arXiv subjects

John Cumings

Publications and source records attributed to John Cumings.

12 recordsLinked to original sources

arXiv2026

Autonomous epitaxial atomic-layer synthesis via real-time computer vision of electron diffraction

Autonomous science platforms which make decisions on the fly are fundamentally changing the outlook for materials development. AI-driven schemes can effectively reduce the total number of iterations needed to arrive at the best stoichiometry for desired properties or optimum synthesis parameters by significant margins. Here, we demonstrate real-time closed-loop autonomous navigation of a multi-dimensional synthesis parameter space for fabricating phase-pure epitaxial films of a metastable functional oxide phase using pulsed laser deposition. Sequential growth iterations in search of the optimized recipe to stabilize the desired crystal phase were performed using frame-by-frame quantitative computer vision of electron diffraction images at the unit-cell level. Our scheme regularly resulted in > 30-fold reduction in the number of experiments compared to comprehensive parameter-space mapping. The real-time workflow developed here can be readily extended to other thin film synthesis platforms opening the door for self-driving atomic-level materials design as well as autonomous semiconductor manufacturing.

cond-mat.mtrl-sci↗

arXiv2025

From plasma to pattern: observation and characterization of periodic structure formation in dielectric breakdown channels of electron-irradiated insulators

Dielectric breakdown of insulators is one of the most common failure modes of electronics in the high-radiation environment of space, but its mechanics remain poorly understood. When electron-irradiated polymethyl methacrylate (PMMA) undergoes breakdown, the resulting channels exhibit striking periodic structures with characteristic wavelengths ~80 μm in the recently identified ivy-mode channels. These previously unobserved modulations offer unique insights into the physics of ultra-fast dielectric breakdown. Through materials characterization and theoretical modeling, we identify the physical instability mechanism responsible for these structures. Raman spectroscopy reveals that carbon deposition correlates with channel width variations, indicating that periodic structure formation occurs during the plasma discharge phase. We evaluated three candidate instability mechanisms: the Asaro-Tiller-Grinfeld instability, the Plateau-Rayleigh instability, and the z-pinch entropy mode. The first two mechanisms operate on incompatible timescales and require unphysical material parameters to match observations. In contrast, the z-pinch entropy mode operates during the nanosecond discharge phase and produces wavelengths consistent with plasma densities of 0.1-1% of solid density and temperatures of 10-100 eV. Current measurements from isolated discharge channels (~200 A) validate theoretical predictions for the entropy mode. These findings establish that the entropy mode plasma instability during the discharge phase, rather than post discharge thermal or mechanical processes, govern periodic structure formation in breakdown channels. This work provides new insights into the physics of dielectric breakdown and establishes a framework for predicting discharge morphology and characteristics in insulators.

physics.app-ph↗

arXiv2025

Electrically insulating materials for centrifugal mirrors

The centrifugal mirror confinement scheme incorporates supersonic rotation into a magnetic mirror device, which stabilizes and heats the plasma. This concept is under investigation in the Centrifugal Mirror Fusion Experiment (CMFX) at the University of Maryland. Plasma rotation is driven by an axial magnetic field and a radial electric field that lead to velocity drifts in the azimuthal direction. An electrically insulating material is required to prevent the applied voltage from shorting on the grounded chamber. Hexagonal boron nitride (hBN) is a promising candidate material for plasma-facing components in future centrifugal mirrors due to its exceptional thermal and electrical properties. However, its performance under intense particle and heat fluxes characteristic of the plasma edge in fusion devices remains largely unexplored. Computational modeling for ion- and neutron-material interactions was carried out with RustBCA and OpenMC, respectively, and predicts relatively good performance in comparison to other insulating materials. Material coupons were then exposed to plasma in PISCES-A at UCSD and CMFX. A load-locked sample feedthrough was constructed and installed on CMFX to test coupons. Two erosion mechanisms were identified -- sputtering and grain ejection -- both of which were more apparent in silicon carbide than hBN.

physics.plasm-ph↗

arXiv2017

Topological frustration of artificial spin ice

Frustrated systems, typically characterized by competing interactions that cannot all be simultaneously satisfied, display rich behaviours not found elsewhere in nature. Artificial spin ice takes a materials-by-design approach to studying frustration, where lithographically patterned bar magnets mimic the frustrated interactions in real materials but are also amenable to direct characterization. Here, we introduce controlled topological defects into square artificial spin ice lattices in the form of lattice edge dislocations and directly observe the resulting spin configurations. We find the presence of a topological defect produces extended frustration within the system caused by a domain wall with indeterminate configuration. Away from the dislocation, the magnets are locally unfrustrated, but frustration of the lattice persists due to its topology. Our results demonstrate the non-trivial nature of topological defects in a new context, with implications for many real systems in which a typical density of dislocations could fully frustrate a canonically unfrustrated system.

cond-mat.mes-hall↗

arXiv2015

FePd$_{3}$ as a material for thermally active artificial spin ice

We introduce FePd$_{3}$ as a new material for studying thermally active artificial spin ice (ASI) systems and use it to investigate both the square and kagome ice geometries. We readily achieve perfect ground state ordering in the square lattice and demonstrate the highest yet degree of monopole charge-ordering in the kagome lattice. We find that smaller lattice constants in the kagome system generally produce larger domains of charge order. Monte Carlo simulations show excellent agreement with our data when a small amount of disorder is included in the simulation.

cond-mat.mes-hall↗

arXiv2012

Dynamics of artificial spin ice: continuous honeycomb network

We model the dynamics of magnetization in an artificial analog of spin ice specializing to the case of a honeycomb network of connected magnetic nanowires. The inherently dissipative dynamics is mediated by the emission, propagation and absorption of domain walls in the links of the lattice. These domain walls carry two natural units of magnetic charge, whereas sites of the lattice contain a unit magnetic charge. Magnetostatic Coulomb forces between these charges play a major role in the physics of the system, as does quenched disorder caused by imperfections of the lattice. We identify and describe different regimes of magnetization reversal in an applied magnetic field determined by the orientation of the applied field with respect to the initial magnetization. One of the regimes is characterized by magnetic avalanches with a 1/n distribution of lengths.

cond-mat.mes-hall↗

arXiv2011

Reducing Disorder in Artificial Kagome Ice

Artificial spin ice has become a valuable tool for understanding magnetic interactions on a microscopic level. The strength in the approach lies in the ability of a synthetic array of nanoscale magnets to mimic crystalline materials, composed of atomic magnetic moments. Unfortunately, these nanoscale magnets, patterned from metal alloys, can show substantial variation in relevant quantities such as coercive field, with deviations up to 6%. By carefully studying the reversal process of artificial kagome ice, we can directly measure the distribution of coercivities, and by switching from disconnected islands to a connected structure, we find that the coercivity distribution can achieve a deviation of only 3.3%. These narrow deviations should allow the observation of behavior that mimics canonical spin-ice materials more closely.

cond-mat.mtrl-sci↗

arXiv2010

Controlling the thermal contact resistance of a carbon nanotube heat spreader

The ability to tune the thermal resistance of carbon nanotube mechanical supports from insulating to conducting could permit the next generation of thermal management devices. Here, we demonstrate fabrication techniques for carbon nanotube supports that realize either weak or strong thermal coupling, selectively. Direct imaging by in-situ electron thermal microscopy shows that the thermal contact resistance of a nanotube weakly-coupled to its support is greater than 250 K*m/W and that this value can be reduced to 4.2(+5.6/-2.1) K*m/W by imbedding the nanotube in metal contacts.

cond-mat.mes-hall↗

arXiv2008

Direct observation of the ice rule in artificial kagome spin ice

Recently, significant interest has emerged in fabricated systems that mimic the behavior of geometrically-frustrated materials. We present the full realization of such an artificial spin ice system on a two-dimensional kagome lattice and demonstrate rigid adherence to the local ice rule by directly counting individual pseudo-spins. The resulting spin configurations show not only local ice rules and long-range disorder, but also correlations consistent with spin ice Monte Carlo calculations. Our results suggest that dipolar corrections are significant in this system, as in pyrochlore spin ice, and they open a door to further studies of frustration in general.

cond-mat.mtrl-sci↗

arXiv2007

Electron Thermal Microscopy

The progress of semiconductor electronics toward ever-smaller length scales and associated higher power densities brings a need for new high-resolution thermal microscopy techniques. Traditional thermal microscopy is performed by detecting infrared radiation with far-field optics, where the resolution is limited by the wavelength of the light. By adopting a serial, local-probe approach, near-field and scanned-probe microscopies can surpass this limit but sacrifice imaging speed. In the same way that electron microscopy was invented to overcome the resolution limits of light microscopy, we here demonstrate a thermal imaging technique that uses an electron microscope to overcome the limits of infrared thermal microscopy, without compromising imaging speed. With this new technique, which we call electron thermal microscopy, temperature is resolved by detecting the liquid-solid transition of arrays of nanoscale islands, producing thermal maps in real-time (30 thermal images per second over a 16um^2 field-of-view). The experimental demonstration is supported by combined electrical and thermal modeling.

cond-mat.mtrl-sci↗

arXiv2007

Kondo Physics in Nanotubes: Magnetic-field dependence and singlet-triplet Kondo

In a single-walled carbon nanotube, we observe the spin-1/2 Kondo effect. The energy of spin-resolved Kondo peaks is proportional to magnetic field at high fields, contrary to recent reports. At lower fields, the energy falls below this linear dependence, in qualitative agreement with theoretical expectations. For even electron occupancy, we observe a spin-1 Kondo effect due to the degeneracy of the triplet ground states. Tuning gate voltage within the same Coulomb diamond drives a transition to a singlet ground state. We also independently tune the energy difference between singlet and triplet states with a magnetic field. The Zeeman splitting thus measured confirms the value of the g-factor measured from the spin-1/2 Kondo feature.

cond-mat.mes-hall↗

arXiv2007

Transport Properties of Carbon Nanotube C$_{60}$ Peapods

We measure the conductance of carbon nanotube peapods from room temperature down to 250mK. Our devices show both metallic and semiconducting behavior at room temperature. At the lowest temperatures, we observe single electron effects. Our results suggest that the encapsulated C$_{60}$ molecules do not introduce substantial backscattering for electrons near the Fermi level. This is remarkable given that previous tunneling spectroscopy measurements show that encapsulated C$_{60}$ strongly modifies the electronic structure of a nanotube away from the Fermi level.

cond-mat.mes-hall↗