arXiv subjects

John M. Doyle

Publications and source records attributed to John M. Doyle.

94 records · Page 6Linked to original sources

arXiv2008

Magnetic trapping of atomic nitrogen (14^N) and cotrapping of NH (X-triplet-Sigma-)

We observe magnetic trapping of atomic nitrogen (14^N) and cotrapping of ground state imidogen (14^NH, X-triplet-Sigma-). Both are loaded directly from a room temperature beam via buffer gas cooling. We trap approximately 1 * 10^11 14^N atoms at a peak density of 5 * 10^11 cm^-3 at 550 mK. The 12 +5/-3 s 1/e lifetime of atomic nitrogen in the trap is limited by elastic collisions with the helium buffer gas. Cotrapping of 14^N and 14^NH is accomplished, with 10^8 NH trapped molecules at a peak density of 10^8 cm^-3. We observe no spin relaxation of nitrogen in collisions with helium.

physics.atom-ph↗

arXiv2008

Time-Domain Measurement of Spontaneous Vibrational Decay of Magnetically Trapped NH

The v = 1 -> 0 radiative lifetime of NH (X triplet-Sigma-, v=1,N=0) is determined to be tau_rad,exp. = 37.0 +/- 0.5 stat +2.0 / -0.8 sys miliseconds, corresponding to a transition dipole moment of |mu_10| = 0.0540 + 0.0009 / -0.0018 Debye. To achieve the long observation times necessary for direct time-domain measurement, vibrationally excited NH (X triplet-Sigma-, v=1,N=0) radicals are magnetically trapped using helium buffer-gas loading. Simultaneous trapping and lifetime measurement of both the NH(v=1, N=0) and NH(v=0,N=0) populations allows for accurate extraction of tau_rad,exp. Background helium atoms are present during our measurement of tau_rad,exp., and the rate constant for helium atom induced collisional quenching of NH(v=1,N=0) was determined to be k_q < 3.9 * 10^-15 cm^3/s. This bound on k_q yields the quoted systematic uncertainty on tau_rad,exp. Using an ab initio dipole moment function and an RKR potential, we also determine a theoretical value of 36.99 ms for this lifetime, in agreement with our experimental value. Our results provide an independent determination of tau_rad,10, test molecular theory, and furthermore demonstrate the efficacy of buffer-gas loading and trapping in determining metastable radiative and collisional lifetimes.

physics.atom-ph↗

arXiv2007

A Bright, Guided Molecular Beam With Hydrodynamic Enhancement

We realize a novel high flux source of cold atoms and molecules employing hydrodynamic enhancement of an effusive aperture at cryogenic temperatures. Molecular oxygen from the source is coupled to a magnetic guide, delivering a cold, continuous, guided flux of 3e12 oxygen molecules per second, with a molecule temperature of a few kelvin. The dynamics of the source are studied by creating and spectroscopically analyzing high-flux beams of atomic ytterbium.

physics.chem-ph↗

arXiv2007

Magnetic trapping and Zeeman relaxation of imidogen (NH X-triplet-Sigma)

Imidogen (NH) radicals are magnetically trapped and their Zeeman relaxation and energy transport collision cross sections with helium are measured. Continuous buffer-gas loading of the trap is direct from a room-temperature molecular beam. The Zeeman relaxation (inelastic) cross section of magnetically trapped electronic, vibrational and rotational ground state imidogen in collisions with He-3 is measured to be 3.8 +/- 1.1 E-19 cm^2 at 710 mK. The NH-He energy transport cross section is also measured, indicating a ratio of diffusive to inelastic cross sections of gamma = 7 E4 in agreement with the recent theory of Krems et al. (PRA 68 051401(R) (2003))

physics.atom-ph↗