arXiv subjects

Jonathan T. Reichanadter

Publications and source records attributed to Jonathan T. Reichanadter.

4 recordsLinked to original sources

arXiv2026

High-Temperature ferromagnetism from site-selective filling in (Fe,Ni)$_{6-δ}$GeTe$_2$

The discovery of high-temperature ferromagnetism in the metallic van der Waals (vdW) system Fe$_N$GeTe$_2$ has brought two-dimensional (2D) magnets into technologically relevant temperature scales. Specifically at N = 5, dilution of magnetic moments by nickel substitution counterintuitively achieves a record high Curie temperature of 478~K. Unraveling the origin of this nickel-substitution-induced enhancement is complicated by the compound's structural complexity, coexistent itinerant and local magnetic contributions, and mesoscopic compositional domains. Through coordinated structural and electronic characterization, we identify that the high-T$_C$ magnetic phase arises from a strain-stabilized Fe$_6$GeTe$_2$ nano-precipitate. Combining first-principles calculations and spin- and angle-resolved photoemission spectroscopy (ARPES), we uncover a site-specific electronic landscape in which interior iron atoms primarily host localized moments while the outer iron atoms neighboring the tellurium layers produce spin-polarized itinerant carriers that cross the vdW gap. The large energy cost associated with homogeneous nickel substitution is found to favor the spontaneous precipitation of the crystallographically and electronically ``clean'' high-T$_C$ phase. Finally, we compare metal-rich vdW magnets with binary magnetic alloys, and discuss the unifying roles of nano-precipitates in stabilizing otherwise unattainable bulk phases. Our work provides mechanistic insights into the record-high T$_C$ ferromagnetism in (Fe,Ni)$_{5+δ}$GeTe$_2$, establishing a rigorous foundation for the atomic engineering of vdW magnetic metals informed by direct electronic signatures.

cond-mat.mtrl-sci↗

arXiv2026

Electronic origin of delicate antiferromagnetism in Fe$_{x}$NbS$_2$

Among the family of intercalated transition-metal dichalcogenides (TMDs), Fe$_{x}$NbS$_2$ is found to possess unique current-induced resistive switching behaviors, tunable antiferromagnetic states, and a commensurate charge order, all of which are tied to a critical Fe doping of $x_c$ = 1/3. However, the electronic origin of such extreme stoichiometry sensitivities remains unclear. Combining angle-resolved photoemission spectroscopy (ARPES) with density functional theory (DFT) calculations, we identify and characterize a dramatic eV-scale electronic restructuring that occurs across the $x_c$. Moment-carrying Fe 3$d_{z^2}$ electrons manifest as narrow bands within 200 meV of the Fermi level, distinct from other transition metal intercalated TMD magnets. These states strongly hybridize with itinerant electrons in TMD layer, rapidly lose coherence above $x_c$ due to correlation-driven effects. This sudden quasiparticle decoherence collapses the Fe-Nb hybridization, which explicitly suppresses the out-of-plane effective Fe-Fe exchange interaction, driving the transformation of the magnetic ground state from an antiferromagnetic stripe phase to a zigzag phase. These observations resemble the exceptional electronic and magnetic sensitivity of strongly correlated systems, and demonstrate that quantifying orbital-specific hybridization via ARPES offers an alternative pathway to evaluate effective magnetic exchange in metallic magnets, complementing inelastic neutron and resonant x-ray scattering probes.

cond-mat.str-el↗

arXiv2025

Dark Metastable Conduction Channels near a Metal-Insulator Transition

Materials that transition between metal and insulator, the two main states that distinguish all solids, are fascinating because they underlie many mysteries at the frontier of solid state physics. In 1T-TaS$_{2}$, the metal-insulator transition is linked to a metastable hidden state arising within a chiral charge density wave (CDW) whose basic nature remains an open question. In this work, we show that pulses of current through these materials create current-carrying filamentary channels that distinguish the 'metallic' hidden state and 'insulating' CDW states. These channels have remained dark to previous measurements, and yet are directly linked to the properties of the hidden state. We leverage the metastability of these conduction channels to demonstrate electrical control of their creation, erasure and location. Our findings show that physical elements, such as boundaries and interfaces, play a key role in the properties of the hidden state characterizing the metal-insulator transition. We suggest new possibilities for in-situ electrical design of synaptic components with possible applications to neuromorphic computing.

cond-mat.str-el↗

arXiv2021

A room temperature polar ferromagnetic metal

The advent of long-range magnetic order in non-centrosymmetric compounds has stimulated interest in the possibility of exotic spin transport phenomena and topologically protected spin textures for applications in next-generation spintronics. This work reports a novel wurtzite-structure polar magnetic metal, identified as AA'-stacked (Fe0.5Co0.5)5-xGeTe2, which exhibits a Neel-type skyrmion lattice as well as a Rashba-Edelstein effect at room temperature. Atomic resolution imaging of the structure reveals a structural transition as a function of Co-substitution, leading to the polar phase at 50% Co. This discovery reveals an unprecedented layered polar magnetic system for investigating intriguing spin topologies and ushers in a promising new framework for spintronics.

cond-mat.mtrl-sci↗