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Jorgen Randrup

Publications and source records attributed to Jorgen Randrup.

At least 19 recordsLinked to original sources

Correlated fission fragment spin dynamics

This study explores the role of nucleon exchange for the generation of the fission fragment angular momenta. For a number of typical fission cases, samples of 10,000 shape evolutions are generated by Langevin simulation and, subsequently, for each such evolution, the nucleon exchange transport theory previously developed for damped nuclear reactions is used to obtain the development of the fragment spin-spin distribution within the Fokker-Planck transport framework. The characteristic evolution of both parallel and perpendicular spin components is discussed. A common feature is that the rotational modes fall out of equilibrium before scission when the temperature rises rapidly while the concurrent shrinking of the neck suppresses further exchange. A number of fission observables are extracted from the event ensembles: the distribution of the magnitude of the fragment spin and its orientation relative to the fission axis, as well as the correlation between the two spins and the distribution of their opening angle. The dependence of these observables on the mass asymmetry is also examined.

nucl-th

Coupled fission fragment angular momenta

Nuclear fission produces fragments whose spins are coupled to the relative angular motion via angular momentum conservation. It is shown how ensembles of such spins can readily be obtained by either direct microcanonical sampling or by sampling of the associated normal modes of rotation. The resulting distribution of the spin-spin opening angle is illustrated in various three- and two- dimensional scenarios and it is demonstrated how recent mutually conflicting model calculations can be well reproduced with different assumptions about the scission geometry.

nucl-th

Directional-dependence of the event-by-event neutron-$\gamma$ multiplicity correlations in $^{252}$Cf(sf)

We differentiate the event-by-event n-$\gamma$ multiplicity data from \ce{^{252}Cf}(sf) with respect to the energies of the emitted particles as well as their relative angles of emission. We determine that neutron emission enhances $\gamma$-ray emission around $0.7$ and $1.2$ MeV, but the only directional alignment was observed for $E_\gamma \leq 0.7$ MeV and tended to be parallel and antiparallel to neutrons emitted in the same event. The emission of $\gamma$ rays at other energies was determined to be nearly isotropic. The presence of the emission and alignment enhancements is explained by positive correlations between neutron emission and quadrupole $\gamma$-ray emission along rotational bands in the de-exciting fragments. This observation corroborates the hypothesis of positive correlations between the angular momentum of a fragment and its intrinsic excitation energy. The results of this work are especially relevant in view of the recent theoretical and experimental interest in the generation of angular momentum in fission. Specifically, we have determined an alignment of the fragments angular momenta in a direction perpendicular to the direction of motion. We interpret the lack of $n$-$\gamma$ angular correlations for fission fragments near closed shells as a weakening of the alignment process for spherical nuclei. Lastly, we have observed that statistical $\gamma$ rays are emitted isotropically, indicating that the average angular momentum removed by this radiation is small. These results, and the analysis tools presented in this work, represent a stepping stone for future analysis of $n$-$\gamma$ emission correlations and their connection to angular momentum properties.

nucl-ex

Angular Momentum of Fission Fragments from Microscopic Theory

During nuclear fission, a heavy nucleus splits into two rotating fragments. The associated angular momentum is large, yet the mechanism of its generation and its dependence on the mass of fragments remain poorly understood. In this Letter, we provide the first microscopic calculations of angular momentum distributions in fission fragments for a wide range of fragment masses. For the benchmark case of $^{239}$Pu($n_{\text{th}}$,f), we find that the angular momentum of the fragments is largely determined by the nuclear shell structure and deformation, and that the heavy fragments therefore typically carry less angular momentum than their light partners. We use the fission model $\tt{FREYA}$ to simulate the emission of neutrons and photons from the fragments. The dependence of the angular momenta on fragment mass after the emission of neutrons and statistical photons is linear for the heavy fragments and either constant or weakly linear for the light fragments, consistent with the universal sawtooth pattern suggested by recent experimental data. Finally, we observe that using microscopic angular momentum distributions modifies the number of emitted photons significantly.

nucl-th

Future of Nuclear Fission Theory

There has been much recent interest in nuclear fission, due in part to a new appreciation of its relevance to astrophysics, stability of superheavy elements, and fundamental theory of neutrino interactions. At the same time, there have been important developments on a conceptual and computational level for the theory. The promising new theoretical avenues were the subject of a workshop held at the University of York in October 2019; this report summarises its findings and recommendations.

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MeV Gamma Rays from Fission: A Distinct Signature of Actinide Production in Neutron Star Mergers

Neutron star mergers (NSMs) are the first verified sites of rapid neutron capture (r-process) nucleosynthesis, and could emit gamma rays from the radioactive isotopes synthesized in the neutron-rich ejecta. These MeV gamma rays may provide a unique and direct probe of the NSM environment as well as insight into the nature of the r process, just as observed gammas from the 56Ni radioactive decay chain provide a window into supernova nucleosynthesis. In this work, we include the photons from fission processes for the first time in estimates of the MeV gamma-ray signal expected from an NSM event. We consider NSM ejecta compositions with a range of neutron richness and find a dramatic difference in the predicted signal depending on whether or not fissioning nuclei are produced. The difference is most striking at photon energies above ~3.5 MeV and at a relatively late time, several days after the merger event, when the ejecta is optically thin. We estimate that a Galactic NSM could be detectable by a next generation gamma-ray detector such as AMEGO in the MeV range, up to ~10^4 days after the merger, if fissioning nuclei are robustly produced in the event.

astro-ph.HE

Using excitation-energy dependent fission yields to identify key fissioning nuclei in r-process nucleosynthesis

We evaluate the impact of using sets of fission yields given by the GEF code for spontaneous (sf), neutron-induced ((n,f)), and beta-delayed (betadf) fission processes which take into account the approximate initial excitation energy of the fissioning compound nucleus. We further explore energy-dependent fission dynamics in the r process by considering the sensitivity of our results to the treatment of the energy sharing and de-excitation of the fission fragments using the FREYA code. We show that the asymmetric-to-symmetric yield trends predicted by GEF can reproduce the high-mass edge of the second r-process peak seen in solar data and examine the sensitivity of this result to the mass model and astrophysical conditions applied. We consider the effect of fission yields and barrier heights on the nuclear heating rates used to predict kilonova light curves. We find that fission barriers influence the contribution of 254Cf spontaneous fission to the heating at ~100 days, such that a light curve observation consistent with such late-time heating would both confirm that actinides were produced in the event and imply the fission barriers are relatively high along the 254Cf beta-feeding path. We lastly determine the key nuclei responsible for setting the r-process abundance pattern by averaging over thirty trajectories from a 1.2--1.4 M_odot neutron star merger simulation. We show it is largely the odd-N nuclei undergoing (Z,N)(n,f) and (Z,N)betadf that control the relative abundances near the second peak. We find the "hot spots" for beta-delayed and neutron-induced fission given all mass models considered and show most of these nuclei lie between the predicted N=184 shell closure and the location of currently available experimental decay data.

nucl-th

Spinodal density enhancements in simulations of relativistic nuclear collisions

We recently introduced a fluid-dynamical model for simulating relativistic nuclear collisions in the presence of a first-order phase transition and made explorative studies of head-on lead-lead collisions. We give here a more detailed account of this novel theoretical tool and carry out more exhaustive studies of the phase-separation dynamics. Extracting the density enhancement caused by the spinodal instabilities, the associated clump size distribution, and the resulting transverse flow velocity, we examine the sensitivity of these quantities to the strength of the gradient term that promotes the phase separation, to the details of the initial density fluctuations that form the seeds for the subsequent amplification, and to the equation of state.

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Spinodal amplification of density fluctuations in fluid-dynamical simulations of relativistic nuclear collisions

Extending a previously developed two-phase equation of state, we simulate head-on relativistic lead-lead collisions with fluid dynamics, augmented with a finite-range term, and study the effects of the phase structure on the evolution of the baryon density. For collision energies that bring the bulk of the system into the mechanically unstable spinodal region of the phase diagram, the density irregularities are being amplified significantly. The resulting density clumping may be exploited as a signal of the phase transition, possibly through an enhanced production of composite particles.

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The Surface Tension of Quark Matter in a Geometrical Approach

The surface tension of quark matter plays a crucial role for the possibility of quark matter nucleation during the formation of compact stellar objects, because it determines the nucleation rate and the associated critical size. However, this quantity is not well known and the theoretical estimates fall within a wide range, $γ_0 \approx 5-300 MeV/fm^2$. We show here that once the equation of state is available one may use a geometrical approach to obtain a numerical value for the surface tension that is consistent with the model approximations adopted. We illustrate this method within the two-flavor linear σmodel and the Nambu--Jona-Lasinio model with two and three flavors. Treating these models in the mean-field approximation, we find $γ_0 \approx 7-30 MeV/fm^2$. Such a relatively small surface tension would favor the formation of quark stars and may thus have significant astrophysical implications. We also investigate how the surface tension decreases towards zero as the temperature is raised from zero to its critical value.

hep-ph

Brownian shape motion on five-dimensional potential-energy surfaces: Nuclear fission-fragment mass distributions

Although nuclear fission can be understood qualitatively as an evolution of the nuclear shape, a quantitative description has proven to be very elusive. In particular, until now, there exists no model with demonstrated predictive power for the fission fragment mass yields. Exploiting the expected strongly damped character of nuclear dynamics, we treat the nuclear shape evolution in analogy with Brownian motion and perform random walks on five-dimensional fission potential-energy surfaces which were calculated previously and are the most comprehensive available. Test applications give good reproduction of highly variable experimental mass yields. This novel general approach requires only a single new global parameter, namely the critical neck size at which the mass split is frozen in, and the results are remarkably insensitive to its specific value.

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Spinodal phase separation in relativistic nuclear collisions

The spinodal amplification of density fluctuations is treated perturbatively within dissipative fluid dynamics for the purpose of elucidating the prospects for this mechanism to cause a phase separation to occur during a relativistic nuclear collision. The present study includes not only viscosity but also heat conduction (whose effect on the growth rates is of comparable magnitude but opposite), as well as a gradient term in the local pressure, and the corresponding dispersion relation for collective modes in bulk matter is derived from relativistic fluid dynamics. A suitable two-phase equation of state is obtained by interpolation between a hadronic gas and a quark-gluon plasma, while the transport coefficients are approximated by simple parametrizations that are suitable at any degree of net baryon density. We calculate the degree of spinodal amplification occurring along specific dynamical phase trajectories characteristic of nuclear collision at various energies. The results bring out the important fact that the prospects for spinodal phase separation to occur can be greatly enhanced by careful tuning of the collision energy to ensure that the thermodynamic conditions associated with the maximum compression lie inside the region of spinodal instability.

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Phase transition dynamics for baryon-dense matter

We construct a simple two-phase equation of state intended to resemble that of compressed baryon-rich matter and then introduce a gradient term in the compressional energy density to take account of fintie-range effects in non-uniform configurations. With this model we study the interface between the two coexisting phases and obtain estimates for the associated interface tension. Subsequently, we incorporate the finite-range equation of state into ideal or viscous fluid dynamics and derive the collective dispersion relation for the mechanically unstable modes of bulk matter in the spinodal region of the thermodynamic phase diagram. Combining these results with time scales extracted from existing dynamical transport simulations, we discuss the prospects for spinodal phase separation to occur in nuclear collisions. We argue that these can be optimized by a careful tuning of the collision energy to maximize the time spent by the bulk of the system inside the mechanically unstable spinodal region of the phase diagram. Our specific numerical estimates suggest cautious optimism that this phenomenon may in fact occur, though a full dynamical simulation is needed for a detailed assessment.

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Optimal conditions for exploring high-density baryonic matter

Using simple parametrizations of the thermodynamic freeze-out parameters extracted from the data over a wide beam-energy range, we reexpress the hadronic freeze-out line in terms of the underlying dynamical quantities, the net baryon density rhoB and the energy density epsilon, which are subject to local conservation laws. This analysis makes it apparent that rhoB exhibits a maximum as the collision energy is decreased. This maximum freeze-out density has muB=400-500 MeV, which is above the critical value, and it is reached for a fixed-target bombarding energy of 20-30 GeV/A.

hep-ph

Signals of spinodal hadronization: strangeness trapping

If the deconfinement phase transformation of strongly interacting matter is of first-order and the expanding chromodynamic matter created in a high-energy nuclear collision enters the corresponding region of phase coexistence, a spinodal phase separation might occur. The matter would then condense into a number of separate blobs, each having a particular net strangeness that would remain approximately conserved during the further evolution. We investigate the effect that such `strangeness trapping' may have on strangeness-related hadronic observables. The kaon multiplicity fluctuations are significantly enhanced and thus provide a possible tool for probing the nature of the phase transition experimentally.

nucl-th

Signals of spinodal phase decomposition in high-energy nuclear collisions

High-energy nuclear collisions produce quark-gluon plasmas that expand and hadronize. If the associated phase transition is of first order then the hadronization should proceed through a spinodal phase separation. We explore here the possibility of identifying the associated clumping by analysis of suitable N-particle momentum correlations.

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Phi-Meson Production at RHIC, Strong Color Fields and Intrinsic Transverse Momenta

We investigate the effects of strong color fields and of the associated enhanced intrinsic transverse momenta on the phi-meson production in ultrarelativistic heavy ion collisions at RHIC. The observed consequences include a change of the spectral slopes, varying particle ratios, and also modified mean transverse momenta. In particular, the composition of the production processes of phi mesons, that is, direct production vs. coalescence-like production, depends strongly on the strength of the color fields and intrinsic transverse momenta and thus represents a sensitive probe for their measurement.

nucl-th

Spinodal decomposition during the hadronization stage at RHIC?

The expansion of strongly interacting matter formed in high-energy nuclear collisions drives the system through the region of phase coexistence. The present study examines the associated spinodal instability and finds that the degree of amplification may be sufficient to raise the prospect of using the spinodal pattern formation as a diagnostic tool for probing the hadronization phase transition.

hep-ph