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Joseph D. Paulsen

Publications and source records attributed to Joseph D. Paulsen.

At least 19 recordsLinked to original sources

Materializing split, mixed, and three-body interactions using rotor-based mechanical hysterons

Interacting hysteretic spins are an appealing model for cyclically-driven athermal disordered matter. Because they provide a basis for storing and processing information from their environment, such models are also being pursued as a framework for intelligent matter. Recent proof-of-concept designs have begun to demonstrate the strong, controlled, pairwise interactions that are necessary for this endeavor. But, it is not yet clear what are the limits---practically or fundamentally---on such interactions. Here we build rotor-based mechanical hysterons that extend the generality of their interactions in three ways: (i) splitting the interaction strength based on the hysteron state, (ii) building a non-reciprocal interaction of mixed sign, and (iii) incorporating tunable three-body effects. We access these effects within a simple, replicable design platform, and we rationalize our results. Our work expands the space of behaviors for designed structures that compute on mechanical inputs.

cond-mat.soft↗

Mechanical hysterons with tunable interactions of general sign

Hysterons are elementary units of hysteresis that underlie many complex behaviors of non-equilibrium matter. Because models of interacting hysterons can describe disordered matter, this suggests that artificial systems could respond to mechanical inputs in precise and targeted ways. Specifying the properties of hysterons and their interactions could thus be a general method for realizing arbitrary non-equilibrium behaviors. Elastic structures including slender beams, creased sheets, and shells are clear candidates for artificial hysterons, but complete control of their interactions has seemed impractical or impossible. Here we report a mechanical hysteron composed of rigid bars and linear springs, which has controllable properties and tunable interactions of general sign that can be reciprocal or non-reciprocal. We derive a mapping from the system parameters to the hysteron properties, and we show how collective behaviors of multiple hysterons can be targeted by adjusting geometric parameters on the fly. By transforming an abstract hysteron model into a physical design platform, our work demonstrates a route toward designed materials that can sense, compute, and respond to their mechanical environment.

cond-mat.soft↗

Single-material 4D-printed shape-morphing structures via spatially patterned strain trapping

A single-step, single-material 4D printing method is developed for programmable structures featuring spatially patterned strain trapping for one-way actuation. This approach enables fabrication on desktop fused filament fabrication 3D printers through a recently developed shape-memory strain programming method, Programming via Printing (PvP), which eliminates the need for secondary post-fabrication programming. Large (up to 50%) and spatially controlled trapped tensile strain programming is achieved by PvP model design, geometric coding, and printing parameter optimization. While contraction naturally arises from printing-induced trapped strain, expansion is introduced via architected lattice designs with patterned strain-enabling a full range of deformation modes. These capabilities, validated at the unit-cell level, are further integrated into larger proof-of-concept structures to demonstrate scalability and practical implementation. This strategy provides an accessible, low-cost, and easily adoptable additive manufacturing approach for diverse functional-material applications.

cond-mat.soft↗

Learning Associations in Reconfigurable Particle Packings via Local Cyclic Driving

We investigate associative-memory behavior in a reconfigurable particle packing programmed by purely local cyclic driving. The system is a two-dimensional bidisperse Lennard--Jones particle assembly with periodic boundaries evolved under athermal quasistatic relaxation. During training, a fixed set of input particles is driven cyclically while output particles are selected on-the-fly by a region-driving rule and driven according to a prescribed flow pattern; during retrieval, only the inputs are driven. Associative-memory performance is quantified by the cosine similarity between realized and target output displacement directions. Unlike physical learning systems with fixed architecture, learning here arises through emergent weight updates: localized rearrangements modify the contact network and reshape the effective mechanical couplings between inputs and outputs. Across task difficulty we identify three regimes. In an easy setting, the intrinsic mechanical response already produces coherent motion in the right-hand region under input-only driving, yielding high performance without training. In a hard setting, the desired mapping conflicts with the dominant collective drift, resulting in low baseline performance and only modest training gains; introducing intermittent relaxation cycles reduces train--retrieval mismatch and improves performance. In an intermediate quadrupolar task, repositioning the input--output geometry stabilizes the desired response and converts initially stochastic trajectories into reproducible learned motions. Together these results identify minimal physical ingredients for association-based functionality in athermally driven particulate media and motivate an association learning phase diagram for reconfigurable matter.

cond-mat.dis-nn↗

Ordered buckling structures in a twisted crimped tube

When a ribbon or tube is twisted far enough it forms buckles and wrinkles. Its new geometry can be strikingly ordered, or hopelessly disordered. Here we study this process in a tube with hybrid boundary conditions: one end a cylinder, and the other end crimped flat like a ribbon, so that the sample resembles a toothpaste tube. The resulting irregular structures and mechanical responses can be dramatically different from those of a ribbon. However, when we form two creases in the tube prior to twisting, we obtain an ordered structure composed of repeating triangular facets oriented at varying angles, and a more elastic torque response, reminiscent of the creased helicoid structure of a twisted ribbon. We measure how the torque and structural evolution depend on parameters such as material thickness and the twist angle. When only part of the tube is pre-creased, the ordered structures are confined to this segment. Surprisingly, in some tubes made from thicker sheets, an ordered structure forms without pre-creasing. This study provides insights into controlling the buckling of thin shells, offering a potential pathway for designing ordered structures in soft materials.

cond-mat.soft↗

Controlling Droplets at the Tips of Fibers

Many complex wetting behaviors of fibrous materials are rooted in the behaviors of individual droplets attached to pairs of fibers. Here, we study the splitting of a droplet held between the tips of two cylindrical fibers. We discover a sharp transition between two post-rupture states, navigated by changing the angle between the rods, in agreement with our bifurcation analysis. Depinning of the bridge contact line can lead to a much larger asymmetry between the volume of liquid left on each rod. This second scenario enables the near-complete transfer of an aqueous glycerol droplet between two identical vinylpolysiloxane fibers. We leverage this response in a device that uses a ruck to pass a droplet along a train of fibers, a proof-of-concept for the geometric control of droplets on deformable, architected surfaces.

physics.flu-dyn↗

Shape of a membrane on a liquid interface with arbitrary curvatures

We study the deformation of a liquid interface with arbitrary principal curvatures by a flat circular sheet. Working first at small slopes, we determine the shape of the sheet analytically in the membrane limit, where the sheet is inextensible yet free to bend and compress. We find that the sheet takes a cylindrical shape on interfaces with negative Gaussian curvature. On interfaces with positive Gaussian curvature, an inner region still adopts a cylindrical shape while the outer region is under azimuthal compression. Numerical energy minimization confirm our predictions and show that this behavior holds for finite slopes. Experiments on a thin polystyrene film at an anisotropic air-water interface show consistent behaviors.

cond-mat.soft↗

Mechanical memories in solids, from disorder to design

Solids are rigid, which means that when left undisturbed, their structures are nearly static. It follows that these structures depend on history -- but it is surprising that they hold readable memories of past events. Here we review the research that has recently flourished around mechanical memory formation, beginning with amorphous solids' various memories of deformation and mesoscopic models based on particle rearrangements. We describe how these concepts apply to a much wider range of solids and glassy matter -- and how they are a bridge to memory and physical computing in mechanical metamaterials. An understanding of memory in all these solids can potentially be the basis for designing or training functionality into materials. Just as important is memory's value for understanding matter whenever it is complex, frustrated, and out of equilibrium.

cond-mat.soft↗

Exact solutions for the wrinkle patterns of confined elastic shells

Complex textured surfaces occur in nature and industry, from fingerprints to lithography-based micropatterns. Wrinkling by confinement to an incompatible substrate is an attractive way of generating reconfigurable patterned topographies, but controlling the often asymmetric and apparently stochastic wrinkles that result remains an elusive goal. Here, we describe a new approach to understanding the wrinkles of confined elastic shells, using a Lagrange multiplier in place of stress. Our theory reveals a simple set of geometric rules predicting the emergence and layout of orderly wrinkles, and explaining a surprisingly generic co-existence of ordered and disordered wrinkle domains. The results agree with numerous test cases across simulation and experiment and represent an elementary geometric toolkit for designing complex wrinkle patterns.

cond-mat.soft↗

A wrinkled cylindrical shell as a tunable locking material

A buckled sheet offers a reservoir of material that can be unfurled at a later time. For sufficiently thin yet stiff materials, this geometric process has a striking mechanical feature: when the slack runs out, the material locks to further extension. Here we establish a simple route to a tunable locking material - a system with an interval where it is freely deformable under a given deformation mode, and where the endpoints of this interval can be changed continuously over a wide range. We demonstrate this type of mechanical response in a thin cylindrical shell subjected to axial twist and compression, and we rationalize our results with a simple geometric model.

cond-mat.soft↗

Interplay of gross and fine structures in strongly-curved sheets

Although thin films are typically manufactured in planar sheets or rolls, they are often forced into three-dimensional shapes, producing a plethora of structures across multiple length-scales. Existing theoretical approaches have made progress by separating the behaviors at different scales and limiting their scope to one. Under large confinement, a geometric model has been proposed to predict the gross shape of the sheet, which averages out the fine features. However, the actual meaning of the gross shape, and how it constrains the fine features, remains unclear. Here, we study a thin-membraned balloon as a prototypical system that involves a doubly curved gross shape with large amplitude undulations. By probing its profiles and cross sections, we discover that the geometric model captures the mean behavior of the film. We then propose a minimal model for the balloon cross sections, as independent elastic filaments subjected to an effective pinning potential around the mean shape. This approach allows us to combine the global and local features consistently. Despite the simplicity of our model, it reproduces a broad range of phenomena seen in the experiments, from how the morphology changes with pressure to the detailed shape of the wrinkles and folds. Our results establish a new route to understanding finite buckled structures over an enclosed surface, which could aid the design of inflatable structures, or provide insight into biological patterns.

cond-mat.soft↗

Propagating irreversibility fronts in cyclically-sheared suspensions

The interface separating a liquid from its vapor phase is diffuse: the composition varies continuously from one phase to the other over a finite length. Recent experiments on dynamic jamming fronts in two dimensions [Waitukaitis et al., Europhysics Letters 102, 44001 (2013)] identified a diffuse interface between jammed and unjammed discs. In both cases, the thickness of the interface diverges as a critical transition is approached. We investigate the generality of this behavior using a third system: a model of cyclically-sheared non-Brownian suspensions. As we sediment the particles towards a boundary, we observe a diffuse traveling front that marks the interface between irreversible and reversible phases. We argue that the front width is linked to a diverging correlation lengthscale in the bulk, which we probe by studying avalanches near criticality. Our results show how diffuse interfaces may arise generally when an incompressible phase is brought to a critical point.

cond-mat.soft↗

Sculpting liquids with ultrathin shells

Thin elastic films can spontaneously attach to liquid interfaces, offering a platform for tailoring their physical, chemical, and optical properties. Current understanding of the elastocapillarity of thin films is based primarily on studies of planar sheets. We show that curved shells can be used to manipulate interfaces in qualitatively different ways. We elucidate a regime where an ultrathin shell with vanishing bending rigidity imposes its own rest shape on a liquid surface, using experiment and theory. Conceptually, the pressure across the interface "inflates" the shell into its original shape. The setup is amenable to optical applications as the shell is transparent, free of wrinkles, and may be manufactured over a range of curvatures.

cond-mat.soft↗

Multiperiodic orbits from interacting soft spots in cyclically-sheared amorphous solids

When an amorphous solid is deformed cyclically, it may reach a steady state in which the paths of constituent particles trace out closed loops that repeat in each driving cycle. A remarkable variant has been noticed in simulations where the period of particle motions is a multiple of the period of driving, but the reasons for this behavior have remained unclear. Motivated by mesoscopic features of displacement fields in experiments on jammed solids, we propose and analyze a simple model of interacting soft spots -- locations where particles rearrange under stress and that resemble two-level systems with hysteresis. We show that multiperiodic behavior can arise among just three or more soft spots that interact with each other, but in all cases it requires frustrated interactions, illuminating this otherwise elusive type of interaction. We suggest directions for seeking this signature of frustration in experiments and for achieving it in designed systems.

cond-mat.soft↗

Geometry underlies the mechanical stiffening and softening of an indented floating film

A basic paradigm underlying the Hookean mechanics of amorphous, isotropic solids is that small deformations are proportional to the magnitude of external forces. However, slender bodies may undergo large deformations even under minute forces, leading to nonlinear responses rooted in purely geometric effects. Here we study the indentation of a polymer film on a liquid bath. Our experiments and simulations support a recently-predicted stiffening response [Vella & Davidovitch, Phys. Rev. E 98, 013003 (2018)], and we show that the system softens at large slopes, in agreement with our theory that addresses small and large deflections. We show how stiffening and softening emanate from nontrivial yet generic features of the stress and displacement fields.

cond-mat.soft↗

Mesoscale structure of wrinkle patterns and defect-proliferated liquid crystalline phases

Thin solids often develop elastic instabilities and subsequently complex, multiscale deformation patterns. Revealing the organizing principles of this spatial complexity has ramifications for our understanding of morphogenetic processes in plant leaves and animal epithelia, and perhaps even the formation of human fingerprints. We elucidate a primary source of this morphological complexity - an incompatibility between an elastically-favored "micro-structure" of uniformly spaced wrinkles and a "macro-structure" imparted through the wrinkle director and dictated by confinement forces. Our theory is borne out of experiments and simulations of floating sheets subjected to radial stretching. By analyzing patterns of grossly radial wrinkles we find two sharply distinct morphologies: defect-free patterns with a fixed number of wrinkles and non-uniform spacing, and patterns of uniformly spaced wrinkles separated by defect-rich buffer zones. We show how these morphological types reflect distinct minima of a Ginzburg-Landau functional - a coarse-grained version of the elastic energy, which penalizes nonuniform wrinkle spacing and amplitude, as well as deviations of their actual director from the axis imposed by confinement. Our results extend the effective description of wrinkle patterns as liquid crystals (H. Aharoni et al., Nat. Commun. 8:15809, 2017), and we highlight a fascinating analogy between the geometry-energy interplay that underlies the proliferation of defects in the mechanical equilibrium of confined sheets and in thermodynamic phases of superconductors and chiral liquid crystals.

cond-mat.soft↗

Crumples as a generic stress-focusing instability in confined sheets

Thin elastic solids are easily deformed into a myriad of three-dimensional shapes, which may contain sharp localized structures as in a crumpled candy wrapper, or have smooth and diffuse features like the undulating edge of a flower. Anticipating and controlling these morphologies is crucial to a variety of applications involving textiles, synthetic skins, and inflatable structures. Here we show that a "wrinkle-to-crumple" transition, previously observed in specific settings, is a ubiquitous response for confined sheets. This unified picture is borne out of a suite of model experiments on polymer films confined to liquid interfaces with spherical, hyperbolic, and cylindrical geometries, which are complemented by experiments on macroscopic membranes inflated with gas. We use measurements across this wide range of geometries, boundary conditions, and lengthscales to quantify several robust morphological features of the crumpled phase, and we build an empirical phase diagram for crumple formation that disentangles the competing effects of curvature and compression. Our results suggest that crumples are a generic microstructure that emerge at large curvatures due to a competition of elastic and substrate energies.

cond-mat.soft↗

Memory formation in matter

Memory formation in matter is a theme of broad intellectual relevance; it sits at the interdisciplinary crossroads of physics, biology, chemistry, and computer science. Memory connotes the ability to encode, access, and erase signatures of past history in the state of a system. Once the system has completely relaxed to thermal equilibrium, it is no longer able to recall aspects of its evolution. Memory of initial conditions or previous training protocols will be lost. Thus many forms of memory are intrinsically tied to far-from-equilibrium behavior and to transient response to a perturbation. This general behavior arises in diverse contexts in condensed matter physics and materials: phase change memory, shape memory, echoes, memory effects in glasses, return-point memory in disordered magnets, as well as related contexts in computer science. Yet, as opposed to the situation in biology, there is currently no common categorization and description of the memory behavior that appears to be prevalent throughout condensed-matter systems. Here we focus on material memories. We will describe the basic phenomenology of a few of the known behaviors that can be understood as constituting a memory. We hope that this will be a guide towards developing the unifying conceptual underpinnings for a broad understanding of memory effects that appear in materials.

cond-mat.soft↗