stars and black holes presents a rich phenomenology that can lead us to a better understanding of their nature and to address more general physics questions: Does general relativity apply in the strong gravity regime? Is spacetime around black holes described by the Kerr metric? This white paper considers how we can investigate these questions by studying reverberation mapping and quasi-periodic oscillations in accreting systems with a combination of high-spectral and high-timing resolution. In the near future, we will be able to study compact objects in the X-rays in a new way: advancements in transition-edge sensors (TES) technology will allow for electron-volt-resolution spectroscopy combined with nanoseconds-precision timing.

astro-ph.HE↗

arXiv2019

Exploring the physics of neutron stars with high-resolution, high-throughput X-ray spectroscopy

The advent of moderately high-resolution X-ray spectroscopy with Chandra and XMM promised to usher in a new age in the study of neutron stars: we thought we would study neutron stars like stars, with resolved absorption spectra revealing their surface chemical composition and physical conditions (e.g. surface gravity, pressure, temperature). Nature, however, did not cooperate in this endeavor, as observations of neutron stars have not revealed verified atomic absorption lines yet. In the near future, advancements in transition-edge sensors (TES) technology will allow for electron-volt-resolution spectroscopy combined with nanoseconds-precision timing. Combining these detectors with collector optics will also us to study neutron stars in much greater detail by achieving high-energy resolution with much larger collecting areas to uncover even weak spectral features over a wide range of the photon energies. Perhaps we will finally be able to study neutron stars like stars.

astro-ph.HE↗

arXiv2018

Studies of Systematic Uncertainties for Simons Observatory: Detector Array Effects

In this proceeding, we present studies of instrumental systematic effects for the Simons Obsevatory (SO) that are associated with the detector system and its interaction with the full SO experimental systems. SO will measure the Cosmic Microwave Background (CMB) temperature and polarization anisotropies over a wide range of angular scales in six bands with bandcenters spanning from 27 GHz to 270 GHz. We explore effects including intensity-to-polarization leakage due to coupling optics, bolometer nonlinearity, uncalibrated gain variations of bolometers, and readout crosstalk. We model the level of signal contamination, discuss proposed mitigation schemes, and present instrument requirements to inform the design of SO and future CMB projects.

astro-ph.IM↗

arXiv2018

Simons Observatory Large Aperture Telescope Receiver Design Overview

The Simons Observatory (SO) will make precision temperature and polarization measurements of the cosmic microwave background (CMB) using a series of telescopes which will cover angular scales between one arcminute and tens of degrees and sample frequencies between 27 and 270 GHz. Here we present the current design of the large aperture telescope receiver (LATR), a 2.4 m diameter cryostat that will be mounted on the SO 6 m telescope and will be the largest CMB receiver to date. The cryostat size was chosen to take advantage of the large focal plane area having high Strehl ratios, which is inherent to the Cross-Dragone telescope design. The LATR will be able to accommodate thirteen optics tubes, each having a 36 cm diameter aperture and illuminating several thousand transition-edge sensor (TES) bolometers. This set of equipment will provide an opportunity to make measurements with unparalleled sensitivity. However, the size and complexity of the LATR also pose numerous technical challenges. In the following paper, we present the design of the LATR and include how we address these challenges. The solutions we develop in the process of designing the LATR will be informative for the general CMB community, and for future CMB experiments like CMB-S4.

astro-ph.IM↗

arXiv2018

The Simons Observatory: Instrument Overview

The Simons Observatory (SO) will make precise temperature and polarization measurements of the cosmic microwave background (CMB) using a set of telescopes which will cover angular scales between 1 arcminute and tens of degrees, contain over 60,000 detectors, and observe at frequencies between 27 and 270 GHz. SO will consist of a 6 m aperture telescope coupled to over 30,000 transition-edge sensor bolometers along with three 42 cm aperture refractive telescopes, coupled to an additional 30,000+ detectors, all of which will be located in the Atacama Desert at an altitude of 5190 m. The powerful combination of large and small apertures in a CMB observatory will allow us to sample a wide range of angular scales over a common survey area. SO will measure fundamental cosmological parameters of our universe, constrain primordial fluctuations, find high redshift clusters via the Sunyaev-Zel`dovich effect, constrain properties of neutrinos, and trace the density and velocity of the matter in the universe over cosmic time. The complex set of technical and science requirements for this experiment has led to innovative instrumentation solutions which we will discuss. The large aperture telescope will couple to a cryogenic receiver that is 2.4 m in diameter and nearly 3 m long, creating a number of technical challenges. Concurrently, we are designing the array of cryogenic receivers housing the 42 cm aperture telescopes. We will discuss the sensor technology SO will use and we will give an overview of the drivers for and designs of the SO telescopes and receivers, with their cold optical components and detector arrays.

astro-ph.IM↗

arXiv2018

Advanced ACTPol TES Device Parameters and Noise Performance in Fielded Arrays

The Advanced ACTPol (AdvACT) upgrade to the Atacama Cosmology Telescope (ACT) features arrays of aluminum manganese transition-edge sensors (TESes) optimized for ground-based observations of the Cosmic Microwave Background (CMB). Array testing shows highly responsive detectors with anticipated in-band noise performance under optical loading. We report on TES parameters measured with impedance data taken on a subset of TESes. We then compare modeled noise spectral densities to measurements. We find excess noise at frequencies around 100 Hz, nearly outside of the signal band of CMB measurements. In addition, we describe full-array noise measurements in the laboratory and in the field for two new AdvACT mid-frequency arrays, sensitive at bands centered on 90 and 150 GHz, and data for the high-frequency array (150/230 GHz) as deployed.

astro-ph.IM↗

arXiv2018

Low Temperature Detectors for CMB Imaging Arrays

We review advances in low temperature detector (LTD) arrays for Cosmic Microwave Background (CMB) polarization experiments, with a particular emphasis on imaging arrays. We briefly motivate the science case, which has spurred a large number of independent experimental efforts. We describe the challenges associated with CMB polarization measurements and how these challenges impact LTD design. Key aspects of an ideal CMB polarization imaging array are developed and compared to the current state-of-the-art. These aspects include dual-polarization-sensitivity, background-limited detection over a 10:1 bandwidth ratio, and frequency independent angular responses. Although existing technology lacks all of this capability, today's CMB imaging arrays achieve many of these ideals and are highly advanced superconducting integrated circuits. Deployed arrays map the sky with pixels that contain elements for beam formation, polarization diplexing, passband definition in multiple frequency channels, and bolometric sensing. Several detector architectures are presented. We comment on the implementation of both transition-edge-sensor bolometers and microwave kinetic inductance detectors for CMB applications. Lastly, we discuss fabrication capability in the context of next-generation instruments that call for $\sim 10^6$ sensors.

astro-ph.IM↗

arXiv2018

Prime-Cam: A first-light instrument for the CCAT-prime telescope

CCAT-prime will be a 6-meter aperture telescope operating from sub-mm to mm wavelengths, located at 5600 meters elevation on Cerro Chajnantor in the Atacama Desert in Chile. Its novel crossed-Dragone optical design will deliver a high throughput, wide field of view capable of illuminating much larger arrays of sub-mm and mm detectors than can existing telescopes. We present an overview of the motivation and design of Prime-Cam, a first-light instrument for CCAT-prime. Prime-Cam will house seven instrument modules in a 1.8 meter diameter cryostat, cooled by a dilution refrigerator. The optical elements will consist of silicon lenses, and the instrument modules can be individually optimized for particular science goals. The current design enables both broadband, dual-polarization measurements and narrow-band, Fabry-Perot spectroscopic imaging using multichroic transition-edge sensor (TES) bolometers operating between 190 and 450 GHz. It also includes broadband kinetic induction detectors (KIDs) operating at 860 GHz. This wide range of frequencies will allow excellent characterization and removal of galactic foregrounds, which will enable precision measurements of the sub-mm and mm sky. Prime-Cam will be used to constrain cosmology via the Sunyaev-Zeldovich effects, map the intensity of [CII] 158 $μ$m emission from the Epoch of Reionization, measure Cosmic Microwave Background polarization and foregrounds, and characterize the star formation history over a wide range of redshifts. More information about CCAT-prime can be found at www.ccatobservatory.org.

astro-ph.IM↗

arXiv2018

First Calorimetric Measurement of Electron Capture in ${}^{193}$Pt with a Transition Edge Sensor

The neutrino mass can be extracted from a high statistics, high resolution calorimetric spectrum of electron capture in ${}^{163}$Ho. In order to better understand the shape of the calorimetric electron capture spectrum, a second isotope was measured with a close to ideal absorber-source configuration. ${}^{193}$Pt was created by irradiating a ${}^{192}$Pt-enriched platinum foil in a nuclear reactor. This Pt-in-Pt absorber was designed to have a nearly ideal absorber-source configuration. The measured ${}^{193}$Pt calorimetric electron-capture spectrum provides an independent check on the corresponding theoretical calculations, which have thus far been compared only for ${}^{163}$Ho. The first experimental and theoretically-calculated spectra from this ${}^{193}$Pt-in-Pt absorber are presented and overlaid for preliminary comparison of theory with experiment.

physics.atom-ph↗

arXiv2018

Tile-and-trim micro-resonator array fabrication optimized for high multiplexing factors

We present a superconducting micro-resonator array fabrication method that is scalable, reconfigurable, and has been optimized for high multiplexing factors. The method uses uniformly sized tiles patterned on stepper photolithography reticles as the building blocks of an array. We demonstrate this technique on a 101-element microwave kinetic inductance detector (MKID) array made from a titanium-nitride superconducting film. Characterization reveals 1.5\% maximum fractional frequency spacing deviations caused primarily by material parameters that vary smoothly across the wafer. However, local deviations exhibit a Gaussian distribution in fractional frequency spacing with a standard deviation of $2.7 \times 10^{-3}$. We exploit this finding to increase the yield of the BLAST-TNG $250 \; μ\text{m}$ production wafer by placing resonators in the array close in both physical and frequency space. This array consists of 1836 polarization-sensitive MKIDs wired in three multiplexing groups. We present the array design and show that the achieved yield is consistent with our model of frequency collisions and is comparable to what has been achieved in other low temperature detector technologies.

physics.ins-det↗

arXiv2017

Microstructure analysis of bismuth absorbers for transition-edge sensor X-ray microcalorimeters

Transition-edge sensors (TESs) as microcalorimeters offer high resolving power, owning to their sharp response and low operating temperature. In the hard X-ray regime and above, the demand for high quantum-efficiency requires the use of absorbers. Bismuth (Bi), owing to its low heat carrier density and high X-ray stopping power, has been widely used as an absorber material for TESs. However, distinct spectral responses have been observed for Bi absorbers deposited via evaporation versus electroplating. Evaporated Bi absorbers are widely observed to have a non-Gaussian tail on the low energy side of measured spectra. In this study, we fabricated Bi absorbers via these two methods, and performed microstructure analysis using scanning electron microscopy (SEM) and X-ray diffraction microscopy. The two types of material showed the same crystallographic structure, but the grain size of the evaporated Bi was about 40 times smaller than that of the electroplated Bi. This distinction in grain size is likely to be the cause of their different spectral responses.

physics.ins-det↗

arXiv2017

Eliminating the non-Gaussian spectral response of X-ray absorbers for transition-edge sensors

Transition-edge sensors (TES) as microcalorimeters for high-energy-resolution X-ray spectroscopy are often fabricated with an absorber made of materials with high Z (for X-ray stopping power) and low heat capacity (for high resolving power). Bismuth represents one of the most compelling options. TESs with evaporated bismuth absorbers have shown spectra with undesirable and unexplained low-energy tails. We have developed TESs with electroplated bismuth absorbers over a gold layer that are not afflicted by this problem and that retain the other positive aspects of this material. To better understand these phenomena, we have studied a series of TESs with gold, gold/evaporated bismuth, and gold/electroplated bismuth absorbers, fabricated on the same die with identical thermal coupling. We show that bismuth morphology is linked to the spectral response of X-ray TES microcalorimeters.

physics.ins-det↗

arXiv2017

L-Edge Spectroscopy of Dilute, Radiation-Sensitive Systems Using a Transition-Edge-Sensor Array

We present X-ray absorption spectroscopy and resonant inelastic X-ray scattering (RIXS) measurements on the iron L-edge of 0.5 mM aqueous ferricyanide. These measurements demonstrate the ability of high-throughput transition-edge-sensor (TES) spectrometers to access the rich soft X-ray (100-2000eV) spectroscopy regime for dilute and radiation-sensitive samples. Our low-concentration data are in agreement with high-concentration measurements recorded by conventional grating-based spectrometers. These results show that soft X-ray RIXS spectroscopy acquired by high-throughput TES spectrometers can be used to study the local electronic structure of dilute metal-centered complexes relevant to biology, chemistry and catalysis. In particular, TES spectrometers have a unique ability to characterize frozen solutions of radiation- and temperature-sensitive samples.

physics.ins-det↗