arXiv subjects

Julian Bergmann

Publications and source records attributed to Julian Bergmann.

6 recordsLinked to original sources

arXiv2025

A pathway towards decentralized studies of radioactive post-lead elements and their applications in beyond standard model physics

Molecules have proven to be sensitive tools for studying physics beyond the standard model, with heavy and deformed nuclei offering decisive sensitivity to parity- and time-reversal-violating effects. However, almost all elements beyond lead, occupying the 6p~to~5f atomic orbitals, lack stable isotopes, hence molecules containing them are referred to as radioactive molecules. Among those, radium monofluoride has seen particular interest, but to date, research on radioactive molecules has mainly been limited to large-scale nuclear facilities. Here, we present a scheme that allows efficient and fast harvest of radioactive ions (including short-lived Ra), and show ion gas-phase reaction studies of singly and doubly charged Ra, Po, and Pb ions with SF$_6$ gas inside an ion trap. Our results show that the chemical reaction rate of Ra$^+$ is in line with trends of other alkaline earth elements, further support by quantum chemical computations. The reaction Ra$^{2+}$ + SF$_6$ $\rightarrow$ RaF${^+}$ + SF$_5^{+}$ achieves an almost unity conversion efficiency, making it particularly suitable for the application for studies in physics beyond the standard model. The scheme enables future decentralized research avenues with short-lived radioactive molecules for fundamental physics research at laboratories without the need for local nuclear reactors or accelerators.

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arXiv2023

Direct mass measurements of neutron-rich zinc and gallium isotopes: an investigation of the formation of the first r-process peak

The prediction of isotopic abundances resulting from the rapid neutron capture process (r-process) requires high-precision mass measurements. Using TITAN's on-line time-of-flight spectrometer, first time mass measurements are performed for $^{83}$Zn and $^{86}$Ga. These measurements reduced uncertainties, and are used to calculate isotopic abundances near the first r-process abundance peak using astrophysical conditions present during a binary neutron star (BNS) merger. Good agreement in abundance across a range of trajectories is found when comparing to several metal-poor stars while also strongly deviating from the solar r-process pattern. These findings point to a high degree of sensitivity to the electron fraction of a BNS merger on the final elemental abundance pattern for certain elements near the first r-process peak while others display universality. We find that small changes in electron fraction can produce distinct abundance patterns that match those of metal-poor stars with different classifications.

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arXiv2023

Mean range bunching of exotic nuclei produced by in-flight fragmentation and fission -- Stopped-beam experiments with increased efficiency

The novel technique of mean range bunching has been developed and applied at the projectile fragment separator FRS at GSI in four experiments of the FAIR phase-0 experimental program. Using a variable degrader system at the final focal plane of the FRS, the ranges of the different nuclides can be aligned, allowing to efficiently implant a large number of different nuclides simultaneously in a gas-filled stopping cell or an implantation detector. Stopping and studying a cocktail beam overcomes the present limitations of stopped-beam experiments. The conceptual idea of mean range bunching is described and illustrated using simulations. In a single setting of the FRS, 37 different nuclides were stopped in the cryogenic stopping cell and were measured in a single setting broadband mass measurement with the multiple-reflection time-of-flight mass spectrometer of the FRS Ion Catcher.

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arXiv2022

Studying Gamow-Teller transitions and the assignment of isomeric and ground states at $N=50$

Direct mass measurements of neutron-deficient nuclides around the $N=50$ shell closure below $^{100}$Sn were performed at the FRS Ion Catcher (FRS-IC) at GSI, Germany. The nuclei were produced by projectile fragmentation of $^{124}$Xe, separated in the fragment separator FRS and delivered to the FRS-IC. The masses of 14 ground states and two isomers were measured with relative mass uncertainties down to $1\times 10^{-7}$ using the multiple-reflection time-of-flight mass spectrometer of the FRS-IC, including the first direct mass measurements of $^{98}$Cd and $^{97}$Rh. A new $Q_\mathrm{EC} = 5437\pm67$ keV was obtained for $^{98}$Cd, resulting in a summed Gamow-Teller (GT) strength for the five observed transitions ($0^+\longrightarrow1^+$) as $B(\text{GT})=2.94^{+0.32}_{-0.28}$. Investigation of this result in state-of-the-art shell model approaches sheds light into a better understanding of the GT transitions in even-even isotones at $N=50$. The excitation energy of the long-lived isomeric state in $^{94}$Rh was determined for the first time to be $293\pm 21$ keV. This, together with the shell model calculations, allows the level ordering in $^{94}$Rh to be understood.

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arXiv2020

Separation of atomic and molecular ions by ion mobility with an RF carpet

Gas-filled stopping cells are used at accelerator laboratories for the thermalization of high-energy radioactive ion beams. Common challenges of many stopping cells are a high molecular background of extracted ions and limitations of extraction efficiency due to space-charge effects. At the FRS Ion Catcher at GSI, a new technique for removal of ionized molecules prior to their extraction out of the stopping cell has been developed. This technique utilizes the RF carpet for the separation of atomic ions from molecular contaminant ions through their difference in ion mobility. Results from the successful implementation and test during an experiment with a 600~MeV/u $^{124}$Xe primary beam are presented. Suppression of molecular contaminants by three orders of magnitude has been demonstrated. Essentially background-free measurement conditions with less than $1~\%$ of background events within a mass-to-charge range of 25 u/e have been achieved. The technique can also be used to reduce the space-charge effects at the extraction nozzle and in the downstream beamline, thus ensuring high efficiency of ion transport and highly-accurate measurements under space-charge-free conditions.

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arXiv2019

A Novel Method for the Measurement of Half-Lives and Decay Branching Ratios of Exotic Nuclei

A novel method for simultaneous measurement of masses, Q-values, isomer excitation energies, half-lives and decay branching ratios of exotic nuclei has been demonstrated. The method includes first use of a stopping cell as an ion trap, combining containment of precursors and decay-recoils for variable durations in a cryogenic stopping cell (CSC), and afterwards the identification and counting of them by a multiple-reflection time-of-flight mass spectrometer (MR-TOF-MS). Feasibility has been established by recording the decay and growth of $^{216}$Po and $^{212}$Pb (alpha decay) and of $^{119m2}$Sb (t$_{1/2}$ = 850$\pm$90 ms) and $^{119g}$Sb (isomer transition), obtaining half-lives and branching ratios consistent with literature values. Hardly any non-nuclear-decay losses have been observed in the CSC for up to $\sim$10 seconds, which exhibits its extraordinary cleanliness. For $^{119}$Sb, this is the first direct measurement of the ground and second isomeric state masses, resolving the discrepancies in previous excitation energy data. These results pave the way for the measurement of branching ratios of exotic nuclei with multiple decay channels.

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