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Juan M. R. Parrondo

Publications and source records attributed to Juan M. R. Parrondo.

At least 19 recordsLinked to original sources

Thermalization in Spatially Extended Open Quantum Systems: Local versus Global Markovian Evolution

We investigate the dynamics of a qubit chain locally coupled to a thermal reservoir, modeled through repeated collisions with particles drawn from a heat bath. Under suitable conditions, the resulting Lindblad equation is thermodynamically consistent -- it drives the system toward thermal equilibrium -- while remaining local at short times. This framework reveals a crossover between the global Lindblad equation derived from the secular approximation in weak-coupling theory and the local dissipative models often employed in the literature, which generally fail to ensure thermodynamic consistency.

quant-ph↗

Sources of nonlinearity in the response of a driven nano-electromechanical resonator

Nanoelectromechanical resonators provide an ideal platform for investigating the interplay between electron transport and nonlinear mechanical motion. Externally driven suspended carbon nanotubes, containing an electrostatically defined quantum dot are especially promising. These devices possess two main sources of nonlinearity: the electromechanical coupling and the intrinsic contributions of the resonator that induce a Duffing-like nonlinear behavior. In this work, we observe the interplay between the two sources across different driving regimes. The main nonlinear feature we observe is the emergence of arch-like resonances in the electronic transport when the resonator is strongly driven. We show that our model is in good agreement with our experimental electron transport measurements on a suspended carbon nanotube. This characterization paves the way for the exploration of nonlinear phenomena using mesoscopic electromechanical resonators.

cond-mat.mes-hall↗

Stability of long-sustained oscillations induced by electron tunneling

Self-oscillations are the result of an efficient mechanism generating periodic motion from a constant power source. In quantum devices, these oscillations may arise due to the interaction between single electron dynamics and mechanical motion. We show that, due to the complexity of this mechanism, these self-oscillations may irrupt, vanish, or exhibit a bistable behaviour causing hysteresis cycles. We observe these hysteresis cycles and characterize the stability of different regimes in both single and double quantum dot configurations. In particular cases, we find these oscillations stable for over 20 seconds, many orders of magnitude above electronic and mechanical characteristic timescales, revealing the robustness of the mechanism at play.

cond-mat.mes-hall↗

Thermodynamics of Information

As early as 1867, two years after the introduction of the concept of entropy by Clausius, Maxwell showed that the limitations imposed by the second law of thermodynamics depend on the information that one possesses about the state of a physical system. A "very observant and neat-fingered being", later on named Maxwell demon by Kelvin, could arrange the molecules of a gas and induce a temperature or pressure gradient without performing work, in apparent contradiction to the second law. One century later, Landauer claimed that "information is physical", and showed that certain processes involving information, like overwriting a memory, need work to be completed and are unavoidably accompanied by heat dissipation. Thermodynamics of information analyzes this bidirectional influence between thermodynamics and information processing. The seminal ideas that Landauer and Bennett devised in the 1970s have been recently reformulated in a more precise and general way by realizing that informational states are out of equilibrium and applying new tools from non-equilibrium statistical mechanics.

cond-mat.stat-mech↗

Thermalization and dephasing in collisional reservoirs

We introduce a wide class of quantum maps that arise in collisional reservoirs and are able to thermalize a system if they operate in conjunction with an additional dephasing mechanism. These maps describe the effect of collisions and induce transitions between populations that obey detailed balance, but also create coherences that prevent the system from thermalizing. We combine these maps with a unitary evolution acting during random Poissonian times between collisions and causing dephasing. We find that, at a low collision rate, the nontrivial combination of these two effects causes thermalization in the system. This scenario is suitable for modeling collisional reservoirs at equilibrium. We justify this claim by identifying the conditions for such maps to arise within a scattering theory approach and provide a thorough characterization of the resulting thermalization process.

quant-ph↗

Ultrastrong coupling between electron tunneling and mechanical motion

The ultrastrong coupling of single-electron tunneling and nanomechanical motion opens exciting opportunities to explore fundamental questions and develop new platforms for quantum technologies. We have measured and modeled this electromechanical coupling in a fully-suspended carbon nanotube device and report a ratio of $g_\mathrm{m}/ω_\mathrm{m} = 2.72 \pm 0.14$, where $g_\mathrm{m}/2π= 0.80\pm 0.04$ GHz is the coupling strength and $ω_\mathrm{m}/2π=294.5$ MHz is the mechanical resonance frequency. This is well within the ultrastrong coupling regime and the highest among all other electromechanical platforms. We show that, although this regime was present in similar fully-suspended carbon nanotube devices, it went unnoticed. Even higher ratios could be achieved with improvement on device design.

cond-mat.mes-hall↗

Quantum scattering as a work source

We consider a collision between a moving particle and a fixed system, each having internal degrees of freedom. We identify the regime where the motion of the particle acts as a work source for the joint internal system, leading to energy changes which preserve the entropy. This regime arises when the particle has high kinetic energy and its quantum state of motion is broad in momentum and narrow in space, whether pure or mixed. In this case, the scattering map ruling the dynamics of the internal degrees of freedom becomes unitary and equivalent to that of a time-dependent interaction between the internal degrees of freedom of the colliding systems. It follows that the kinetic energy lost by the particle during the autonomous quantum collision coincides with the work performed by the time-dependent interaction. Recently, collisions with particles were shown to act as heat sources under suitable conditions; here we show that they can also act as work sources. This opens interesting perspectives for quantum thermodynamics formulations within scattering theory.

quant-ph↗

Inferring work by quantum superposing forward and time-reversal evolutions

The study of thermodynamic fluctuations allows one to relate the free energy difference between two equilibrium states with the work done on a system through processes far from equilibrium. This finding plays a crucial role in the quantum regime, where the definition of work becomes non-trivial. Based on these relations, here we develop a simple interferometric method allowing a direct estimation of the work distribution and the average dissipative work during a driven thermodynamic process by superposing the forward and time-reversal evolutions of the process. We show that our scheme provides useful upper bounds on the average dissipative work even without full control over the thermodynamic process, and we propose methodological variations depending on the possible experimental limitations encountered. Finally, we exemplify its applicability by an experimental proposal for implementing our method on a quantum photonics system, on which the thermodynamic process is performed through polarization rotations induced by liquid crystals acting in a discrete temporal regime.

quant-ph↗

Non-Abelian Quantum Transport and Thermosqueezing Effects

Modern quantum experiments provide examples of transport with non-commuting quantities, offering a tool to understand the interplay between thermal and quantum effects. Here we set forth a theory for non-Abelian transport in the linear response regime. Our key insight is to use generalized Gibbs ensembles with non-commuting charges as the basic building blocks and strict charge-preserving unitaries in a collisional setup. The linear response framework is then built using a collisional model between two reservoirs. We show that the transport coefficients obey Onsager reciprocity. Moreover, we find that quantum coherence, associated to the non-commutativity, acts so as to reduce the net entropy production, when compared to the case of commuting transport. This therefore provides a clear connection between quantum coherent transport and dissipation. As an example, we study heat and squeezing fluxes in bosonic systems, characterizing a set of thermosqueezing coefficients with potential applications in metrology and heat-to-work conversion in the quantum regime.

quant-ph↗

Quantum collisional thermostats

Collisional reservoirs are becoming a major tool for modelling open quantum systems. In their simplest implementation, an external agent switches on, for a given time, the interaction between the system and a specimen from the reservoir. Generically, in this operation the external agent performs work onto the system, preventing thermalization when the reservoir is at equilibrium. One can recover thermalization by considering an autonomous global setup where the reservoir particles colliding with the system possess a kinetic degree of freedom. The drawback is that the corresponding scattering problem is rather involved. Here, we present a formal solution of the problem in one dimension and for flat interaction potentials. The solution is based on the transfer matrix formalism and allows one to explore the symmetries of the resulting scattering map. One of these symmetries is micro-reversibility, which is a condition for thermalization. We then introduce two approximations of the scattering map that preserve these symmetries and, consequently, thermalize the system. These relatively simple approximate solutions constitute models of quantum thermostats and are useful tools to study quantum systems in contact with thermal baths. We illustrate their accuracy in a specific example, showing that both are good approximations of the exact scattering problem even in situations far from equilibrium. Moreover, one of the models consists of the removal of certain coherences plus a very specific randomization of the interaction time. These two features allow one to identify as heat the energy transfer due to switching on and off the interaction. Our results prompt the fundamental question of how to distinguish between heat and work from the statistical properties of the exchange of energy between a system and its surroundings.

quant-ph↗

Dissipation reduction and information-to-measurement conversion in DNA pulling experiments with feedback protocols

Information-to-energy conversion with feedback measurement stands as one of the most intriguing aspects of the thermodynamics of information in the nanoscale. To date, experiments have focused on feedback protocols for work extraction. Here we address the novel case of dissipation reduction in non-equilibrium systems with feedback. We perform pulling experiments on DNA hairpins with optical tweezers, with a general feedback protocol based on multiple measurements that includes either discrete-time or continuous-time feedback. While feedback can reduce dissipation, it remains unanswered whether it also improves free energy determination (information-to-measurement conversion). We define thermodynamic information Υ as the natural logarithm of the feedback efficacy, a quantitative measure of the efficiency of information-to-energy and information-to-measurement conversion in feedback protocols. We find that discrete and continuous-time feedback reduces dissipation by roughly kBTΥ without improvement in free energy determination. Remarkably, a feedback strategy (defined as a correlated sequence of feedback protocols) further reduces dissipation, enhancing information-to-measurement efficiency. Our study underlines the role of temporal correlations to develop feedback strategies for efficient information-to-energy conversion in small systems.

cond-mat.stat-mech↗

Quantifying entropy production in active fluctuations of the hair-cell bundle from time irreversibility and uncertainty relations

We introduce lower bounds for the rate of entropy production of an active stochastic process by quantifying the irreversibility of stochastic traces obtained from mesoscopic degrees of freedom. Our measures of irreversibility reveal signatures of time's arrow and provide bounds for entropy production even in the case of active fluctuations that have no drift. We apply these irreversibility measures to experimental recordings of spontaneous hair-bundle oscillations in mechanosensory hair cells from the ear of the bullfrog. By analysing the fluctuations of only the tip position of hair bundles, we reveal irreversibility in active oscillations and estimate an associated rate of entropy production of at least $\sim 3 k_{\rm B}$/s, on average. Applying thermodynamic uncertainty relations, we predict that measuring both the tip position of the hair bundle and the mechano-electrical transduction current that enters the hair cell leads to tighter lower bounds for the rate of entropy production, up to $\sim 10^3 k_{\rm B}$/s in the oscillatory regime.

cond-mat.stat-mech↗

Thermalization induced by quantum scattering

We use quantum scattering theory to study a fixed quantum system Y subject to collisions with massive particles X described by wave-packets. We derive the scattering map for system Y and show that the induced evolution crucially depends on the width of the incident wave-packets compared to the level spacing in Y . If Y is non-degenerate, sequential collisions with narrow wave-packets cause Y to decohere. Moreover, an ensemble of narrow packets produced by thermal effusion causes Y to thermalize. On the other hand, broad wave-packets can act as a source of coherences for Y , even in the case of an ensemble of incident wave-packets given by the effusion distribution, preventing thermalization. We illustrate our findings on several simple examples and discuss the consequences of our results in realistic experimental situations.

quant-ph↗

Micro-reversibility and thermalization with collisional baths

Micro-reversibility, that is, the time reversal symmetry exhibited by microscopic dynamics, plays a central role in thermodynamics and statistical mechanics. It is used to prove fundamental results such as Onsager reciprocal relations or fluctuation theorems. From micro-reversibility one can also prove that isolated systems and systems in contact with a thermal bath relax to micro-canonical and canonical ensembles, respectively. However, a number of problems arise when trying to reproduce this proof for classical and quantum collisional baths, consisting of particles from an equilibrium reservoir interacting with a localized system via collisions. In particular, it is not completely clear which distribution for the velocities of the incident particles warrants thermalization. Here, we clarify these issues by showing that Liouville's theorem is a necessary condition for micro-reversibility in classical and semi-classical scenarios. As a consequence, one must take into account all the canonical coordinates and momenta, including the position of the incident particles. Taking into account the position modifies the effective probability distribution of the velocity of the particles that interact with the system, which is no longer Maxwellian. We finally show an example of seemingly plausible collision rules that nonetheless violate the Liouville theorem and allow one to design machines that beat the second law of thermodynamics.

cond-mat.stat-mech↗

Inferring broken detailed balance in the absence of observable currents

Identifying dissipation is essential for understanding the physical mechanisms underlying nonequilibrium processes. {In living systems, for example, the dissipation is directly related to the hydrolysis of fuel molecules such as adenosine triphosphate (ATP)}. Nevertheless, detecting broken time-reversal symmetry, which is the hallmark of dissipative processes, remains a challenge in the absence of observable directed motion, flows, or fluxes. Furthermore, quantifying the entropy production in a complex system requires detailed information about its dynamics and internal degrees of freedom. Here we introduce a novel approach to detect time irreversibility and estimate the entropy production from time-series measurements, even in the absence of observable currents. We apply our technique to two different physical systems, namely, a partially hidden network and a molecular motor. Our method does not require complete information about the system dynamics and thus provides a new tool for studying nonequilibrium phenomena.

cond-mat.stat-mech↗

Autonomous thermal machine for amplification and control of energetic coherence

We present a model for an autonomous quantum thermal machine comprised of two qubits capable of manipulating and even amplifying the local coherence in a non-degenerate external system. The machine uses only thermal resources, namely, contact with two heat baths at different temperatures, and the external system has a non-zero initial amount of coherence. The method we propose allows for an interconversion between energy, both work and heat, and coherence in an autonomous configuration working in out-of-equilibrium conditions. This model raises interesting questions about the role of fundamental limitations on transformations involving coherence and opens up new possibilities in the manipulation of coherence by autonomous thermal machines.

quant-ph↗

Quantum fluctuation theorems for arbitrary environments: adiabatic and non-adiabatic entropy production

We analyze the production of entropy along non-equilibrium processes in quantum systems coupled to generic environments. First, we show that the entropy production due to final measurements and the loss of correlations obeys a fluctuation theorem in detailed and integral forms. Second, we discuss the decomposition of the entropy production into two positive contributions, adiabatic and non-adiabatic, based on the existence of invariant states of the local dynamics. Fluctuation theorems for both contributions hold only for evolutions verifying a specific condition of quantum origin. We illustrate our results with three relevant examples of quantum thermodynamic processes far from equilibrium.

quant-ph↗

Fluctuation-dissipation theorem for non-equilibrium quantum systems

The fluctuation-dissipation theorem (FDT) is a central result in statistical physics, both for classical and quantum systems. It establishes a relationship between the linear response of a system under a time-dependent perturbation and time correlations of certain observables in equilibrium. Here we derive a generalization of the theorem which can be applied to any Markov quantum system and makes use of the symmetric logarithmic derivative (SLD). There are several important benefits from our approach. First, such a formulation clarifies the relation between classical and quantum versions of the equilibrium FDT. Second, and more important, it facilitates the extension of the FDT to arbitrary quantum Markovian evolutions, as given by quantum maps. Third, it brings out the full connection between the FDT and the Quantum Fisher information, the figure of merit in quantum metrology.

quant-ph↗