SearcharxivSearch

arXiv subjects

Joonho Jang

Publications and source records attributed to Joonho Jang.

14 recordsLinked to original sources

Superconductivity near quarter and half filling of a strongly correlated triangular Hubbard band in twisted trilayer WSe2

The triangular-lattice Hubbard model is one of the paradigmatic settings for studying correlated electronic systems with geometric frustration that can give rise to a variety of phases. Recently, twisted bilayer TMD systems have emerged as attractive experimental platforms for realising such a model in the moderate-correlation regime. Alternating twisted trilayer TMD systems are expected to realise stronger correlations than bilayer systems owing to their mirror symmetry. Here we report the discovery of superconductivity near quarter- and half-filling, together with various correlated phases, in alternating twisted trilayer WSe2 (TTWSe2). At half filling, a robust correlated insulating state persists over a broad range of displacement fields, signalling the strongly correlated regime. Upon doping, superconductivity emerges over an extended region of the phase diagram. Near quarter filling, another superconducting state appears flanked by correlated metals. Our results establish the TTWSe2 system as a compelling platform for studying strongly correlated triangular-lattice Hubbard physics.

cond-mat.supr-con

Evidence for electron localisation in a moir\'e-of-moir\'e superlattice

The localisation of electrons in a lattice potential is an quantum-mechanical phenomenon and is often associated with remarkable physical properties of solids involving electron spins, electric polarisations and topological effects. In particular, even a small amount of distortion of the lattice potential can localise otherwise-delocalised quantum states in low-dimensional electron systems, dramatically influencing their thermodynamic properties and charge-transport behaviour. Study of such electron localisation induced by an aperiodic lattice potential remains exceptionally challenging in solid-state systems, since extrinsic disorders can trivially trap electrons in potential minima near disorders, obscuring the underlying quantum-mechanical origin of localisation phenomena. Van der Waals heterostructures can provide an alternative route for explorations of the phenomena via the emergence of superlattice potentials generated by rotating and stacking individual layers. Here, we report strong signatures of electron localisation in helical trilayer graphene, where the interplay of two moir\'e patterns gives rise to a moir\'e-of-moir\'e superlattice with distinct regions of moir\'e-periodic and moir\'e-aperiodic potentials. Remarkably, our measurements reveal the presence of double moir\'e-induced bands and high-order Brown-Zak oscillations, which are direct reflections of the periodic region with two constituent moir\'e patterns, and a superimposed anomalous hysteretic signal attributable to the aperiodic region. The data strongly suggest that electron wave functions are partially localised driven by the loss of a periodic lattice potential. Our work provides insight into the effects of spatially inhomogeneous lattice potentials on the low-dimensional electronic states and introduces a promising approach to control electron localisation for practical applications in solid-state devices.

cond-mat.mes-hall

Interaction of moire-induced quantum Hall channels in a locally gated graphene junction

Manipulating electron quantum 1D channels is an important element in the field of quantum information due to their ballistic and phase coherence properties. In GaAs and graphene based two dimensional gas systems, these edge channels have been investigated with both integer and fractional quantum Hall effects, contributing to the realization of electron interferometer and anyon braiding. Often, at the p-n junction in the quantum Hall (QH) regime, the presence of a depletion region due to a band gap or the formation of gaps between the zeroth Landau levels (zLL) suppresses interaction between the co-propagating edge channels of opposing doping regimes and helps to preserve the phase coherence of the channels. Here, we observe a new type of p-n junction in hexagonal boron nitride aligned graphene that lacks both the zLL and band gap. In this system, a van Hove singularity (vHS) emerges at the p-n junctions under magnetic fields of several Tesla, owing to the doping inversion near the secondary Dirac point. By fabricating devices with independently tunable global bottom and local top gates, we enable the study of interactions between p-type and n-type QH edge channels through magnetic breakdown associated with the vHS. These findings provide valuable insights into the interactions of superlattice-induced QH edge channels in hBN-aligned graphene.

cond-mat.mes-hall

Local thermodynamic DOS measurement and twist-angle mapping in graphene-hBN superlattices

Moir\'e patterns arising from twisted van der Waals stacks fundamentally reshape their electronic properties, enabling band-structure engineering that has driven rapidly growing interest in this field. In studying electronic properties, however, structural disorder present in real devices often leads to twist-angle inhomogeneity and obscures angle-dependent electronic effects when measured with bulk-averaged measurements. Probes that can access local thermodynamic response of the electronic systems with high sensitivity would be highly valuable. Here, we adopt Kelvin probe force microscopy (KPFM) to locally investigate graphene-hBN superlattices. By additionally modulating the chemical potential of the system, we obtain the inverse compressibility with high signal-to-noise ratio, enabling extraction of the local thermodynamic DOS. From this information, we determine the local twist angle along the device and find that twist-angle deviations are strongly correlated with bubble-induced strain features. Furthermore, by simultaneously tracking the offsets in the contact potential difference and in the net charge, we identify which interface within the heterostructure hosts the trapped bubbles. This capability to identify local electro-chemical environments provides a practical tool for strain-based studies and future device designs utilizing nanoscale engineering in moir\'e systems.

cond-mat.mes-hall

Cryogen-free variable-temperature Kelvin probe force microscopy for probing local chemical potential in a graphene heterostructure

We report the development of a variable-temperature Kelvin probe force microscopy (KPFM) system capable of stable and highly sensitive operation over a wide temperature range based on a GM-cooler-based cryogen-free cryostat. The system incorporates a custom-designed phase-locked loop and automatic gain control, along with passive vibration isolation, enabling precise measurements of local chemical potential even under cryogenic conditions. We demonstrate the performance of this setup by measuring hBN encapsulated monolayer graphene (MLG), revealing spatially resolved electronic inhomogeneities and charge puddles. Our measurements clearly capture temperature-dependent variations in the chemical potential near the charge neutrality point (CNP), consistent with the linear band dispersion of MLG and interaction-driven renormalization of Fermi velocity. This work highlights the robust sensitivity and stability of our system, making it a versatile local probe of quantum phases in van der Waals heterostructures.

physics.app-ph

Interplay of canted antiferromagnetism and nematic order in Mott insulating Sr2Ir1-xRhxO4

Sr2IrO4 is one of the prime candidates for realizing exotic quantum spin orders owing to the subtle combination of spin-orbit coupling and electron correlation. Sensitive local magnetization measurement can serve as a powerful tool to study these kinds of systems with multiple competing spin orders since the comprehensive study of the spatially-varying magnetic responses provide crucial information of their energetics. Here, using sensitive magneto-optical Kerr effect measurements and spin Hamiltonian model calculations, we show that Sr2IrO4 has non-trivial domain structures which cannot be understood by conventional antiferromagnetism. This unconventional magnetic response exhibits broken symmetry along the Ir-O-Ir bond direction and is enhanced upon spin-flip transition or Rh-doping. Our analysis, based on possible stacking patterns of spins, shows that introduction of an additional rotational-symmetry breaking is essential to describe the magnetic behavior of Sr2Ir1-xRhxO4, providing strong evidence for a nematic hidden order phase in this highly correlated spin-orbit Mott insulator.

cond-mat.mtrl-sci

Effect of lattice relaxation on electronic spectra of helically twisted trilayer graphene: Large-scale atomistic simulation approach

Twisted trilayer graphene hosts two moir\'e superlattices originating from two interfaces between graphene layers. However, the system is generally unstable to lattice relaxation at small twist angles and is expected to show a significantly modified electronic band structure. In particular, a helical trilayer graphene - whose two twisted angles have the same sign - provides an attractive platform with a flat band isolated by large energy gaps near the magic angle, but the interplay between the lattice and the electronic degrees of freedom is not well understood. Here, we performed a large-scale molecular dynamics simulation to study the lattice relaxation of helical trilayer graphenes and evaluated their electronic spectra with a tight-binding model calculation. The comparison of the electronic spectra both with and without the lattice relaxation reveals how the lattice relaxation significantly modifies the electronic spectra particularly near the charge neutrality point. We also investigated the local density of states to visualize the spatially-varying electronic spectra that accords with domain patterns of moir\'e lattice stackings. We propose these characteristic spectral features in the electronic degrees of freedom of a relaxed helical trilayer graphene to be confirmed by scanning probe techniques, such as scanning single-electron transistors and scanning tunneling microscopes.

cond-mat.mes-hall

Characterization of a graphene-hBN superlattice field effect transistor

Graphene provides a unique platform for hosting high quality 2D electron systems. Encapsulating graphene with hexagonal boron nitride (hBN) to shield it from noisy environments offers the potential to achieve ultrahigh performance nanodevices, such as photodiodes and transistors. However, the absence of a bandgap at the Dirac point presents challenges for using this system as a useful transistor. In this study, we investigated the functionality of hBN-aligned monolayer graphene as a field effect transistor (FET). By precisely aligning the hBN and graphene, bandgaps open at the first Dirac point and at the hole-doped induced Dirac point via an interfacial moir\'e potential. To characterize this as a submicrometer scale FET, we fabricated a global bottom gate to tune the density of a conducting channel and a local top gate to switch off this channel. This demonstrated that the system could be tuned to an optimal on/off ratio regime by separately controlling the gates. These findings provide a valuable reference point for the further development of FETs based on graphene heterostructures.

cond-mat.mes-hall

Interplay of valley, layer and band topology towards interacting quantum phases in moir\'e bilayer graphene

In Bernal-stacked bilayer graphene (BBG), the Landau levels give rise to an intimate connection between valley and layer degrees of freedom. Adding a moir\'e superlattice potential enriches the BBG physics with the formation of topological minibands - potentially leading to tunable exotic quantum transport. Here, we present magnetotransport measurements of a high-quality bilayer graphene-hexagonal boron nitride (hBN) heterostructure. The zero-degree alignment generates a strong moir\'e superlattice potential for the electrons in BBG and the resulting Landau fan diagram of longitudinal and Hall resistance displays a Hofstadter butterfly pattern with a high level of detail. We demonstrate that the intricate relationship between valley and layer degrees of freedom controls the topology of moir\'e-induced bands, significantly influencing the energetics of interacting quantum phases in the BBG superlattice. We further observe signatures of field-induced correlated insulators, helical edge states and clear quantizations of interaction-driven topological quantum phases, such as symmetry broken Chern insulators.

cond-mat.mes-hall

Quantum spin nematic phase in a square-lattice iridate

Spin nematic (SN) is a magnetic analog of classical liquid crystals, a fourth state of matter exhibiting characteristics of both liquid and solid. Particularly intriguing is a valence-bond SN, in which spins are quantum entangled to form a multi-polar order without breaking time-reversal symmetry, but its unambiguous experimental realization remains elusive. Here, we establish a SN phase in the square-lattice iridate Sr$_2$IrO$_4$, which approximately realizes a pseudospin one-half Heisenberg antiferromagnet (AF) in the strong spin-orbit coupling limit. Upon cooling, the transition into the SN phase at T$_C$ $\approx$ 263 K is marked by a divergence in the static spin quadrupole susceptibility extracted from our Raman spectra, and concomitant emergence of a collective mode associated with the spontaneous breaking of rotational symmetries. The quadrupolar order persists in the antiferromagnetic (AF) phase below T$_N$ $\approx$ 230 K, and becomes directly observable through its interference with the AF order in resonant x-ray diffraction, which allows us to uniquely determine its spatial structure. Further, we find using resonant inelastic x-ray scattering a complete breakdown of coherent magnon excitations at short-wavelength scales, suggesting a resonating-valence-bond-like quantum entanglement in the AF state. Taken together, our results reveal a quantum order underlying the N\'eel AF that is widely believed to be intimately connected to the mechanism of high temperature superconductivity (HTSC).

cond-mat.str-el

Strong interlayer charge transfer due to exciton condensation in an electrically-isolated GaAs quantum well bilayer

We introduce a design of electrically isolated floating bilayer GaAs quantum wells (QW) in which application of a large gating voltage controllably and highly reproducibly induces charges that remain trapped in the bilayer after removal of the gating voltage. At smaller gate voltages, the bilayer is fully electrically isolated from external electrodes by thick insulating barriers. This design permits full control of the total and differential densities of two coupled 2D electron systems. The floating bilayer design provides a unique approach for studying systems inaccessible by simple transport measurements. It also provides the ability to measure the charge transfer between the layers, even when the in-plane resistivities of the 2D systems diverge. We measure the capacitance and inter-layer tunneling spectra of the QW bilayer with independent control of the top and bottom layer electron densities. Our measurements display strongly enhanced inter-layer tunneling current at the total filling factor of 1, a signature of exciton condensation of a strongly interlayer-correlated bilayer system. With fully tunable densities of individual layers, the floating bilayer QW system provides a versatile platform to access previously unavailable information on the quantum phases in electron bilayer systems.

cond-mat.mes-hall

Full Momentum and Energy Resolved Spectral Function of a 2D Electronic System

The single-particle spectral function measures the density of electronic states (DOS) in a material as a function of both momentum and energy, providing central insights into phenomena such as superconductivity and Mott insulators. While scanning tunneling microscopy (STM) and other tunneling methods have provided partial spectral information, until now only angle-resolved photoemission spectroscopy (ARPES) has permitted a comprehensive determination of the spectral function of materials in both momentum and energy. However, ARPES operates only on electronic systems at the material surface and cannot work in the presence of applied magnetic fields. Here, we demonstrate a new method for determining the full momentum and energy resolved electronic spectral function of a two-dimensional (2D) electronic system embedded in a semiconductor. In contrast with ARPES, the technique remains operational in the presence of large externally applied magnetic fields and functions for electronic systems with zero electrical conductivity or with zero electron density. It provides a direct high-resolution and high-fidelity probe of the dispersion and dynamics of the interacting 2D electron system. By ensuring the system of interest remains under equilibrium conditions, we uncover delicate signatures of many-body effects involving electron-phonon interactions, plasmons, polarons, and a novel phonon analog of the vacuum Rabi splitting in atomic systems.

cond-mat.mes-hall

Sharp Tunneling Resonance from the Vibrations of an Electronic Wigner Crystal

Photoemission and tunneling spectroscopies measure the energies at which single electrons can be added to or removed from an electronic system. Features observed in such spectra have revealed electrons coupling to vibrational modes of ions both in solids and in individual molecules. Here we report the discovery of a sharp resonance in the tunneling spectrum of a 2D electron system. Its behavior suggests that it originates from vibrational modes, not involving ionic motion, but instead arising from vibrations of spatial ordering of the electrons themselves. In a two-dimensional electronic system at very low temperatures and high magnetic fields, electrons can either condense into a variety of quantum Hall phases or arrange themselves into a highly ordered Wigner crystal lattice. Such spatially ordered phases of electrons are often electrically insulating and delicate and have proven very challenging to probe with conventional methods. Using a unique pulsed tunneling method capable of probing electron tunneling into insulating phases, we observe a sharp peak with dependencies on energy and other parameters that fit to models for vibrations of a Wigner crystal. The remarkable sharpness of the structure presents strong evidence of the existence of a Wigner crystal with long correlation length.

cond-mat.str-el

Detection of Individual Vortices in Micron-Size Sr2RuO4 Rings by Phase-Locked Cantilever Magnetometry

We describe a feedback-based dynamic cantilever magnetometry technique capable of achieving high magnetic moment sensitivity with low applied fields. Using this technique, we have observed periodic entry of vortices into mesoscopic Sr2RuO4 rings. The quantized jump in the magnetic moment of the particle produced by individual vortices was measured with a resolution of 7x10^-16 e.m.u. at an applied field of 1 Oe.

cond-mat.supr-con