SearcharxivSearch

arXiv subjects

Juemin Yi

Publications and source records attributed to Juemin Yi.

3 recordsLinked to original sources

Universal 3:1 Scaling of Quantum-Confined Stark Spectra Revealed by a Three-Dimensional Profile

We report that the quantum-confined Stark effect spectrum exhibits a nearly rigid redshift while preserving its characteristic peak spacing patterns when increasing the electric field strength F. Using InGaN as a model system, we uncover two electric-field-independent scaling laws for the spectral peaks in both the sub-bandgap and above-bandgap regions and the coefficient ratio is near 3:1. With a novel three-dimensional (3D) visualization, we reveal that the sub-bandgap peak spacings scale as $\frac{12π\hbar^2}{L^2\sqrt{m_em_h}}$ while the above-bandgap peak spacings scale as $\frac{4π\hbar^2}{L^2\sqrt{m_em_h}}$, explaining the origin of the 3:1 ratio. This scaling behavior, validated in both InGaN and GaAs systems and at electroluminescence working conditions, shows that increasing F only expands the energy range and increases the number of peaks without altering the spacing. Beyond these laws, the 3D profile offers new insights into the Tauc background, Franz-Keldysh oscillations and coherence length, providing a powerful tool for the design and diagnostics of electro-optic devices.

cond-mat.mtrl-sci

Femtosecond field-driven on-chip unidirectional electronic currents in nonadiabatic tunnelling regime

Recently, asymmetric plasmonic nanojunctions [Karnetzky et. al., Nature Comm. 2471, 9 (2018)] have shown promise as on-chip electronic devices to convert femtosecond optical pulses to current bursts, with a bandwidth of multi-terahertz scale, although yet at low temperatures and pressures. Such nanoscale devices are of great interest for novel ultrafast electronics and opto-electronic applications. Here, we operate the device in air and at room temperature, revealing the mechanisms of photoemission from plasmonic nanojunctions, and the fundamental limitations on the speed of optical-to-electronic conversion. Inter-cycle interference of coherent electronic wavepackets results in a complex energy electron distribution and birth of multiphoton effects. This energy structure, as well as reshaping of the wavepackets during their propagation from one tip to the other, determine the ultrafast dynamics of the current. We show that, up to some level of approximation, the electron flight time is well-determined by the mean ponderomotive velocity in the driving field.

cond-mat.mes-hall

Strong spatial and spectral localization of surface plasmons in individual randomly disordered gold nanosponges

Porous nanosponges, percolated with a three-dimensional network of 10-nm sized ligaments, recently emerged as promising substrates for plasmon-enhanced spectroscopy and (photo-)catalysis. Experimental and theoretical work suggests surface plasmon localization in some hot-spot modes as the physical origin of their unusual optical properties, but so far the existence of such hot-spots has not been proven. Here we use scattering-type scanning near-field nano-spectroscopy on individual gold nanosponges to reveal spatially and spectrally confined modes with 10 nanometer localization lengths by mapping the local optical density of states. High quality factors of individual hot-spots of more than 40 are demonstrated. A statistical analysis of near-field intensity fluctuations unveils plasmonics in the strong localization regime. The observed field localization and enhancement make such nanosponges an appealing platform for a variety of applications ranging from nonlinear optics to strong-coupling physics.

cond-mat.mes-hall