arXiv subjects

Joshua Klose

Publications and source records attributed to Joshua Klose.

7 recordsLinked to original sources

arXiv2026

International Optical Clock Comparison Using the European Optical Fiber Network

Optical clocks have achieved remarkable estimated fractional frequency uncertainties reaching the $10^{-18}$ level and below, enabling applications in fundamental physics, general relativity, and geodesy. However, the challenge of verifying the international consistency of optical clocks remains critical as efforts intensify toward redefining the SI second based on an optical transition or transitions. We report on a two-month international clock comparison campaign involving seven optical clocks in four national metrology institutes (INRIM, LNE-OP, NPL, and PTB) connected via the optical fiber network established in Europe. The campaign resulted in optical frequency ratios with uncertainties ranging from $7.7\times10^{-18}$ to $6.1\times10^{-17}$. Among the results, the $^{171}$Yb$^+$(E3) clocks at NPL and PTB demonstrated agreement within an uncertainty of $7.7\times10^{-18}$, marking the first international verification of two independently developed optical clocks below one part in $10^{17}$. The operation of the $^{199}$Hg clock at LNE-OP (formerly LNE-SYRTE) resulted in frequency ratios with improved uncertainties with $^{171}$Yb$^+$(E3), $^{171}$Yb, and $^{87}$Sr optical clocks. These results provide input for the redefinition of the second and underscore how fiber-linked clock networks can advance metrology and scientific applications.

physics.atom-ph↗

arXiv2026

An Al$^+$ clock with $1.6\times10^{-18}$ systematic uncertainty and its frequency ratios

Advances in optical clocks motivate a redefinition of the second, requiring rigorous evaluations of systematic uncertainties and robust consistency among the clocks. Here, we report the full evaluation of the systematic frequency shifts of an $^{27}\mathrm{Al}^+$ single-ion clock, and the measurement of its absolute frequency and frequency ratio with a $^{87}$Sr optical lattice clock at PTB. The evaluated total systematic fractional frequency uncertainty is $1.6\times10^{-18}$, mainly limited by the accuracy of the relevant atomic coefficients and by background gas collisions. The absolute frequency of the clock has been measured to be $ν_{\mathrm{Al}^+}=1 121 015 393 207 859.19(24)\,$Hz, obtained by comparison with two primary caesium fountain clocks at PTB. The frequency ratio between the Al and Sr optical clocks has been determined to be $ν_{\mathrm{Al}^+}/ν_{^{87}\mathrm{Sr}}=2.611 701 431 781 462 668(36)$, limited by the accuracy of the Sr clock. This ratio differs by $8.6σ$ and $1.2σ$ from the 2021 and 2025 frequency ratio published by the BACON collaboration, respectively. These results represent an important contribution toward a future redefinition of the second using optical clocks, and underscore the importance of independent measurements of clock-candidate frequency ratios across different institutions.

physics.atom-ph↗

arXiv2025

A high-stability optical clock based on a continuously ground-state cooled Al$^+$ ion without compromising its accuracy

Single ion optical clocks have shown systematic frequency uncertainties below $10^{-18}$, but typically require more than one week of averaging to achieve a corresponding statistical uncertainty. This time can be reduced with longer probe times, but comes at the cost of a higher time-dilation shift due to motional heating of the ions in the trap. We show that sympathetic ground-state cooling using electromagnetically-induced transparency (EIT) of an \Al clock ion via a co-trapped \Ca ion during clock interrogation suppresses the heating of the ions. \Al can be kept close to the motional ground state, independent from the chosen interrogation time, at a relative time dilation shift of $(-1.69\pm0.20)\times10^{-18}$. The \Ca cooling light introduces an additional light shift on the \Al clock transition of $(-9.27\pm 1.03)\times10^{-18}$. We project that the uncertainty of this light shift can be further reduced by nearly an order of magnitude. This sympathetic cooling enables seconds of interrogation time with $10^{-19}$ motional and cooling laser-induced uncertainties for \Al and can be employed in other ion clocks as well.

physics.atom-ph↗

arXiv2025

Entanglement-enhanced optical ion clock

Entangled states hold the promise of improving the precision and accuracy of quantum sensors. We experimentally demonstrate that spectroscopy of an optical clock transition using entangled states can outperform its classical counterpart. Two ^{40}\text{Ca}^{+} ions are entangled in a quantum state with vanishing first-order magnetic field sensitivity, extending the coherence time of the atoms and enabling near lifetime-limited probe times of up to 550 ms. In our protocol, entangled ions reach the same instability as uncorrelated ions, but at half the probe time, enabling faster cycle times of the clock. We run two entangled ^{40}\text{Ca}^{+} ions as an optical clock and compare its frequency instability with a ^{87}\text{Sr} lattice clock. The instability of the entangled ion clock is below a clock operated with classically correlated states for all probe times. We observe instabilities below the theoretically expected quantum projection noise limit of two uncorrelated ions for interrogation times below 100 ms. The lowest fractional frequency instability of 7e-16 / sqrt(tau / 1 s) is reached for 250 ms probe time, limited by residual phase noise of the probe laser. This represents the lowest instability reported to date for a ^{40}\text{Ca}^{+} ion clock.

physics.atom-ph↗

arXiv2025

Coordinated international comparisons between optical clocks connected via fiber and satellite links

Optical clocks provide ultra-precise frequency references that are vital for international metrology as well as for tests of fundamental physics. To investigate the level of agreement between different clocks, we simultaneously measured the frequency ratios between ten optical clocks in six different countries, using fiber and satellite links. This is the largest coordinated comparison to date, from which we present a subset of 38 optical frequency ratios and an evaluation of the correlations between them. Four ratios were measured directly for the first time, while others had significantly lower uncertainties than previously achieved, supporting the advance towards a redefinition of the second and the use of optical standards for international time scales.

physics.atom-ph↗

arXiv2024

International comparison of optical frequencies with transportable optical lattice clocks

Optical clocks have improved their frequency stability and estimated accuracy by more than two orders of magnitude over the best caesium microwave clocks that realise the SI second. Accordingly, an optical redefinition of the second has been widely discussed, prompting a need for the consistency of optical clocks to be verified worldwide. While satellite frequency links are sufficient to compare microwave clocks, a suitable method for comparing high-performance optical clocks over intercontinental distances is missing. Furthermore, remote comparisons over frequency links face fractional uncertainties of a few $10^{-18}$ due to imprecise knowledge of each clock's relativistic redshift, which stems from uncertainty in the geopotential determined at each distant location. Here, we report a landmark campaign towards the era of optical clocks, where, for the first time, state-of-the-art transportable optical clocks from Japan and Europe are brought together to demonstrate international comparisons that require neither a high-performance frequency link nor information on the geopotential difference between remote sites. Conversely, the reproducibility of the clocks after being transported between countries was sufficient to determine geopotential height offsets at the level of 4 cm. Our campaign paves the way for redefining the SI second and has a significant impact on various applications, including tests of general relativity, geodetic sensing for geosciences, precise navigation, and future timing networks.

physics.atom-ph↗

arXiv2022

Experimental determination of the E2-M1 polarizability of the strontium clock transition

To operate an optical lattice clock at a fractional uncertainty below $10^{-17}$, one must typically consider not only electric-dipole (E1) interaction between an atom and the lattice light field when characterizing the resulting lattice light shift of the clock transition but also higher-order multipole contributions, such as electric-quadrupole (E2) and magnetic-dipole (M1) interactions. However, strongly incompatible values have been reported for the E2-M1 polarizability difference of the clock states $(5s5p)\,{}^{3}\mathrm{P}_{0}$ and $(5s^2)\,{}^{1}\mathrm{S}_{0}$ of strontium [Ushijima et al., Phys. Rev. Lett. 121 263202 (2018); Porsev et al., Phys. Rev. Lett. 120, 063204 (2018)]. This largely precludes operating strontium clocks with uncertainties of few $10^{-18}$, as the resulting lattice light shift corrections deviate by up to $1 \times 10^{-17}$ from each other at typical trap depths. We have measured the E2-M1 polarizability difference using our ${}^{87}\mathrm{Sr}$ lattice clock and find a value of $Δα_{\mathrm{qm}} = -987^{+174}_{-223} \; \mathrm{μHz}$. This result is in very good agreement with the value reported by Ushijima et al.

physics.atom-ph↗