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Johannes Eberle

Publications and source records attributed to Johannes Eberle.

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Color Centers and Hyperbolic Phonon Polaritons in Hexagonal Boron Nitride: A New Platform for Quantum Optics

Hyperbolic phonon polaritons (HPPs) in hexagonal boron nitride (hBN) confine mid-infrared light to deep-subwavelength scales and may offer a powerful route to strong light-matter interactions. Generation and control of HPPs are typically accessed using classical near-field probes, which limits experiments at the quantum level.A complementary frontier in hBN research focuses on color centers: bright, stable, atomically localized emitters that have rapidly emerged as a promising platform for solid-state quantum optics. Here we establish a key connection between these two directions by developing a cavity-QED framework in which a single hBN color center serves as a quantum source of HPPs. We quantify the emitter-HPP interaction and analyze two generation schemes. The first is spontaneous emission into the phonon sideband, which can produce single-HPP events and, in ultrathin slabs, becomes single-mode with an enhanced decay rate. The second is a stimulated Raman process that provides frequency selectivity, tunable conversion rate, and narrowband excitation. This drive launches spatially confined, ray-like HPPs that propagate over micrometer distances. We also outline a two-emitter correlation measurement that can directly test the single-polariton character of these emissions. By connecting color-center quantum optics with hyperbolic polaritonics, our approach enables quantum emitters to act as on-chip quantum sources and controls for HPPs, while HPPs provide long-range channels that couple spatially separated emitters. Together, these capabilities point to a new direction for mid-infrared photonic experiments that unite strong coupling, spectral selectivity, and spatial reach within a single material system.

cond-mat.mes-hall

A defect in diamond with millisecond-scale spin relaxation time at room temperature

Spin defects in diamond are promising platforms for quantum sensing. The longest electron spin relaxation times ($T_1$) at room temperature for solid-state defects are observed in nitrogen vacancy centers in diamond, which can reach 6.67 ms, and substitutional nitrogen ("P1 centers") in diamond, which exhibit a $T_1$ of 2 ms. No other solid-state defect has exhibited millisecond-scale spin relaxation times at room temperature thus far. Here, we characterize the spin properties of the WAR5 defect in diamond with pulsed electron spin resonance. The observed $T_1$ is one of the longest for solid-state spin defects: 0.97(27) ms at room temperature and 14.38(19) min at 4 K. The observed coherence time ($T_2$) is 246(7) $μ$s, which can be extended to 6.49(34) ms at 4 K with dynamical decoupling. Furthermore, we demonstrate optical spin polarization with a range of wavelengths from 405 nm to 500 nm and propose potential zero-phonon line candidates.

cond-mat.mtrl-sci

Cooperative Emission from Quantum Emitters in Hexagonal Boron Nitride Layers

Collective light emission from many-body quantum systems is a cornerstone of quantum optics, yet its implementation in solid-state platforms operating under ambient conditions remains highly challenging. Large-bandgap van der Waals materials such as hexagonal boron nitride (hBN) host stable room-temperature single-photon emitters with narrow linewidths across a broad spectral range. However, cooperative radiative effects in this system have not been previously explored. Here we demonstrate collective emission from quantum-emitter ensembles in hBN layers when the emitters are nearly indistinguishable and positioned within a sub-wavelength proximity. Using confocal microscopy and a Hanbury Brown-Twiss (HBT) configuration, we identify both isolated emitters and ensembles activated by localized electron-beam irradiation. Time-resolved photoluminescence measurements reveal a superlinear intensity enhancement and a pronounced acceleration of the radiative decay in tightly confined ensembles, with lifetimes approaching the temporal resolution of our experimental system (about 500 ps), compared to approximately 1.85 ns for single emitters or large, spatially extended ensembles. Complementary second-order photon-correlation measurements exhibit sub-Poissonian antidip consistent with emission from a few indistinguishable emitters. The simultaneous observation of lifetime shortening and enhanced emission provides direct evidence of cooperative emission at room temperature, achieved without optical cavities or cryogenic cooling. These results establish optically active defect ensembles in hBN as a scalable solid-state platform for engineered collective quantum optics in two-dimensional materials, opening avenues toward ultrabright superradiant light sources and nonclassical photonic states for quantum technologies.

quant-ph

Single Photon Emitters in Ultra-Thin Hexagonal Boron Nitride Layers

Single-photon emitters (SPE) in hexagonal boron nitride (h-BN) are promising for applications ranging from single-photon sources to quantum sensors. Previous studies exclusively focused on the generation and characterization of SPEs in relatively thick h-BN layers ($\geq$ 30 nm). However, for electrical and magnetic sensing applications, the thickness of the h-BN limits the attainable spatial resolution. Here, we report the observation of blue-wavelength emitters (B-centers) activated by electron beam irradiation in ultra-thin ($\simeq$ 3 nm) h-BN. These SPEs in ultra-thin flakes exhibit reduced brightness, broader zero-phonon line, and enhanced photobleaching. Remarkably, upon encapsulation in thicker h-BN, we restore their brightness, narrow linewidth 230$μ$eV at 5K, resolution limited), suppress photobleaching, and confirm single-photon emission with $ g^{(2)}(0) < 0.4$ at room temperature. The possibility of generating SPEs in a few-layer h-BN and their subsequent incorporation into a van der Waals heterostructure paves the way for achieving quantum sensing with unprecedented nanometer-scale spatial resolution.

cond-mat.mes-hall