arXiv subjects

Jonathan B. Curtis

Publications and source records attributed to Jonathan B. Curtis.

At least 19 recordsLinked to original sources

arXiv2026

Probing Time Reversal Symmetry Breaking using a Nonlinear Superconducting Ring Resonator

Time-reversal symmetry breaking (TRSB) has been central to detecting exotic phases of matter. Here, we leverage the circuit electrodynamics capabilities of superconducting devices to propose a novel scheme based on a multimode superconducting ring resonator for sensitive probing of TRSB in quantum materials. A ring resonator enables nonlinear cross-interactions between the modes which act as an built-in amplifiers to be harnessed for enhanced sensing. Using a driven-dissipative model, we explore the nonlinear dynamics of a two-mode superconducting circuit with self- and cross-Kerr nonlinearities under conditions near the bifurcation threshold. By mapping the optimal parameter regimes, we show that even when the photon occupation numbers are subjected to different initial conditions, they can be driven into a symmetric configuration which is broken even with weak TRSB. Through full quantum analysis we demonstrate that the Kerr-nonlinear interactions up-convert the magnetic effects of material-resonator hybrid system, enhancing the probing of TRSB. Our findings highlight the utility of superconducting microwave resonators outside of quantum information processing, as a tool for probing exotic states of matter.

quant-ph↗

arXiv2026

Universal magnetic energy scale in the doped Fermi-Hubbard model

Magnetic correlations of doped Mott insulators hold the key to the unusual characteristics of many quantum materials. Recent experiments with ultracold atoms in optical lattices have provided new information about the magnetic properties of the Fermi-Hubbard model on a square lattice. We demonstrate that recent measurements indicate that a single doping-dependent energy scale determines both static correlations and dynamical response of these systems. To understand these experimental findings, we employ a self-consistent formalism to describe the coupling between antiferromagnetic magnons and doped holes, and we uncover the emergence of a universal magnetic energy scale at finite doping, which we denote by $J^*$. We present the single- and two-magnon spectral properties at finite doping and discuss the appearance of a bimagnon peak in lattice-modulation spectroscopy, at frequencies set by $J^*$. Furthermore, we argue that this same energy scale sets the onset of pseudogap phenomena, leading to the hypothesis $k_BT^* = c J^*$, with $c$ an order one number. We identify another low-energy scale emerging from our analysis of magnetic excitations, and argue that it controls the stability of Néel order at the lowest temperatures, ultimately driving a transition to an incommensurate spin-density-wave at finite doping. We discuss the relation between this low-energy scale and the nature of fermionic quasiparticles. Our analysis suggests that stability of the commensurate antiferromagentic phase at finite doping can be controlled experimentally by introducing additional quasiparticle broadening via disorder or low-frequency noise.

cond-mat.str-el↗

arXiv2025

Exciton collective modes in a bilayer of axion insulator $\text{MnBi}_2 \text{Te}_4$

We investigate the emergence of an exciton condensate and associated collective modes in a bilayer configuration of $\text{MnBi}_2\text{Te}_4$, an antiferromagnetic topological insulator and van der Waals material, recognized for hosting axion physics. Utilizing a minimal low-energy Hamiltonian for the two layer system which is gapped by the intrinsic Néel order, we first employ mean-field theory to establish the conditions for exciton condensation. Our analysis identifies a nonzero, spin-singlet exciton order parameter which is tuned by external displacement field, temperature, and Coulomb attraction. Beyond the mean-field, we explore collective mode fluctuations in the uncondensed phase via many-body perturbation theory and the random phase approximation. From this, we derive the exciton spectral function which allows for a direct comparison between theoretical prediction and experimental observation. We detail how the softening of the collective mode peak is a function of the competition between interlayer detuning and thermal fluctuations. This work elucidates how the unique topological and magnetic environment of $\text{MnBi}_2\text{Te}_4$ offers a tunable platform for the realization and manipulation of exciton condensates and the corresponding collective excitations. Our findings contribute to understanding the interplay of topology and bosonic condensates, which could inspire application in optically accessing topological properties, dissipationless transport, and gate-tunable optoelectronics.

cond-mat.mtrl-sci↗

arXiv2025

Casimir Stabilization of Fluctuating Electronic Nematic Order

Vacuum cavity control of quantum materials is the engineering of quantum materials systems through electromagnetic zero-point fluctuations. In this work we articulate a generic mechanism for vacuum optical control of correlated electronic order: Casimir control, where the zero-point energy of the electromagnetic continuum, the Casimir energy, depends on the properties of the material system. To assess the experimental viability of this mechanism we focus on the Casimir stabilization of fluctuating nematic order. In nematic Fermi liquids, different orientations of the electronic order are often energetically degenerate. Thus, while local domains of fixed orientation may form, thermal disordering inhibits long range order. By engineering the electromagnetic environment of the electronic system, however, we show that the Casimir energy can be used as a tool to preferentially stabilize particular orientations of the nematic order. As a concrete example, we examine the interplay between a birefringent crystal -- which sources an anisotropic electromagnetic environment -- and a quantum Hall stripe system, an archetypal nematic Fermi fluid. We show that for experimentally feasible setups, the anisotropy induced by the orientation dependent Casimir energy can be $10^4$ times larger than other mechanisms known to stabilize quantum Hall stripes. This finding convincingly implies that our setting may be realized with currently available experimental technology. Having demonstrated that the Casimir energy can be used to stabilize fluctuating nematic order, we close by discussing the implications for recent terahertz cavity experiments on quantum Hall stripes, as well as pave the road towards broader Casimir control of competing correlated electronic phases.

cond-mat.str-el↗

arXiv2025

Non-Gaussian Noise Magnetometry Using Local Spin Qubits

Atomic scale qubits, as may be realized in nitrogen vacancy (NV) centers in diamond, offer the opportunity to study magnetic field noise with nanometer scale spatial resolution. Using these spin qubits, one can learn a great deal about the magnetic-field noise correlations, and correspondingly the collective-mode spectra, in quantum materials and devices. However, to date these tools have been essentially restricted to studying Gaussian noise processes -- equivalent to linear-response. In this work we will show how to extend these techniques beyond the Gaussian regime and show how to unambiguously measure higher-order magnetic noise cumulants in a local, spatially resolved way. We unveil two protocols for doing this; the first uses a single spin-qubit and different dynamical decoupling sequences to extract non-Markovian and non-Gaussian spin-echo noise. The second protocol uses two-qubit coincidence measurements to study spatially non-local cumulants in the magnetic noise. We then demonstrate the utility of these protocols by considering a model of a bath of non-interacting two-level systems, as well as a model involving spatially correlated magnetic fluctuations near a second-order Ising phase transition. In both cases, we highlight how this technique can be used to measure in a real many-body system how fluctuation dynamics converge towards the central limit theorem as a function of effective bath size. We then conclude by discussing some promising applications and extensions of this method.

quant-ph↗

arXiv2025

Cavity QED Control of Quantum Hall Stripes

Controlling quantum phases of materials with vacuum field fluctuations in engineered cavities is a novel route towards the optical control of emergent phenomena. We demonstrate, using magnetotransport measurements of a high-mobility two-dimensional electron gas, striking cavity-induced anisotropies in the electronic transport, including the suppression of the longitudinal resistance well below the resistivity at zero magnetic field. Our cavity-induced effects occur at ultra-low temperatures (< 200 mK) when the magnetic field lies between quantized Hall plateaus. We interpret our results as arising from the stabilization of thermally-disordered quantum Hall stripes. Our work presents a clear demonstration of the cavity QED control of a correlated electronic phase.

cond-mat.mes-hall↗

arXiv2024

Quantum geometry induced microwave enhancement of flat band superconductivity

Photo-control of correlated phases is central to advancing and manipulating novel functional properties of quantum materials. Here, we explore microwave enhancement of superconductivity in flat bands through generation of nonequilibrium quasiparticles at subgap frequencies. In conventional superconductors, it is known to occur via radiation absorption determined by fermi velocity, which however is small in flat bands resulting in quenched quasiparticle excitations. Strikingly, in contrast to the conventional paradigm we show a non-vanishing microwave absorption in flat band systems enabled by Bloch quantum geometry leading to superconducting gap enhancement, underscoring the band-geometric origin of nonequilibrium flat band superconductivity. Specifically, we demonstrate this in twisted bilayer graphene, a promising candidate material, and find significant gap enhancement near critical temperature. This work highlights that the nonequilibrium dynamics of materials with non-trivial flat bands as a promising area for future experimental and theoretical investigation.

cond-mat.supr-con↗

arXiv2024

Terahertz field-induced nonlinear coupling of two magnon modes in an antiferromagnet

Magnons are quantized collective spin-wave excitations in magnetically ordered materials. Revealing their interactions among these collective modes is crucial for the understanding of fundamental many-body effects in such systems and the development of high-speed information transport and processing devices based on them. Nevertheless, identifying couplings between individual magnon modes remains a long-standing challenge. Here, we demonstrate spectroscopic fingerprints of anharmonic coupling between distinct magnon modes in an antiferromagnet, as evidenced by coherent photon emission at the sum and difference frequencies of the two modes. This discovery is enabled by driving two magnon modes coherently with a pair of tailored terahertz fields and then disentangling a mixture of nonlinear responses with different origins. Our approach provides a route for generating nonlinear magnon-magnon mixing.

cond-mat.mtrl-sci↗

arXiv2024

Dynamic magnetic phase transition induced by parametric magnon pumping

Uncovering pathways to optically drive magnetic order-disorder transitions on ultrashort timescales can lead to the realization of novel out-of-equilibrium quantum phenomena. A long-sought pathway is to directly excite a highly non-thermal energy-momentum distribution of magnons, bypassing both charge and lattice degrees of freedom. However, this remains elusive owing to the weak coupling and large momentum mismatch between photons and magnons. Here we demonstrate strong parametric excitation of magnons across the entire Brillouin zone of the antiferromagnetic insulator Sr$_2$Cu$_3$O$_4$Cl$_2$ by periodically modulating the superexchange interaction with the electric field of light. The excitation efficiency is greatly enhanced by tuning to the van Hove singularity in the magnon spectrum, sufficient to transiently collapse the antiferromagnetic state using a pulsed laser field of 10$^9$ V/m. The order parameter recovery timescale increases by over 1000 times as a function of excitation density, reflecting a crossover from high- to low-energy magnon dominated decay dynamics. This electric-field induced parametric magnon pumping mechanism is applicable to a broad range of magnetic insulators and opens up the possibility of dynamically engineering magnon distributions by design.

cond-mat.str-el↗

arXiv2024

Probing the Berezinskii-Kosterlitz-Thouless vortex unbinding transition in two-dimensional superconductors using local noise magnetometry

The melting of quasi-long-range superconductivity in two spatial dimensions occurs through the proliferation and unbinding of vortex-antivortex pairs -- a phenomenon known as the Berezinskii-Kosterlitz-Thouless (BKT) transition. Although signatures of this transition have been observed in bulk measurements, these experiments are often complicated, ambiguous, and unable to resolve the rich physics of the vortex unbinding transition. Here we show that local noise magnetometry is a sensitive, noninvasive probe that can provide direct information about the scale-dependent vortex dynamics. In particular, by resolving the distance and temperature dependence of the magnetic noise, it may be possible to experimentally study the renormalization group flow equations of the vortex gas and track the onset of vortex unbinding in situ. Specifically, we predict i) a nonmonotonic dependence of the noise on temperature and ii) the local noise is almost independent of the sample-probe distance at the BKT transition. We also show that noise magnetometry can distinguish Gaussian superconducting order-parameter fluctuations from topological vortex fluctuations and can detect the emergence of unbound vortices. The weak distance dependence at the BKT transition can also be used to distinguish it from quasiparticle background noise. Our predictions may be within experimental reach for a number of unconventional superconductors.

cond-mat.supr-con↗

arXiv2023

Probing Electromagnetic Nonreciprocity with Quantum Geometry of Photonic States

Reciprocal and nonreciprocal effects in dielectric and magnetic materials provide crucial information about the microscopic properties of electrons. However, experimentally distinguishing the two has proven to be challenging, especially when the associated effects are extremely small. To this end, we propose a contact-less detection using a cross-cavity device where a material of interest is placed at its centre. We show that the optical properties of the material, such as Kerr and Faraday rotation, or, birefringence, manifest in the coupling between the cavities' electromagnetic modes and in the shift of their resonant frequencies. By calculating the dynamics of a geometrical photonic state, we formulate a measurement protocol based on the quantum metric and quantum process tomography that isolates the individual components of the material's complex refractive index and minimizes the quantum mechanical Cramér-Rao bound on the variance of the associated parameter estimation. Our approach is expected to be applicable across a broad spectrum of experimental platforms including Fock states in optical cavities, or, coherent states in microwave and THz resonators.

physics.optics↗

arXiv2023

Local Fluctuations in Cavity Control of Ferroelectricity

Control of quantum matter through resonant electromagnetic cavities is a promising route towards establishing control over material phases and functionalities. Quantum paraelectric insulators -- materials which are nearly ferroelectric -- are particularly promising candidate systems for this purpose since they have strongly fluctuating collective modes which directly couple to the electric field. In this work we explore this possibility in a system comprised of a quantum paraelectric sandwiched between two high-quality metal mirrors, realizing a Fabry-Perot type cavity. By developing a full multimode, continuum description we are able to study the effect of the cavity in a spatially resolved way for a variety of system sizes and temperatures. Surprisingly, we find that once a continuum of transverse modes are included the cavity ends up suppressing ferroelectric correlations. This effect arises from the screening out of transverse photons at the cavity boundaries and as a result is confined to the surface of the paraelectric sample. We also explore the temperature dependence of this effect and find it vanishes at high temperatures, indicating it is a purely quantum mechanical effect. We connect our result to calculations of Casimir and Van der Waals forces, which we argue are closely related to the dipolar fluctuations in the quantum paraelectric. Our results are based on a general formalism and are expected to be widely applicable, paving the way towards studies of the quantum electrodynamics of heterostructures featuring multiple materials and phases.

cond-mat.mes-hall↗

arXiv2023

Theory for Anomalous Terahertz Emission in Striped Cuprate Superconductors

Recent experiments in the doped cuprates La$_{2-x}$Ba$_x$CuO$_4$ have revealed the emission of anomalous terahertz radiation after impulsive optical excitation. Here, we theoretically investigate the nonlinear electrodynamics of such striped superconductors and explore the origin of the observed radiation. We argue that photoexcitation is converted into a photocurrent by a second-order optical nonlinearity, which is activated by the breaking of inversion symmetry in certain stripe configurations. We point out the importance of including Umklapp photocurrents modulated at the stripe periodicity itself, which impulsively drive surface Josephson plasmons and lead to a resonant structure of outgoing radiation, consistent with the experiments. We speculate on the utility of the proposed mechanism in the context of generating tunable terahertz radiation.

cond-mat.supr-con↗

arXiv2023

Absence of Weak Localization on Negative Curvature Surfaces

The interplay between disorder and quantum interference leads to a wide variety of physical phenomena including celebrated Anderson localization -- the complete absence of diffusive transport due to quantum interference between different particle trajectories. In two dimensions, any amount of disorder is thought to induce localization of all states at long enough length scales, though this may be prevented if bands are topological or have strong spin-orbit coupling. In this note, we present a simple argument providing another mechanism for disrupting localization: by tuning the underlying curvature of the manifold on which diffusion takes place. We show that negative curvature manifolds contain a natural infrared cut off for the probability of self returning paths. We provide explicit calculations of the Cooperon -- directly related to the weak-localization corrections to the conductivity -- in hyperbolic space. It is shown that constant negative curvature leads to a rapid growth in the number of available trajectories a particle can coherently traverse in a given time, reducing the importance of interference effects and restoring classical diffusive behavior even in the absence of inelastic collisions. We conclude by arguing that this result may be amenable to experimental verification through the use of quantum simulators.

cond-mat.dis-nn↗

arXiv2023

Terahertz field-driven magnon upconversion in an antiferromagnet

Tailored light excitation and nonlinear control of lattice vibrations have emerged as powerful strategies to manipulate the properties of quantum materials out of equilibrium. Generalizing the use of coherent phonon-phonon interactions to nonlinear couplings among other types of collective modes would open unprecedented opportunities in the design of novel dynamic functionalities in solids. For example, the collective excitations of magnetic order -- magnons -- can carry information with little energy dissipation, and their coherent and nonlinear control would provide an attractive route to achieve collective-mode-based information processing and storage in forthcoming spintronics and magnonics. Here, we discover that intense terahertz (THz) fields can initiate processes of magnon upconversion mediated by an intermediate magnetic resonance. By using a suite of advanced spectroscopic tools, including a newly demonstrated two-dimensional (2D) THz polarimetry technique enabled by single-shot detection, we unveil the unidirectional nature of coupling between distinct magnon modes of a canted antiferromagnet. Calculations of spin dynamics further suggest that this coupling is a universal feature of antiferromagnets with canted magnetic moments. These results demonstrate a route to inducing desirable energy transfer pathways and THz-induced coupling between coherent magnons in solids and pave the way for a new era in the development of ultrafast control of magnetism.

cond-mat.mtrl-sci↗

arXiv2023

The bulk van der Waals layered magnet CrSBr is a quasi-1D material

Correlated quantum phenomena in one-dimensional (1D) systems that exhibit competing electronic and magnetic order are of strong interest for studying fundamental interactions and excitations, such as Tomonaga-Luttinger liquids and topological orders and defects with properties completely different from the quasiparticles expected in their higher-dimensional counterparts. However, clean 1D electronic systems are difficult to realize experimentally, particularly magnetically ordered systems. Here, we show that the van der Waals layered magnetic semiconductor CrSBr behaves like a quasi-1D material embedded in a magnetically ordered environment. The strong 1D electronic character originates from the Cr-S chains and the combination of weak interlayer hybridization and anisotropy in effective mass and dielectric screening with an effective electron mass ratio of $m^e_X/m^e_Y \sim 50$. This extreme anisotropy experimentally manifests in strong electron-phonon and exciton-phonon interactions, a Peierls-like structural instability and a Fano resonance from a van Hove singularity of similar strength of metallic carbon nanotubes. Moreover, due to the reduced dimensionality and interlayer coupling, CrSBr hosts spectrally narrow (1 meV) excitons of high binding energy and oscillator strength that inherit the 1D character. Overall, CrSBr is best understood as a stack of weakly hybridized monolayers and appears to be an experimentally attractive candidate for the study of exotic exciton and 1D correlated many-body physics in the presence of magnetic order.

cond-mat.mes-hall↗

arXiv2023

Finite-Momentum Instability of Dynamical Axion Insulator

The chiral anomaly is a striking signature of quantum effects which lead to the non-conservation of a classically conserved current, specifically the chiral currents in systems of fermions. In condensed matter systems, the chiral anomaly can be realized in Weyl semimetals, which then exhibit a signature electromagnetic response associated to anomaly due to the separation of the Weyl points in momentum space. In the presence of strong interactions however, a Weyl semimetal phase can give rise to an ordered phase, and spontaneously break the chiral symmetry. This then leads to a Goldstone mode which can have intrinsic dynamics and fluctuations, leading to a dynamical chiral anomaly response -- a situation known as a dynamical axion insulator. Here we consider a simple model of this dynamical axion insulator and calculate the equations of motion for the Goldstone mode. Surprisingly, we find that the Goldstone mode appears to exhibit a negative phase stiffness, signalling a further instability of the system towards finite momentum. This is expected to lead to very strong fluctuations of the anomalous response. We suggest a long-wavelength theory of Lifschitz type which may govern the axion dynamics in this system and comment on possible signatures of this model.

cond-mat.str-el↗

arXiv2022

Surface Cooper pair spin waves in triplet superconductors

We study the electrodynamics of spin triplet superconductors including dipolar interactions, which give rise to an interplay between the collective spin dynamics of the condensate and orbital Meissner screening currents. Within this theory, we identify a class of spin waves that originate from the coupled dynamics of the spin-symmetry breaking triplet order parameter and the electromagnetic field. In particular, we study magnetostatic spin wave modes that are localized to the sample surface. We show that these surface modes can be excited and detected using experimental techniques such as microwave spin wave resonance spectroscopy or nitrogen-vacancy magnetometry, and propose that the detection of these modes offers a means for the identification of spin triplet superconductivity.

cond-mat.supr-con↗