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Josep Ingla-Aynés

Publications and source records attributed to Josep Ingla-Aynés.

At least 19 recordsLinked to original sources

Magnetic exchange coupled nonreciprocal devices for cryogenic memory

As computing power demands continue to grow, superconducting electronics present an opportunity to reduce power consumption by increasing the energy efficiency of digital logic and memory. A key milestone for scaling this technology is the development of efficient superconducting memories. Such devices should be nonvolatile, scalable to high integration density and memory capacity, enable fast and low-power reading and writing operations, and be compatible with the digital logic. We present a versatile device platform to develop such nonvolatile memory devices consisting of an exchange-coupled ultra-thin superconductor encapsulated between two ferromagnetic insulators (FIs). The superconducting exchange coupling, which is tuneable by the relative alignment between the FI magnetizations, enables the switching of superconductivity on and off. We exploit this mechanism to create a superconducting nonvolatile memory where single-cell writing is realized using heat-assisted magnetic recording, and explain how it can become a contender for state-of-the-art superconducting memories. Furthermore, below their critical temperatures, the memory elements show a marked nonreciprocity, with zero magnetic field superconducting diode efficiencies exceeding $\pm$60%, showing the versatility of the proposed devices for superconducting computing.

cond-mat.supr-con↗

Tunable Kondo effect in a bilayer graphene quantum channel

The interaction between itinerant electrons and localized spins is key to a wide range of electronic phenomena. Of particular interest is the regime where the interacting electrons exhibit both spin and valley degeneracy, resulting in SU(4) Kondo physics. However, this regime is challenging to realize in typical mesoscopic systems because it requires a strong interaction between electrons, resulting in a Kondo temperature ($T_\mathrm{K}$) significantly larger than the spin and valley splittings. Here, we present conductance measurements of a quantum point contact (QPC) in bilayer graphene (BLG). Beyond the expected quantized conductance plateaus, which reflect spin and valley degeneracy, we observe an additional subband, known as `0.7 anomaly' exhibiting signatures of Kondo physics and a $T_\mathrm{K}$ ranging from approximately 0.5 up to 2.4 K at zero magnetic field, corresponding to Kondo energies between 40 and 200 $μ$eV. Given that the spin-orbit splitting in BLG is between 40 and 80 $μ$eV, we argue that these results are consistent with a transition between four-fold degenerate SU(4) and two-fold degenerate spin-valley locked SU(2) Kondo effects. Furthermore, we break the valley degeneracy of the lowest subband by an out-of-plane magnetic field and show that Kondo signatures remain present, indicating a transition from SU(4) to a valley-polarized SU(2) Kondo effect, and showing the versatility of BLG QPCs for exploring many-body effects.

cond-mat.mes-hall↗

Interplay of energy and charge transfer in WSe2/CrSBr heterostructures

Van der Waals heterostructures (vdWHs) composed of transition-metal dichalcogenides (TMDs) and layered magnetic semiconductors offer great opportunities to manipulate exciton and valley properties of TMDs. Here, we present magneto-photoluminescence (PL) studies in a WSe2 monolayer (ML) on a CrSBr crystal, an anisotropic layered antiferromagnetic semiconductor. Our results reveal unique behavior of each of the ML-WSe2 PL peaks under magnetic field that is distinct from the pristine case. An intriguing feature is the clear enhancement of the PL intensity that we observe each time the external magnetic field tunes the energy of an exciton in CrSBr into resonance with one of the optical states of WSe2. This result suggests a magnetic field-controlled resonant energy transfer (RET) beyond other effects reported in similar structures. Our work provides deep insight on the importance of different mechanisms into magnetic vdWHs and underscores its great potential for light harvesting and emission enhancement of two-dimensional materials.

cond-mat.mtrl-sci↗

Quantum Spin Hall Effect in Magnetic Graphene

A promising approach to attain long-distance coherent spin propagation is accessing topological spin-polarized edge states in graphene. Achieving this without external magnetic fields necessitates engineering graphene band structure, obtainable through proximity effects in van der Waals heterostructures. In particular, proximity-induced staggered potentials and spin-orbit coupling are expected to form a topological bulk gap in graphene with gapless helical edge states that are robust against disorder. In this work, we detect the spin-polarized helical edge transport in graphene at zero external magnetic field, allowed by the proximity of an interlayer antiferromagnet, CrPS$_4$. We show the coexistence of the quantum spin Hall (QSH) states and magnetism in graphene, where the induced spin-orbit and exchange couplings also give rise to a large anomalous Hall (AH) effect. The detection of the QSH states at zero external magnetic field, together with the AH signal that persists up to room temperature, opens the route for practical applications of magnetic graphene in quantum spintronic circuitries.

cond-mat.mes-hall↗

Control of charge-spin interconversion in van der Waals heterostructures with chiral charge density waves

A charge density wave (CDW) represents an exotic state in which electrons are arranged in a long range ordered pattern in low-dimensional materials. Although our understanding of the fundamental character of CDW has been enriched after extensive studies, its relationship with functional phenomena remains relatively limited. Here, we show an unprecedented demonstration of a tunable charge-spin interconversion (CSI) in graphene/1T-TaS$_2$ van der Waals heterostructures by manipulating the distinct CDW phases in 1T-TaS$_2$. Whereas CSI from spins polarized in all three directions are observed in the heterostructure when the CDW phase does not show commensurability, the output of one of the components disappears and the other two are enhanced when the CDW phase becomes commensurate. The experimental observation is supported by first-principles calculations, which evidence that chiral CDW multidomains are at the origin of the switching of CSI. Our results uncover a new approach for on-demand CSI in low-dimensional systems, paving the way for advanced spin-orbitronic devices.

cond-mat.mtrl-sci↗

Highly Efficient Superconducting Diodes and Rectifiers for Quantum Circuitry

Superconducting electronics is essential for energy-efficient quantum and classical high-end computing applications. Towards this goal, non-reciprocal superconducting circuit elements, such as superconducting diodes (SDs) can fulfill many critical needs. SDs have been the subject of multiple studies, but integrating several SDs in a superconducting circuit remains a challenge. Here we implement the first SD bridge with multiple SDs exhibiting reproducible characteristics operating at temperatures of a few Kelvin. We demonstrate its functionality as a full wave rectifier using elemental superconductors and insulating ferromagnets, with efficiency up to 43%, and ac to dc signal conversion capabilities at frequencies up to 40 kHz. Our results show a pathway with a highly scalable thin film platform for nonreciprocal superconducting circuits. They could significantly reduce energy consumption as well as decohering thermal and electromagnetic noise in quantum computing.

cond-mat.supr-con↗

Gate-tunable spin Hall effect in an all-light-element heterostructure: graphene with copper oxide

Graphene is a light material for long-distance spin transport due to its low spin-orbit coupling, which at the same time is the main drawback to exhibit a sizeable spin Hall effect. Decoration by light atoms has been predicted to enhance the spin Hall angle in graphene while retaining a long spin diffusion length. Here, we combine a light metal oxide (oxidized Cu) with graphene to induce the spin Hall effect. Its efficiency, given by the product of the spin Hall angle and the spin diffusion length, can be tuned with the Fermi level position, exhibiting a maximum (1.8 $\pm$ 0.6 nm at 100 K) around the charge neutrality point. This all-light-element heterostructure shows a larger efficiency than conventional spin Hall materials. The gate-tunable spin Hall effect is observed up to room temperature. Our experimental demonstration provides an efficient spin-to-charge conversion system free from heavy metals and compatible with large-scale fabrication.

cond-mat.mes-hall↗

A ballistic electron source with magnetically-controlled valley polarization in bilayer graphene

The achievement of valley-polarized electron currents is a cornerstone for the realization of valleytronic devices. Here, we report on ballistic coherent transport experiments where two opposite quantum point contacts (QPCs) are defined by electrostatic gating in a bilayer graphene (BLG) channel. By steering the ballistic currents with an out-of-plane magnetic field we observe two current jets, a consequence of valley-dependent trigonal warping. Tuning the BLG carrier density and number of QPC modes (m) with a gate voltage we find that the two jets are present for m=1 and up to m=6, indicating the robustness of the effect. Semiclassical simulations which account for size quantization and trigonal warping of the Fermi surface quantitatively reproduce our data without fitting parameters, confirming the origin of the signals. In addition, our model shows that the ballistic currents collected for non-zero magnetic fields are valley-polarized independently of m, but their polarization depends on the magnetic field sign, envisioning such devices as ballistic current sources with tuneable valley-polarization.

cond-mat.mes-hall↗

Out-of-plane spin-to-charge conversion at low temperatures in graphene/MoTe$_2$ heterostructures

Multi-directional spin-to-charge conversion - in which spin polarizations with different orientations can be converted into a charge current in the same direction - has been demonstrated in low-symmetry materials and interfaces. This is possible because, in these systems, spin to charge conversion can occur in unconventional configurations in which spin polarization and charge current where charge current, spin current and polarization do not need to be mutually orthogonal. Here, we explore, in the low temperature regime, the spin-to-charge conversion in heterostructures of graphene with the low-symmetry 1T' phase of MoTe$_2$. First, we observe the emergence of charge conversion for out-of-plane spins at temperatures below 100 K. This unconventional component is allowed by the symmetries of both MoTe$_2$ and graphene and likely arises from spin Hall effect in the spin-orbit proximitized graphene. Moreover, we examine the low-temperature evolution of non-local voltage signals arising from the charge conversion of the two in-plane spin polarizations, which have been previously observed at higher temperature. As a result, we report omni-directional spin-to-charge conversion - for all spin polarization orientations - in graphene/MoTe${_2}$ heterostructures at low temperatures.

cond-mat.mes-hall↗

Specular electron focusing between gate-defined quantum point contacts in bilayer graphene

We report on multiterminal measurements in a ballistic bilayer graphene (BLG) channel where multiple spin and valley-degenerate quantum point contacts (QPCs) are defined by electrostatic gating. By patterning QPCs of different shapes and along different crystallographic directions, we study the effect of size quantization and trigonal warping on the transverse electron focusing (TEF) spectra. Our TEF spectra show eight clear peaks with comparable amplitude and weak signatures of quantum interference at the lowest temperature, indicating that reflections at the gate-defined edges are specular and transport is phase coherent. The temperature dependence of the scattering rate indicates that electron-electron interactions play a dominant role in the charge relaxation process for electron doping and temperatures below 100 K. The achievement of specular reflection, which is expected to preserve the pseudospin information of the electron jets, is promising for the realization of ballistic interconnects for new valleytronic devices.

cond-mat.mes-hall↗

Unconventional charge-to-spin conversions in graphene/MoTe2 van der Waals heterostructures

Spin-charge interconversion (SCI) is a central phenomenon to the development of spintronic devices from materials with strong spin-orbit coupling (SOC). In the case of materials with high crystal symmetry, the only allowed SCI processes are those where the spin current, charge current and spin polarization directions are orthogonal to each other. Consequently, standard SCI experiments are designed to maximize the signals arising from the SCI processes with conventional mutually orthogonal geometry. However, in low-symmetry materials, certain non-orthogonal SCI processes are also allowed. Since the standard SCI experiment is limited to charge current flowing only in one direction in the SOC material, certain allowed SCI configurations remain unexplored. In this work, we performed a thorough SCI study in a graphene-based lateral spin valve combined with low-symmetry MoTe$_2$. Due to a very low contact resistance between the two materials, we could detect SCI signals using both a standard configuration, where the charge current is applied along the MoTe$_2$, and a recently introduced (3D-current) configuration, where the charge current flow can be controlled in three directions within the heterostructure. As a result, we observed three different SCI components, one orthogonal and two non-orthogonal, giving new insight into the SCI processes in low-symmetry materials. The large SCI signals obtained at room temperature, along with the versatility of the 3D-current configuration, provide feasibility and flexibility to the design of the next generation of spin-based devices.

cond-mat.mes-hall↗

Omnidirectional spin-to-charge conversion in graphene/NbSe$_2$ van der Waals heterostructures

The conversion of spin currents polarized in different directions into charge currents is a keystone for novel spintronic devices. Van der Waals heterostructures with tailored symmetry are a very appealing platform for such a goal. Here, by performing nonlocal spin precession experiments, we demonstrate the spin-to-charge conversion (SCC) of spins oriented in all three directions (x, y, and z). By analyzing the magnitude and temperature dependence of the signal in different configurations, we argue that the different SCC components measured are likely due to spin-orbit proximity and broken symmetry at the twisted graphene/NbSe$_2$ interface. Such efficient omnidirectional SCC opens the door to the use of new architectures in spintronic devices, from spin-orbit torques that can switch any magnetization to the magnetic state readout of magnetic elements pointing in any direction.

cond-mat.mes-hall↗

Reliability of spin-to-charge conversion measurements in graphene-based lateral spin valves

Understanding spin physics in graphene is crucial for developing future two-dimensional spintronic devices. Recent studies show that efficient spin-to-charge conversions via either the inverse spin Hall effect or the inverse Rashba-Edelstein effect can be achieved in graphene by proximity with an adjacent spin-orbit coupling material. Lateral spin valve devices, made up of a graphene Hall bar and ferromagnets, are best suited for such studies. Here, we report that signals mimicking the inverse Rashba-Edelstein effect can be measured in pristine graphene possessing negligible spin-orbit coupling, confirming that these signals are unrelated to spin-to-charge conversion. We identify either the anomalous Hall effect in the ferromagnet or the ordinary Hall effect in graphene induced by stray fields as the possible sources of this artefact. By quantitatively comparing these options with finite-element-method simulations, we conclude the latter better explains our results. Our study deepens the understanding of spin-to-charge conversion measurement schemes in graphene, which should be taken into account when designing future experiments.

cond-mat.mes-hall↗

Electrical control of valley-Zeeman spin-orbit coupling-induced spin precession at room temperature

The ultimate goal of spintronics is achieving electrically controlled coherent manipulation of the electron spin at room temperature to enable devices such as spin field-effect transistors. With conventional materials, coherent spin precession has been observed in the ballistic regime and at low temperatures only. However, the strong spin anisotropy and the valley character of the electronic states in 2D materials provide unique control knobs to manipulate spin precession. Here, by manipulating the anisotropic spin-orbit coupling in bilayer graphene by the proximity effect to WSe$_2$, we achieve coherent spin precession in the absence of an external magnetic field, even in the diffusive regime. Remarkably, the sign of the precessing spin polarization can be tuned by a back gate voltage and by a drift current. Our realization of a spin field-effect transistor at room temperature is a cornerstone for the implementation of energy-efficient spin-based logic.

cond-mat.mes-hall↗

Gate tunability of highly efficient spin-to-charge conversion by spin Hall effect in graphene proximitized with WSe$_2$

The proximity effect opens ways to transfer properties from one material into another and is especially important in two-dimensional materials. In van der Waals heterostructures, transition metal dichalcogenides (TMD) can be used to enhance the spin-orbit coupling of graphene leading to the prediction of gate controllable spin-to-charge conversion (SCC). Here, we report for the first time and quantify the SHE in graphene proximitized with WSe$_2$ up to room temperature. Unlike in other graphene/TMD devices, the sole SCC mechanism is the spin Hall effect and no Rashba-Edelstein effect is observed. Importantly, we are able to control the SCC by applying a gate voltage. The SCC shows a high efficiency, measured with an unprecedented SCC length larger than 20 nm. These results show the capability of two-dimensional materials to advance towards the implementation of novel spin-based devices and future applications.

cond-mat.mes-hall↗

Spin Hall Effect in Bilayer Graphene Combined with an Insulator up to Room Temperature

Spin-orbit coupling in graphene can be enhanced by chemical functionalization, adatom decoration or proximity with a van der Waals material. As it is expected that such enhancement gives rise to a sizeable spin Hall effect, a spin-to-charge current conversion phenomenon of technological relevance, it has sparked wide research interest. However, it has only been measured in graphene/transition metal dichalcogenide van der Waals heterostructures with limited scalability. Here, we experimentally demonstrate spin Hall effect up to room temperature in bilayer graphene combined with a nonmagnetic insulator, an evaporated bismuth oxide layer. The measured spin Hall effect raises most likely from an extrinsic mechanism. With a large spin-to-charge conversion efficiency, scalability, and ease of integration to electronic devices, we show a promising material heterostructure suitable for spin-based device applications.

cond-mat.mes-hall↗

Large multi-directional spin-to-charge conversion in low symmetry semimetal MoTe$_2$ at room temperature

Efficient and versatile spin-to-charge current conversion is crucial for the development of spintronic applications, which strongly rely on the ability to electrically generate and detect spin currents. In this context, the spin Hall effect has been widely studied in heavy metals with strong spin-orbit coupling. While the high crystal symmetry in these materials limits the conversion to the orthogonal configuration, unusual configurations are expected in low symmetry transition metal dichalcogenide semimetals, which could add flexibility to the electrical injection and detection of pure spin currents. Here, we report the observation of spin-to-charge conversion in MoTe$_2$ flakes, which are stacked in graphene lateral spin valves. We detect two distinct contributions arising from the conversion of two different spin orientations. In addition to the conventional conversion where the spin polarization is orthogonal to the charge current, we also detect a conversion where the spin polarization and the charge current are parallel. Both contributions, which could arise either from bulk spin Hall effect or surface Edelstein effect, show large efficiencies comparable to the best spin Hall metals and topological insulators. Our finding enables the simultaneous conversion of spin currents with any in-plane spin polarization in one single experimental configuration.

cond-mat.mes-hall↗

Room temperature spin Hall effect in graphene/MoS$_2$ van der Waals heterostructures

Graphene is an excellent material for long distance spin transport but allows little spin manipulation. Transition metal dichalcogenides imprint their strong spin-orbit coupling into graphene via proximity effect, and it has been predicted that efficient spin-to-charge conversion due to spin Hall and Rashba-Edelstein effects could be achieved. Here, by combining Hall probes with ferromagnetic electrodes, we unambiguously demonstrate experimentally spin Hall effect in graphene induced by MoS$_2$ proximity and for varying temperature up to room temperature. The fact that spin transport and spin Hall effect occur in different parts of the same material gives rise to a hitherto unreported efficiency for the spin-to-charge voltage output. Remarkably for a single graphene/MoS$_2$ heterostructure-based device, we evidence a superimposed spin-to-charge current conversion that can be indistinguishably associated with either the proximity-induced Rashba-Edelstein effect in graphene or the spin Hall effect in MoS$_2$. By comparing our results to theoretical calculations, the latter scenario is found the most plausible one. Our findings pave the way towards the combination of spin information transport and spin-to-charge conversion in two-dimensional materials, opening exciting opportunities in a variety of future spintronic applications.

cond-mat.mes-hall↗