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Jonas Arnold

Publications and source records attributed to Jonas Arnold.

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Bad Metal Behavior and Lifshitz Transition of a Nagaoka Ferromagnet

Using an extension of the fermionic functional renormalization group for systems where strong correlations give rise to projected Hilbert spaces we calculate the phase diagram and the electronic spectral function of the Hubbard model at infinite on-site repulsion. For a square lattice with nearest-neighbor hopping we find that the ground state evolves from a paramagnetic Fermi liquid at low densities via a state with antiferromagnetic stripe order at intermediate densities to an extended Nagaoka ferromagnet at high densities. The single-particle spectral function of the Nagaoka ferromagnet exhibits a flat but rather broad band characteristic for an incoherent non-Fermi liquid. We identify two distinct ferromagnetic regimes separated by a Lifshitz transition.

cond-mat.str-el

Functional renormalization group for extremely correlated electrons

At strong on-site repulsion $ U $, the fermionic Hubbard model realizes an extremely correlated electron system. In this regime, it is natural to derive the low-energy physics with the help of non-canonical operators acting on a projected Hilbert space without double occupancies. Using a strong-coupling functional renormalization group technique, we study the physics of such extreme correlations in the strict $ U = \infty $ limit, where only kinematic interactions due to the Hilbert space projection remain. For nearest-neighbor hopping on a square lattice, we find that the electronic spectrum is significantly renormalized, with bandwidth and quasi-particle residue strongly decreasing with increasing electron density. On the other hand, damping and particle-hole asymmetry increase, while a polaronic continuum forms in the hole sector, below the single-particle band. Fermi liquid phenomenology applies only at low densities, where the system remains paramagnetic. At higher densities, we find a bad metal with strong magnetic correlations, indicating that the ground state is the Nagaoka ferromagnet at high densities and a stripe antiferromagnet at intermediate densities. Both in the paramagnetic and the ferromagnetic regimes, we observe a violation of Luttinger's theorem.

cond-mat.str-el

Atomic-Scale Quantum Control of Single Spin Defects in a Two-Dimensional Semiconductor

Individual spin defects in solids are promising building blocks for quantum technologies, but their deterministic creation, individual addressability, and operation near surfaces remain major challenges. Two-dimensional materials provide an attractive alternative, as their single-layer thickness enables direct atomic-scale access to defect states. Here, we demonstrate single-spin control of solid-state defects in a two-dimensional semiconductor by a combination of scanning tunneling microscopy and electron spin resonance. We create and manipulate individual sulfur vacancies and carbon substitution defects in monolayer molybdenum disulfide and characterize their spin dynamics, including coherent control, at the single-defect level. Using atomic manipulation, we further engineer and probe spin-spin interactions between defect pairs. Our results demonstrate deterministic creation, addressability, coherent manipulation, and controlled coupling of individual spin defects within a single experimental platform. This establishes atomically engineered spin defects in two-dimensional semiconductors as a versatile class of controllable solid-state quantum systems and opens a route towards tailored quantum sensing experiments.

cond-mat.mes-hall

Functional renormalization group without functional integrals: implementing Hilbert space projections for strongly correlated electrons via Hubbard X-operators

Exact functional renormalization group (FRG) flow equations for quantum systems can be derived directly within an operator formalism without using functional integrals. This simple insight opens new possibilities for applying FRG methods to models for strongly correlated electrons with projected Hilbert spaces, such as quantum spin models, the $t$-$J$ model, or the Hubbard model at infinite on-site repulsion. By representing these models in terms of Hubbard X-operators, we derive exact flow equations for the time-ordered correlation functions of the X-operators (X-FRG), which allow us to calculate the electronic correlation functions in the projected Hilbert space of these models. The Hubbard-I approximation for the single-particle Green function of the Hubbard model is recovered from a trivial truncation of the flow equations where the two-point vertex is approximated by its atomic limit. We use our approach to calculate the quasi-particle residue and damping in the ``hidden Fermi liquid'' state of the Hubbard model at infinite on-site repulsion where the Hamiltonian consists only of the projected kinetic energy.

cond-mat.str-el

Spin functional renormalization group for dimerized quantum spin systems

We investigate dimerized quantum spin systems using the spin functional renormalization group approach proposed by Krieg and Kopietz [Phys. Rev. B 99, 060403(R) (2019)] which directly focuses on the physical spin correlation functions and avoids the representation of the spins in terms of fermionic or bosonic auxiliary operators. Starting from decoupled dimers as initial condition for the renormalization group flow equations, we obtain the spectrum of the triplet excitations as well as the magnetization in the quantum paramagnetic, ferromagnetic, and thermally disordered phases at all temperatures. Moreover, we compute the full phase diagram of a weakly coupled dimerized spin system in three dimensions, including the correct mean field critical exponents at the two quantum critical points.

cond-mat.str-el