arXiv subjects

Juan P. Garrahan

Publications and source records attributed to Juan P. Garrahan.

At least 145 records · Page 8Linked to original sources

arXiv2013

Kinetic constraints, hierarchical relaxation and onset of glassiness in strongly interacting and dissipative Rydberg gases

We show that the dynamics of a laser driven Rydberg gas in the limit of strong dephasing is described by a master equation with manifest kinetic constraints. The equilibrium state of the system is uncorrelated but the constraints in the dynamics lead to spatially correlated collective relaxation reminiscent of glasses. We study and quantify the evolution towards equilibrium in one and two dimensions, and analyze how the degree of glassiness and the relaxation time are controlled by the interaction strength between Rydberg atoms. We also find that spontaneous decay of Rydberg excitations leads to an interruption of glassy relaxation that takes the system to a highly correlated non-equilibrium stationary state. The results presented here, which are in principle also applicable other systems such as polar molecules and atoms with large magnetic dipole moments, show that the collective behavior of cold atomic and molecular ensembles can be similar to that found in soft condensed-matter systems.

physics.atom-ph↗

arXiv2013

Transition in coupled replicas may not imply a finite temperature ideal glass transition in glass forming systems

A key open question in the glass transition field is whether a finite temperature thermodynamic transition to the glass state exists or not. Recent simulations of coupled replicas in atomistic models have found signatures of a static transition as a function of replica coupling. This can be viewed as evidence of an associated thermodynamic glass transition in the uncoupled system. We demonstrate here that a different interpretation is possible. We consider the triangular plaquette model, an interacting spin system which displays (East model-like) glassy dynamics in the absence of any static transition. We show that when two replicas are coupled there is a curve of equilibrium phase transitions, between phases of small and large overlap, in the temperature-coupling plane (located on the self-dual line of an exact temperature/coupling duality of the system) which ends at a critical point. Crucially, in the limit of vanishing coupling the finite temperature transition disappears, and the uncoupled system is in the disordered phase at all temperatures. We discuss interpretation of atomistic simulations in light of this result.

cond-mat.stat-mech↗

arXiv2013

Fluctuating observation time ensembles in the thermodynamics of trajectories

The dynamics of stochastic systems, both classical and quantum, can be studied by analysing the statistical properties of dynamical trajectories. The properties of ensembles of such trajectories for long, but fixed, times are described by large-deviation (LD) rate functions. These LD functions play the role of dynamical free-energies: they are cumulant generating functions for time-integrated observables, and their analytic structure encodes dynamical phase behaviour. This "thermodynamics of trajectories" approach is to trajectories and dynamics what the equilibrium ensemble method of statistical mechanics is to configurations and statics. Here we show that, just like in the static case, there is a variety of alternative ensembles of trajectories, each defined by their global constraints, with that of trajectories of fixed total time being just one of these. We show that an ensemble of trajectories where some time-extensive quantity is constant (and large) but where total observation time fluctuates, is equivalent to the fixed-time ensemble, and the LD functions that describe one ensemble can be obtained from those that describe the other. We discuss how the equivalence between generalised ensembles can be exploited in path sampling schemes for generating rare dynamical trajectories.

cond-mat.stat-mech↗

arXiv2013

Comment on "Is there a breakdown of the Stokes-Einstein relation in Kinetically Constrained Models at low temperature?" by O. Blondel and C. Toninelli, arXiv:1307.1651

We consider the diffusion constant, D, of a probe particle coupled to the East model, extending previous numerical results for this model to encompass a total of twelve orders of magnitude in relaxation time, τ. Our considerations thus cover the full range of relaxation times relevant to experimental studies of reversible glass formers. Throughout this range, we show that the results of the model are consistent with a fractional Stokes-Einstein law, D \propto τ^{-ξ} with ξ \approx 0.77. The same data can also be fit by relating Dτ to the East model excitation concentration q, specifically, Dτ \sim 1/q^α with α \approx 1.6. In either case, breakdown of the Stokes-Einstein relation in this kinetically constrained model is unquestionable and large.

cond-mat.stat-mech↗

arXiv2013

Dynamical phase transitions, time-integrated observables and geometry of states

We show that there exist dynamical phase transitions (DPTs), as defined in [Phys. Rev. Lett. 110 135704 (2013)], in the transverse-field Ising model (TFIM) away from the static quantum critical points. We study a class of special states associated with singularities in the generating functions of time-integrated observables found in [Phys. Rev. B 88 184303 (2013)]. Studying the dynamics of these special states under the evolution of the TFIM Hamiltonian, we find temporal non-analtyicities in the initial-state return probability associated with dynamical phase transitions. By calculating the Berry phase and Chern number we show the set of special states have interesting geometric features similar to those associated with static quantum critical points.

cond-mat.stat-mech↗

arXiv2013

Rare-event trajectory ensemble analysis reveals metastable dynamical phases in lattice proteins

We explore the dynamical large-deviations of a lattice heteropolymer model of a protein by means of path sampling of trajectories. We uncover the existence of non-equilibrium dynamical phase-transitions in ensembles of trajectories between active and inactive dynamical phases, whose nature depends on properties of the interaction potential. When the full heterogeneity of interactions due to the amino-acid sequence is preserved, as in a fully interacting model or in a heterogeneous version of the Gō model where only native interactions are considered, the transition is between the equilibrium native state and a highly native but kinetically trapped state. In contrast, for the homogeneous Gō model, where there is a single native energy and the sequence plays no role, the dynamical transition is a direct consequence of the static bi-stability between unfolded and native states. In the heterogeneous case the native-active and native-inactive states, despite their static similarity, have widely varying dynamical properties, and the transition between them occurs even in lattice proteins whose sequences are designed to make them optimal folders.

cond-mat.soft↗

arXiv2013

Trajectory phase transitions and dynamical Lee-Yang zeros of the Glauber-Ising chain

We examine the generating function of the time-integrated energy for the one-dimensional Glauber-Ising model. At long times, the generating function takes on a large-deviation form and the associated cumulant generating function has singularities corresponding to continuous trajec- tory (or "space-time") phase transitions between paramagnetic trajectories and ferromagnetically or anti-ferromagnetically ordered trajectories. In the thermodynamic limit, the singularities make up a whole curve of critical points in the complex plane of the counting field. We evaluate analyti- cally the generating function by mapping the generator of the biased dynamics to a non-Hermitian Hamiltonian of an associated quantum spin chain. We relate the trajectory phase transitions to the high-order cumulants of the time-integrated energy which we use to extract the dynamical Lee-Yang zeros of the generating function. This approach offers the possibility to detect continuous trajectory phase transitions from the finite-time behaviour of measurable quantities.

cond-mat.stat-mech↗

arXiv2013

Calorimetric glass transition explained by hierarchical dynamic facilitation

The glass transition refers to the non-equilibrium process by which an equilibrium liquid is transformed to a non-equilibrium disordered solid, or vice versa. Associated response functions, such as heat capacities, are markedly different on cooling than on heating, and the response to melting a glass depends markedly on the cooling protocol by which the glass was formed. This paper shows how this irreversible behavior can be interpreted quantitatively in terms of an East-model picture of localized excitations (or soft spots) in which molecules can move with a specific direction, and from which excitations with the same directionality of motion can appear or disappear in adjacent regions. As a result of this facilitated dynamics, excitations become correlated in a hierarchical fashion. These correlations are manifested in the dynamic heterogeneity of the supercooled liquid phase. While equilibrium thermodynamics is virtually featureless, a non-equilibrium glass phase emerges when the model is driven out of equilibrium with a finite cooling rate. The correlation length of this emergent phase is large and increases with decreasing cooling rate. A spatially and temporally resolved fictive temperature encodes memory of its preparation. Parameters characterizing the model can be determined from reversible transport data, and with these parameters, predictions of the model agree well with irreversible differential scanning calorimetry.

cond-mat.soft↗

arXiv2013

Perspective: The Glass Transition

We provide here a brief perspective on the glass transition field. It is an assessment, written from the point of view of theory, of where the field is and where it seems to be heading. We first give an overview of the main phenomenological characteristics, or "stylised facts", of the glass transition problem, i.e. the central observations that a theory of the physics of glass formation should aim to explain in a unified manner. We describe recent developments, with a particular focus on real space properties, including dynamical heterogeneity and facilitation, the search for underlying spatial or structural correlations, and the relation between the thermal glass transition and athermal jamming. We then discuss briefly how competing theories of the glass transition have adapted and evolved to account for such real space issues. We consider in detail two conceptual and methodological approaches put forward recently, that aim to access the fundamental critical phenomenon underlying the glass transition, be it thermodynamic or dynamic in origin, by means of biasing of ensembles, of configurations in the thermodynamic case, or of trajectories in the dynamic case. We end with a short outlook.

cond-mat.stat-mech↗

arXiv2012

Dynamical Phases in the Full Counting Statistics of the Resonant-Level Model

We present a thermodynamic formalism to study the full counting statistics (FCS) of charge transport through a quantum dot coupled to two leads in the resonant-level model. We show that a close analogue of equilibrium phase transitions exists for the statistics of transferred charge; by tuning an appropriate `counting field', crossovers to different dynamical phases are possible. Our description reveals a mapping between the FCS of a given device and current measurements over a range of devices with different dot-lead coupling strengths. Further insight into features in the FCS is found by studying the occupation of the dot conditioned on the transported charge between the leads.

cond-mat.stat-mech↗

arXiv2012

Time-integrated observables as order parameters for dynamical phase transitions in closed quantum systems

The dynamical behaviour of many-body systems is often richer than what can be anticipated from their static properties. Here we show that in closed quantum systems this becomes evident by considering time-integrated observables as order parameters. In particular, the analytic properties of their generating functions, as estimated by full-counting statistics, allow to identify dynamical phases, i.e. phases with specific fluctuation properties of time-integrated observables, and to locate the transitions between these phases. We discuss in detail the case of the quantum Ising chain in a transverse field. We show that this model displays a continuum of quantum dynamical transitions, of which the static transition is just an end point. These singularities are not a consequence of particular choices of initial conditions or other external non-equilibrium protocols such as quenches in coupling constants. They can be probed generically through quantum jump statistics of an associated open problem, and for the case of the quantum Ising chain we outline a possible experimental realisation of this scheme by digital quantum simulation with cold ions.

cond-mat.stat-mech↗

arXiv2012

Characterization of dynamical phase transitions in quantum jump trajectories beyond the properties of the stationary state

We describe how to characterize dynamical phase transitions in open quantum systems from a purely dynamical perspective, namely, through the statistical behavior of quantum jump trajectories. This approach goes beyond considering only properties of the steady state. While in small quantum systems dynamical transitions can only occur trivially at limiting values of the controlling parameters, in many-body systems they arise as collective phenomena and within this perspective they are reminiscent of thermodynamic phase transitions. We illustrate this in open models of increasing complexity: a three-level system, a dissipative version of the quantum Ising model, and the micromaser. In these examples dynamical transitions are accompanied by clear changes in static behavior. This is however not always the case, and in general dynamical phase behavior needs to be uncovered by observables which are strictly dynamical, e.g. dynamical counting fields. We demonstrate this via the example of a class of models of dissipative quantum glasses, whose dynamics can vary widely despite having identical (and trivial) stationary states.

cond-mat.stat-mech↗

arXiv2012

Trajectory phase transitions, Lee-Yang zeros, and high-order cumulants in full counting statistics

We investigate Lee-Yang zeros of generating functions of dynamical observables and establish a general relation between phase transitions in ensembles of trajectories of stochastic many-body systems and the time evolution of high-order cumulants of such observables. This connects dynamical free-energies for full counting statistics in the long-time limit, which can be obtained via large-deviation methods and whose singularities indicate dynamical phase transitions, to observables that are directly accessible in simulation and experiment. As an illustration we consider facilitated spin models of glasses and show that from the short-time behavior of high-order cumulants it is possible to infer the existence and location of dynamical or "space-time" transitions in these systems.

cond-mat.stat-mech↗

arXiv2012

Thermodynamics of Quadrature Trajectories in Open Quantum Systems

We apply a large-deviation method to study the diffusive trajectories of the quadrature operators of light within a reservoir connected to dissipative quantum systems. We formulate the study of quadrature trajectories in terms of characteristic operators and show that in the long time limit the statistics of such trajectories obey a large-deviation principle. We take our motivation from homodyne detection schemes which allow the statistics of quadrature operator of the light field to be measured. We illustrate our approach with four examples of increasing complexity: a driven two-level system, a `blinking' three-level system, a pair of weakly-coupled two-level driven systems, and the micromaser. We discuss how quadrature operators can serve as alternative order parameters for the classification of dynamical phases, which is particularly useful in cases where the statistics of quantum jumps cannot distinguish between such phases. The formalism we introduce also allows us to analyse the properties of the light emitted by quantum jump trajectories which fluctuate far from the typical dynamics.

cond-mat.stat-mech↗

arXiv2012

Phase Transitions in Trajectories of a Superconducting Single-Electron Transistor Coupled to a Resonator

Recent progress in the study of dynamical phase transitions has been made with a large-deviation approach to study trajectories of stochastic jumps using a thermodynamic formalism. We study this method applied to an open quantum system consisting of a superconducting single-electron transistor, near the Josephson quasiparticle resonance, coupled to a resonator. We find that the dynamical behavior shown in rare trajectories can be rich even when the mean dynamical activity is small and thus the formalism gives insights into the form of fluctuations. The structure of the dynamical phase diagram found from the quantum-jump trajectories of the resonator is studied and we see that sharp transitions in the dynamical activity may be related to the appearance and disappearance of bistabilities in the state of the resonator as system parameters are changed. We also demonstrate that for a fast resonator, the trajectories of quasiparticles are similar to the resonator trajectories.

quant-ph↗

arXiv2012

Random and ordered phases of off-lattice rhombus tiles

We study the covering of the plane by non-overlapping rhombus tiles, a problem well-studied only in the limiting case of dimer coverings of regular lattices. We go beyond this limit by allowing tiles to take any position and orientation on the plane, to be of irregular shape, and to possess different types of attractive interactions. Using extensive numerical simulations we show that at large tile densities there is a phase transition from a fluid of rhombus tiles to a solid packing with broken rotational symmetry. We observe self-assembly of broken-symmetry phases, even at low densities, in the presence of attractive tile-tile interactions. Depending on tile shape and interactions the solid phase can be random, possessing critical orientational fluctuations, or crystalline. Our results suggest strategies for controlling tiling order in experiments involving `molecular rhombi'.

cond-mat.stat-mech↗

arXiv2012

Facilitated spin models of dissipative quantum glasses

We introduce a class of dissipative quantum spin models with local interactions and without quenched disorder that show glassy behaviour. These models are the quantum analogs of the classical facilitated spin models. Just like their classical counterparts, quantum facilitated models display complex glassy dynamics despite the fact that their stationary state is essentially trivial. In these systems, dynamical arrest is a consequence of kinetic constraints and not of static ordering. These models display a quantum version of dynamic heterogeneity: the dynamics towards relaxation is spatially correlated despite the absence of static correlations. Associated dynamical fluctuation phenomena such as decoupling of timescales is also observed. Moreover, we find that close to the classical limit quantum fluctuations can enhance glassiness, as recently reported for quantum liquids.

cond-mat.stat-mech↗

arXiv2012

Inactive dynamical phase of a symmetric exclusion process on a ring

We investigate the nature of the dynamically inactive phase of a simple symmetric exclusion process on a ring. We find that as the system's activity is tuned to a lower-than-average value the particles progressively lump into a single cluster, thereby forming a kink in the density profile. All dynamical regimes, and their finite size range of validity, are explicitly determined.

cond-mat.stat-mech↗