arXiv subjects

Jonathan Keeling

Publications and source records attributed to Jonathan Keeling.

At least 55 records · Page 3Linked to original sources

arXiv2020

Multimode Organic Polariton Lasing

We present a beyond-mean-field approach to predict the nature of organic polariton lasing, accounting for all relevant photon modes in a planar microcavity. Starting from a microscopic picture, we show how lasing can switch between polaritonic states resonant with the maximal gain, and those at the bottom of the polariton dispersion. We show how the population of non-lasing modes can be found, and by using two-time correlations, we show how the photoluminescence spectrum (of both lasing and non-lasing modes) evolves with pumping and coupling strength, confirming recent experimental work on the origin of blueshift for polariton lasing.

cond-mat.quant-gas↗

arXiv2020

Crescent states in charge-imbalanced polariton condensates

We study two-dimensional charge-imbalanced electron-hole systems embedded in an optical microcavity. We find that strong coupling to photons favors states with pairing at zero or small center of mass momentum, leading to a condensed state with spontaneously broken time-reversal and rotational symmetry, and unpaired carriers that occupy an anisotropic crescent-shaped sliver of momentum space. The crescent state is favoured at moderate charge imbalance, while a Fulde--Ferrel--Larkin--Ovchinnikov-like state --- with pairing at large center of mass momentum --- occurs instead at strong imbalance. The crescent state stability results from long-range Coulomb interactions in combination with extremely long-range photon-mediated interactions.

cond-mat.quant-gas↗

arXiv2019

Atom-only descriptions of the driven-dissipative Dicke model

We investigate how to describe the dissipative spin dynamics of the driven-dissipative Dicke model, describing $N$ two-level atoms coupled to a cavity mode, after adiabatic elimination of the cavity mode. To this end, we derive a Redfield master equation which goes beyond the standard secular approximation and large detuning limits. We show that the secular (or rotating wave) approximation and the large detuning approximation both lead to inadequate master equations, that fail to predict the Dicke transition or the damping rates of the atomic dynamics. In contrast, the full Redfield theory correctly predicts the phase transition and the effective atomic damping rates. Our work provides a reliable framework to study the full quantum dynamics of atoms in a multimode cavity, where a quantum description of the full model becomes intractable.

quant-ph↗

arXiv2019

Introduction to the Dicke model: from equilibrium to nonequilibrium, and vice versa

The Dicke model describes the coupling between a quantized cavity field and a large ensemble of two-level atoms. When the number of atoms tends to infinity, this model can undergo a transition to a superradiant phase, belonging to the mean-field Ising universality class. The superradiant transition was first predicted for atoms in thermal equilibrium and was recently realized with a quantum simulator made of atoms in an optical cavity, subject to both dissipation and driving. In this Progress Report, we offer an introduction to some theoretical concepts relevant to the Dicke model, reviewing the critical properties of the superradiant phase transition, and the distinction between equilibrium and nonequilibrium conditions. In addition, we explain the fundamental difference between the superradiant phase transition and the more common lasing transition. Our report mostly focuses on the steady states of atoms in single-mode optical cavities, but we also mention some aspects of real-time dynamics, as well as other quantum simulators, including superconducting qubits, trapped ions, and using spin-orbit coupling for cold atoms. These realizations differ in regard to whether they describe equilibrium or non-equilibrium systems.

quant-ph↗

arXiv2018

Fluorescence spectrum and thermalization in a driven coupled cavity array

We calculate the fluorescence spectra of a driven lattice of coupled cavities. To do this, we extend methods of evaluating two-time correlations in infinite lattices to open quantum systems; this allows access to momentum resolved fluorescence spectrum. We illustrate this for a driven-dissipative transverse field anisotropic XY model. By studying the fluctuation dissipation theorem, we find the emergence of a quasi-thermalized steady state with a temperature dependent on system parameters; for blue detuned driving, we show this effective temperature is negative. In the low excitation density limit, we compare these numerical results to analytical spin-wave theory, providing an understanding of the form of the distribution function and the origin of quasi-thermalization.

cond-mat.other↗

arXiv2018

Emergent and broken symmetries of atomic self-organization arising from Gouy phase shifts in multimode cavity QED

Optical cavities can induce photon-mediated interactions among intracavity-trapped atoms. Multimode cavities provide the ability to tune the form of these interactions, e.g., by inducing a nonlocal, sign-changing term to the interaction. By accounting for the Gouy phase shifts of the modes in a nearly degenerate, confocal, Fabry-Perot cavity, we provide a theoretical description of this interaction, along with additional experimental confirmation to complement that presented in the companion paper, Ref. [1]. Furthermore, we show that this interaction should be written in terms of a complex order parameter, allowing for a U(1)-symmetry to emerge. This symmetry corresponds to the phase of the atomic density wave arising from self-organization when the cavity is transversely pumped above a critical threshold power. We theoretically and experimentally show how this phase depends on the position of the Bose-Einstein condensate (BEC) within the cavity and discuss mechanisms that break the U(1)-symmetry and lock this phase. We then consider alternative Fabry-Perot multimode cavity geometries (i.e., beyond the confocal) and schemes with more than one pump laser and show that these provide additional capabilities for tuning the cavity-meditated interaction among atoms, including the ability to restore the U(1)-symmetry despite the presence of symmetry-breaking effects. These photon-mediated interactions may be exploited for realizing quantum liquid crystalline states and spin glasses using multimode optical cavities.

cond-mat.quant-gas↗

arXiv2018

Sign-changing photon-mediated atom interactions in multimode cavity QED

Sign-changing interactions constitute a crucial ingredient in the creation of frustrated many-body systems such as spin glasses. We present here the demonstration of a photon-mediated sign-changing interaction between Bose-Einstein condensed (BEC) atoms in a confocal cavity. The interaction between two atoms is of an unusual, nonlocal form proportional to the cosine of the inner product of the atoms' position vectors. This interaction arises from the differing Gouy phase shifts of the cavity's degenerate modes. Moreover, these Gouy phase anomalies induce an extra pattern of Z_2-symmetry-breaking in the atomic density-wave self-ordering that arises from a nonequilibrium Dicke-type phase transition in the system. This state is detected via the holographic imaging of the cavity's superradiant emission. Together with Ref. [1], we explore this interaction's influence on superradiant phase transitions in multimode cavities. Employing this interaction in cavity QED spin systems may enable the creation of artificial spin glasses and quantum neural networks.

cond-mat.quant-gas↗

arXiv2018

Efficient non-Markovian quantum dynamics using time-evolving matrix product operators

In order to model realistic quantum devices it is necessary to simulate quantum systems strongly coupled to their environment. To date, most understanding of open quantum systems is restricted either to weak system-bath couplings, or to special cases where specific numerical techniques become effective. Here we present a novel general numerical approach to efficiently describe the time evolution of a quantum system coupled to a non-Markovian environment. We demonstrate the power and flexibility of our method by numerically identifying the localisation transition of the Ohmic spin-boson model, and considering a model with widely separated environmental timescales arising for a pair of spins embedded in a common environment.

quant-ph↗

arXiv2018

Organic polariton lasing and the weak- to strong-coupling crossover

Following experimental realizations of room temperature polariton lasing with organic molecules, we present a microscopic model that allows us to explore the crossover from weak to strong matter-light coupling. We consider a non-equilibrium Dicke-Holstein model, including both strong coupling to vibrational modes and strong matter-light coupling, providing the phase diagram of this model in the thermodynamic limit. We discuss the mechanism of polariton lasing, uncovering a process of self-tuning, and identify the relation and distinction between regular dye lasers and organic polariton lasers.

cond-mat.quant-gas↗

arXiv2018

Spinor self-ordering of a quantum gas in a cavity

We observe the joint spin-spatial (spinor) self-organization of a two-component BEC strongly coupled to an optical cavity. This unusual nonequilibrium Hepp-Lieb-Dicke phase transition is driven by an off-resonant two-photon Raman transition formed from a classical pump field and the emergent quantum dynamical cavity field. This mediates a spinor-spinor interaction that, above a critical strength, simultaneously organizes opposite spinor states of the BEC on opposite checkerboard configurations of an emergent 2D lattice. The resulting spinor density-wave polariton condensate is observed by directly detecting the atomic spin and momentum state and by holographically reconstructing the phase of the emitted cavity field. The latter provides a direct measure of the spin state, and a spin-spatial domain wall is observed. The photon-mediated spin interactions demonstrated here may be engineered to create dynamical gauge fields and quantum spin glasses.

cond-mat.quant-gas↗

arXiv2018

Spectroscopic probes of quantum many-body correlations in polariton microcavities

We investigate the many-body states of exciton-polaritons that can be observed by pump-probe spectroscopy. Here, a weak-probe `spin-down' polariton is introduced into a coherent state of `spin-up' polaritons created by a strong pump. We show that the $\downarrow$ impurities become dressed by excitations of the $\uparrow$ medium, and form new polaronic quasiparticles that feature two-point and three-point many-body quantum correlations, which, in the low density regime, arise from coupling to the vacuum biexciton and triexciton states respectively. In particular, we find that these correlations generate additional branches and avoided crossings in the $\downarrow$ optical transmission spectrum that have a characteristic dependence on the $\uparrow$-polariton density. Our results thus demonstrate a way to directly observe correlated many-body states in an exciton-polariton system that go beyond classical mean-field theories.

cond-mat.quant-gas↗

arXiv2018

Orientational alignment in Cavity Quantum Electrodynamics

We consider the orientational alignment of dipoles due to strong matter light coupling, for a non-vanishing density of excitations. We compare various approaches to this problem in the limit of large numbers of emitters, and show that direct Monte Carlo integration, mean-field theory, and large deviation methods match exactly in this limit. All three results show that orientational alignment develops in the presence of a macroscopically occupied polariton mode, and that the dipoles asymptotically approach perfect alignment in the limit of high density or low temperature.

cond-mat.mes-hall↗

arXiv2018

Coherence protection in coupled quantum systems

The interaction of a quantum system with its environment causes decoherence, setting a fundamental limit on the suitability of a system for quantum information processing. However, we show that if the quantum system consists of coupled parts with different internal energy scales then the interaction of one part with a thermal bath need not lead to loss of coherence from the other. Remarkably, we find that the protected part can become more coherent when the coupling to the bath becomes stronger or the temperature is raised. Our theory will enable the design of decoherence-resistant hybrid quantum computers.

quant-ph↗

arXiv2018

Generalized classes of continuous symmetries in two-mode Dicke models

As recently realized experimentally [Léonard et al., Nature 543, 87 (2017)], one can engineer models with continuous symmetries by coupling two cavity modes to trapped atoms, via a Raman pumping geometry. Considering specifically cases where internal states of the atoms couple to the cavity, we show an extended range of parameters for which continuous symmetry breaking can occur, and we classify the distinct steady states and time-dependent states that arise for different points in this extended parameter regime.

cond-mat.quant-gas↗

arXiv2017

Superradiant and Lasing States in Driven-Dissipative Dicke Models

We present the non-equilibrium phase diagram of a model which can demonstrate both Dicke--Hepp--Lieb superradiance and regular lasing by varying the coherent and incoherent driving terms. We find that the regions in the phase diagram corresponding to superradiance and standard lasing are always separated by a normal region. We analyse the behaviour of the system using a combination of exact numerics based on permutation symmetry of the density matrix for small to intermediate numbers of molecules, and second order cumulant equations for large numbers of molecules. We find that the nature of the photon distribution in the superradiant and lasing states are very similar, but the emission spectrum is very different. We also show that in the presence of both coherent and incoherent driving, a period-doubling route to a chaotic state occurs.

cond-mat.quant-gas↗

arXiv2017

Exact states and spectra of vibrationally dressed polaritons

Strong coupling between light and matter is possible with a variety of organic materials. In contrast to the simpler inorganic case, organic materials often have a complicated spectrum, with vibrationally dressed electronic transitions. Strong coupling to light competes with this vibrational dressing, and if strong enough, can suppress the entanglement between electronic and vibrational degrees of freedom. By exploiting symmetries, we can perform exact numerical diagonalization to find the polaritonic states for intermediate numbers of molecules, and use these to define and validate accurate expressions for the lower polariton states and strong-coupling spectrum in the thermodynamic limit. Using this approach, we find that vibrational decoupling occurs as a sharp transition above a critical matter-light coupling strength. We also demonstrate how the polariton spectrum evolves with the number of molecules, recovering classical linear optics results only at large $N$.

cond-mat.mes-hall↗

arXiv2017

Polarization dynamics in a photon BEC

It has previously been shown that a dye-filled microcavity can produce a Bose-Einstein condensate of photons. Thermalization of photons is possible via repeated absorption and re-emission by the dye molecules. In this paper, we theoretically explore the behavior of the polarization of light in this system. We find that in contrast to the near complete thermalization between different spatial modes of light, thermalization of polarization states is expected to generally be incomplete. We show that the polarization degree changes significantly from below to above threshold, and explain the dependence of polarization on all relevant material parameters.

cond-mat.mes-hall↗

arXiv2017

Tunable-range, photon-mediated atomic interactions in multimode cavity QED

Optical cavity QED provides a platform with which to explore quantum many-body physics in driven-dissipative systems. Single-mode cavities provide strong, infinite-range photon-mediated interactions among intracavity atoms. However, these global all-to-all couplings are limiting from the perspective of exploring quantum many-body physics beyond the mean-field approximation. The present work demonstrates that local couplings can be created using multimode cavity QED. This is established through measurements of the threshold of a superradiant, self-organization phase transition versus atomic position. Specifically, we experimentally show that the interference of near-degenerate cavity modes leads to both a strong and tunable-range interaction between Bose-Einstein condensates (BECs) trapped within the cavity. We exploit the symmetry of a confocal cavity to measure the interaction between real BECs and their virtual images without unwanted contributions arising from the merger of real BECs. Atom-atom coupling may be tuned from short range to long range. This capability paves the way toward future explorations of exotic, strongly correlated systems such as quantum liquid crystals and driven-dissipative spin glasses.

cond-mat.quant-gas↗