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Joshua E. S. Socolar

Publications and source records attributed to Joshua E. S. Socolar.

At least 19 recordsLinked to original sources

Quasicrystalline structure of the Smith monotile tilings

Tiling models can reveal unexpected ways in which local constraints give rise to exotic long-range spatial structure. The recently discovered Hat monotile (and its mirror image) has been shown to be aperiodic~[Smith et al., arXiv:2303.10798 (2023)]; it can tile the plane with no holes or overlaps, but cannot do so periodically. We show that the structure enforced by the local space-filling constraints is quasiperiodic with hexagonal (C6) rotational symmetry. Although this symmetry is compatible with periodicity, the incommensurate ratio characterizing the quasiperiodicity stays locked to the golden mean as the tile parameters are continuously varied. We analyze a modification of the metatiles introduced by Smith et al. that yields a set of ``Key tiles'' that can be constructed as projections of a subset of six-dimensional hypercubic lattice points onto the two-dimensional tiling plane. We analytically compute the diffraction pattern of a set of unit masses placed at the tiling vertices, establishing the quasiperiodic nature of the tiling. We point out several unusual features of the family of Key tilings and associated Hat tilings, including the tile rearrangements associated with the phason degree of freedom associated with incommensurate density waves, which exhibit novel features that may influence the elastic properties of a material in which atoms or larger particles spontaneously exhibit the symmetries of the Hat tiling.

cond-mat.mtrl-sci↗

Microscopic Reversibility and Emergent Elasticity in Ultrastable Granular Systems

In a recent paper [Phys. Rev. X 12, 031021], we reported experimental observations of ``ultrastable'' states in a shear-jammed granular system subjected to small-amplitude cyclic shear. In such states, all the particle positions and contact forces are reproduced after each shear cycle so that a strobed image of the stresses and particle positions appears static. In the present work, we report further analyses of data from those experiments to characterize both global and local responses of ultrastable states within a shear cycle, not just the strobed dynamics. We find that ultrastable states follow a power-law relation between shear modulus and pressure with an exponent $β\approx 0.5$, reminiscent of critical scaling laws near jamming. We also examine the evolution of contact forces measured using photoelasticimetry. We find that there are two types of contacts: non-persistent contacts that reversibly open and close; and persistent contacts that never open \yiqiu{and display no measurable sliding}. We show that the non-persistent contacts make a non-negligible contribution to the emergent shear modulus. We also analyze the spatial correlations of the stress tensor and compare them to the predictions of a recent theory of the emergent elasticity of granular solids, the Vector Charge Theory of Granular mechanics and dynamics (VCTG) [Phys. Rev. Lett. 125, 118002, arXiv:2204.11811]. We show that our experimental results can be fit well by VCTG, assuming uniaxial symmetry of the contact networks. The fits reveal that the response of the ultrastable states to additional applied stress is substantially more isotropic than that of the original shear-jammed states. Our results provide important insight into the mechanical properties of frictional granular solids created by shear.

cond-mat.soft↗

Ultra-stable shear jammed granular material

Dry granular materials such as sand, gravel, pills, or agricultural grains, can become rigid when compressed or sheared. At low density, one can distort the shape of a container of granular material without encountering any resistance. Under isotropic compression, the material will reach a certain {\it jamming} density and then resist further compression. {\em Shear jamming} occurs when resistance to shear emerges in a system at a density lower than the jamming density, and the elastic properties of such states have important implications for industrial and geophysical processes. We report on experimental observations of changes in the mechanical properties of a shear-jammed granular material subjected to small-amplitude, quasi-static cyclic shear. We study a layer of plastic discs confined to a shear cell, using photoelasticimetry to measure all inter-particle vector forces. For sufficiently small cyclic shear amplitudes and large enough initial shear, the material evolves to an unexpected "ultra-stable" state in which all the particle positions and inter-particle contact forces remain unchanged after each complete shear cycle for thousands of cycles. The stress response of these states to small imposed shear is nearly elastic, in contrast to the original shear jammed state.

cond-mat.soft↗

Random logic networks: from classical Boolean to quantum dynamics

We investigate dynamical properties of a quantum generalization of classical reversible Boolean networks. The state of each node is encoded as a single qubit, and classical Boolean logic operations are supplemented by controlled bit-flip and Hadamard operations. We consider synchronous updating schemes in which each qubit is updated at each step based on stored values of the qubits from the previous step. We investigate the periodic or quasiperiodic behavior of quantum networks, and we analyze the propagation of single site perturbations through the quantum networks with input degree one. A non-classical mechanism for perturbation propagation leads to substantially different evolution of the Hamming distance between the original and perturbed states.

quant-ph↗

Stress propagation in locally loaded packings of disks and pentagons

The mechanical strength and flow of granular materials can depend strongly on the shapes of individual grains. We report quantitative results obtained from photoelasticimetry experiments on locally loaded, quasi-two-dimensional granular packings of either disks or pentagons exhibiting stick-slip dynamics. Packings of pentagons resist the intruder at significantly lower packing fractions than packings of disks, transmitting stresses from the intruder to the boundaries over a smaller spatial extent. Moreover, packings of pentagons feature significantly fewer back-bending force chains than packings of disks. Data obtained on the forward spatial extent of stresses and back-bending force chains collapse when the packing fraction is rescaled according to the packing fraction of steady state open channel formation, though data on intruder forces and dynamics do not collapse. We comment on the influence of system size on these findings and highlight connections with the dynamics of the disks and pentagons during slip events.

cond-mat.soft↗

Two approaches to quantification of force networks in particulate systems

The interactions between particles in particulate systems are organized in `force networks', mesoscale features that bridge between the particle scale and the scale of the system as a whole. While such networks are known to be crucial in determining the system wide response, extracting their properties, particularly from experimental systems, is difficult due to the need to measure the interparticle forces. In this work, we show by analysis of the data extracted from simulations that such detailed information about interparticle forces may not be necessary, as long as the focus is on extracting the most dominant features of these networks. The main finding is that a reasonable understanding of the time evolution of force networks can be obtained from incomplete information such as total force on the particles. To compare the evolution of the networks based on the completely known particle interactions and the networks based on incomplete information (total force each grain) we use tools of algebraic topology. In particular we will compare simple measures defined on persistence diagrams that provide useful summaries of the force network features.

cond-mat.soft↗

Yielding, Rigidity, and Tensile Stress in Sheared Columns of Hexapod Granules

Granular packings of non-convex or elongated particles can form free-standing structures like walls or arches. For some particle shapes, such as staples, the rigidity arises from interlocking of pairs of particles, but the origins of rigidity for non-interlocking particles remains unclear. We report on experiments and numerical simulations of sheared columns of "hexapods," particles consisting of three mutually orthogonal sphero-cylinders whose centers coincide. We vary the length-to-diameter aspect ratio, $α$, of the sphero-cylinders and subject the packings to quasistatic direct shear. For small $α$, we observe a finite yield stress. For large $α$, however, the column becomes rigid when sheared, supporting stresses that increase sharply with increasing strain. Analysis of X-ray micro-computed tomography (Micro-CT) data collected during the shear reveals that the stiffening is associated with a tilted, oblate cluster of hexapods near the nominal shear plane in which particle deformation and average contact number both increase. Simulation results show that the particles are collectively under tension along one direction even though they do not interlock pairwise. These tensions comes from contact forces carrying large torques, and they are perpendicular to the compressive stresses in the packing. They counteract the tendency to dilate, thus stabilize the particle cluster.

cond-mat.soft↗

Intruder in a two-dimensional granular system: Effects of dynamic and static basal friction on stick-slip and clogging dynamics

We discuss the results of simulations of an intruder pulled through a two-dimensional granular system by a spring, using a model designed to lend insight into the experimental findings described by Kozlowski et al. [Phys. Rev. E, 100, 032905 (2019)]. In that previous study the presence of basal friction between the grains and the base was observed to change the intruder dynamics from clogging to stick-slip. Here we first show that our simulation results are in excellent agreement with the experimental data for a variety of experimentally accessible friction coefficients governing interactions of particles with each other and with boundaries. Then, we use simulations to explore a broader range of parameter space, focusing on the friction between the particles and the base. We consider a range of both static and dynamic basal friction coefficients, which are difficult to vary smoothly in experiments. The simulations show that dynamic friction strongly affects the stick-slip behaviour when the coefficient is decreased below 0.1, while static friction plays only a marginal role in the intruder dynamics.

cond-mat.soft↗

Dynamics of a grain-scale intruder in a two-dimensional granular medium with and without basal friction

We report on a series of experiments in which a grain-sized intruder is pushed by a spring through a 2D granular material comprised of photoelastic disks in a Couette geometry. We study the intruder dynamics as a function of packing fraction for two types of supporting substrates: a frictional glass plate and a layer of water for which basal friction forces are negligible. We observe two dynamical regimes: intermittent flow, in which the intruder moves freely most of the time but occasionally gets stuck, and stick-slip dynamics, in which the intruder advances via a sequence of distinct, rapid events. When basal friction is present, we observe a smooth crossover between the two regimes as a function of packing fraction, and we find that reducing the interparticle friction coefficient causes the stick-slip regime to shift to higher packing fractions. When basal friction is eliminated, we observe intermittent flow at all accessible packing fractions. For all cases, we present results for the statistics of stick events, the intruder velocity, and the force exerted on the intruder by the grains. Our results indicate the qualitative importance of basal friction at high packing fractions and suggest a possible connection between intruder dynamics in a static material and clogging dynamics in granular flows.

cond-mat.soft↗

Shear jammed, fragile, and steady states in homogeneously strained granular materials

We study the jamming phase diagram of sheared granular material using a novel Couette shear set-up with multi-ring bottom. The set-up uses small basal friction forces to apply a volume-conserving linear shear with no shear band to a granular system composed of frictional photoelastic discs. The set-up can generate arbitrarily large shear strain due to its circular geometry, and the shear direction can be reversed, allowing us to measure a feature that distinguishes shear-jammed from fragile states. We report systematic measurements of the stress, strain and contact network structure at phase boundaries that have been difficult to access by traditional experimental techniques, including the yield stress curve and the jamming curve close to $ϕ_{SJ}\approx 0.74$, the smallest packing fraction supporting a shear-jammed state. We observe fragile states created under large shear strain over a range of $ϕ< ϕ_{SJ}$. We also find a transition in the character of the quasi-static steady flow centered around $ϕ_{SJ}$ on the yield curve as a function of packing fraction. Near $ϕ_{SJ}$, the average contact number, fabric anisotropy, and non-rattler fraction all show a change of slope. Above $ϕ_{F}\approx 0.7$ the steady flow shows measurable deviations from the basal linear shear profile, and above $ϕ_c\approx 0.78$ the flow is localized in a shear band.

cond-mat.soft↗

Jamming transition in non-spherical particle systems: pentagons vs. disks

We investigate the jamming transition in a quasi-2D granular material composed of regular pentagons or disks subjected to quasistatic uniaxial compression. We report six major findings based on experiments with monodisperse photoelastic particles with static friction coefficient $μ\approx 1$. (1) For both pentagons and disks, the onset of rigidity occurs when the average coordination number of non-rattlers, $Z_{nr}$ , reaches 3, and the dependence of $Z_{nr}$ on the packing fraction $ϕ$ changes again when $Z_{nr}$ reaches 4. (2) Though the packing fractions $ϕ_{c1}$ and $ϕ_{c2}$ at these transitions differ from run to run, for both shapes the data from all runs with different initial configurations collapses when plotted as a function of the non-rattler fraction. (3) The averaged values of $ϕ_{c1}$ and $ϕ_{c2}$ for pentagons are around 1% smaller than those for disks. (4) Both jammed pentagons and disks show Gamma distribution of the Voronoi cell area with same parameters. (5) The jammed pentagons have similar translational order for particle centers but slightly less orientational order for contacting pairs comparing to jammed disks. (6) For jammed pentagons, the angle between edges at a face-to-vertex contact point shows a uniform distribution and the size of a cluster connected by face-to-face contacts shows a power-law distribution.

cond-mat.soft↗

Hyperuniformity and anti-hyperuniformity in one-dimensional substitution tilings

We consider the scaling properties characterizing the hyperuniformity (or anti-hyperuniformity) of long wavelength fluctuations in a broad class of one-dimensional substitution tilings. We present a simple argument that predicts the exponent $α$ governing the scaling of Fourier intensities at small wavenumbers, tilings with $α>0$ being hyperuniform, and confirm with numerical computations that the predictions are accurate for quasiperiodic tilings, tilings with singular continuous spectra, and limit-periodic tilings. Tilings with quasiperiodic or singular continuous spectra can be constructed with $α$ arbitrarily close to any given value between $-1$ and $3$. Limit-periodic tilings can be constructed with $α$ between $-1$ and $1$ or with Fourier intensities that approach zero faster than any power law.

cond-mat.stat-mech↗

Phase diagram and aggregation dynamics of a monolayer of paramagnetic colloids

We have developed a tunable colloidal system and a corresponding simulation model for studying the phase behavior of particles assembling under the influence of long-range magnetic interactions. A monolayer of paramagnetic particles is subjected to a spatially uniform magnetic field with a static perpendicular component and rapidly rotating in-plane component. The sign and strength of the interactions vary with the tilt angle $θ$ of the rotating magnetic field. For a purely in-plane field, $θ=90^{\circ}$, interactions are attractive and the experimental results agree well with both equilibrium and out-of-equilibrium predictions based on a two-body interaction model. For tilt angles $50^{\circ}\lesssim θ\lesssim 55^{\circ}$, the two-body interaction gives a short-range attractive and long-range repulsive (SALR) interaction, which predicts the formation of equilibrium microphases. In experiments, however, a different type of assembly is observed. Inclusion of three-body (and higher-order) terms in the model does not resolve the discrepancy. We thus further characterize the anomalous behavior by measuring the time-dependent cluster size distribution.

cond-mat.soft↗

Hyperuniformity of Quasicrystals

Hyperuniform systems, which include crystals, quasicrystals and special disordered systems, have attracted considerable recent attention, but rigorous analyses of the hyperuniformity of quasicrystals have been lacking because the support of the spectral intensity is dense and discontinuous. We employ the integrated spectral intensity, $Z(k)$, to quantitatively characterize the hyperuniformity of quasicrystalline point sets generated by projection methods. The scaling of $Z(k)$ as $k$ tends to zero is computed for one-dimensional quasicrystals and shown to be consistent with independent calculations of the variance, $σ^2(R)$, in the number of points contained in an interval of length $2R$. We find that one-dimensional quasicrystals produced by projection from a two-dimensional lattice onto a line of slope $1/τ$ fall into distinct classes determined by the width of the projection window. For a countable dense set of widths, $Z(k) \sim k^4$; for all others, $Z(k)\sim k^2$. This distinction suggests that measures of hyperuniformity define new classes of quasicrystals in higher dimensions as well.

cond-mat.stat-mech↗

Mechanical Graphene

We present a model of a mechanical system with a vibrational mode spectrum identical to the spectrum of electronic excitations in a tight-binding model of graphene. The model consists of point masses connected by elastic couplings, called "tri-bonds," that implement certain three-body interactions, which can be tuned by varying parameters that correspond to the relative hopping amplitudes on the different bond directions in graphene. In the mechanical model, this is accomplished by varying the location of a pivot point that determines the allowed rigid rotations of a single tri-bond. The infinite system constitutes a Maxwell lattice, with the number of degrees of freedom equal to the number of constraints imposed by the tri-bonds. We construct the equilibrium and compatibility matrices and analyze the model's phase diagram, which includes spectra with Weyl points for some placements of the pivot and topologically polarized phases for others. We then discuss the edge modes and associated states of self stress for strips cut from the periodic lattice. Finally, we suggest a physical realization of the tri-bond, which allows access to parameter regimes not available to experiments on (strained) graphene and may be used to create other two-dimensional mechanical metamaterials with different spectral features.

cond-mat.soft↗

Local growth of icosahedral quasicrystalline tilings

Icosahedral quasicrystals (IQCs) with extremely high degrees of translational order have been produced in the laboratory and found in naturally occurring minerals, yet questions remain about how IQCs form. In particular, the fundamental question of how locally determined additions to a growing cluster can lead to the intricate long-range correlations in IQCs remains open. In answer to this question, we have developed an algorithm that is capable of producing a perfectly ordered IQC, yet relies exclusively on local rules for sequential, face-to-face addition of tiles to a cluster. When the algorithm is seeded with a special type of cluster containing a defect, we find that growth is forced to infinity with high probability and that the resultant IQC has a vanishing density of defects. The geometric features underlying this algorithm can inform analyses of experimental systems and numerical models that generate highly ordered quasicrystals.

cond-mat.mtrl-sci↗

Sparse phonon modes of a limit-periodic structure

Limit-periodic structures are well ordered but nonperiodic, and hence have nontrivial vibrational modes. We study a ball and spring model with a limit-periodic pattern of spring stiffnesses and identify a set of extended modes with arbitrarily low participation ratios, a situation that appears to be unique to limit-periodic systems. The balls that oscillate with large amplitude in these modes live on periodic nets with arbitrarily large lattice constants. By studying periodic approximants to the limit-periodic structure, we present numerical evidence for the existence of such modes, and we give a heuristic explanation of their structure.

cond-mat.mtrl-sci↗

Hard sphere packings within cylinders

The packing of hard spheres (HS) of diameter $σ$ in a cylinder has been used to model experimental systems, such as fullerenes in nanotubes and colloidal wire assembly. Finding the densest packings of HS under this type of confinement, however, grows increasingly complex with the cylinder diameter, $D$. Little is thus known about the densest achievable packings for $D>2.873σ$. In this work, we extend the identification of the packings up to $D=4.00σ$ by adapting Torquato-Jiao's adaptive-shrinking-cell formulation and sequential-linear-programming (SLP) technique. We identify 17 new structures, almost all of them chiral. Beyond $D\approx2.85σ$, most of the structures consist of an outer shell and an inner core that compete for being close packed. In some cases, the shell adopts its own maximum density configuration, and the stacking of core spheres within it is quasiperiodic. In other cases, an interplay between the two components is observed, which may result in simple periodic structures. In yet other cases, the very distinction between core and shell vanishes, resulting in more exotic packing geometries, including some that are three-dimensional extensions of structures obtained from packing hard disks in a circle.

cond-mat.soft↗