arXiv subjects

John E. Sader

Publications and source records attributed to John E. Sader.

17 recordsLinked to original sources

arXiv2026

Settling of chiral particles in a turbulent flow

Chiral particles are experimentally investigated while settling inwater with various turbulence intensity levels. The locations and orientations of the particles are tracked over time, allowing the close investigation of the particles' settling dynamics. The generated turbulent flow is measured using laser Doppler anemometry (LDA), and the turbulence strength varies between experiments in the range $0 \leq Re_λ\leq 250$. Starting with quiescent particle settling, the chiral particle's orientation dynamics are studied, revealing a preferred alignment and a strong translation-rotation coupling. The particle chirality determines the preferred rotation direction, though the alignment and translation-rotation coupling gradually vanish with increasing turbulence. We identify multiple settling modes for the chiral particles, which are characterised by the evolution of the rotation angles. Finally, a theoretical model assuming a simplified chiral particle in Stokes flow clarifies the emergence of each settling mode.

physics.flu-dyn↗

arXiv2025

Optically Actuated Transitions in Multimodal, Bistable Micromechanical Oscillators

We experimentally demonstrate a new class of optomechanical nonlinearities in weakly damped micromechanical resonators, arising from the interplay between the Duffing nonlinearity, intermodal coupling, and thermal fluctuations. Within the bistable regime of a single Duffing mode driven by radiation pressure forces, we observe stochastically generated sidebands, originating from thermal fluctuations around equilibrium trajectories in phase space, and exploit these sidebands to induce probabilistic transitions between bistable states using weak secondary acoustic excitation. Extending this framework to multimodal interactions, we show that nonlinear modes coupling within the same resonator leads to similar transitions due to parametric modulation around the noise-excited sidebands as a result of frequency mixing. Simultaneously, abrupt changes in displacements of modes cause their instantaneous energy exchange rates to span five orders of magnitude. These findings open new avenues for reconfigurable optomechanical networks, nonreciprocal energy transport, and precision sensing based on dynamically tunable mechanical nonlinearities.

physics.optics↗

arXiv2025

Visual anemometry of natural vegetation from their leaf motion

High-resolution, near-ground wind-speed data are critical for improving the accuracy of weather predictions and climate models,$^{1-3}$ supporting wildfire control efforts,$^{4-7}$ and ensuring the safe passage of airplanes during takeoff and landing maneouvers.$^{8,9}$ Quantitative wind speed anemometry generally employs on-site instrumentation for accurate single-position data or sophisticated remote techniques such as Doppler radar for quantitative field measurements. It is widely recognized that the wind-induced motion of vegetation depends in a complex manner on their structure and mechanical properties, obviating their use in quantitative anemometry.$^{10-14}$ We analyze measurements on a host of different vegetation showing that leaf motion can be decoupled from the leaf's branch and support structure, at low-to-moderate wind speed, $U_{wind}$. This wind speed range is characterized by a leaf Reynolds number, enabling the development of a remote, quantitative anemometry method based on the formula, $U_{wind}\approx740\sqrt{μU_{leaf}/ρD}$, that relies only on the leaf size $D$, its measured fluctuating (RMS) speed $U_{leaf}$, the air viscosity $μ$, and its mass density $ρ$. This formula is corroborated by a first-principles model and validated using a host of laboratory and field tests on diverse vegetation types, ranging from oak, olive, and magnolia trees through to camphor and bullgrass. The findings of this study open the door to a new paradigm in anemometry, using natural vegetation to enable remote and rapid quantitative field measurements at global locations with minimal cost.

physics.flu-dyn↗

arXiv2024

Data-driven fingerprint nanomechanical mass spectrometry

Fingerprint analysis is a ubiquitous tool for pattern recognition with applications spanning from geolocation and DNA analysis to facial recognition and forensic identification. Central to its utility is the ability to provide accurate identification without an a priori mathematical model for the pattern. We report a data-driven fingerprint approach for nanoelectromechanical systems mass spectrometry (NEMS-MS) that enables mass measurements of particles and molecules using complex, uncharacterized nanoelectromechanical devices of arbitrary specification. NEMS-MS is based on the frequency shifts of the NEMS vibrational modes induced by analyte adsorption. The sequence of frequency shifts constitutes a fingerprint of this adsorption, which is directly amenable to pattern matching. Two current requirements of NEMS-based mass spectrometry are: (1) a priori knowledge or measurement of the device mode-shapes, and (2) a mode-shape-based model that connects the induced modal frequency shifts to mass adsorption. This may not be possible for advanced NEMS with three-dimensional mode-shapes and nanometer-sized features. The advance reported here eliminates this impediment, thereby allowing device designs of arbitrary specification and size to be employed. This enables the use of advanced NEMS devices with complex vibrational modes, which offer unprecedented prospects for attaining the ultimate detection limits of nanoelectromechanical mass spectrometry.

physics.ins-det↗

arXiv2024

Direct Radiation Pressure Measurements for Lightsail Membranes

Ultrathin lightsails propelled by laser radiation pressure to relativistic speeds are currently the most promising route for flyby-based exoplanet exploration. However, there has been a notable lack of experimental characterization of key parameters essential for lightsail propulsion. Therefore, a model platform for optomechanical characterization of lightsail prototypes made from realistic materials is needed. We propose an approach for simultaneous measurement of optical forces and driving powers, which capitalizes on the multiphysics dynamics induced by the driving laser beam. By modelling the lightsail with a 50-nm thick silicon nitride membrane suspended by compliant micromechanical springs, we quantify force from off-resonantly driven displacement and power from heating-induced mechanical mode softening. This approach allows us to calibrate the measured forces to the driving powers by operating the device as a mechanical bolometer. We report radiation pressure forces of 80 fN using a collimated pump beam of 100 W/cm2 and noise-robust common-path interferometry. As lightsails will inevitably experience non-normal forces, we quantify the effects of incidence angle and spot size on the optical force and explain the nonintuitive trend by edge scattering. Our results provide a framework for comprehensive lightsail characterization and laboratory optomechanical manipulation of macroscopic objects by radiation pressure forces.

physics.optics↗

arXiv2021

Squeeze-film effect on atomically thin resonators in the high-pressure limit

The resonance frequency of membranes depends on the gas pressure due to the squeeze-film effect, induced by the compression of a thin gas film that is trapped underneath the resonator by the high frequency motion. This effect is particularly large in low-mass graphene membranes, which makes them promising candidates for pressure sensing applications. Here, we study the squeeze-film effect in single layer graphene resonators and find that their resonance frequency is lower than expected from models assuming ideal compression. To understand this deviation, we perform Boltzmann and continuum finite-element simulations, and propose an improved model that includes the effects of gas leakage and can account for the observed pressure dependence of the resonance frequency. Thus, this work provides further understanding of the squeeze-film effect and provides further directions into optimizing the design of squeeze-film pressure sensors from 2D materials.

cond-mat.mes-hall↗

arXiv2020

Inertial and viscous flywheel sensing of nanoparticles

Rotational dynamics often challenge physical intuition while enabling unique realizations, from the rotor of a gyroscope that maintains its orientation regardless of the outer gimbals, to a tennis racket that rotates around its handle when tossed face-up in the air. In the context of inertial mass sensing, which can measure mass with atomic precision, rotational dynamics are normally considered a complication hindering measurement interpretation. Here, we exploit the rotational dynamics of a microfluidic device to develop a new modality in inertial resonant sensing. Combining theory with experiments, we show that this modality normally measures the volume of the particle while being insensitive to its density. Paradoxically, particle density only emerges when fluid viscosity becomes dominant over inertia. We explain this paradox via a viscosity-driven, hydrodynamic coupling between the fluid and the particle that activates the rotational inertia of the particle, converting it into a viscous flywheel. This modality now enables the simultaneous measurement of particle volume and mass in fluid, using a single, high-throughput measurement.

physics.flu-dyn↗

arXiv2020

The measurement of Navier slip on individual nanoparticles in liquid

The Navier slip condition describes the motion of a liquid, relative to a neighboring solid surface, with its characteristic Navier slip length being a constitutive property of the solid-liquid interface. Measurement of this slip length is complicated by its small magnitude, expected in the nanometer range based on molecular simulations. Here, we report an experimental technique that interrogates the Navier slip length on individual nanoparticles immersed in liquid, with sub-nanometer precision. Proof-of-principle experiments on individual, citrate-stabilized, gold nanoparticles in water give a constant slip length of 2.7$\pm$0.6 nm (95% C.I.) - independent of particle size. Achieving this feature of size independence is central to any measurement of this constitutive property, which is facilitated through the use of individual particles of varying radii. This demonstration motivates studies that can now validate the wealth of existing molecular simulation data on slip.

cond-mat.soft↗

arXiv2020

Dynamics of an inverted cantilever plate at moderate angle of attack

The dynamics of a cantilever plate clamped at its trailing edge and placed at a moderate angle ($α\leq 30^{\circ}$) to a uniform flow are investigated experimentally and numerically, and a large experimental data set is provided. The dynamics are shown to differ significantly from the zero-angle-of-attack case, commonly called the inverted-flag configuration. Four distinct dynamical regimes arise at finite angles: a small oscillation around a small-deflection equilibrium (deformed regime), a small-amplitude flapping motion, a large-amplitude flapping motion and a small oscillation around a large-deflection equilibrium (deflected regime). The small-amplitude flapping motion appears gradually as the flow speed is increased and is consistent with a limit-cycle oscillation caused by the quasi-steady fluid forcing. The large-amplitude flapping motion is observed to appear at a constant critical flow speed that is independent of angle of attack. Its characteristics match those of the large-amplitude vortex-induced vibration present at zero angle of attack. The flow speed at which the plate enters the deflected regime decreases linearly as the angle of attack is increased, causing the flapping motion to disappear for angles of attack greater than $α\approx 28^{\circ}$. Finally, the effect of aspect ratio on the plate dynamics is considered, with reduced aspect ratio plates being shown to lack sharp distinctions between regimes.

physics.flu-dyn↗

arXiv2019

Strong Vibrational Coupling in Room Temperature Plasmonic Resonators

Strong vibrational coupling has been realized in a variety of mechanical systems from cavity optomechanics to electromechanics.$^{1, 2, 3, 4, 5}$ It is an essential requirement for enabling quantum control over the vibrational states.$^{6, 7, 8, 9, 10, 11}$ The majority of the mechanical systems that have been studied to date are vibrational resonances of dielectric or semiconductor nanomaterials coupled to optical modes.$^{12, 13, 14, 15}$ While there are fewer studies of coupling between two mechanical modes,$^{3, 9}$ particularly, there have been no experimental observation of strong coupling of the ultra-high frequency acoustic modes of plasmonic nanostructures, due to the rapid energy dissipation in these systems. Here we realized strong vibrational coupling in ultra-high frequency plasmonic nanoresonators by increasing the vibrational quality factors by an order of magnitude. This is achieved through blocking an energy dissipation pathway in the form of out-going acoustic waves. We achieved the highest frequency quality factor products of $\mathbf{f}\times\mathbf{Q}=1.0\times10^{13}$ Hz for the fundamental mechanical modes in room temperature plasmonic nanoresonators reported to date, which exceeds the value of $0.1\times10^{13}$ Hz required for ground state cooling. Avoided crossing were observed between the vibrational modes of two plasmonic nanoresonators with a coupling rate of $\mathbf{g}=7.5\pm 1.2$ GHz, an order of magnitude larger than the dissipation rates. The intermodal strong coupling was consistent with theoretical calculations using a coupled oscillator model. Our results expanded the strong coupling systems for mechanical resonators and enabled a platform for future observation and control of the quantum behavior of phonon modes in metallic nanoparticles.

physics.app-ph↗

arXiv2019

Mass measurement of graphene using quartz crystal microbalances

Current wafer-scale fabrication methods for graphene-based electronics and sensors involve the transfer of single-layer graphene by a support polymer. This often leaves some polymer residue on the graphene, which can strongly impact its electronic, thermal, and mechanical resonance properties. To assess the cleanliness of graphene fabrication methods, it is thus of considerable interest to quantify the amount of contamination on top of the graphene. Here, we present a methodology for direct measurement of the mass of the graphene sheet using quartz crystal microbalances (QCM). By monitoring the QCM resonance frequency during removal of graphene in an oxygen plasma, the total mass of the graphene and contamination is determined with sub-graphene-monolayer accuracy. Since the etch-rate of the contamination is higher than that of graphene, quantitative measurements of the mass of contaminants below, on top, and between graphene layers are obtained. We find that polymer-based dry transfer methods can increase the mass of a graphene sheet by a factor of 10. The presented mass measurement method is conceptually straightforward to interpret and can be used for standardized testing of graphene transfer procedures in order to improve the quality of graphene devices in future applications.

cond-mat.mes-hall↗

arXiv2018

Effect of morphology on the large-amplitude flapping dynamics of an inverted flag in a uniform flow

The stability of a cantilevered elastic sheet in a uniform flow has been studied extensively due to its importance in engineering and its prevalence in natural structures. Varying the flow speed can give rise to a range of dynamics including limit cycle behaviour and chaotic motion of the cantilevered sheet. Recently, the "inverted flag" configuration - a cantilevered elastic sheet aligned with the flow impinging on its free edge - has been observed to produce large-amplitude flapping over a finite band of flow speeds. This flapping phenomenon has been found to be a vortex-induced vibration, and only occurs at sufficiently large Reynolds numbers. In all cases studied, the inverted flag has been formed from a cantilevered sheet of rectangular morphology, i.e. the planform of its elastic sheet is a rectangle. Here, we investigate the effect of the inverted flag's morphology on its resulting stability and dynamics. We choose a trapezoidal planform which is explored using experiment and an analytical theory for the divergence instability of an inverted flag of arbitrary morphology. Strikingly, for this planform we observe that the flow speed range over which flapping occurs scales approximately with the flow speed at which the divergence instability occurs. This provides a means by which to predict and control flapping. In a biological setting, leaves in a wind can also align themselves in an inverted flag configuration. Motivated by this natural occurrence we also study the effect of adding an artificial "petiole" (a thin elastic stalk that connects the sheet to the clamp) on the inverted flag's dynamics. We find that the petiole serves to partially decouple fluid forces from elastic forces and increases the freedom by which the flapping dynamics can be tuned. These results highlight the intricacies of the flapping instability and account for some of the varied dynamics of leaves in nature.

physics.flu-dyn↗

arXiv2017

Plasmonic Hot-Carrier Extraction: Mechanisms of Electron Emission

When plasmonic nanoparticles are coupled with semiconductors, highly energetic hot carriers can be extracted from the metal-semiconductor interface for various applications in light energy conversion. Hot charge-carrier extraction upon plasmon decay using such an interface has been argued to occur after the formation of an intermediate electron population with a uniform momentum distribution. The efficiency of the charge separation process is thus discussed to be limited by this spatial homogeneity in certain plasmon-induced applications. Here we demonstrate using visible pump, near-infrared probe transient absorption spectroscopy that increases in the contact area between metal and semiconductor leads to an increase in the quantum yield for hot electron injection that is inconsistent with the homogeneous energy-momentum distribution of hot-electrons. Instead, further analysis of the experimental data suggests that the highly energetic electrons are emitted across the interface via a surface charge emission mechanism that occurs via a plasmon excitation

physics.chem-ph↗

arXiv2017

Interatomic force laws that corrupt their own measurement

Atomically-resolved imaging and force measurements using the atomic force microscope (AFM) are performed most commonly in a frequency-modulation (FM) mode. This has led to spectacular results, including direct observation of the atomic structure of complex molecules and quantification of chemical and frictional forces at the atomic scale. We address here a critical question: Is recovery of force from the measured frequency shift experienced by the AFM cantilever ill-posed - that is, unreliable in the presence of (unavoidable) measurement uncertainty? Resolution of this issue underlies all force measurements using FM-AFM, but remains outstanding. It is shown that concavity of the force law's distance dependence controls ill-posed behavior, with a rapid concavity change corrupting force measurements by inducing spurious and unphysical effects - such rapid change is not uncommon. Practical conditions to eliminate ill-posed behavior are formulated which are verified experimentally. This study lays the foundations for robust atomically-resolved force spectroscopy and future work that will seek to regularize ill-posed force measurements.

cond-mat.mes-hall↗

arXiv2016

A virtual instrument to standardise the calibration of atomic force microscope cantilevers

Atomic force microscope (AFM) users often calibrate the spring constants of cantilevers using functionality built into individual instruments. This is performed without reference to a global standard, which hinders robust comparison of force measurements reported by different laboratories. In this article, we describe a virtual instrument (an internet-based initiative) whereby users from all laboratories can instantly and quantitatively compare their calibration measurements to those of others - standardising AFM force measurements - and simultaneously enabling non-invasive calibration of AFM cantilevers of any geometry. This global calibration initiative requires no additional instrumentation or data processing on the part of the user. It utilises a single website where users upload currently available data. A proof-of-principle demonstration of this initiative is presented using measured data from five independent laboratories across three countries, which also allows for an assessment of current calibration.

physics.ins-det↗

arXiv2015

Photo-induced electron transfer in the strong coupling regime: Waveguide-plasmon polaritons

Reversible exchange of photons between a material and an optical cavity can lead to the formation of hybrid light--matter states where material properties such as the work function\cite{Hutchison_AM2013a}, chemical reactivity\cite{Hutchison_ACIE2012a}, ultra--fast energy relaxation \cite{Salomon_ACIE2009a,Gomez_TJOPCB2012a} and electrical conductivity\cite{Orgiu_NM2015a} of matter differ significantly to those of the same material in the absence of strong interactions with the electromagnetic fields. Here we show that strong light--matter coupling between confined photons on a semiconductor waveguide and localised plasmon resonances on metal nanowires modifies the efficiency of the photo--induced charge--transfer rate of plasmonic derived (hot) electrons into accepting states in the semiconductor material. Ultra--fast spectroscopy measurements reveal a strong correlation between the amplitude of the transient signals, attributed to electrons residing in the semiconductor, and the hybridization of waveguide and plasmon excitations.

physics.optics↗

arXiv2012

Stress-Induced Variations in the Stiffness of Micro- and Nanocantilever Beams

The effect of surface stress on the stiffness of cantilever beams remains an outstanding problem in the physical sciences. While numerous experimental studies report significant stiffness change due to surface stress, theoretical predictions are unable to rigorously and quantitatively reconcile these observations. In this Letter, we present the first controlled measurements of stress-induced change in cantilever stiffness with commensurate theoretical quantification. Simultaneous measurements are also performed on equivalent clamped-clamped beams. All experimental results are quantitatively and accurately predicted using elasticity theory. We also present conclusive experimental evidence for invalidity of the longstanding and unphysical axial force model, which has been widely applied to interpret measurements using cantilever beams. Our findings will be of value in the development of micro- and nanoscale resonant mechanical sensors.

cond-mat.mes-hall↗