SearcharxivSearch

arXiv subjects

Jozef Strecka

Publications and source records attributed to Jozef Strecka.

At least 19 recordsLinked to original sources

Thermal phase transitions in a mixed-spin Ising model on the Lieb lattice: Exact results beyond zero magnetic field

We investigate the ground-state and finite-temperature properties of a mixed spin-1/2 and spin-1 Ising model on a decorated square (Lieb) lattice incorporating a uniaxial single-ion anisotropy and magnetic field. By employing the generalized decoration-iteration transformation, the model is mapped exactly onto an effective spin-1/2 Ising model on the square lattice characterized by an effective nearest-neighbor interaction and an effective field. The studied model consequently becomes exactly solvable even for finite values of the applied magnetic field whenever the effective field vanishes. The ground-state analysis reveals three distinct phases: ferrimagnetic phase (FRI), disordered phase (DP), and ferromagnetic (FM) phase. The ground-state boundary between FRI and DP phases gives rise to a dome-shaped surface of discontinuous thermal phase transitions, which is terminated by a line of Ising-type critical points associated with continuous thermal phase transitions. Both continuous and discontinuous thermal phase transitions belong to the exactly solvable parameter regime defined by a vanishing effective field in spite of the fact that the applied magnetic field is finite. Two consecutive discontinuous thermally-induced reentrant phase transitions DP-FRI-DP are identified in a narrow parameter region. The exact analytical predictions including reentrance, field- and thermally-driven phase transitions are independently verified by classical Monte Carlo simulations.

cond-mat.stat-mech

Still life in a classic Blume-Capel model: pseudo-transitions in a spin-1 diamond chain

We exactly investigate the ground-state, magnetic, and thermodynamic properties of a spin-1 Blume-Capel diamond chain in a magnetic field by means of the transfer-matrix method. After establishing the complete ground-state phase diagram and characterizing each ground-state spin configuration, we examine the finite-temperature behavior in the vicinity of selected phase boundaries and triple points. It is demonstrated that an extremely small energy gap between a nondegenerate ground state and competing macroscopically degenerate low-lying excited states gives rise to entropically-driven pseudo-transitions. These pseudo-transitions manifest themselves through abrupt but continuous changes in the magnetization and entropy resembling discontinuous jumps, while the magnetic susceptibility and specific heat exhibit exceptionally sharp yet finite peaks resembling divergences. Our results provide the exact evidence that pseudo-transitions can also emerge in the classical spin-1 Blume-Capel model and thereby extend the class of one-dimensional spin systems known to display pseudo-transitions.

cond-mat.stat-mech

Katsura-Nagaosa-Balatsky magnetoelectricity in molecular magnets: Bipartite entanglement transfer by means of rotating electric field

We investigate quantum entanglement in a spin-1/2 Heisenberg trimer with spin-induced electric polarization described by the Katsura-Nagaosa-Balatsky (KNB) mechanism in the presence of external magnetic and electric fields. The electric field is assumed to lie in the plane of the magnetic ions, allowing its strength and orientation to be tuned independently. We analyze both bipartite and tripartite entanglement and demonstrate that the spin-electric-field coupling provides an efficient mechanism for controlling quantum correlations within the molecular nanomagnet. Depending on the electric-field parameters, the bipartite entanglement can be significantly enhanced or suppressed, while the multipartite entanglement exhibits a rich dependence on the microscopic spin-electric coupling. Most notably, we demonstrate that a rotating in-plane electric field of constant magnitude induces a controllable transfer of bipartite entanglement between different spin pairs. In the symmetric case of homogeneous exchange interactions and uniform KNB coupling, this transfer is found to be nearly ideal, with the bipartite negativity approaching its theoretical maximum for one spin pair while simultaneously vanishing for the remaining pairs. We show that the efficiency of the transfer can be tailored through the exchange interactions, bond geometry, and nonuniform spin-electric coupling. These results establish molecular nanomagnets with KNB spin-electric coupling as a promising platform for the electrical manipulation, steering, and localization of quantum entanglement at the molecular scale.

cond-mat.other

Continuous and discontinuous transitions in the Ising-Heisenberg model on the extended Lieb lattice in a magnetic field

The spin-1/2 Ising-Heisenberg model on the extended Lieb lattice in a magnetic field is exactly mapped onto an effective spin-1/2 Ising model on the square lattice. The ground-state phase diagram comprises the quantum antiferromagnetic (QAF), quantum monomer-dimer (MD), classical ferrimagnetic (FRI), and classical ferromagnetic phase. The MD-FRI ground-state phase boundary extends to finite temperatures as a dome-shaped surface of discontinuous thermal transitions bounded by a line of Ising critical points. The QAF phase is enclosed by a surface of continuous thermal transitions evolving from the QAF-MD and QAF-FRI ground-state phase boundaries. Monte Carlo simulations fully confirm the existence and nature of both continuous and discontinuous thermal phase transitions obtained by exact and approximate analytical calculations.

cond-mat.stat-mech

Magnetoelastic signatures of thermal and quantum phase transitions in a deformable Ising chain under a longitudinal and transverse magnetic field

We investigate a deformable spin-1/2 Ising chain subjected to either a longitudinal or a transverse magnetic field, which incorporates a magnetoelastic coupling linearly dependent on a lattice distortion parameter. Within the harmonic and static adiabatic approximations, the variational Gibbs free energy is evaluated exactly using transfer-matrix and Jordan-Wigner fermionization techniques and then minimized self-consistently with respect to the lattice distortion parameter. This approach enables a unified description of magnetic and elastic properties including the magnetization, magnetic susceptibility, lattice distortion, inverse compressibility, and relative change in the sound velocity. In a longitudinal magnetic field, the deformable Ising chain displays a line of discontinuous thermal phase transitions terminating at a critical point. The discontinuous transitions are accompanied by metastable states, which give rise to a hysteresis loop at low temperatures. In contrast, the deformable Ising chain in a transverse field undergoes exclusively a continuous quantum phase transition at zero temperature with no indication of thermal phase transitions. The magnetic susceptibility and inverse compressibility exhibit cusp- and dip-like anomalies at discontinuous phase transitions, while a diverging susceptibility and vanishing inverse compressibility characterize the continuous phase transitions. An elastic softening of the deformable chain near thermal and quantum phase transitions manifest itself also through a significant sound attenuation.

cond-mat.stat-mech

Magnetization plateaus, spin-canted orders and field-induced transitions in a spin-1/2 Heisenberg antiferromagnet on a distorted diamond-decorated honeycomb lattice

We investigate the spin-1/2 Heisenberg antiferromagnet on a distorted diamond-decorated honeycomb lattice in an external magnetic field. By combining density-matrix renormalization group, sign-problem-free quantum Monte Carlo in a mixed dimer-monomer basis, exact diagonalization, and an effective lattice-gas approach, we determine the ground-state phase diagram and analyze the finite-temperature magnetization process. The model hosts a rich variety of frustration-induced quantum phases including a quantum ferrimagnetic phase of Lieb-Mattis type, a quantum ferromagnetic phase, a spin-canted phase, a monomer-dimer phase, a dimer-tetramer liquid, a dimer-tetramer solid, and two distinct one-dimensional-crossover phases of ferromagnetic and ferrimagnetic character. Depending on the lattice distortion, we identify robust magnetization plateaus at 0, 1/4, 1/2, and 3/4 of the saturation magnetization originating from competing local dimer and tetramer singlets. Finite-temperature QMC data reveal how thermal fluctuations progressively smear the plateau structure, while the effective lattice-gas description reliably captures the corresponding low-temperature behavior.

cond-mat.stat-mech

Approaching Kasteleyn transition in frustrated quantum Heisenberg antiferromagnets

We show that the Kasteleyn transition, the abrupt proliferation of infinite strings of defects in classical dimer and related models, can also be relevant for frustrated 2d quantum magnets. This is explicitly demonstrated in a phase of the spin-1/2 Heisenberg diamond-decorated honeycomb lattice where a family of exact eigenstates built as products of dimer and plaquette singlets can be mapped onto the dimer coverings of the honeycomb lattice. The low-temperature properties of this phase are accurately described by an effective dimer model with anisotropic activities and a small, tunable density of monomers, leading to an arbitrarily sharp crossover version of the Kasteleyn transition. The generalization to other geometries and the possibility to realize this model in organo-metallic compounds are briefly discussed.

cond-mat.stat-mech

Unveiling the degeneracy of bound magnon crystals from magnetic and thermodynamic features of the spin-1/2 Heisenberg octahedral chain

Magnetic, thermodynamic, and magnetocaloric properties of a spin-1/2 Heisenberg octahedral chain with three distinct exchange interactions are investigated in an external magnetic field using the variational method, extended localized-magnon approach, and exact diagonalization. Variational arguments rigorously establish two distinct fragmented phases in the frustrated regime. In the former phase all four spins of each square plaquette form a collective plaquette singlet, whereas in the latter phase two dimer singlets are formed along diagonals of each square plaquette. These bound two-magnon states, supplemented with three localized one-magnon states, enable us to elaborate a generalized localized-magnon theory that is applicable in a frustrated regime across the entire field range as confirmed by comparison with exact diagonalization data. The concept of localized magnons provides a consistent description of low-temperature magnetization curves featuring intermediate one-fifth and three-fifths plateaus, which intersect each other at temperature-independent crossing points determined by the relative degeneracies of competing bound-magnon phases. Field variations of the specific heat reveal a pronounced double-peak structure near each field-driven transition with peak heights depending on the relative degeneracies of the respective bound-magnon states. Our results demonstrate that the system supports highly efficient cooling via adiabatic demagnetization, making it a promising candidate for magnetocaloric refrigeration.

cond-mat.stat-mech

Fingerprints of cluster-based Haldane and bound-magnon states in a spin-1 Heisenberg diamond chain

We investigate magnetic and thermodynamic properties of a spin-1 Heisenberg diamond chain in a magnetic field using a combination of analytical and numerical methods including the variational approach, exact diagonalization, density-matrix renormalization group, localized-magnon theory, and quantum Monte Carlo simulations. In the unfrustrated regime, the model exhibits a quantum ferrimagnetic phase that captures key magnetic features of the nickel-based polymeric compound [Ni3(OH)2(C4H2O4)(H2O)4].2H2O such as a at minimum in the temperature dependence of the susceptibility times temperature product and an intermediate one-third magnetization plateau. In the frustrated regime, we uncover a rich variety of unconventional quantum phases including uniform and cluster-based Haldane states, fragmented monomer-dimer phase, and bound-magnon crystals. Analysis of the adiabatic temperature change and magnetic Gruneisen parameter reveals an enhanced magnetocaloric effect near field-induced transitions between these exotic quantum phases. Additionally, we demonstrate that the frustrated spin-1 diamond chain can operate as an efficient working medium of a quantum Stirling engine, which approaches near-optimal efficiency when driven into these unconventional quantum states.

cond-mat.stat-mech

Enhancing fidelity in teleportation of a two-qubit state via a quantum communication channel formed by spin-1/2 Ising-Heisenberg trimer chains due to a magnetic field

We demonstrate that two independent spin-1/2 Ising-Heisenberg trimer chains provide an effective platform for the quantum teleportation of any entangled two-qubit state through the quantum communication channel formed by two Heisenberg dimers. The reliability of this quantum channel is assessed by comparing the concurrences, which quantify a strength of the bipartite entanglement of the initial input state and the readout output state. Additionally, we rigorously calculate quantities fidelity and average fidelity to evaluate the quality of the teleportation protocol depending on temperature and magnetic field. It is evidenced that the efficiency of quantum teleportation of arbitrary entangled two-qubit state through this quantum communication channel can be significantly enhanced by moderate magnetic fields. This enhancement can be attributed to the magnetic-field-driven transition from a quantum antiferromagnetic phase to a quantum ferrimagnetic phase, which supports realization of a fully entangled quantum channel suitable for efficient quantum teleportation. The polymeric trimer chains Cu3(P2O6OH)2 are proposed as an experimental resource of this quantum communication channel, which provides an efficient platform for realization of the quantum teleportation up to moderate temperatures 40 K and extremely high magnetic fields 80 T.

quant-ph

Thermodynamic properties of the macroscopically degenerate tetramer-dimer phase of the spin-1/2 Heisenberg model on the diamond-decorated square lattice

The spin-1/2 Heisenberg antiferromagnet on the diamond-decorated square lattice in the presence of a magnetic field displays various quantum phases including the Lieb-Mattis ferrimagnetic, dimer-tetramer, monomer-dimer, and spin-canted phases, in addition to the trivial fully saturated state. Thermodynamic properties of this model are investigated using several complementary analytical and numerical methods such as exact diagonalization up to the systems of 40 spins, an effective monomer-dimer description, sign-problem-free quantum Monte Carlo simulations for up to 180 spins, and a decoupling approximation. Our particular attention is focused on the parameter region favoring the dimer-tetramer phase. This ground state can be represented by a classical hard-dimer model on the square lattice and retains a macroscopic degeneracy even under a magnetic field. However, the description of the low-temperature thermodynamics close to the boundary between the macroscopically degenerate dimer-tetramer and the non-degenerate monomer-dimer phases requires an extended classical monomer-dimer lattice-gas model. Anomalous thermodynamic properties emerging in the vicinity of the dimer-tetramer phase are studied in detail. Under the adiabatic demagnetization we detect an enhanced magnetocaloric effect promoting an efficient cooling to absolute zero temperature, provided that the system reaches the dimer-tetramer ground state at zero field.

cond-mat.str-el

Pseudo-transition between antiferromagnetic and charge orders in a minimal spin-pseudospin model of one-dimensional cuprates

This study rigorously investigates the phenomenon of a pseudo-transition in a minimal spinpseudospin model, serving as a simplified model of one-dimensional cuprate chains [CuO]n, by making use of the transfer-matrix method. The studied spin-pseudospin model of one-dimensional cuprate chains [CuO]n reveals a peculiar pseudo-transition between a charged-ordered phase and an antiferromagnetic phase, which is accompanied with anomalous behavior of magnetic and thermodynamic quantities. While the entropy and short-range correlations undergo near the pseudo-transition steep continuous changes reminiscent of a discontinuous phase transition, the specific heat displays a sizable sharp peak akin to a continuous phase transition.

cond-mat.stat-mech

Quantum Magnetism in Fe2Cu2 Polymeric Branched Chains: Insights from Exactly Solved Ising-Heisenberg Model

The spin-1/2 Ising-Heisenberg branched chain, inspired by the magnetic structure of three isostructural polymeric coordination compounds [(Tp)2Fe2(CN)6X(bdmap)Cu2(H2O)].H2O to be further denoted as Fe2Cu2 (Tp = tris(pyrazolyl)hydroborate, bdmapH = 1,3-bis(dimethylamino)-2-propanol, HX = acetic acid, propionic acid or trifluoroacetic acid), is rigorously studied using the transfer-matrix method. The overall ground-state phase diagram reveals three distinct phases: a quantum antiferromagnetic phase, a quantum ferrimagnetic phase and a classical ferromagnetic phase. In the zero-temperature magnetization curve, two quantum ground states are manifested as intermediate plateaus at zero and half of the saturation magnetization, while the magnetization reaches its saturated value within the classical ferromagnetic phase. The bipartite entanglement between nearest-neighbor Heisenberg spins is more pronounced in the quantum ferrimagnetic phase compared to the quantum antiferromagnetic phase due to a fully polarized nature of the Ising spins. A reasonable agreement between theoretical predictions for the spin-1/2 Ising-Heisenberg branched chain and experimental data measured for a temperature dependence of the magnetic susceptibility and a low-temperature magnetization curve suggests strong antiferromagnetic coupling between nearest-neighbor CuII-CuII magnetic ions and moderately strong ferromagnetic coupling between nearest-neighbor CuII-FeIII magnetic ions in the polymeric compounds Fe2Cu2. A thermal entanglement between nearest-neighbor CuII-CuII magnetic ions persists up to a relatively high threshold temperature T = 224 K and undergoes a transient magnetic-field-driven strengthening.

cond-mat.stat-mech

Room-temperature entanglement of the nickel-radical molecular complex (Et3NH)[Ni(hfac)2L]

The bipartite entanglement is comprehensively investigated in the mononuclear molecular complex (Et3NH)[Ni(hfac)2L]L, where HL denotes 2-(2-hydroxy-3-methoxy-5-nitrophenyl)-4,4,5,5-tetramethyl-4,5-dihydro-1H-imidazol-3-oxide-1-oxyl and hfacH stands for hexafluoroacetylacetone. From the magnetic point of view, the molecular compound (Et3NH)[Ni(hfac)2L] consists of an exchange-coupled spin-1 Ni2+ magnetic ion and a spin-1/2 nitronyl-nitroxide radical substituted nitrophenol. The nickel-radical molecular complex affords an experimental realization of a mixed spin-(1/2, 1) Heisenberg dimer with a strong antiferromagnetic exchange coupling J/kB = 505 K and two distinct g-factors gRad=2.005 and gNi=2.275. By adopting this set of magnetic parameters we demonstrate that the Zeeman splitting of a quantum ferrimagnetic ground-state doublet due to a weak magnetic field may substantially reinforce the strength of bipartite entanglement at low temperatures. The molecular compound (Et3NH)[Ni(hfac)2L] maintains sufficiently strong thermal entanglement even at room temperature, vanishing only above 546 K. Specifically, the thermal entanglement in the nickel-radical molecular complex retains approximately 40% of the maximum value corresponding to perfectly entangled Bell states at room temperature, which implies that this magnetic compound provides suitable platform of a molecular qubit with potential implications for room-temperature quantum computation and quantum information processing.

cond-mat.mtrl-sci

Magnetic analogue of liquid-gas phase transition of water: case study of a spin-1/2 Ising-Heisenberg model on a diamond-decorated square lattice

The spin-1/2 Ising-Heisenberg model on a diamond-decorated square lattice exhibits an intriguing temperature-driven phase transition in a magnetic field between a classical ferrimagnetic phase and a quantum monomer-dimer phase. A generalized decoration-iteration transformation accurately maps the considered model to an effective spin-1/2 Ising model on a square lattice with temperature-dependent effective interactions and field, whereby the effective field vanishes at the phase boundary separating the classical ferrimagnetic phase from the quantum monomer-dimer phase. Typical features of the magnetization, magnetic susceptibility and specific heat in the vicinity of discontinuous and continuous thermal phase transitions between the classical ferrimagnetic phase and the quantum monomer-dimer phase are elucidated.

cond-mat.stat-mech

Thermal entanglement of a geometrically frustrated spin-1 Heisenberg diamond cluster

Thermal entanglement of a geometrically frustrated spin-1 Heisenberg diamond cluster is examined within the framework of the exact diagonalization method by computing the measure of entanglement negativity. The calculated exact analytical results are applied in order to obtain theoretical prediction of the robustness of bipartite thermal entanglement of the tetranuclear nickel complex [Ni4(CO3)2(aetpy)8](ClO4)4 (aetpy = 2-aminoethyl-pyridine) against rising temperature and magnetic field.

cond-mat.stat-mech

Thermal first-order phase transitions, Ising critical points, and reentrance in the Ising-Heisenberg model on the diamond-decorated square lattice in a magnetic field

The thermal phase transitions of a spin-1/2 Ising-Heisenberg model on the diamond-decorated square lattice in a magnetic field are investigated using a decoration-iteration transformation and classical Monte Carlo simulations. A generalized decoration-iteration transformation maps this model exactly onto an effective classical Ising model on the square lattice with temperature-dependent effective nearest-neighbor interactions and magnetic field strength. The effective field vanishes along a ground-state phase boundary of the original model, separating a ferrimagnetic and a quantum monomer-dimer phase. At finite temperatures this phase boundary gives rise to an exactly solvable surface of discontinuous (first-order) phase transitions, which terminates in a line of Ising critical points. The existence of discontinuous reentrant phase transitions within a narrow parameter regime is reported and explained in terms of the low-energy excitations from both phases. These exact results, obtained from the mapping to the zero-field effective Ising model are corroborated by classical Monte Carlo simulations of the effective model.

cond-mat.stat-mech

Phases of the spin-1/2 Heisenberg antiferromagnet on the diamond-decorated square lattice in a magnetic field

The spin-1/2 Heisenberg antiferromagnet on the frustrated diamond-decorated square lattice is known to feature various zero-field ground-state phases, consisting of extended monomer-dimer and dimer-tetramer ground states as well as a ferrimagnetic regime. Using a combination of analytical arguments, density matrix renormalization group (DMRG), exact diagonalization, as well as sign-problem-free quantum Monte Carlo (QMC) calculations, we investigate the properties of this system and the related Lieb lattice in the presence of a finite magnetic field, addressing both the ground-state phase diagram as well as several thermodynamic properties. In addition to the zero-field ground states, we find at high magnetic field a spin-canted phase with a continuously rising magnetization for increasing magnetic field strength, as well as the fully polarized paramagnetic phase. At intermediate field strength, we identify a first-order quantum phase transition line between the ferrimagnetic and the monomer-dimer regime. This first-order line extends to finite temperatures, terminating in a line of critical points that belong to the universality class of the two-dimensional Ising model.

cond-mat.str-el