arXiv subjects

Jonah S. Peter

Publications and source records attributed to Jonah S. Peter.

7 recordsLinked to original sources

arXiv2026

Chiral superfluorescence from perovskite superlattices at room temperature

Superfluorescence (SF) is the collective emission of intense, coherent light from an interacting ensemble of quantum emitters1-4. While SF has been observed in several solid-state materials5-8, the spontaneous generation of circularly polarized SF from chiral materials (chiral SF) has not been realized9,10. Here, we report the first observation of chiral SF originating from edge states in large-area (>100 um * 100 um) vertically aligned chiral perovskite superlattices at room-temperature. Theoretical quantum optics calculations describe the transition from initially unpolarized, incoherent spontaneous emission to a coherent chiral SF state, quantitatively reproducing both the experimentally observed generation of circular polarization (up to ~14%) and its reversal in sign with opposite material handedness. Moreover, we show that both the intensity and the degree of circular polarization of chiral SF can be modulated by a weak magnetic field, enabling precise control over solid-state quantum light emission at room temperature. Our findings demonstrate an interplay between chirality and many-body quantum coherence, thereby revealing promising new directions for chirality-controlled quantum-optical applications.

physics.optics↗

arXiv2026

Light-induced Self-Organization in Cooperative Free Space Atomic Arrays

We investigate how laser-driven, cooperative dipole-dipole interactions in weakly trapped atomic arrays give rise to self-organized configurations. Starting from an analytically tractable two-emitter system, we identify the possible steady-state spatial arrangements accessible to the atoms. We then extend this analysis to larger ensembles in both linear and ring geometries. In linear chains, we demonstrate the emergence of topologically nontrivial dimerized configurations across a range of initial interatomic spacings. In ring geometries, we find that the system undergoes self-organized contraction and expansion, enabling access to length scales below those set by the trapping lattice. Our results demonstrate that collective light-matter interactions in free space can spontaneously generate modified ordered geometries, even when the emitters are initially separated by distances larger than their transition wavelength.

quant-ph↗

arXiv2024

Chirality-induced emergent spin-orbit coupling in topological atomic lattices

Spin-orbit coupling is of fundamental interest in both quantum optical and condensed matter systems alike. In this work, we show that optically induced electronic excitations in lattices of V-type atoms exhibit an emergent spin-orbit coupling when the geometry is chiral. This spin-orbit coupling arises naturally from the electric dipole interaction between the atomic sites and leads to a nontrivial topology for the lattice band structure. Using a general quantum optical model, we determine analytically the conditions that give rise to spin-orbit coupling and characterize the behavior under various symmetry transformations. We demonstrate that chirality-induced spin-orbit coupling can result from either the chirality of the underlying lattice geometry or the combination of an achiral lattice with a suitably chosen external quantization axis. We then discuss how these results are influenced by dissipation, which breaks time-reversal symmetry and illuminates the distinction between true and false chirality. Our results demonstrate that chiral atom arrays are a robust platform for realizing spin-orbit-coupled topological states of matter.

quant-ph↗

arXiv2024

Examining the quantum signatures of optimal excitation energy transfer

Light-harvesting via the transport and trapping of optically-induced electronic excitations is of fundamental interest to the design of new energy efficient quantum technologies. Using a paradigmatic quantum optical model, we study the influence of coherence, entanglement, and cooperative dissipation on the transport and capture of excitation energy. In particular, we demonstrate that the rate of energy extraction is optimized under conditions that minimize the quantum coherence and entanglement of the system. We show that this finding is not limited to disordered or high temperature systems but is instead a fundamental consequence of spontaneous parity time-reversal symmetry breaking associated with the quantum-to-classical transition. We then examine the effects of vibrational fluctuations, revealing a strong dephasing assisted transport enhancement for delocalized excitations in the presence of cooperative interactions. Our results highlight the rich, emergent behavior associated with decoherence and may be relevant to the study of biological photosynthetic antenna complexes or to the design of room-temperature quantum devices.

quant-ph↗

arXiv2023

Chirality Dependent Photon Transport and Helical Superradiance

Chirality, or handedness, is a geometrical property denoting a lack of mirror symmetry. Chirality is ubiquitous in nature and is associated with the non-reciprocal interactions observed in complex systems ranging from biomolecules to topological materials. Here, we demonstrate that chiral arrangements of dipole-coupled atoms or molecules can facilitate the unidirectional transport of helical photonic excitations without breaking time-reversal symmetry. We show that such helicity dependent transport stems from an emergent spin-orbit coupling induced by the chiral geometry, which results in nontrivial topological properties. We also examine the effects of collective dissipation and find that many-body coherences lead to helicity dependent photon emission: an effect we call helical superradiance. Our results demonstrate an intimate connection between chirality, topology, and photon helicity that may contribute to molecular photodynamics in nature and could be probed with near-term quantum simulators.

quant-ph↗

arXiv2023

Detection of HCN and diverse redox chemistry in the plume of Enceladus

The Cassini spacecraft observed that Saturn's moon Enceladus possesses a series of jets erupting from its South Polar Terrain. Previous studies of in situ data collected by Cassini's Ion and Neutral Mass Spectrometer (INMS) have identified H$_2$O, CO$_2$, CH$_4$, NH$_3$, and H$_2$ within the plume of ejected material. Identification of minor species in the plume remains an ongoing challenge, owing to the large number of possible combinations that can be used to fit the INMS data. Here, we present the detection of several new compounds of strong importance to the habitability of Enceladus, including HCN, C$_2$H$_2$, C$_3$H$_6$, and C$_2$H$_6$. Our analyses of the low velocity INMS data, coupled with our detailed statistical framework, enable discrimination between previously ambiguous species in the plume by alleviating the effects of high dimensional model fitting. Together with plausible mineralogical catalysts and redox gradients derived from surface radiolysis, these compounds could potentially support extant microbial communities or drive complex organic synthesis leading to the origin of life.

astro-ph.EP↗

arXiv2022

Nano-scale simulation of neuronal damage by galactic cosmic rays

The effects of complex, mixed-ion radiation fields on neuronal function remain largely unexplored. Here, we present a complete analysis of the nano-scale physics associated with broad-spectrum galactic cosmic ray (GCR) irradiation in a realistic cornu ammonis 1 (CA1) pyramidal neuron geometry. We simulate the entire 33 ion-energy beam fluence distribution currently in use at the NASA Space Radiation Laboratory galactic cosmic ray simulator (GCRSim). We use the TOol for PArticle Simulation (TOPAS) and TOPAS-nBio Monte Carlo-based track structure simulation toolkits to assess the dosimetry, physics processes, and fluence statistics of different neuronal compartments at the nanometer scale. We also make comparisons between the full GCRSim distribution and a simplified 6 ion-energy spectrum (SimGCRSim). We show that across all physics processes, ionizations mediate the majority of the energy deposition $(68 \pm 1\%)$, though vibrational excitations are the most abundant ($70 \pm 2\%$ of all energy deposition events). We report that neuronal energy deposition by proton and $α$-particle tracks declines approximately hyperbolically with increasing primary particle energy at mission-relevant energies. We also demonstrate an inverted exponential relationship between dendritic segment irradiation probability and neuronal absorbed dose. Finally, we find that there are no significant differences in the average physical responses between the GCRSim and SimGCRSim fluence distributions. To our knowledge, this is the first nano-scale simulation study of a realistic neuron geometry using the GCRSim and SimGCRSim fluence distributions. The results presented here are expected to aid in the interpretation of future experimental results and help guide future study designs.

physics.med-ph↗