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Juan Carlos Cuevas

Publications and source records attributed to Juan Carlos Cuevas.

At least 19 recordsLinked to original sources

Nonreciprocal Magnon Hanle Effect in Antiferromagnetic $α$-Fe$_2$O$_3$

The precession of the magnon pseudospin about the equilibrium pseudofield, the latter capturing the nature of magnonic eigenexcitations in an antiferromagnet, gives rise to the magnon Hanle effect. Its realization via electrically injected and detected spin transport in an antiferromagnetic insulator demonstrates its high potential for devices and as a convenient probe for magnon eigenmodes and the underlying spin interactions in the antiferromagnet. Here, we observe a non-reciprocity in the Hanle signal measured in alpha-Fe2O3 using two spatially separated Pt electrodes as spin injector and detector. Interchanging their roles alters the detected magnon spin signal. The recorded difference depends on the applied magnetic field and reverses sign when the signal passes its nominal maximum at the so-called compensation field. Our findings unlock the high potential of antiferromagnetic magnonics towards the realization of electronics-inspired phenomena.

cond-mat.mes-hall↗

Continuous Tuning of the Charge-Phase Uncertainty in a Josephson Junction

Quantum mechanics constrains conjugate observables from being simultaneously measurable with arbitrary precision. In a Josephson junction, these are the transferred electric charge and the quantum-mechanical phase difference between the superconducting domains. Which of them fluctuates determines the supercurrent: a dissipative trickle of single Cooper pairs in one limit, a coherent dissipationless flow in the other. Bridging both regimes in one device remained elusive because the Josephson and charging energies are fixed at fabrication. Here, we use the tunable tunnel junction of a scanning tunneling microscope at millikelvin temperature to vary their ratio continuously over many orders of magnitude. In this way, we monitor the smooth transition between incoherent and coherent Cooper pair flow in a single junction, revealing the quantum-to-classical transition in a controlled way.

cond-mat.supr-con↗

Stereochemical Vacuum Gap Explains Out-of-Plane Thermal Insulation in MXenes

Two-dimensional MXenes are promising materials for thermal management and spectral camouflage, combining low out-of-plane thermal conductivity with low infrared emissivity and mechanical robustness. Yet the near-order-of-magnitude spread in experimental out-of-plane thermal conductivity measurements (0.14-0.8 W/mK) and the systematic overestimation by simulations point to a fundamental gap in our understanding of heat transport in these materials. Here, we argue these differences originate in the overlooked role of heterogeneous surface terminations. Using Non-Equilibrium Molecular Dynamics simulations of Ti3C2Tx, we show that this discrepancy arises from a stereochemically induced vacuum gap between adjacent layers, formed when surface terminations of different sizes coexist. Even minor deviations from homogeneous terminations drastically suppress out-of-plane thermal conductivity, bringing simulated values into quantitative agreement with experiment. We also show that thermal conductivity scales strongly with the atomic density, and that introducing bulky surface terminations, including residual water, reduces the thermal conductivity to 0.3 W/mK, an order of magnitude below homogeneous termination values and below the minimum thermal conductivity limit predicted for disordered solids. Thus, we propose a chemistry-driven route to engineer thermal transport in MXenes.

cond-mat.mtrl-sci↗

Yu-Shiba-Rusinov States in Ising Superconductors

The nature of the superconducting state in two-dimensional transition-metal dichalcogenides remains under active debate. A widely used description invokes so-called \textit{Ising superconductivity}. In this work, we investigate theoretically this pairing state by employing single magnetic impurities as local probes of the superconducting condensate. We analyze the formation of Yu-Shiba-Rusinov bound states in the presence of Ising spin-orbit coupling and an in-plane magnetic field to study how their spectral properties encode the underlying pairing structure. We identify distinct features in the bound-state spectrum and tunneling response that differentiate this system from conventional superconductors. Our results demonstrate that magnetic impurities provide a sensitive probe of the structure of the superconducting state and yield experimentally accessible signatures of unconventional aspects of Ising superconductivity.

cond-mat.supr-con↗

Transparency-controlled multiple charge transfer in superconducting junctions with local shot-noise scanning tunneling spectroscopy

Charge transport in superconducting junctions at finite voltages is governed by Andreev reflections, including multiple Andreev reflections, which are processes that enable multiple charge transfer, a hallmark that shot noise can directly quantify. Since the effective charge extracted from shot noise measurements varies with the transparency of the junction, systematic control of transparency is essential but experimentally challenging. Here, we present shot noise scanning tunneling microscopy measurements enabled by a newly developed amplifier, allowing access to different transparency regimes. We perform shot noise measurements on Pb(111) with tunable transparency at 2.2 K and observe that the shot noise evolves from a single electron tunneling regime to multiple charge transfer regime as transparency increases. Our results are quantitatively consistent with theoretical simulations of Andreev reflections and multiple Andreev reflections for a single-channel system. These results establish junction transparency as the key parameter governing the evolution of charge transport and demonstrate that noise-STM is a powerful platform for investigating microscopic charge transport mechanisms with controlled junction transparency at the atomic scale.

cond-mat.supr-con↗

The role of charge in thermodynamic uncertainty relations

We demonstrate that the charge value of transport mechanisms heavily impacts the validity of thermodynamic uncertainty relations (TURs). Specifically, we show within the framework of full counting statistics, that the recently established quantum TUR can be violated by the presence of transport processes that carry more than one charge, like Andreev reflection processes in normal metal-superconductor junctions. We propose a modified quantum TUR, which incorporates the charge value and demonstrate that this charge-dependent quantum TUR can only be violated if the highest charge transport process exceeds this charge value. In particular, we establish that the breaking of the quantum TUR solely originates from the charge value of the highest charge transport process. Namely, our analytical considerations do not invoke the existence of superconductivity, and these considerations generally hold for non-interacting electronic transport which can be described by the scattering formalism.

cond-mat.mes-hall↗

Full Counting Statistics of Yu-Shiba-Rusinov Bound States

With the help of scanning tunneling microscopy (STM) it has become possible to address single magnetic impurities on superconducting surfaces and to investigate the peculiar properties of the in-gap states known as Yu-Shiba-Rusinov (YSR) states. However, until very recently YSR states were only investigated with conventional tunneling spectroscopy, missing the crucial information contained in other transport properties such as shot noise. Here, we adapt the concept of full counting statistics (FCS) to provide a very deep insight into the spin-dependent transport in these hybrid systems. We illustrate the power of FCS by analyzing different situations in which YSR states show up including single-impurity junctions, as well as double-impurity systems where one can probe the tunneling between individual YSR states. The FCS concept allows us to unambiguously identify every tunneling process that plays a role in these situations. Moreover, FCS provides all the relevant transport properties, including current, shot noise and all the cumulants of the current distribution. Our approach can reproduce the experimental results recently reported on the shot noise of a single-impurity junction with a normal STM tip. We also predict the signatures of resonant (and non-resonant) multiple Andreev reflections in the shot noise of single-impurity junctions with two superconducting electrodes. In the case of double-impurity junctions we show that the direct tunneling between YSR states is characterized by a strong reduction of the Fano factor that reaches a minimum value of 7/32, a new fundamental result in quantum transport. The FCS approach presented here can be naturally extended to investigate the spin-dependent superconducting transport in a variety of situations, and it is also suitable to analyze multi-terminal superconducting junctions, irradiated contacts, and many other basic situations.

cond-mat.mes-hall↗

Quartet Tomography in Multiterminal Josephson Junctions

We investigate the detection of quartets in hybrid multiterminal Josephson junctions. Using simple models of quantum dots coupled to superconducting leads, we find that quartets are ubiquitous and show how to rigorously extract their contribution to the current-phase relation (CPR). We also demonstrate that quartets are closely related to the hybridization of Andreev bound states (ABSs) in these systems and propose a method to identify quartets directly in ABS spectra. We illustrate our method by analyzing the spectroscopic measurements of the ABS spectrum in a three-terminal Josephson junction realized in an InAs/Al heterostructure. Our analysis strongly suggests the existence of quartets in the studied hybrid system.

cond-mat.supr-con↗

Thermodynamic uncertainty relations in superconducting junctions

Quantum conductors attached to metallic reservoirs have been demonstrated to overcome the thermodynamic uncertainty relation (TUR), a trade-off relation between the amount of dissipation and the absence of charge and heat current fluctuations. Here, we report large TUR violations when superconducting reservoirs replace metallic ones. The coexistence of different transport processes, namely (multiple) Andreev reflection, where electrons and their retro-reflected holes create Cooper pairs, in addition to the normal quasiparticle transport is identified as the source for such TUR breakdowns. The large TUR violation is a remarkable advantage for building low dissipative and highly stable quantum thermal machines.

cond-mat.mes-hall↗

Signatures of superconducting Higgs mode in irradiated Josephson junctions

The Higgs mode, originally proposed in the context of superconductivity, corresponds to oscillations of the amplitude of the superconducting order parameter. Recent THz-domain optical studies have found signatures consistent with the Higgs mode, but its unambiguous detection is still challenging. We predict that the existence of the Higgs mode can be unambiguously revealed by standard measurements of the transport characteristics in microwave-irradiated asymmetric and transparent Josephson junctions. One signature of the Higgs mode in a Josephson junction is the microwave-induced enhancement of the second harmonic of the equilibrium current-phase relation (at zero DC bias voltage), whose sign differs from its expected value in the absence of the Higgs mode. As the radiation frequency is varied, this enhancement exhibits resonant behavior when the microwave frequency is tuned across the Higgs mass. The second signature that we propose is the enhancement of the second harmonic of the AC Josephson current at finite DC voltage bias, which can be probed in a customary analysis of the Shapiro steps in a microwave-irradiated junction.

cond-mat.supr-con↗

Sextets in four-terminal Josephson junctions

Multiterminal superconducting junctions have revitalized the investigation of the Josephson effect. One of the most interesting aspects of these hybrid systems is the occurrence of multi-Cooper pair tunneling processes that have no analog in two-terminal devices. Such correlated tunneling events are also intimately connected to the Andreev bound states (ABSs) supported by these structures. Josephson junctions with four superconducting terminals have attracted special attention because they are predicted to support ABSs with nontrivial topological properties. Here, we present a theoretical study of sextets, which are correlated tunneling processes involving three Cooper pairs and four different superconducting terminals. We investigate how sextets can be identified from the analysis of the current-phase relation, we show how sextets are connected to the hybridization of ABSs, and we discuss their existence in recent experiments on four-terminal devices realized in hybrid Al/InAs heterostructures.

cond-mat.supr-con↗

Nonclassical Photon-Assisted Transport in Superconducting Tunnel Junctions

Advances in circuit quantum electrodynamics have enabled the generation of arbitrary nonclassical microwave states and paved the way for addressing novel physics questions. Here, we present a theoretical study of the electrical current in a Josephson tunnel junction interacting with a nonclassical electromagnetic environment. This allows us to generalize classical transport phenomena like photon-assisted tunneling and Shapiro steps to the quantum regime. We predict that the analysis of the supercurrent in such a setup enables the complete reconstruction of quantum states of the electromagnetic environment, something that is not possible with normal tunnel junctions.

cond-mat.mes-hall↗

From local to collective superconductivity in proximitized graphene

The superconducting proximity effect induces pairing correlations in metallic systems via Andreev scattering. This effect is particularly intriguing in graphene, as it enables two-dimensional superconductivity that is tunable through doping. Understanding how superconducting correlations propagate within the metal is crucial to unveiling the key factors behind this tunability. Here, we employ scanning tunneling microscopy to investigate the energy and length scales of the proximity effect induced by Pb islands on graphene. Using tip-induced manipulation, we assemble S/N/S junctions with tunable N-region spacing and explore the evolution of the proximitized state in the confined normal region. We find that different doping levels can lead to either localized or collective superconducting states. By combining our experimental results with quasiclassical theory, we demonstrate that interface conductance plays a key role in determining the strength and coherence length of pairing correlations and inter-island coupling. Our findings provide new insights into the design of novel superconducting states and the control of their properties.

cond-mat.mes-hall↗

Exploring the energy spectrum of a four-terminal Josephson junction: Towards topological Andreev band structures

Hybrid multiterminal Josephson junctions (JJs) are expected to harbor a novel class of Andreev bound states (ABSs), including topologically nontrivial states in four-terminal devices. In these systems, topological phases emerge when ABSs depend on at least three superconducting phase differences, resulting in a three-dimensional (3D) energy spectrum characterized by Weyl nodes at zero energy. Here, we realize a four-terminal JJ in a hybrid Al/InAs heterostructure, where ABSs form a synthetic 3D band structure. We probe the energy spectrum using tunneling spectroscopy and identify spectral features associated with the formation of a tri-Andreev molecule, a bound state whose energy depends on three superconducting phases and, therefore, is able to host topological ABSs. The experimental observations are well described by a numerical model. The calculations predict the appearance of four Weyl nodes at zero energy within a gap smaller than the experimental resolution. These topological states are theoretically predicted to remain stable within an extended region of the parameter space, well accessible by our device. These findings establish an experimental foundation to study high-dimensional synthetic band structures in multiterminal JJs, and to realize topological Andreev bands.

cond-mat.mes-hall↗

Deep Reinforcement Learning for Radiative Heat Transfer Optimization Problems

Reinforcement learning is a subfield of machine learning that is having a huge impact in the different conventional disciplines, including physical sciences. Here, we show how reinforcement learning methods can be applied to solve optimization problems in the context of radiative heat transfer. We illustrate their use with the optimization of the near-field radiative heat transfer between multilayer hyperbolic metamaterials. Specifically, we show how this problem can be formulated in the language of reinforcement learning and tackled with a variety of algorithms. We show that these algorithms allow us to find solutions that outperform those obtained using physical intuition. Overall, our work shows the power and potential of reinforcement learning methods for the investigation of a wide variety of problems in the context of radiative heat transfer and related topics.

physics.optics↗

Theory of Electron Spin Resonance in Scanning Tunneling Microscopy

Electron spin resonance (ESR) spectroscopy in scanning tunneling microscopy (STM) has enabled probing the electronic structure of single magnetic atoms and molecules on surfaces with unprecedented energy resolution, as well as demonstrating coherent manipulation of single spins. Despite this remarkable success, the field could still be greatly advanced by a more quantitative understanding of the ESR-STM physical mechanisms. Here, we present a theory of ESR-STM which quantitatively models not only the ESR signal itself, but also the full background tunneling current, from which the ESR signal is derived. Our theory is based on a combination of Green's function techniques to describe the electron tunneling and a quantum master equation for the dynamics of the spin system along with microwave radiation interacting with both the tunneling current and the spin system. We show that this theory is able to quantitatively reproduce the experimental results for a spin-1/2 system (TiH molecules on MgO) across many orders of magnitude in tunneling current, providing access to the relaxation and decoherence rates that govern the spin dynamics due to intrinsic mechanisms and to the applied bias voltage. More importantly, our work establishes that: (i) sizable ESR signals, which are a measure of microwave-induced changes in the junction magnetoresistance, require surprisingly high tip spin polarizations, (ii) the coupling of the magnetization dynamics to the microwave field gives rise to the asymmetric ESR spectra often observed in this spectroscopy. Additionally, our theory provides very specific predictions for the dependence of the relaxation and decoherence times on the bias voltage and the tip-sample distance. Finally, with the help of electromagnetic simulations, we find that the transitions in our ESR-STM experiments can be driven by the ac magnetic field at the junction.

cond-mat.mes-hall↗

Microscopic theory of supercurrent suppression by gate-controlled surface depairing

Recently gate-mediated supercurrent suppression in superconducting nano-bridges has been reported in many experiments. This could be either a direct or an indirect gate effect. The microscopic understanding of this observation is not clear till now. Using the quasiclassical Green's function method, we show that a small concentration of magnetic impurities at the surface of the bridges can significantly help to suppress superconductivity and hence the supercurrent inside the systems while applying a gate field. This is because the gate field can enhance the depairing through the exchange interaction between the magnetic impurities at the surface and the superconductor. We also obtain a \emph{symmetric} suppression of the supercurrent with respect to the gate field, a signature of a direct gate effect. Future experiments can verify our predictions by modifying the surface with magnetic impurities.

cond-mat.mes-hall↗

DC Josephson effect between two Yu-Shiba-Rusinov bound states

Motivated by recent experiments [Nat. Phys. $\textbf{16}$, 1227 (2020)], we present here a theoretical study of the DC Josephson effect in a system comprising two magnetic impurities coupled to their respective superconducting electrodes and which exhibit Yu-Shiba-Rusinov (YSR) states. We make use of a mean-field Anderson model with broken spin symmetry to compute the supercurrent in this system for an arbitrary range of parameters (coupling between the impurities, orientation of the impurity spins, etc.). We predict a variety of physical phenomena such as (i) the occurrence of multiple $0-π$ transitions in the regime of weak coupling that can be induced by changing the energy of the YSR states or the temperature; (ii) the critical current strongly depends on the relative orientation of the impurity spins and it is maximized when the spins are either parallel or antiparallel, depending on the ground state of the impurities; and (iii) upon increasing the coupling between impurities, triplet superconductivity is generated in the system and it is manifested in a highly nonsinusoidal current-phase relation. In principle, these predictions can be tested experimentally with the existing realization of this system and the main lessons of this work are of great relevance for the field of superconducting spintronics.

cond-mat.supr-con↗