arXiv subjects

John H. Gaida

Publications and source records attributed to John H. Gaida.

5 recordsLinked to original sources

arXiv2025

Roadmap for Quantum Nanophotonics with Free Electrons

Over the past century, continuous advancements in electron microscopy have enabled the synthesis, control, and characterization of high-quality free-electron beams. These probes carry an evanescent electromagnetic field that can drive localized excitations and provide high-resolution information on material structures and their optical responses, currently reaching the sub-ångström and few-meV regime. Moreover, combining free electrons with pulsed light sources in ultrafast electron microscopy adds temporal resolution in the sub-femtosecond range while offering enhanced control of the electron wave function. Beyond their exceptional capabilities for time-resolved spectromicroscopy, free electrons are emerging as powerful tools in quantum nanophotonics, on par with photons in their ability to carry and transfer quantum information, create entanglement within and with a specimen, and reveal previously inaccessible details on nanoscale quantum phenomena. This Roadmap outlines the current state of this rapidly evolving field, highlights key challenges and opportunities, and discusses future directions through a collection of topical sections prepared by leading experts.

cond-mat.mes-hall↗

arXiv2023

Attosecond electron microscopy by free-electron homodyne detection

Time-resolved electron microscopy aims at tracking nanoscale excitations and dynamic states of matter with a temporal resolution ultimately reaching the attosecond regime. Periodically time-varying fields in an illuminated specimen cause free-electron inelastic scattering, which enables the spectroscopic imaging of near-field intensities. However, access to the evolution of nanoscale fields and structures within the light cycle requires a sensitivity to the optical phase. Here, we introduce Free-Electron Homodyne Detection (FREHD) as a universally applicable approach to electron microscopy of phase-resolved optical responses at high spatiotemporal resolution. In this scheme, a phase-controlled reference interaction serves as the local oscillator to extract arbitrary sample-induced modulations of a free-electron wave function. We demonstrate this principle through the phase-resolved imaging of plasmonic fields with few-nanometer spatial and sub-cycle temporal resolutions. Due to its sensitivity to both phase- and amplitude-modulated electron beams, FREHD measurements will be able to detect and amplify weak signals stemming from a wide variety of microscopic origins, including linear and nonlinear optical polarizations, atomic and molecular resonances and attosecond-modulated structure factors.

physics.optics↗

arXiv2023

Coulomb-correlated electron number states in a transmission electron microscope beam

We demonstrate the generation of Coulomb-correlated pair, triple and quadruple states of free electrons by femtosecond photoemission from a nanoscale field emitter inside a transmission electron microscope. Event-based electron spectroscopy allows a spatial and spectral characterization of the electron ensemble emitted by each laser pulse. We identify distinctive energy and momentum correlations arising from acceleration-enhanced interparticle energy exchange, revealing strong few-body Coulomb interactions at an energy scale of about two electronvolts. State-sorted beam caustics show a discrete increase in virtual source size and longitudinal source shift for few-electron states, associated with transverse momentum correlations. We observe field-controllable electron antibunching, attributed primarily to transverse Coulomb deflection. The pronounced spatial and spectral characteristics of these electron number states allow filtering schemes that control the statistical distribution of the pulse charge. In this way, the fraction of specific few-electron states can be actively suppressed or enhanced, facilitating the preparation of highly non-Poissonian electron beams for microscopy and lithography, including future heralding schemes and correlated multi-electron probing.

cond-mat.mes-hall↗

arXiv2021

Pinning and gyration dynamics of magnetic vortices revealed by correlative Lorentz and bright-field imaging

Topological magnetic textures are of great interest in various scientific and technological fields. To allow for precise control of nanoscale magnetism, it is of great importance to understand the role of intrinsic defects in the host material. Here, we use conventional and time-resolved Lorentz microscopy to study the effect of grain size in polycrystalline permalloy films on the pinning and gyration orbits of vortex cores inside magnetic nanoislands. To assess static pinning, we use in-plane magnetic fields to shift the core across the island while recording its position. This enables us to produce highly accurate two-dimensional maps of pinning sites. Based on this technique, we can generate a quantitative map of the pinning potential for the core, which we identify as being governed by grain boundaries. Furthermore, we investigate the effects of pinning on the dynamic behavior of the vortex core using stroboscopic Lorentz microscopy, harnessing a new photoemission source that accelerates image acquisition by about two orders of magnitude. We find characteristic changes to the vortex gyration in the form of increased dissipation and enhanced bistability in samples with larger grains.

cond-mat.mes-hall↗

arXiv2017

Polarized photoluminescence clocks ultrafast pseudospin relaxation in graphene

Electronic states in 2D materials can exhibit pseudospin degrees of freedom, which allow for unique carrier-field interaction scenarios. Here, we investigate ultrafast sublattice pseudospin relaxation in graphene by means of polarization-resolved photoluminescence spectroscopy. Comparison with microscopic Boltzmann simulations allows to determine a lifetime of the optically aligned pseudospin distribution of $12\pm 2\,\text{fs}$. This experimental approach extends the toolbox of graphene pseudospintronics, providing novel means to investigate pseudospin dynamics in active devices or under external fields.

cond-mat.mes-hall↗