arXiv subjects

Jordan R. Stone

Publications and source records attributed to Jordan R. Stone.

15 recordsLinked to original sources

arXiv2023

Sub-Doppler spectroscopy of quantum systems through nanophotonic spectral translation of electro-optic light

An outstanding challenge for deployable quantum technologies is the availability of high-resolution laser spectroscopy at the specific wavelengths of ultranarrow transitions in atomic and solid-state quantum systems. Here, we demonstrate a powerful spectroscopic tool that synergistically combines high resolution with flexible wavelength access, by showing that nonlinear nanophotonics can be readily pumped with electro-optic frequency combs to enable highly coherent spectral translation with essentially no efficiency loss. Third-order (\c{hi}(3)) optical parametric oscillation in a silicon nitride microring enables nearly a million optical frequency comb pump teeth to be translated onto signal and idler beams; while the comb tooth spacing and bandwidth are adjustable through electro-optic control, the signal and idler carrier frequencies are widely tuneable through dispersion engineering. We then demonstrate the application of these devices to quantum systems, by performing sub-Doppler spectroscopy of the hyperfine transitions of a Cs atomic vapor with our electro-optically-driven Kerr nonlinear light source. The generality, robustness, and agility of this approach as well as its compatibility with photonic integration are expected to lead to its widespread applications in areas such as quantum sensing, telecommunications, and atomic clocks.

physics.optics↗

arXiv2022

Wavelength-Accurate Nonlinear Conversion through Wavenumber Selectivity in Photonic Crystal Resonators

Integrated nonlinear wavelength converters transfer optical energy from lasers or quantum emitters to other useful colors, but chromatic dispersion limits the range of achievable wavelength shifts. Moreover, because of geometric dispersion, fabrication tolerances reduce the accuracy with which devices produce specific target wavelengths. Here, we report nonlinear wavelength converters whose operation is not contingent on dispersion engineering; yet, the output wavelengths are controlled with high accuracy. In our scheme, coherent coupling between counter-propagating waves in a photonic crystal microresonator induces a photonic bandgap that isolates (in dispersion space) specific wavenumbers for nonlinear gain. We first demonstrate the wide applicability of this strategy to parametric nonlinear processes, by simulating its use in third harmonic generation, dispersive wave formation in Kerr microcombs, and four-wave mixing Bragg scattering. In experiments, we demonstrate Kerr optical parametric oscillators in which such wavenumber-selective coherent coupling designates the signal mode. As a result, differences between the targeted and realized signal wavelengths are <0.3 percent. Moreover, leveraging the bandgap-protected wavenumber selectivity, we continuously tune the output frequencies by nearly 300 GHz without compromising efficiency. Our results will bring about a paradigm shift in how microresonators are designed for nonlinear optics, and they make headway on the larger problem of building wavelength-accurate light sources using integrated photonics.

physics.optics↗

arXiv2022

Efficient chip-based optical parametric oscillators from 590 nm to 1150 nm

Optical parametric oscillators are widely used to generate coherent light at frequencies not accessible by conventional laser gain. However, chip-based parametric oscillators operating in the visible spectrum have suffered from pump-to-signal conversion efficiencies typically less than 0.1 %. Here, we demonstrate efficient optical parametric oscillators based on silicon nitride photonics that address frequencies between 260 THz (1150 nm) and 510 THz (590 nm). Pumping silicon nitride microrings near 385 THz (780 nm) yields monochromatic signal and idler waves with unprecedented output powers in this wavelength range. We estimate on-chip output powers (separately for the signal and idler) between 1 mW and 5 mW and conversion efficiencies reaching approximately 15 %. Underlying this improved performance is our development of pulley waveguides for broadband near-critical coupling, which exploits a fundamental connection between the waveguide-resonator coupling rate and conversion efficiency. Finally, we find that mode competition reduces conversion efficiency at high pump powers, thereby constraining the maximum realizable output power. Our work proves that optical parametric oscillators built with integrated photonics can produce useful amounts of visible laser light with high efficiency.

physics.optics↗

arXiv2021

Inverse-designed multi-dimensional silicon photonic transmitters

Modern microelectronic processors have migrated towards parallel computing architectures with many-core processors. However, such expansion comes with diminishing returns exacted by the high cost of data movement between individual processors. The use of optical interconnects has burgeoned as a promising technology that can address the limits of this data transfer. While recent pushes to enhance optical communication have focused on developing wavelength-division multiplexing technology, this approach will eventually saturate the usable bandwidth, and new dimensions of data transfer will be paramount to fulfill the ever-growing need for speed. Here we demonstrate an integrated intra- and inter-chip multi-dimensional communication scheme enabled by photonic inverse design. Using inverse-designed mode-division multiplexers, we combine wavelength- and mode- multiplexing and send massively parallel data through nano-photonic waveguides and optical fibres. Crucially, as we take advantage of an orthogonal optical basis, our approach is inherently scalable to a multiplicative enhancement over the current state of the art.

physics.app-ph↗

arXiv2021

Conversion efficiency in Kerr microresonator optical parametric oscillators: From three modes to many modes

We study optical parametric oscillations in Kerr-nonlinear microresonators, revealing an intricate solution space -- parameterized by the pump-to-signal conversion efficiency -- that arises from an interplay of nonlinear processes. Using a three-mode approximation, we derive an efficiency-maximizing relation between pump power and frequency mismatch. To move beyond a three-mode approximation, a necessity for geometries such as integrated microring resonators, we numerically simulate the Lugiato-Lefever Equation that accounts for the full spectrum of nonlinearly-coupled resonator modes. We observe and characterize two nonlinear phenomena linked to parametric oscillations in multi-mode resonators: Mode competition and cross phase modulation-induced modulation instability. Both processes may impact conversion efficiency. Finally, we show how to increase the conversion efficiency by tuning the microresonator loss rates. Our analysis will guide microresonator designs that aim for high conversion efficiency and output power.

physics.optics↗

arXiv2021

Ultra-Broadband Kerr Microcomb Through Soliton Spectral Translation

Broad bandwidth and stable microresonator frequency combs are critical for accurate and precise optical frequency measurements in a compact and deployable format. Typically, broad bandwidths (e.g., octave spans) are achieved by tailoring the microresonator's geometric dispersion. However, geometric dispersion engineering alone may be insufficient for sustaining bandwidths well beyond an octave. Here, we introduce the novel concept of synthetic dispersion, in which a second pump laser effectively alters the dispersion landscape to create Kerr soliton microcombs that extend far beyond the anomalous geometric dispersion region. Through detailed numerical simulations, we show that the synthetic dispersion model captures the system's key physical behavior, in which the second pump enables non-degenerate four-wave mixing that produces new dispersive waves on both sides of the spectrum. We experimentally demonstrate these concepts by pumping a silicon nitride microring resonator at 1060 nm and 1550 nm to generate a single soliton microcomb whose bandwidth approaches two octaves (137 THz to 407 THz) and whose phase coherence is verified through beat note measurements. Such ultra-broadband microcombs provide new opportunities for full microcomb stabilization in optical frequency synthesis and optical atomic clocks, while the synthetic dispersion concept can extend microcomb operation to wavelengths that are hard to reach solely through geometric dispersion engineering.

physics.optics↗

arXiv2020

Harnessing Dispersion in Soliton Microcombs to Mitigate Thermal Noise

We explore intrinsic thermal noise in soliton microcombs, revealing thermodynamic correlations induced by nonlinearity and group-velocity dispersion. A suitable dispersion design gives rise to control over thermal-noise transduction from the environment to a soliton microcomb. We present simulations with the Lugiato-Lefever equation (LLE), including temperature as a stochastic variable. By systematically tuning the dispersion, we suppress repetition-rate frequency fluctuations by up to 50 decibels for different LLE soliton solutions. In an experiment, we observe a measurement-system-limited 15-decibel reduction in the repetition-rate phase noise for various settings of the pump-laser frequency, and our measurements agree with a thermal-noise model. Finally, we compare two octave-spanning soliton microcombs with similar optical spectra and offset frequencies, but with designed differences in dispersion. Remarkably, their thermal-noise-limited carrier-envelope-offset frequency linewidths are 1 MHz and 100 Hz, which demonstrates an unprecedented potential to mitigate thermal noise. Our results guide future soliton-microcomb design for low-noise applications, and, more generally, they illuminate emergent properties of nonlinear, multi-mode optical systems subject to intrinsic fluctuations.

physics.optics↗

arXiv2020

Generating octave-bandwidth soliton frequency combs with compact, low-power semiconductor lasers

We report a comprehensive study of low-power, octave-bandwidth, single-soliton microresonator frequency combs in both the 1550 nm and 1064 nm bands. Our experiments utilize fully integrated silicon-nitride Kerr microresonators, and we demonstrate direct soliton generation with widely available distributed-Bragg-reflector lasers that provide less than 40 mW of chip-coupled laser power. We report measurements of soliton thermal dynamics and demonstrate how rapid laser-frequency control, consistent with the thermal timescale of a microresonator, facilitates stabilization of octave-bandwidth soliton combs. Moreover, since soliton combs are completely described by fundamental linear and nonlinear dynamics of the intraresonator field, we demonstrate the close connection between modeling and generation of octave-bandwidth combs. Our experiments advance the development of self-referenced frequency combs with integrated-photonics technology, and comb-laser sources with tens of terahertz pulse bandwidth across the near-infrared.

physics.optics↗

arXiv2019

Thermal decoherence and laser cooling of Kerr microresonator solitons

Thermal noise is ubiquitous in microscopic systems and in high-precision measurements. Controlling thermal noise, especially using laser light to apply dissipation, substantially affects science in revealing the quantum regime of gases, in searching for fundamental physics, and in realizing practical applications. Recently, nonlinear light-matter interactions in microresonators have opened up new classes of microscopic devices. A key example is Kerr-microresonator frequency combs; so-called soliton microcombs not only explore nonlinear science but also enable integrated-photonics devices, such as optical synthesizers, optical clocks, and data-communications systems. Here, we explore how thermal noise leads to fundamental decoherence of soliton microcombs. We show that a particle-like soliton exists in a state of thermal equilibrium with its silicon-chip-based resonator. Therefore the soliton microcomb's modal linewidth is thermally broadened. Our experiments utilize record sensitivity in carrier-envelope-offset frequency detection in order to uncover this regime of strong thermal-noise correlations. Furthermore, we have discovered that passive laser cooling of the soliton reduces thermal decoherence to far below the ambient-temperature limit. We implement laser cooling by microresonator photothermal forcing, and we observe cooling of the frequency-comb light to an effective temperature of 84 K. Our work illuminates inherent connections between nonlinear photonics, microscopic physical fluctuations, and precision metrology that could be harnessed for innovative devices and methods to manipulate light.

physics.optics↗

arXiv2018

Direct Kerr-frequency-comb atomic spectroscopy

Microresonator-based soliton frequency combs - microcombs - have recently emerged to offer low-noise, photonic-chip sources for optical measurements. Owing to nonlinear-optical physics, microcombs can be built with various materials and tuned or stabilized with a consistent framework. Some applications require phase stabilization, including optical-frequency synthesis and measurements, optical-frequency division, and optical clocks. Partially stabilized microcombs can also benefit applications, such as oscillators, ranging, dual-comb spectroscopy, wavelength calibration, and optical communications. Broad optical bandwidth, brightness, coherence, and frequency stability have made frequency-comb sources important for studying comb-matter interactions with atoms and molecules. Here, we explore direct microcomb atomic spectroscopy, utilizing a cascaded, two-photon 1529-nm atomic transition of rubidium. Both the microcomb and the atomic vapor are implemented with planar fabrication techniques to support integration. By fine and simultaneous control of the repetition rate and carrier-envelope-offset frequency of the soliton microcomb, we obtain direct sub-Doppler and hyperfine spectroscopy of the $4^2D_{5/2}$ manifold. Moreover, the entire set of microcomb modes are stabilized to this atomic transition, yielding absolute optical-frequency fluctuations of the microcomb at the kilohertz-level over a few seconds and < 1 MHz day-to-day accuracy. Our work demonstrates atomic spectroscopy with microcombs and provides a rubidium-stabilized microcomb laser source, operating across the 1550 nm band for sensing, dimensional metrology, and communication.

physics.optics↗

arXiv2018

A Kerr-microresonator optical clockwork

Kerr microresonators generate interesting and useful fundamental states of electromagnetic radiation through nonlinear interactions of continuous-wave (CW) laser light. Using photonic-integration techniques, functional devices with low noise, small size, low-power consumption, scalable fabrication, and heterogeneous combinations of photonics and electronics can be realized. Kerr solitons, which stably circulate in a Kerr microresonator, have emerged as a source of coherent, ultrafast pulse trains and ultra-broadband optical-frequency combs. Using the f-2f technique, Kerr combs support carrier-envelope-offset phase stabilization for optical synthesis and metrology. In this paper, we introduce a Kerr-microresonator optical clockwork based on optical-frequency division (OFD), which is a powerful technique to transfer the fractional-frequency stability of an optical clock to a lower frequency electronic clock signal. The clockwork presented here is based on a silicon-nitride (Si$_3$N$_4$) microresonator that supports an optical-frequency comb composed of soliton pulses at 1 THz repetition rate. By electro-optic phase modulation of the entire Si$_3$N$_4$ comb, we arbitrarily generate additional CW modes between the Si$_3$N$_4$ comb modes; operationally, this reduces the pulse train repetition frequency and can be used to implement OFD to the microwave domain. Our experiments characterize the residual frequency noise of this Kerr-microresonator clockwork to one part in $10^{17}$, which opens the possibility of using Kerr combs with high performance optical clocks. In addition, the photonic integration and 1 THz resolution of the Si$_3$N$_4$ frequency comb makes it appealing for broadband, low-resolution liquid-phase absorption spectroscopy, which we demonstrate with near infrared measurements of water, lipids, and organic solvents.

physics.optics↗

arXiv2018

Kerr-microresonator solitons from a chirped background

We demonstrate protected single-soliton formation and operation in a Kerr microresonator using a phase-modulated pump laser. Phase modulation gives rise to spatially varying effective loss and detuning parameters, which in turn lead to an operation regime in which multi-soliton degeneracy is lifted and a single soliton is the only observable behavior. Direct excitation of single solitons is indicated by observed reversal of the characteristic 'soliton step.' Phase modulation also enables precise control of the soliton pulse train's properties, and measured dynamics agree closely with simulations. We show that the technique can be extended to high repetition-frequency Kerr solitons through subharmonic phase modulation. These results facilitate straightforward generation and control of Kerr-soliton microcombs for integrated photonics systems.

physics.optics↗

arXiv2017

Kerr-microresonator solitons for accurate carrier-envelope-frequency stabilization

Carrier-envelope phase stabilization of optical pulses enables exquisitely precise measurements by way of direct optical-frequency synthesis, absolute optical-to-microwave phase conversion, and control of ultrafast waveforms. We report such phase stabilization for Kerr-microresonator frequency combs integrated on silicon chips, and verify their fractional-frequency inaccuracy at <3x10-16. Our work introduces an interlocked Kerr-comb configuration comprised of one silicon-nitride and one silica microresonator, which feature nearly harmonic repetition frequencies and can be generated with one laser. These frequency combs support an ultrafast-laser regime with few-optical-cycle, 1-picosecond-period soliton pulses and a total dispersive-wave-enhanced bandwidth of 170 THz, while providing a stable phase-link between the optical and microwave domains. To accommodate low-power and mobile application platforms, our phase-locked frequency-comb system operates with <250 mW of chip-coupled power. Our work establishes Kerr-microresonator combs as a viable technology for applications like optical-atomic timekeeping, optical synthesis, and related directions.

physics.optics↗

arXiv2017

Optical-frequency measurements with a Kerr-microcomb and photonic-chip supercontinuum

Dissipative solitons formed in Kerr microresonators may enable chip-scale frequency combs for precision optical metrology. Here we explore the creation of an octave-spanning, 15-GHz repetition-rate microcomb suitable for both f-2f self-referencing and optical-frequency comparisons across the near infrared. This is achieved through a simple and reliable approach to deterministically generate, and subsequently frequency stabilize, soliton pulse trains in a silica-disk resonator. Efficient silicon-nitride waveguides provide a supercontinuum spanning 700 to 2100 nm, enabling both offset-frequency stabilization and optical-frequency measurements with >100 nW per mode. We demonstrate the stabilized comb by performing a microcomb-mediated comparison of two ultrastable optical-reference cavities.

physics.optics↗

arXiv2016

Stably accessing octave-spanning microresonator frequency combs in the soliton regime

Microresonator frequency combs can be an enabling technology for optical frequency synthesis and timekeeping in low size, weight, and power architectures. Such systems require comb operation in low-noise, phase-coherent states such as solitons, with broad spectral bandwidths (e.g., octave-spanning) for self-referencing to detect the carrier-envelope offset frequency. However, stably accessing such states is complicated by thermo-optic dispersion. For example, in the Si3N4 platform, precisely dispersion-engineered structures can support broadband operation, but microsecond thermal time constants have necessitated fast pump power or frequency control to stabilize the solitons. In contrast, here we consider how broadband soliton states can be accessed with simple pump laser frequency tuning, at a rate much slower than the thermal dynamics. We demonstrate octave-spanning soliton frequency combs in Si3N4 microresonators, including the generation of a multi-soliton state with a pump power near 40 mW and a single-soliton state with a pump power near 120 mW. We also develop a simplified two-step analysis to explain how these states are accessed in a thermally stable way without fast control of the pump laser, and outline the required thermal properties for such operation. Our model agrees with experimental results as well as numerical simulations based on a Lugiato-Lefever equation that incorporates thermo-optic dispersion. Moreover, it also explains an experimental observation that a member of an adjacent mode family on the red-detuned side of the pump mode can mitigate the thermal requirements for accessing soliton states.

physics.optics↗