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Julian Kaiser

Publications and source records attributed to Julian Kaiser.

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Anisotropic magnetoelastic coupling in the honeycomb magnet Na$_3$Co$_2$SbO$_6$

We present magnetization and dilatometry measurements on the honeycomb cobaltate Na$_3$Co$_2$SbO$_6$ and map out its detailed field-temperature phase diagram down to sub-Kelvin temperatures. Our data for in-plane magnetic fields show a strongly anisotropic $c^{*}$-axis lattice response, which is dominated by the variation of Co--O--Co bond angles according to \textit{ab initio} calculations. At $T = 0.4$~K, the magnetization $M(B)$ exhibits step-like features that are also highly anisotropic. In the case of $B \parallel b$, a small hysteresis observed around the second field-induced magnetic transition ($B_{c2}$) indicates its first-order character, whereas divergence of the magnetic Gr\"uneisen parameter at $B_{c2}$ is suppressed upon cooling and signals the absence of quantum critical behavior upon entering the field-polarized state. None of our thermodynamic measurements provide evidence for a field-induced quantum spin liquid state near or above $B_{c2}$.

cond-mat.str-el

Elastoresistance as probe of strain-controlled entropy from Kondo scattering

Heavy-fermion metals are prototype correlated electron systems for the study of Kondo entanglement and quantum criticality. We use the symmetry decomposed elastoresistance to uncover the fingerprints of strain-dependent Kondo scattering as function of temperature and magnetic field in the prototypical tetragonal Kondo lattice YbRh$_2$Si$_2$. By combining longitudinal and transverse resistance measurements under uniaxial strain applied along the tetragonal $[100]$ and $[110]$ directions, we obtain the elastoresistive responses in the $A_{1g}$, $B_{1g}$, and $B_{2g}$ symmetry channels. While the responses in the symmetry-breaking channels are negligible, the isotropic $A_{1g}$ elastoresistance displays characteristic sign changes and approaches huge values at low temperatures. Scaling analysis and comparison with linear thermal expansion measurements reveals that the elastoresistance probes the contribution of Kondo scattering to the strain dependence of magnetic entropy and signals strain-controlled quantum criticality upon cooling to 2 K.

cond-mat.str-el

Intermediate field-induced phase of the honeycomb magnet BaCo$_2$(AsO$_4$)$_2$

We use magnetometry, calorimetry, and high-resolution capacitive dilatometry, as well as single-crystal neutron diffraction to explore temperature-field phase diagram of the anisotropic honeycomb magnet BaCo$_2$(AsO$_4)_2$. Our data reveal four distinct ordered states observed for in-plane magnetic fields. Of particular interest is the narrow region between 0.51 and 0.55 T that separates the up-up-down order from the fully polarized state and coincides with the field range where signatures of the spin-liquid behavior have been reported. We show that magnetic Bragg peaks persist in this intermediate phase, thus ruling out its spin-liquid nature. However, the simultaneous nonmonotonic evolution of nuclear Bragg peaks suggests the involvement of the lattice, witnessed also in other regions of the phase diagram where large changes in the sample length are observed upon entering the magnetically ordered states. Our data highlight the importance of lattice effects in BaCo$_2$(AsO$_4)_2$.

cond-mat.str-el

Metallic conductivity on Na-deficient structural domain walls in the spin-orbit Mott insulator Na$_2$IrO$_3$

Honeycomb Na$_2$IrO$_3$ is a prototype spin-orbit Mott insulator and Kitaev magnet. We report a combined structural and electrical resistivity study of Na$_2$IrO$_3$ single crystals. Laue back-scattering diffraction indicates twinning with $\pm 120^\circ$ rotation around the $c^*$-axis while scanning electron microscopy displays nanothin lines parallel to all three b-axis orientations of twin domains. Energy dispersive x-ray analysis line-scans across such domain walls indicate no change of the Ir signal intensity, i.e. intact honeycomb layers, while the Na intensity is reduced down to $\sim 2/3$ of its original value at the domain walls, implying significant hole doping. Utilizing focused-ion-beam micro-sectioning, the temperature dependence of the electrical resistance of individual domain walls is studied. It demonstrates the tuning through the metal-insulator transition into a correlated-metal ground state by increasing hole doping.

cond-mat.str-el