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Julien Tailleur

Publications and source records attributed to Julien Tailleur.

At least 55 records · Page 3Linked to original sources

Lamellar to micellar phases and beyond: when tactic active systems admit free-energy functionals

We consider microscopic models of active particles whose velocities, rotational diffusivities, and tumbling rates depend on the gradient of a local field, which is either externally imposed or depends on all particle positions. Despite the fundamental differences between active and passive dynamics at the microscopic scale, we show that a large class of such tactic active systems admit fluctuating hydrodynamics equivalent to those of interacting Brownian colloids in equilibrium. We exploit this mapping to show how taxis may lead to the lamellar and micellar phases observed for soft repulsive colloids. In the context of chemotaxis, we show how the competition between chemoattractant and chemorepellent may lead to a bona-fide equilibrium liquid-gas phase separation in which a loss of thermodynamic stability of the fluid signals the onset of a chemotactic collapse.

cond-mat.soft↗

Surface Tensions between Active Fluids and Solid Interfaces: bare vs dressed

We analyze the surface tension exerted at the interface between an active fluid and a solid boundary in terms of tangential forces. Focusing on active systems known to possess an equation of state for the pressure, we show that interfacial forces are of a more complex nature. Using a number of macroscopic setups, we show that the surface tension is a combination of an equation-of-state abiding part and of setup-dependent contributions. The latter arise from generic setup-dependent steady currents which "dress" the measurement of the "bare" surface tension. The former shares interesting properties with its equilibrium counterpart, and can be used to generalize the Young-Laplace law to active systems. We finally show how a suitably designed probe can directly access this bare surface tensions, which can also be computed using a generalized Virial formula.

cond-mat.soft↗

Activated escape of a self-propelled particle from a metastable state

We study the noise-driven escape of active Brownian particles (ABPs) and run-and-tumble particles (RTPs) from confining potentials. In the small noise limit, we provide an exact expression for the escape rate in term of a variational problem in any dimension. For RTPs in one dimension, we obtain an explicit solution, including the first sub-leading correction. In two dimensions we solve the escape from a quadratic well for both RTPs and ABPs. In contrast to the equilibrium problem we find that the escape rate depends explicitly on the full shape of the potential barrier, and not only on its height. This leads to a host of unusual behaviors. For example, when a particle is trapped between two barriers it may preferentially escape over the higher one. Moreover, as the self-propulsion speed is varied, the escape route may discontinuously switch from one barrier to the other, leading to a dynamical phase transition.

cond-mat.soft↗

Optimizing active work: Dynamical phase transitions, collective motion, and jamming

Active work measures how far the local self-forcing of active particles translates into real motion. Using Population Monte Carlo methods, we investigate large deviations in the active work for repulsive active Brownian disks. Minimizing the active work generically results in dynamical arrest; in contrast, despite the lack of aligning interactions, trajectories of high active work correspond to a collectively moving, aligned state. We use heuristic and analytic arguments to explain the origin of dynamical phase transitions separating the arrested, typical, and aligned regimes.

cond-mat.stat-mech↗

Non-Gaussian noise without memory in active matter

Modeling the dynamics of an individual active particle invariably involves an isotropic noisy self-propulsion component, in the form of run-and-tumble motion or variations around it. This nonequilibrium source of noise is neither white---there is persistence---nor Gaussian. While emerging collective behavior in active matter has hitherto been attributed to the persistent ingredient, we focus on the non-Gaussian ingredient of self-propulsion. We show that by itself, that is without invoking any memory effect, it is able to generate particle accumulation close to boundaries and effective attraction between otherwise repulsive particles, a mechanism which generically leads to motility-induced phase separation in active matter.

cond-mat.stat-mech↗

Generalized thermodynamics of Motility-Induced Phase Separation: Phase equilibria, Laplace pressure, and change of ensembles

Motility-induced phase separation (MIPS) leads to cohesive active matter in the absence of cohesive forces. We present, extend and illustrate a recent generalized thermodynamic formalism which accounts for its binodal curve. Using this formalism, we identify both a generalized surface tension, that controls finite-size corrections to coexisting densities, and generalized forces, that can be used to construct new thermodynamic ensembles. Our framework is based on a nonequilibrium generalization of the Cahn-Hilliard equation and we discuss its application to active particles interacting either via quorum-sensing interactions or directly through pairwise forces.

cond-mat.stat-mech↗

Optimized Diffusion of Run-and-Tumble Particles in Crowded Environments

We study the transport of self-propelled particles in dynamic complex environments. To obtain exact results, we introduce a model of run-and-tumble particles (RTPs) moving in discrete time on a $d$-dimensional cubic lattice in the presence of diffusing hard core obstacles. We derive an explicit expression for the diffusivity of the RTP, which is exact in the limit of low density of fixed obstacles. To do so, we introduce a generalization of Kac's theorem on the mean return times of Markov processes, which we expect to be relevant for a large class of lattice gas problems. Our results show the diffusivity of RTPs to be nonmonotonic in the tumbling probability for low enough obstacle mobility. These results prove the potential for optimization of the transport of RTPs in crowded and disordered environments with applications to motile artificial and biological systems.

cond-mat.stat-mech↗

Sedimentation of self-propelled Janus colloids: polarization and pressure

We study experimentally-using Janus colloids-and theoretically-using Active Brownian Particles- the sedimentation of dilute active colloids. We first confirm the existence of an exponential density profile. We show experimentally the emergence of a polarized steady state outside the effective equilibrium regime, i.e. when v_s is not much smaller than the propulsion speed. The experimental distribution of polarization is very well described by the theoretical prediction with no fitting parameter. We then discuss and compare three different definitions of pressure for sedimenting particles: the weight of particles above a given height, the flux of momentum and active impulse, and the force density measured by pressure gauges.

cond-mat.soft↗

Generalized Thermodynamics of Phase Equilibria in Scalar Active Matter

Motility-induced phase separation (MIPS) arises generically in fluids of self-propelled particles when interactions lead to a kinetic slowdown at high densities. Starting from a continuum description of scalar active matter, akin to a generalized Cahn-Hilliard equation, we give a general prescription for the mean densities of coexisting phases in flux-free steady states that amounts, at a hydrodynamics scale, to extremizing an effective free energy. We illustrate our approach on two well-known models: self-propelled particles interacting either through a density-dependent propulsion speed or via direct pairwise forces. Our theory accounts quantitatively for their phase diagrams, providing a unified description of MIPS.

cond-mat.stat-mech↗

Exact Hydrodynamic Description of Active Lattice Gases

We introduce a class of lattice gas models of active matter systems whose hydrodynamic description can be derived exactly. We illustrate our approach by considering two systems exhibiting two of the most studied collective behaviours in active matter: the motility-induced phase separation and the transition to collective motion. In both cases, we derive coupled partial differential equation describing the dynamics of the local density and polarization fields and show how they quantitatively predict the emerging properties of the macroscopic lattice gases.

cond-mat.stat-mech↗

Mechanical pressure and momentum conservation in dry active matter

We relate the breakdown of equations of states for the mechanical pressure of generic dry active systems to the lack of momentum conservation in such systems. We show how sources and sinks of momentum arise generically close to confining walls. These typically depend on the interactions of the container with the particles, which makes the mechanical pressure a container-dependent quantity. We show that an equation of state is recovered if the dynamics of the orientation of active particles are decoupled from other degrees of freedom and lead to an apolar bulk steady-state. This is related to the fact that the mean steady-state active force density is the divergence of the flux of "active impulse", an observable which measures the mean momentum particles will receive from the substrate in the future.

cond-mat.stat-mech↗

Extraction du solvant d'un hydrogel par des gouttes de bactéries B. subtilis

We observe that small drops of a Bacillus subtilis suspension deposited on agar strongly increase in volume while similar bacteria-void drops do not. By measuring the bacterial concentration within the drop at different heights, we show that the biomass increase due to the constant bacterial cell-division is too small to explain the drop bloating. Rather, the increased volume is caused by the presence of surfactin - a surfactant produced by the bacteria - which induces a water flow out of the environment by an osmotic capillary effect. The required concentration is very low (< 1 mM), four orders of magnitude smaller than the concentration of, for example, glucose to produce a similar effect. The ability of B. subtilis to extract water from its environment probably contributes to collective migration modes like mass swarming. It also gives rise to a new displacement mode independent of cellular motility: By combining the osmotic and wetting effects of the surfactant, B. subtilis can actively induce the sliding of the bacterial colony on substrates tilted by angles as small as 0.1 degrees.

cond-mat.soft↗

Active depinning of bacterial droplets: the collective surfing of Bacillus subtilis

How systems are endowed with migration capacity is a fascinating question with implications ranging from the design of novel active systems to the control of microbial populations. Bacteria, which can be found in a variety of environments, have developed among the richest set of locomotion mechanisms both at the microscopic and collective levels. Here, we uncover experimentally a new mode of collective bacterial motility in humid environment through the depinning of bacterial droplets. While capillary forces are notoriously enormous at the bacterial scale, even capable of pinning water droplets of millimetric size on inclined surfaces, we show that bacteria are able to harness a variety of mechanisms to unpin contact lines, hence inducing a collective slipping of the colony across the surface. Contrary to flagella-dependent migration modes like swarming we show that this much faster `colony surfing' still occurs in mutant strains of \textit{Bacillus subtilis} lacking flagella. The active unpinning seen in our experiments relies on a variety of microscopic mechanisms which could each play an important role in the migration of microorganisms in humid environment.

physics.bio-ph↗

Entropy production in field theories without time reversal symmetry: Quantifying the non-equilibrium character of active matter

Active matter systems operate far from equilibrium due to the continuous energy injection at the scale of constituent particles. At larger scales, described by coarse-grained models, the global entropy production rate S quantifies the probability ratio of forward and reversed dynamics and hence the importance of irreversibility at such scales: it vanishes whenever the coarse-grained dynamics of the active system reduces to that of an effective equilibrium model. We evaluate S for a class of scalar stochastic field theories describing the coarse-grained density of self-propelled particles without alignment interactions, capturing such key phenomena as motility-induced phase separation. We show how the entropy production can be decomposed locally (in real space) or spectrally (in Fourier space), allowing detailed examination of the spatial structure and correlations that underly departures from equilibrium. For phase-separated systems, the local entropy production is concentrated mainly on interfaces with a bulk contribution that tends to zero in the weak-noise limit. In homogeneous states, we find a generalized Harada-Sasa relation that directly expresses the entropy production in terms of the wavevector-dependent deviation from the fluctuation-dissipation relation between response functions and correlators. We discuss extensions to the case where the particle density is coupled to a momentum-conserving solvent, and to situations where the particle current, rather than the density, should be chosen as the dynamical field. We expect the new conceptual tools developed here to be broadly useful in the context of active matter, allowing one to distinguish when and where activity plays an essential role in the dynamics.

cond-mat.stat-mech↗

Active particles with soft and curved walls: Equation of state, ratchets, and instabilities

We study, from first principles, the pressure exerted by an active fluid of spherical particles on general boundaries in two dimensions. We show that, despite the non-uniform pressure along curved walls, an equation of state is recovered upon a proper spatial averaging. This holds even in the presence of pairwise interactions between particles or when asymmetric walls induce ratchet currents, which are accompanied by spontaneous shear stresses on the walls. For flexible obstacles, the pressure inhomogeneities lead to a modulational instability as well as to the spontaneous motion of short semi-flexible filaments. Finally, we relate the force exerted on objects immersed in active baths to the particle flux they generate around them.

cond-mat.stat-mech↗

How far from equilibrium is active matter?

Active matter systems are driven out of thermal equilibrium by a lack of generalized Stokes-Einstein relation between injection and dissipation of energy at the microscopic scale. We consider such a system of interacting particles, propelled by persistent noises, and show that, at small but finite persistence time, their dynamics still satisfy a time-reversal symmetry. To do so, we compute perturbatively their steady-state measure and show that, for short persistent times, the entropy production rate vanishes. This endows such systems with an effective Fluctuation-Dissipation theorem akin to that of thermal equilibrium systems. Last we show how interacting particle systems with viscous drags and correlated noises can be seen as in equilibrium with a visco-elastic bath but driven out of equilibrium by non-conservative forces, hence providing an energetic insight on the departure of active systems from equilibrium.

cond-mat.stat-mech↗

Lyapunov exponents of stochastic systems---from micro to macro

Lyapunov exponents of dynamical systems are defined from the rates of divergence of nearby trajectories. For stochastic systems, one typically assumes that these trajectories are generated under the "same noise realization". The purpose of this work is to critically examine what this expression means. For Brownian particles, we consider two natural interpretations of the noise: intrinsic to the particles or stemming from the fluctuations of the environment. We show how they lead to different distributions of the largest Lyapunov exponent as well as different fluctuating hydrodynamics for the collective density field. We discuss, both at microscopic and macroscopic levels, the limits in which these noise prescriptions become equivalent. We close this paper by providing an estimate of the largest Lyapunov exponent and of its fluctuations for interacting particles evolving with the Dean-Kawasaki dynamics.

cond-mat.stat-mech↗