arXiv subjects

John Wilkinson

Publications and source records attributed to John Wilkinson.

8 recordsLinked to original sources

arXiv2026

Future perspective of muons; a quantum particle measuring quantum processes

Although considered a niche technique, muon spectroscopy provides a unique and complementary insight into a range of different materials from hard condensed matter to biological samples and everything in between. In matter, the muon has a mass of $\frac{1}{9}~m_p$ or $207~m_e$, and is a local probe of quantum states that can provide a focus on the bulk properties of materials. While often interpreted in a classical framework, the muon is itself a quantum particle and it is increasingly common for researchers to take account of this when thinking about muon spectroscopy experiments. In this perspective, we focus on the power of using this quantum treatment of muon spectroscopy, which is a key future direction for the technique.

cond-mat.other↗

arXiv2026

Multistage development of short-range spin correlations and weak magnetic order in the two coupled trillium lattices of K2Fe2(MoO4)(PO4)2

Trillium lattices, where magnetic ions form a chiral network of corner-sharing triangles, offer a three-dimensional magnetic framework that can host fragile classical spin-liquid states. Herein, we report on the magnetization, specific heat, electron spin resonance (ESR), and muon spin relaxation ($\mu$SR) of K$_{2}$Fe$_{2}$(MoO$_{4}$)(PO$_{4}$)$_{2}$ single crystals. Magnetization measurements reveal strong antiferromagnetic interactions coexisting with weak magnetic order at $T_{\rm N} = 5.2$~K, as evidenced by a $\lambda$-like anomaly observed in the magnetic susceptibility, a critical enhancement of the muon spin relaxation rate and the wipeout of the ESR signal as the temperature approaches $T_{\rm N}$. Above $T_{\rm N}$, two distinct developments of short-range spin correlations are identified at $T_{\rm H} = 34$~K and $T_{\rm L} = 10$~K, supported by magnetic specific heat anomalies and the temperature dependence of the ESR linewidth and $g$-factor. Upon cooling below $T_{\rm N}$, an anomaly appears at $T^{*} = 3.2$~K in thermodynamic observables and the muon spin relaxation rate, indicative of spin reorientation driven by residual interactions. Despite the presence of magnetic order, $\mu$SR experiments reveal dynamically fluctuating spins persisting even in the ordered state. Moreover, the suppression of $T_{\rm N}$ under applied magnetic fields ($\mu_{0}H \geq 2$~T) suggests that K$_{2}$Fe$_{2}$(MoO$_{4}$)(PO$_{4}$)$_{2}$ constitutes a promising candidate for exploring field-induced spin-liquid behavior in three-dimensionally coupled trillium lattices.

cond-mat.str-el↗

arXiv2026

Measuring AI Agents' Progress on Multi-Step Cyber Attack Scenarios

We evaluate the autonomous cyber-attack capabilities of frontier AI models on two purpose-built cyber ranges-a 32-step corporate network attack and a 7-step industrial control system attack-that require chaining heterogeneous capabilities across extended action sequences. By comparing seven models released over an eighteen-month period (August 2024 to February 2026) at varying inference-time compute budgets, we observe two capability trends. First, model performance scales log-linearly with inference-time compute, with no observed plateau-increasing from 10M to 100M tokens yields gains of up to 59%, requiring no specific technical sophistication from the operator. Second, each successive model generation outperforms its predecessor at fixed token budgets: on the corporate network range, average steps completed at 10M tokens rose from 1.7 (GPT-4o, August 2024) to 9.8 (Opus 4.6, February 2026). The best single run completed 22 of 32 steps, corresponding to roughly 6 of the estimated 14 hours a human expert would need. On the industrial control system range, performance remains limited, though the most recent models are the first to reliably complete steps, averaging 1.2-1.4 of 7 (max 3).

cs.AI↗

arXiv2026

Quantifying Frontier LLM Capabilities for Container Sandbox Escape

Large language models (LLMs) increasingly act as autonomous agents, using tools to execute code, read and write files, and access networks, creating novel security risks. To mitigate these risks, agents are commonly deployed and evaluated in isolated "sandbox" environments, often implemented using Docker/OCI containers. We introduce SANDBOXESCAPEBENCH, an open benchmark that safely measures an LLM's capacity to break out of these sandboxes. The benchmark is implemented as an Inspect AI Capture the Flag (CTF) evaluation utilising a nested sandbox architecture with the outer layer containing the flag and no known vulnerabilities. Following a threat model of a motivated adversarial agent with shell access inside a container, SANDBOXESCAPEBENCH covers a spectrum of sandboxescape mechanisms spanning misconfiguration, privilege allocation mistakes, kernel flaws, and runtime/orchestration weaknesses. We find that, when vulnerabilities are added, LLMs are able to identify and exploit them, showing that use of evaluation like SANDBOXESCAPEBENCH is needed to ensure sandboxing continues to provide the encapsulation needed for highly-capable models.

cs.CR↗

arXiv2025

Novel Quantum Spin Liquid States in the $S = {\frac{1}{2}}$ Three-Dimensional Compound Y$_{3}$Cu$_{2}$Sb$_{3}$O$_{14}$

The three-dimensional $S = {\frac{1}{2}}$ system Y$_{3}$Cu$_{2}$Sb$_{3}$O$_{14}$ consists of two inequivalent Cu$^{2+}$ sites, each forming an edge shared triangular lattice. Our magnetic susceptibility $\chi(T)$, specific heat $C_p(T)$, $^{89}$Y nuclear magnetic resonance (NMR), muon spin relaxation ($\upmu\mathrm{SR}$), and electron spin resonance (ESR) measurements on this system confirm the absence of any long-range magnetic ordering and the persistence of spin dynamics down to 0.077 K. In $^{89}$Y NMR we find an anomaly at about 120 K which we suggest arises from a fraction of the spins condensing into a singlet (a valence bond solid VBS) state. A plateau in the muon relaxation rate is observed between 60 K and 10 K (signifying the VBS state from a fraction of the spins) followed by an increase and another plateau below about 1 K (presumably signifying the quantum spin liquid state from all the spins). Our density functional theory calculations find a dominant antiferromagnetic interaction along the body diagonal with inequivalent Cu(1) and Cu(2) ions alternately occupying the corners of the cube. All other near-neighbour interactions between the Cu ions are also found to be antiferromagnetic and are thought to drive the frustration.

cond-mat.str-el↗

arXiv2025

Effects of Ru-doping on the magnetism of Ag3LiIr2O6, a candidate Kitaev quantum spin liquid

We report our investigations on Ag3LiIr1.4Ru0.6O6, which results from the Ru substitution in the Kitaev quantum spin liquid candidate Ag3LiIr2O6. It crystallizes in the monoclinic C2/m space group like its parent compound, Ag3LiIr2O6. Our susceptibility measurements reveal an effective moment = 2.6 muB, which is higher than the moments of the parent compound and less than that of the Ru-analog (Ag3LiRu2O6), suggesting the presence of magnetic Ir4+ (Jeff= 1/2) and Ru4+ (S=1). Bulk magnetic susceptibility suggests long-range order (LRO)at T~20 K, whereas no clear signature is present in the heat capacity. Likewise, there is a loss of the 7Li NMR spectral intensity around T~20 K as expected at the onset of LRO, but a complete wipe-out is not seen in contrast to the result in Ag3LiIr2O6. There is also a T~20 K anomaly in the 7Li NMR relaxation rate and also a fall in the 7Li NMR shift with decreasing temperature. These results suggest LRO at T~20 K in Ag3LiIr1.4Ru0.6O6. However, at low-T below 10 K, we observe a power law variation in magnetic heat capacity and spin lattice relaxation rate, temperature-independent-7K, and no further loss of the 7Li NMR spectral intensity. These results might suggest the persistence or stabilisation of a quantum spin liquid-like phase, perhaps from a fraction of the sample in Ag3LiIr1.4Ru0.6O6 below 10 K. Our muon spin relaxation measurements suggest ordering around 20 K, consistent with our other probes. It appears that the main effect of Ru-substitution is to shift the LRO to a higher temperature in comparison with Ag3LiIr2O6, though there are signatures of a novel phase below about 10 K.

cond-mat.str-el↗

arXiv2024

(H,Li)$_{6}$Ru$_{2}$O$_{6}$ : a possible zero-field Ru$^{3+}$-based Kitaev Quantum Spin Liquid

We report the synthesis and properties of (H,Li)$_{6}$Ru$_{2}$O$_{6}$, which is shown to be a $J_{\text{eff}}=\frac{1}{2}$ system made out of Ru$^{3+}$ moments in a honeycomb geometry. Bulk magnetization, heat capacity, nuclear magnetic resonance (NMR), and muon spin relaxation ($\mu$SR) rule out the presence of static moments or any spin glass phase down to 84 mK. All techniques suggest a crossover to a liquid-like state below about 40 K. The $^{7}$Li nuclear magnetic resonance (NMR) shift data suggest a non-zero $T$-independent spin susceptibility at low $T$. In zero field, $C_m/T$ shows $T^{-0.9}$ divergence which is consistent with vacancy-induced effects on low-energy excitations of the pristine Kitaev spin liquid. With field, power-law variations in the $^{7}$Li NMR spin-lattice relaxation rate 1/T$_{1}$ and magnetic heat capacity $C_{m}$ show quantitatively new scaling behaviors. A two-step entropy release in heat capacity is also observed putatively from $Z_{2}$ flux (low-$T$ step) and itinerant Majorana fermions (high-$T$ step). Based on these findings, we propose that (H,Li)$_{6}$Ru$_{2}$O$_{6}$ realizes a Kitaev spin liquid with no evidence of inherent magnetic ordering in zero field unlike $\alpha$-RuCl$_{3}$ where approximately $8$ Tesla field is required to suppress magnetic order.

cond-mat.str-el↗

arXiv2018

Isotope Harvesting at FRIB: Additional opportunities for scientific discovery

The Facility for Rare Isotope Beams (FRIB) at Michigan State University provides a unique opportunity to access some of the nation's most specialized scientific resources: radioisotopes. An excess of useful radioisotopes will be formed as FRIB fulfills its basic science mission of providing rare isotope beams. In order for the FRIB beams to reach high-purity, many of the isotopes are discarded and go unused. If harvested, the unused isotopes could enable cutting-edge research for diverse applications ranging from medical therapy and diagnosis to nuclear security. Given that FRIB will have the capability to create about 80 percent of all possible atomic nuclei, harvesting at FRIB will provide a fast path for access to a vast array of isotopes of interest in basic and applied science investigations. To fully realize this opportunity, infrastructure investment is required to enable harvesting and purification of otherwise unused isotopes. An investment in isotope harvesting at FRIB will provide the nation with a powerful resource for development of crucial isotope applications.

physics.ins-det↗