arXiv subjects

John W. Rosenberg

Publications and source records attributed to John W. Rosenberg.

3 recordsLinked to original sources

arXiv2026

Sensing single molecule magnets with nitrogen vacancy centers

Single-molecule magnets (SMMs) are molecules that can function as nanoscale magnets with potential use as magnetic memory bits. While SMMs can retain magnetization at low temperatures, characterizing them on surface and at room temperature remains challenging and requires specialized nanoscale techniques. Here, we use single nitrogen-vacancy (NV) centers in diamond as highly sensitive, broadband magnetic field sensors to detect the magnetic noise of cobalt-based SMMs deposited on a diamond surface. We measure the NV relaxation and decoherence times at 296 K and at 5-8 K, observing a significant influence of the SMMs on them. From this, we can infer the SMMs' magnetic noise spectral density (NSD) and underlying magnetic properties. Moreover, we observe the effect of an applied magnetic field on the SMMs' NSD at low temperatures. The method provides nanoscale sensitivity for characterizing SMMs under realistic conditions relevant to their use as surface-bound memory units.

quant-ph↗

arXiv2025

Witnessing non-stationary and non-Markovian environments with a quantum sensor

Quantum sensors offer exceptional sensitivity to nanoscale magnetic fluctuations, where non-stationary effects -- such as spin diffusion -- and non-Markovian dynamics arising from coupling to few environmental degrees of freedom play critical roles. Because fully reconstructing the microscopic structure of realistic spin baths is often infeasible, a practical challenge is to identify the dynamical features that are actually encoded in the sensor's decoherence signal. Here, we demonstrate how quantum sensors can operationally characterize the statistical nature of environmental noise, distinguishing between stationary and non-stationary behaviors, as well as Markovian and non-Markovian dynamics. Using nitrogen-vacancy (NV) centers in diamond as a platform, we develop a physical noise model that captures the essential dynamical features of realistic environments relevant to sensor observables -- independently of the microscopic bath details -- and provides analytical predictions for Ramsey decay across different regimes. These predictions are experimentally validated through controlled noise injection with tunable correlation properties. Our results showcase the capability of quantum sensors to isolate and identify key dynamical properties of complex environments, without requiring full microscopic bath reconstruction. This work clarifies the operational signatures of non-stationarity and non-Markovian behavior at the nanoscale and lays the foundation for strategies that mitigates decoherence while exploiting environmental dynamics for enhanced quantum sensing.

quant-ph↗

arXiv2019

Phase protection of Fano-Feshbach resonances

Decay of bound states due to coupling with free particle states is a general phenomenon occurring at energy scales from MeV in nuclear physics to peV in ultracold atomic gases. Such a coupling gives rise to Fano-Feshbach resonances (FFR) that have become key to understanding and controlling interactions - in ultracold atomic gases, but also between quasiparticles such as microcavity polaritons. The energy positions of FFR were shown to follow quantum chaotic statistics. In contrast, lifetimes which are the fundamental property of a decaying state, have so far escaped a similarly comprehensive understanding. Here we show that a bound state, despite being resonantly coupled to a scattering state, becomes protected from decay whenever the relative phase is a multiple of $π$. We observe this phenomenon by measuring lifetimes spanning four orders of magnitude for FFR of spin-orbit excited molecular ions with merged beam and electrostatic trap experiments. Our results provide a blueprint for identifying naturally long-lived states in a decaying quantum system.

physics.atom-ph↗