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Jonathan Stensberg

Publications and source records attributed to Jonathan Stensberg.

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Finite-momentum Cooper plasmons in superconducting terahertz microcavities

The phase mode of a superconductor's order parameter encodes fundamental information about pairing and dissipation, but is typically inaccessible at low frequencies due to the Anderson-Higgs mechanism. Superconducting samples thinner than the London penetration depth, however, support a gapless phase mode whose dispersion can be reshaped by a proximal screening layer. Here, we theoretically and experimentally show that this screened phase mode in a superconducting thin film integrated into on-chip terahertz circuitry naturally forms a superconducting microcavity that hosts resonant finite-momentum standing waves of supercurrent density, which we term Cooper plasmons. We measure two Cooper plasmons in a superconducting NbN microcavity and demonstrate that their resonance frequencies and linewidths independently report the density of participating carriers and plasmon's dissipation at finite momenta. Our results reveal an emergent collective mode of an integrated superconductor-circuit system and establish design principles for engineering or suppressing Cooper plasmons in superconducting terahertz devices and circuits.

cond-mat.supr-con

Persistent Fluctuating Superconductivity and Planckian Dissipation in Fe(Te,Se)

Increasingly intricate phase diagrams in new classes of superconductors host fascinating interactions between superconductivity, diverse quantum phases, and quantum critical dynamics. The native superfluids, however, often exhibit much lower density and much greater inhomogeneity than conventional superfluids. This may render the superconductivity susceptible to fluctuations that are ordinarily assumed to be frozen out far below the superconducting transition temperature $T_c$, calling into question the degree to which the superconducting state is fully coherent. In this work, we leverage terahertz spectroscopy to demonstrate strongly fluctuating superconductivity in topological compositions of the multiband iron-based superconductor Fe(Te,Se). These fluctuations are found to persist undiminished far below $T_c$ and converge upon the limit of Planckian dissipation above $T_c$. These results indicate that extended quantum fluctuations dominate the electrodynamics of both the superconducting and Planckian-dissipative precursor states of Fe(Te,Se), and demonstrate that the assumption of phase coherence must be rigorously validated in emerging classes of unconventional superconductors.

cond-mat.supr-con

Purcell enhancement of photogalvanic currents in a van der Waals plasmonic self-cavity

Cavities provide a means to manipulate the optical and electronic responses of quantum materials by selectively enhancing light-matter interaction at specific frequencies and momenta. While cavities typically involve external structures, exfoliated flakes of van der Waals (vdW) materials can form intrinsic self-cavities due to their small finite dimensions, confining electromagnetic fields into plasmonic cavity modes, characterized by standing-wave current distributions. While cavity-enhanced phenomena are well-studied at optical frequencies, the impact of self-cavities on nonlinear electronic responses--such as photogalvanic currents--remains largely unexplored, particularly in the terahertz regime, critical for emerging ultrafast optoelectronic technologies. Here, we report a self-cavity-induced Purcell enhancement of photogalvanic currents in the vdW semimetal WTe$_2$. Using ultrafast optoelectronic circuitry, we measured coherent near-field THz emission resulting from nonlinear photocurrents excited at the sample edges. We observed enhanced emission at finite frequencies, tunable via excitation fluence and sample geometry, which we attribute to plasmonic interference effects controlled by the cavity boundaries. We developed an analytical theory that captures the cavity resonance conditions and spectral response across multiple devices. Our findings establish WTe$_2$ as a bias-free, geometry-tunable THz emitter and demonstrate the potential of self-cavity engineering for controlling nonlinear, nonequilibrium dynamics in quantum materials.

cond-mat.mes-hall

Observation of Coherent Ferron Emission and Propagation

Excitation of ordered quantum phases gives rise to collective modes and quasiparticles, as exemplified by spin waves and magnons emerging from magnetic order. Extending this paradigm to ferroelectric materials suggests the existence of polarization waves and their fundamental quanta, ferrons. Here, we report the generation and transport of polarization waves, i.e., coherent ferrons, in the van der Waals ferroelectric material NbOI2. Upon excitation by a short laser pulse, the polarization wave emits intense and narrow-band terahertz (THz) radiation at the ferroelectric transverse optical phonon frequency, modulates the ferroelectric order parameter, and propagates uniaxially along the polar axis at hypersonic velocities of ~105 m/s. These long-lived, uniaxial, and dipole-carrying polarization waves may find applications in narrow-band THz emission, ferronic information processing, and coherent electric control.

cond-mat.mtrl-sci

Observation of terahertz second harmonic generation from Dirac surface states in the topological insulator Bi$_2$Se$_3$

We report the observation of second harmonic generation with high conversion efficiency $\sim 0.005\%$ in the terahertz regime from thin films of the topological insulator Bi$_2$Se$_3$ that exhibit the linear photogalvanic effect, measured via time-domain terahertz spectroscopy and terahertz emission, respectively. As neither phenomena is observable from topologically trivial In-doped Bi$_2$Se$_3$, and since no enhancement is observed when subject to band bending, the efficient thickness-independent nonliear responses are attributable to the Dirac fermions of topological surface states of Bi$_2$Se$_3$. This observation of intrinsic terahertz second harmonic generation in an equilibrium system unlocks the full suite of both even and odd harmonic orders in the terahertz regime and opens new pathways to probing quantum geometry via intraband nonlinear processes. We hope our work will motivate the theoretical development of a full treatment of second harmonic generation for probing the quantum geometry in various inversion-breaking topological and twisted materials.

cond-mat.str-el

Observation of the superconducting proximity effect from surface states in SmB$_6$/YB$_6$ thin film heterostructures via terahertz spectroscopy

The AC conduction of epitaxially-grown SmB$_6$ thin films and superconducting heterostructures of SmB$_6$/YB$_6$ are investigated via time domain terahertz spectroscopy. A two-channel model of thickness-dependent bulk states and thickness-independent surface states accurately describes the measured conductance of bare SmB$_6$ thin films, demonstrating the presence of surface states in SmB$_6$. While the observed reductions in the simultaneously-measured superconducting gap, transition temperature, and superfluid density of SmB$_6$/YB$_6$ heterostructures relative to bare YB$_6$ indicate the penetration of proximity-induced superconductivity into the SmB$_6$ overlayer; the corresponding SmB$_6$-thickness independence between different heterostructures indicates that the induced superconductivity is predominantly confined to the interface surface state of the SmB$_6$. This study demonstrates the ability of terahertz spectroscopy to probe proximity-induced superconductivity at an interface buried within a heterostructure, and our results show that SmB$_6$ behaves as a predominantly insulating bulk surrounded by conducting surface states in both the normal and induced-superconducting states in both terahertz and DC responses, which is consistent with the topological Kondo insulator picture.

cond-mat.mtrl-sci

Giant intrinsic anomalous terahertz Faraday rotation in the magnetic Weyl semimetal Co$_2$MnGa at room temperature

We report measurement of terahertz anomalous Hall conductivity and Faraday rotation in the magnetic Weyl semimetal Co$_2$MnGa thin films as a function of the magnetic field, temperature and thickness, using time-domain terahertz spectroscopy. The terahertz conductivity shows a thickness-independent anomalous Hall conductivity of around 600 $\Omega^{-1}\cdot cm^{-1}$ at room temperature, and it is also frequency-independent from 0.2-1.5 THz. The magnitude of the longitudinal and Hall conductivities, the weak spin-orbit coupling, and the very close positioning of Weyl points to the chemical potential all satisfy the criteria for intrinsic anomalous Hall conductivity. First-principle calculation also supports the frequency-independent intrinsic anomalous Hall conductivity at low frequency. We also find a thickness-independent Faraday rotation of 59 ($\pm6$) mrad at room temperature, which comes from the intrinsic Berry curvature contribution. In the thinnest 20 nm sample, the Faraday rotation divided by the sample thickness reaches around 3 mrad/nm due to Berry curvature, and is the largest reported at room temperature. The giant Verdet constant of the order of 10 $^{6}$ rad m $^{-1}$ T $^{-1}$ at room temperature and the large Hall angle around 8.5 $\%$ from 0.2-1.5 THz indicates that Co$_2$MnGa is promising for THz spintronics at room temperature.

cond-mat.mtrl-sci