arXiv subjects

Joseph H. D. Munns

Publications and source records attributed to Joseph H. D. Munns.

6 recordsLinked to original sources

arXiv2026

Optical probing of phononic properties of a tin-vacancy color center in diamond

The coherence characteristics of a tin-vacancy color center (SnV) in diamond are investigated through optical means, including linewidth broadening effects and coherent population trapping (CPT) between the ground state orbital levels. Spectral analysis is required as due to the large spin-orbit splitting of the orbital ground states, thermalization between the ground states occurs at rates that are impractical to measure directly in the time domain. First, by implementing a temperature-dependent linewidth broadening measurement, including the challenging-to-measure D transition, phononic coupling coefficients are determined. These measurements are performed on an emitter with a lifetime-limited linewidth and atom-like properties, making the measurement representative for high-quality SnVs. Next, a CPT-type experiment is carried out to independently analyze thermal decoherence processes at 4 K. The spectral information is transformed into its conjugate variable time, providing picosecond resolution and revealing an orbital depolarization timescale of ${\sim30{\rm~ps}}$. Consequences of the investigated dynamics are then used to estimate spin dephasing times limited by thermal effects.

quant-ph↗

arXiv2026

SUPER and femtosecond spin-conserving coherent excitation of a tin-vacancy color center in diamond

The coherent excitation of an optically active spin system is one of the key elements in the engineering of a spin-photon interface. Using the novel SUPER scheme, we coherently control the main optical transition of a tin-vacancy color center in diamond with nonresonant ultrashort optical pulses. Furthermore, we implement a femtosecond control scheme using resonant pulses for achieving record short quantum gates applied to diamond color centers. We simulate the applicability of the SUPER scheme to spin qubits and experimentally investigate spin mixing. Finally, we propose a spin-spin entanglement scheme in a scenario where the excitation with broadband pulses is incompatible with spin-selective excitation. The employed ultrafast quantum gates open up a new regime of quantum control with solid-state color centers, enabling multi-gate operations and efficient spectral filtering of the excitation laser from deterministically prepared coherent photons.

quant-ph↗

arXiv2025

Quantum Electrometer for Time-Resolved Material Science at the Atomic Lattice Scale

The detection of individual charges plays a crucial role in fundamental material science and the advancement of classical and quantum high-performance technologies that operate with low noise. However, resolving charges at the lattice scale in a time-resolved manner has not been achieved so far. Here, we present the development of an electrometer with 60 ns acquisition steps, leveraging on the spectroscopy of an optically-active spin defect embedded in a solid-state material with a non-linear Stark response. By applying our approach to diamond, a widely used platform for quantum technology applications, we can distinguish the distinct charge traps at the lattice scale, quantify their impact on transport dynamics and noise generation, analyze relevant material properties, and develop strategies for material optimization.

physics.app-ph↗

arXiv2023

Deterministic Creation of Large Photonic Multipartite Entangled States with Group-IV Color Centers in Diamond

Measurement-based quantum computation relies on single qubit measurements of large multipartite entangled states, so-called lattice-graph or cluster states. Graph states are also an important resource for quantum communication, where tree cluster states are a key resource for one-way quantum repeaters. A photonic realization of this kind of state would inherit many of the benefits of photonic platforms, such as very little dephasing due to weak environmental interactions and the well-developed infrastructure to route and measure photonic qubits. In this work, a linear cluster state and GHZ state generation scheme is developed for group-IV color centers. In particular, this article focuses on an in-depth investigation of the required control operations, including the coherent spin and excitation gates. We choose an off-resonant Raman scheme for the spin gates, which can be much faster than microwave control. We do not rely on a reduced level scheme and use efficient approximations to design high-fidelity Raman gates. We benchmark the spin-control and excitation scheme using the tin vacancy color center coupled to a cavity, assuming a realistic experimental setting. Additionally, the article investigates the fidelities of the Raman and excitation gates in the presence of radiative and non-radiative decay mechanisms. Finally, a quality measure is devised, which emphasizes the importance of fast and high-fidelity spin gates in the creation of large entangled photonic states.

quant-ph↗

arXiv2021

Optimized diamond inverted nanocones for enhanced color center to fiber coupling

Nanostructures can be used for boosting the light outcoupling of color centers in diamond; however, the fiber coupling performance of these nanostructures is rarely investigated. Here, we use a finite element method for computing the emission from color centers in inverted nanocones and the overlap of this emission with the propagation mode in a single-mode fiber. Using different figures of merit, the inverted nanocone parameters are optimized to obtain maximal fiber coupling efficiency, free-space collection efficiency, or rate enhancement. The optimized inverted nanocone designs show promising results with 66% fiber coupling or 83% free-space coupling efficiency at the tin-vacancy center zero-phonon line wavelength of 619 nm. Moreover, when evaluated for broadband performance, the optimized designs show 55% and 76% for fiber coupling and free-space efficiencies respectively, for collecting the full tin-vacancy emission spectrum at room temperature. An analysis of fabrication insensitivity indicates that these nanostructures are robust against imperfections. For maximum emission rate into a fiber mode, a design with a Purcell factor of 2.34 is identified. Finally, possible improvements offered by a hybrid inverted nanocone, formed by patterning into two different materials, are investigated, and increases the achievable fiber coupling efficiency to 71%.

quant-ph↗

arXiv2019

Raman Quantum Memory with Built-In Suppression of Four-wave Mixing Noise

Quantum memories are essential for large-scale quantum information networks. Along with high efficiency, storage lifetime and optical bandwidth, it is critical that the memory add negligible noise to the recalled signal. A common source of noise in optical quantum memories is spontaneous four-wave mixing. We develop and implement a technically simple scheme to suppress this noise mechanism by means of quantum interference. Using this scheme with a Raman memory in warm atomic vapour we demonstrate over an order of magnitude improvement in noise performance. Furthermore we demonstrate a method to quantify the remaining noise contributions and present a route to enable further noise suppression. Our scheme opens the way to quantum demonstrations using a broadband memory, significantly advancing the search for scalable quantum photonic networks.

quant-ph↗