arXiv subjects

Jonathan D. Hood

Publications and source records attributed to Jonathan D. Hood.

15 recordsLinked to original sources

arXiv2026

Few-Body Decay Dynamics in Colloidal CsPbI3 Quantum-Dot Clusters

Colloidal perovskite quantum dots combine bright emission with the ability to self- assemble into closely spaced structures, enabling radiative dynamics to be studied from isolated emitters to few-dot clusters. Here, we characterize CsPbI3 perovskite quan- tum dots from isolated emitters to self-assembled clusters containing up to ten dots. We estimate the number of emitters in each cluster using a combination of photon autocorrelation, blinking statistics, and emission brightness. Compared with isolated dots, clusters containing two or more emitters exhibit biexponential decay, with a short lifetime that decreases with emitter number and an additional long-lived component. Photon-correlation Fourier spectroscopy shows that the single-dot emission remains far from the lifetime-limited regime. Nevertheless, we observe emitter-number-dependent decay dynamics even in this low-coherence regime. Together, these measurements es- tablish self-assembled perovskite quantum-dot clusters as a platform for studying how collective optical behavior emerges between the single-emitter and ensemble limits

quant-ph↗

arXiv2026

First order Maxwell operator formalism for macroscopic quantum electrodynamics

Standard macroscopic QED is built on the second-order Green's function for the electric field and discards open-system boundary terms. Here we develop a first-order electromagnetic operator approach that retains both $\mathbf{E}$ and $\mathbf{H}$ and keeps those boundary terms, naturally leading to a quantum input-output formalism. We recast Maxwell's equations as an operator equation for the dual field $\mathit{E}$=$[\mathbf{E},\mathbf{H}]^T$, whose first-order Green operator $g$ propagates the electromagnetic state between surfaces. Symmetries of the Maxwell operator under energy and reciprocal inner products yield the propagation formula, Lorentz reciprocity, and a generalized optical theorem, with minimal vector calculus. Quantizing via a Heisenberg-Langevin approach for absorptive, dispersive media yields two independent quantum noise sources: bulk Langevin operators from material absorption and input-output field operators at the boundary. Expressing the interior field in terms of these operators and the Green propagator yields an exact closed commutation relation $[{\mathit{E}},{\mathit{E}}^\dagger]\propto \mathrm{Im}\,g$, consistent with the fluctuation-dissipation theorem. This identity holds even when dielectrics extend to the boundary, as in waveguide input-output problems, and enables quantum input-output descriptions of complex photonic structures where the Green's function is obtained numerically, extending the framework beyond cavities and waveguides.

quant-ph↗

arXiv2026

Vapor Phase Assembly of Molecular Emitter Crystals for Photonic Integrated Circuits

Organic molecules embedded in an organic matrix exhibit lifetime-limited optical coherence and bright emission at cryogenic temperatures below 3 K. Here we present a simple vapor-phase growth method for synthesizing optically thin DBT-doped anthracene crystals that are compatible with integrated nanophotonics. The crystals are ~200 nm thick with sub-nm surface roughness and a tunable lateral dimension of up to 200 $μ$m. The molecular transitions remain narrow and spectrally stable, with inhomogeneous broadening below 100 GHz, comparable to DBT in bulk anthracene. The dopant density is tunable up to several hundred molecules per $μ$m$^2$, ensuring emitters within the near-field of nanophotonic structures. We demonstrate that the crystals can be micropositioned onto integrated photonic devices with the molecular dipole aligned to the optical mode. This approach opens a path toward on-chip single-photon sources and collective many-emitter effects.

quant-ph↗

arXiv2025

Many-Body Entanglement in Solid-State Emitters

The preparation and control of quantum states lie at the heart of quantum information science (QIS). Recent advances in solid-state quantum emitters (QEs) and nanophotonics have transformed the landscape of quantum photonic technologies, enabling scalable generation of quantum states of light and matter. A new frontier in solid-state quantum photonics is the engineering of many-body interactions between QEs and photons to achieve robust coherence and controllable many-body entanglement. These entangled states, including photonic graph and cluster states, superradiant emission, and emergent quantum phases, are promising for quantum computation, sensing, and simulation. However, intrinsic inhomogeneities and decoherence in solid-state platforms pose significant challenges to realize such complex entangled states. This review provides an overview of the fundamental many-body interactions and dynamics at the light-matter interfaces of solid-state QEs, and discusses recent advances in mitigating decoherence and harnessing robust many-body coherence.

quant-ph↗

arXiv2025

Cavity QED with molecular defects coupled to a photonic crystal cavity

We implement permanent spectral tuning to bring lifetime-limited emitters into collective resonance within an integrated photonic cavity. This addresses a fundamental challenge in solid-state cavity QED: combining multiple coherent quantum emitters with scalable nanophotonics. Our hybrid approach decouples emitter synthesis from nanophotonic fabrication using straightforward techniques that make cavity QED broadly accessible. High doping densities allow us to couple several coherent emitters to a single cavity mode, while optically-induced frequency shifting provides long-lived spectral control. By tuning two molecules into resonance, we demonstrate controlled formation of collective quantum states, establishing a scalable platform for many-body cavity QED. This opens pathways toward chemically-designed quantum systems where optical properties are engineered through synthetic chemistry.

quant-ph↗

arXiv2025

Narrow-Line Electric Quadrupole Cooling And Background-Free Imaging Of A Single Cs Atom With Spatially Structured Light

We demonstrate background-free imaging and sideband cooling of a single 133Cs atom via the narrow-line 6S1/2 to 5D5/2 electric quadrupole transition in a 1064 nm optical tweezer. The 5D5/2 state decays through the 6P3/2 state to the ground state, emitting an 852 nm wavelength photon that allows for background-free imaging. By encoding both spin and orbital angular momentum onto the 685 nm excitation light, we achieve background-free fluorescence histograms with 99.58(3)% fidelity by positioning the atom at the dark center of a vortex beam. Tuning the tweezer polarization ellipticity realizes a magic trap for the stretched F = 4, mF = 4 to F' = 6, mF' = 6 cycling transition. We cool to 5 uK in a 1.1 mK trap and outline a strategy for ground-state cooling. We compare cooling performance across different sideband regimes, while also exploring how the orbital angular momentum of structured light controls the selection rules for quadrupole transitions. These results expand the toolbox for high-fidelity quantum control and cooling in alkali-atom tweezer arrays.

physics.atom-ph↗

arXiv2024

A Generalized Theory for Optical Cooling of a Trapped Atom with Spin

Cooling atoms to the ground-state of optical tweezers is becoming increasingly important for high-fidelity imaging, cooling, and molecular assembly. While extensive theoretical work has been conducted on cooling in free space, fewer studies have focused on cooling in bound states. In this work, we present a unified formalism for optical cooling mechanisms in neutral atom tweezers, including resolved and unresolved sideband cooling with different trapping potentials, polarization gradient cooling, gray molasses cooling, $Λ$-enhanced gray molasses cooling, and Raman sideband cooling. We perform simulations and demonstrate good agreement with a simplified spin model. We derive and discuss the fundamental limits of each cooling mechanism and propose new strategies for achieving ground-state cooling in optical tweezers. Our findings provide valuable insights into optimizing cooling schemes for neutral atoms in optical tweezers, paving the way for minimizing thermal decoherence in Rydberg and molecular gates and improving efficiencies of molecular assembly.

physics.atom-ph↗

arXiv2023

Superradiant and subradiant states in lifetime-limited organic molecules through laser-induced tuning

An array of radiatively coupled emitters is an exciting new platform for generating, storing, and manipulating quantum light. However, the simultaneous positioning and tuning of multiple lifetime-limited emitters into resonance remains a significant challenge. Here we report the creation of superradiant and subradiant entangled states in pairs of lifetime-limited and sub-wavelength spaced organic molecules by permanently shifting them into resonance with laser-induced tuning. The molecules are embedded as defects in an organic nanocrystal. The pump light redistributes charges in the nanocrystal and dramatically increases the likelihood of resonant molecules. The frequency spectra, lifetimes, and second-order correlation agree with a simple quantum model. This scalable tuning approach with organic molecules provides a pathway for observing collective quantum phenomena in sub-wavelength arrays of quantum emitters.

quant-ph↗

arXiv2023

High resolution photoassociation spectroscopy of the excited $c^3Σ_{1}^+$ potential of $^{23}$Na$^{133}$Cs

We report on photoassociation spectroscopy probing the $c^3Σ_{1}^+$ potential of the bi-alkali NaCs molecule, identifying eleven vibrational lines between $v' = 0$ and $v' = 25$ of the excited $c^3Σ_{1}^+$ potential, and resolving their rotational and hyperfine structure. The observed lines are assigned by fitting to an effective Hamiltonian model of the excited state structure with rotational and hyperfine constants as free parameters. We discuss unexpected broadening of select vibrational lines, and its possible link to strong spin-orbit coupling of the $c^3Σ_{1}^+$ potential with the nearby $b^3Π_1$ and $B^1Π_1$ manifolds. Finally we report use of the $v' = 22$ line as an intermediate state for two-photon transfer of weakly bound Feshbach molecules to the rovibrational ground state of the $X^1Σ^+$ manifold.

physics.atom-ph↗

arXiv2020

Coherent optical creation of a single molecule

We report coherent association of atoms into a single weakly bound NaCs molecule in an optical tweezer through an optical Raman transition. The Raman technique uses a deeply bound electronic excited intermediate state to achieve a large transition dipole moment while reducing photon scattering. Starting from two atoms in their relative motional ground state, we achieve an optical transfer efficiency of 69%. The molecules have a binding energy of 770.2MHz at 8.83(2)G. This technique does not rely on Feshbach resonances or narrow excited-state lines and may allow a wide range of molecular species to be assembled atom-by-atom.

physics.atom-ph↗

arXiv2020

Reduction of laser intensity noise over 1 MHz band for single atom trapping

We reduce the intensity noise of laser light by using an electro-optic modulator and a cousto-optic modulator in series. The electro-optic modulator reduces noise at high frequency(10 kHz to 1 MHz), while the acousto-optic modulator sets the average power of the light and reduces noise at low frequency (up to 10 kHz). The light is then used to trap single sodium atoms in an optical tweezer, where the lifetime of the atoms is limited by parametric heating due to laser noise at twice the trapping frequency. With our noise eater, the noise is reduced by up to 15 dB at these frequencies, and the lifetime is increased by an order of magnitude to around 6 seconds. Our technique is general and acts directly on the laser beam, expanding laser options for sensitive optical trapping applications.

physics.atom-ph↗

arXiv2020

Forming a single molecule by magnetoassociation in an optical tweezer

We demonstrate the formation of a single NaCs molecule in an optical tweezer by magnetoassociation through an s-wave Feshbach resonance at 864.11(5)G. Starting from single atoms cooled to their motional ground states, we achieve conversion efficiencies of 47(1)%, and measure a molecular lifetime of 4.7(7)ms. By construction, the single molecules are predominantly (77(5)%) in the center-of-mass motional ground state of the tweezer. Furthermore, we produce a single p-wave molecule near 807G by first preparing one of the atoms with one quantum of motional excitation. Our creation of a single weakly bound molecule in a designated internal state in the motional ground state of an optical tweezer is a crucial step towards coherent control of single molecules in optical tweezer arrays.

physics.atom-ph↗

arXiv2020

Multichannel interactions of two atoms in an optical tweezer

The multichannel Na-Cs interactions are characterized by a series of measurements using two atoms in an optical tweezer, along with a multichannel quantum defect theory (MQDT). The triplet and singlet scattering lengths are measured by performing Raman spectroscopy of the Na-Cs motional states and least-bound molecular state in the tweezer. Magnetic Feshbach resonances are observed for only two atoms at fields which agree well with the MQDT. Our methodology, which promotes the idea of an effective theory of interaction, can be a key step towards the understanding and the description of more complex interactions. The tweezer-based measurements in particular will be an important tool for atom-molecule and molecule-molecule interactions, where high densities are experimentally challenging and where the interactions can be dominated by intra-species processes.

physics.atom-ph↗

arXiv2019

Molecular assembly of ground state cooled single atoms

We demonstrate full quantum state control of two species of single atoms using optical tweezers and assemble the atoms into a molecule. Our demonstration includes 3D ground-state cooling of a single atom (Cs) in an optical tweezer, transport by several microns with minimal heating, and merging with a single Na atom. Subsequently, both atoms occupy the simultaneous motional ground state with 61(4)\% probability. This realizes a sample of exactly two co-trapped atoms near the phase-space-density limit of one, and allows for efficient stimulated-Raman transfer of a pair of atoms into a molecular bound state of the triplet electronic ground potential $a^3Σ^+$. The results are key steps toward coherent creation of single ultracold molecules, for future exploration of quantum simulation and quantum information processing.

physics.atom-ph↗

arXiv2018

Motional Ground State Cooling Outside the Lamb-Dicke Regime

We report Raman sideband cooling of a single sodium atom to its three-dimensional motional ground state in an optical tweezer. Despite a large Lamb-Dicke parameter, high initial temperature, and large differential light shifts between the excited state and the ground state, we achieve a ground state population of $93.5(7)$% after $53$ ms of cooling. Our technique includes addressing high-order sidebands, where several motional quanta are removed by a single laser pulse, and fast modulation of the optical tweezer intensity. We demonstrate that Raman sideband cooling to the 3D motional ground state is possible, even without tight confinement and low initial temperature.

physics.atom-ph↗