arXiv subjects

Joris Van de Vondel

Publications and source records attributed to Joris Van de Vondel.

16 recordsLinked to original sources

arXiv2026

Cryogenic Voltage Control of Magnetism in Silicon-Integrated \newline SrTiO$_3$/Fe Heterostructures

Cryogenic electronics forms a rapidly emerging research domain for high-performance and power-efficient computing applications. Incorporating nanomagnetic components in cryogenic circuitry adds highly valuable functionality, facilitating downscaling, reducing energy consumption and introducing time-reversal symmetry breaking. Furthermore, low-temperature environments enhance magnetic stability and switching efficiency at nanoscale dimensions, reinforcing the potential of cryogenic nanomagnets. To fully leverage these opportunities, magnetic control schemes require alternative options to current-based writing, which is the main bottleneck regarding power consumption and downscaling. In this regard, voltage-based gating of the magnetic state could drastically enhance operational efficiency and integration density. In this work, we investigate cryogenic Voltage Control of Magnetism (VCM) in epitaxial SrTiO$_3$/Fe thin film heterostructures on a CMOS compatible Si substrate. We demonstrate and quantify voltage-controlled modifications of the magnetic domain structure, consistent with electric field-controlled magnetic anisotropy at the Fe/SrTiO$_3$ interface. These findings provide a viable material system for the development of next-generation magnetic domain-based devices for classical and quantum computing.

cond-mat.mes-hall↗

arXiv2026

Engineering Magnetic Anisotropy in Permalloy Films via Atomic Force Nanolithography

Atomic force nanolithography provides a precise method for sculpting magnetic thin films, enabling controlled engineering of magnetic anisotropy in soft ferromagnets at the microscale. We demonstrate that nanoscale groove arrays patterned into permalloy (Ni80Fe20) films induce a robust in-plane uniaxial anisotropy, with the easy axis aligned along the groove direction. The anisotropy field is shown to increase with decreasing groove period and increasing engraving depth, offering continuous tunability of magnetic hardness within a single fabrication step. Artificially engraved microstructures further allow domain configurations and domain-wall trajectories to be directed along predefined pathways, exemplified by the creation of a chessboard-like magnetic landscape. Owing to its adaptability to diverse ferromagnetic materials and arbitrary corrugation geometries, this approach provides a versatile platform for tailoring in-plane magnetic anisotropy. Concrete applications are demonstrated in the design of magnonic elements and anisotropic magnetoresistance sensors.

cond-mat.mtrl-sci↗

arXiv2025

Stoichiometry and Thickness of Epitaxial SrTiO$_{3}$ on Silicon (001): an Investigation of Physical, Optical and Electrical Properties

Strontium titanate (SrTiO$_{3}$, STO) stands out as a promising material for various electronic applications thanks to its exceptional dielectric properties. Molecular beam epitaxy is one of the few techniques which allows epitaxial growth of STO directly on industry-relevant silicon substrates. However, maintaining precise stoichiometry and high crystalline quality in this process remains a significant challenge. Establishing this is essential to obtain STO with bulk-like dielectric properties and to minimize leakage current and optical absorbance. In this study, the importance of cationic stoichiometry and the effect of thickness are investigated for STO thin films epitaxially grown on silicon. We employed real-time reflection high-energy electron diffraction (RHEED) as a feedback loop mechanism to counteract Sr source oxidation and maintain a constant flux. Additionally, high-temperature post-growth annealing treatments in O$_{2}$ were investigated to promote layer relaxation and reduce oxygen vacancy concentration, thereby improving the physical, electrical, and optical properties of stoichiometric STO. As a result, high-quality STO thin films exceeding 100 nm were successfully fabricated featuring a bulk-like out-of-plane lattice parameter and refractive index, as well as rocking curve full width at half maximum below 0.2°, smooth surface (R$_{q}$ < 0.2 nm) and a leakage current density below 1E-7 A/cm$^{2}$.

cond-mat.mtrl-sci↗

arXiv2025

Nonvolatile Cryogenic Phase Slip Memory with Single-Shot Readout

The demand for cryogenic memory components is driven by the need for ultra-fast, low-power, and highly reliable computing systems. Phase slip-based devices promise to fulfill all these requirements, with potential applications in both classical and quantum information processing. However, previous implementations have faced challenges due to inefficient writing and readout schemes. In this work, we address these limitations with a simple device design and measurement techniques inspired by circuit quantum electrodynamics. We present a memory element that stores information in the winding of a high-kinetic inductance superconducting loop, inductively coupled to a coplanar waveguide resonator. Using single-shot measurements, we achieve a readout fidelity of 99.698\% with an active measurement time of just 25 ns.

cond-mat.supr-con↗

arXiv2024

DC-operated Josephson junction arrays as a cryogenic on-chip microwave measurement platform

Providing radio frequency (RF) signals to circuits working in cryogenic conditions requires bulky and expensive transmission cabling interfacing specialized RF electronics anchored at room temperature. Superconducting Josephson junction arrays (JJAs) can change this paradigm by placing the RF source and detector inside the chip. In this work, we demonstrate that DC-biased JJAs can emit signals in the C-band frequency spectrum and beyond. We fabricate reproducible JJAs comprised of amorphous MoGe or NbTiN superconducting islands and metallic Au weak links. Temperature, magnetic fields, applied currents, and device design are explored to control the operation of the RF sources, while we also identify important features that affect the ideal source behavior. Combined with the proven ability of these JJAs to detect microwave radiation, these sources allow us to propose a fully DC-operated cryogenic on-chip measurement platform that is a viable alternative to the high-frequency circuitry currently required for several quantum applications.

cond-mat.supr-con↗

arXiv2024

Non-Invasive Readout of the Kinetic Inductance of Superconducting Nanostructures

The energy landscape of multiply connected superconducting structures is ruled by fluxoid quantization due to the implied single-valuedness of the complex wave function. The transitions and interaction between these energy states, each defined by a specific phase winding number, are governed by classical and/or quantum phase slips. Understanding these events requires the ability to probe, non-invasively, the state of the ring. Here, we employ a niobium resonator to examine the superconducting properties of an aluminum loop. By applying a magnetic field, adjusting temperature, and altering the loop's dimensions via focused ion beam milling, we correlate resonance frequency shifts with changes in the loop's kinetic inductance. This parameter is a unique indicator of the superconducting condensate's state, facilitating the detection of phase slips in nanodevices and providing insights into their dynamics. Our method presents a proof-of-principle spectroscopic technique with promising potential for investigating the Cooper pair density in inductively coupled superconducting nanostructures.

physics.app-ph↗

arXiv2024

Al$_3$Sc thin films for advanced interconnect applications

Al$_x$Sc$_{1-x}$ thin films have been studied with compositions around Al$_3$Sc ($x$ = 0.75) for potential interconnect metallization applications. As-deposited 25 nm thick films were x-ray amorphous but crystallized at 190°C, followed by recrystallization at 440°C. After annealing at 500°C, 24 nm thick stoichiometric Al$_3$Sc showed a resistivity of 12.6 $μΩ$cm, limited by a combination of grain boundary and point defect (disorder) scattering. Together with ab initio calculations that found a mean free path of the charge carriers of 7 nm for stoichiometric Al$_3$Sc, these results indicate that Al$_3$Sc bears promise for future interconnect metallization schemes. Challenges remain in minimizing the formation of secondary phases as well as in the control of the non-stoichiometric surface oxidation and interfacial reactions with underlying dielectrics.

cond-mat.mtrl-sci↗

arXiv2023

Catastrophic magnetic flux avalanches in NbTiN superconducting resonators

Macroscopic superconducting components are an important building block of various quantum circuits. Since several of the envisioned applications require exposure to magnetic fields, it is of utmost importance to explore the impact of magnetic fields on their performance. Here we explore the complex pattern of magnetic field penetration and identify its impact on the resonance frequency of NbTiN superconducting resonators by combining magneto-optical imaging and high-frequency measurements. At temperatures below approximately half of the superconducting critical temperature, the development of magnetic flux avalanches manifests itself as a noisy response in the field-dependent resonance frequency. Magneto-optical imaging reveals different regimes and distinguishes the impact of avalanches in the ground plane and resonator. Our findings demonstrate that superconducting resonators represent a valuable tool to investigate magnetic flux dynamics. Moreover, the current blooming of niobium-based superconducting radio-frequency devices makes this report timely by unveiling the severe implications of magnetic flux dynamics.

cond-mat.supr-con↗

arXiv2022

Nanobridge SQUIDs as multilevel memory elements

With the development of novel computing schemes working at cryogenic temperatures, superconducting memory elements have become essential. In this context, superconducting quantum interference devices (SQUIDs) are promising candidates, as they may trap different discrete amounts of magnetic flux. We demonstrate that a field-assisted writing scheme allows such a device to operate as a multilevel memory by the readout of eight distinct vorticity states at zero magnetic field. We present an alternative mechanism based on single phase slips which allows to switch the vorticity state while preserving superconductivity. This mechanism provides a possibly deterministic channel for flux control in SQUID-based memories, under the condition that the field-dependent energy of different vorticity states are nearby.

cond-mat.supr-con↗

arXiv2022

Metastable states and hidden phase slips in nanobridge SQUIDs

We fabricated an asymmetric nanoscale SQUID consisting of one nanobridge weak link and one Dayem bridge weak link. The current phase relation of these particular weak links is characterized by multivaluedness and linearity. While the latter is responsible for a particular magnetic field dependence of the critical current (so-called vorticity diamonds), the former enables the possibility of different vorticity states (phase winding numbers) existing at one magnetic field value. In experiments the observed critical current value is stochastic in nature, does not necessarily coincide with the current associated with the lowest energy state and critically depends on the measurement conditions. In this work, we unravel the origin of the observed metastability as a result of the phase dynamics happening during the freezing process and while sweeping the current. Moreover, we employ special measurement protocols to prepare the desired vorticity state and identify the (hidden) phase slip dynamics ruling the detected state of these nanodevices. In order to gain insights into the dynamics of the condensate and, more specifically the hidden phase slips, we performed time-dependent Ginzburg-Landau simulations.

cond-mat.supr-con↗

arXiv2018

Restoring self-limited growth of single-layer graphene on copper foil via backside coating

The growth of single-layer graphene (SLG) by chemical vapor deposition (CVD) on copper surfaces is very popular because of the self-limiting effect that prevents the growth of few-layer graphene (FLG). However, the reproducibility of the CVD growth of homogeneous SLG remains a major challenge, especially if one wants to avoid heavy surface treatments, monocrystalline substrates and expensive equipment to control the atmosphere inside the growth system. We demonstrate here that backside tungsten coating of copper foil allows the exclusive growth of SLG with full coverage by atmospheric pressure CVD implemented in a vacuum-free outfit. We show that the absence of FLG patches is related to the absence of decomposition of methane on the backside and consequently to the suppression of C diffusion through copper. In the perspective of large-scale production of graphene, this approach constitutes a significant improvement to the traditional CVD growth process since (1) a tight control of the hydrocarbon flow is no longer required to avoid FLG formation and, consequently, (2) the growth duration necessary to reach full coverage can be dramatically shortened.

cond-mat.mtrl-sci↗

arXiv2018

Determination of the spin-lifetime anisotropy in graphene using oblique spin precession

We determine the spin-lifetime anisotropy of spin-polarized carriers in graphene. In contrast to prior approaches, our method does not require large out-of-plane magnetic fields and thus it is reliable for both low- and high-carrier densities. We first determine the in-plane spin lifetime by conventional spin precession measurements with magnetic fields perpendicular to the graphene plane. Then, to evaluate the out-of-plane spin lifetime, we implement spin precession measurements under oblique magnetic fields that generate an out-of-plane spin population. We find that the spin-lifetime anisotropy of graphene on silicon oxide is independent of carrier density and temperature down to 150 K, and much weaker than previously reported. Indeed, within the experimental uncertainty, the spin relaxation is isotropic. Altogether with the gate dependence of the spin lifetime, this indicates that the spin relaxation is driven by magnetic impurities or random spin-orbit or gauge fields.

cond-mat.mes-hall↗

arXiv2017

Direct visualization of vortex ice in a nanostructured superconductor

Artificial ice systems have unique physical properties promising for potential applications. One of the most challenging issues in this field is to find novel ice systems that allows a precise control over the geometries and many-body interactions. Superconducting vortex matter has been proposed as a very suitable candidate to study artificial ice, mainly due to availability of tunable vortex-vortex interactions and the possibility to fabricate a variety of nanoscale pinning potential geometries. So far, a detailed imaging of the local configurations in a vortex-based artificial ice system is still lacking. Here we present a direct visualization of the vortex ice state in a nanostructured superconductor. By using the scanning Hall probe microscopy, a large area with the vortex ice ground state configuration has been detected, which confirms the recent theoretical predictions for this new ice system. Besides the defects analogous to artificial spin ice systems, other types of defects have been visualized and identified. We also demonstrate the possibility to realize different types of defects by varying the magnetic field.

cond-mat.dis-nn↗

arXiv2017

Stick-slip Phenomena and Memory Effects in Moving Vortex Matter

Manipulating vortices in non-conventional superconductors is nowadays a challenging path toward controlling functionalities for superconducting nanodevices. Here, we directly observe and control single vortex core trajectories with unmatched resolution using a new scanning tunneling spectroscopy at very low temperature. Our data show the depinning threshold of a Bragg-glass in a weakly disordered superconductor, a clean 2H-NbSe2 crystal. We first experimentally capture the linear and collective response, the Campbell regime. Upon strong drives, the oscillating trajectories perform a series of stick-slip motions that mimics the lattice periodicity. We then theoretically elucidate this peculiar non-linear regime by solving the Langevin dynamics equations. We additionally explore the impact of initial conditions and reveal an enhancement of the long-range correlations with the cooling procedure. Finally, our work establishes a connection between theory of vortex pinning, memory effects and vortex lineshapes, thus offering a new platform to investigate the relationship between viscous media and individual controllable objects in any many-body systems.

cond-mat.supr-con↗

arXiv2017

Nanoscale assembly of superconducting vortices with scanning tunnelling microscope tip

Vortices play a crucial role in determining the properties of superconductors as well as their applications. Therefore, characterization and manipulation of vortices, especially at the single vortex level, is of great importance. Among many techniques to study single vortices, scanning tunneling microscopy (STM) stands out as a powerful tool, due to its ability to detect the local electronic states and high spatial resolution. However, local control of superconductivity as well as the manipulation of individual vortices with the STM tip is still lacking. Here we report a new function of the STM, namely to control the local pinning in a superconductor through the heating effect. Such effect allows us to quench the superconducting state at nanoscale, and leads to the growth of vortex-clusters whose size can be controlled by the bias voltage. We also demonstrate the use of an STM tip to assemble single quantum vortices into desired nanoscale configurations.

cond-mat.supr-con↗

arXiv2016

Magnetic Dipoles at Topological Defects in the Meissner State of a Nanostructured Superconductor

In a magnetic field, superconductivity is manifested by total magnetic field expulsion (Meissner effect) or by the penetration of integer multiples of the flux quantum Φ_0. Here we present experimental results revealing magnetic dipoles formed by Meissner current flowing around artificially introduced topological defects (lattice of antidots). By using scanning Hall probe microscopy, we have detected ordered magnetic dipole lattice generated at spatially periodic antidots in a Pb superconducting film. While the conventional homogeneous Meissner state breaks down, the total magnetic flux of the magnetic dipoles remains quantized and is equal to zero. The observed magnetic dipoles strongly depend on the intensity and direction of the locally flowing Meissner current, making the magnetic dipoles an effective way to monitor the local supercurrent. We have also investigated the first step of the vortex depinning process, where, due to the generation of magnetic dipoles, the pinned Abrikosov vortices are deformed and shifted from their original pinning sites.

cond-mat.supr-con↗