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Jun Miyawaki

Publications and source records attributed to Jun Miyawaki.

6 recordsLinked to original sources

Divergence between long- and short-wavelength magnon damping in spinel ferrites

The realization of practical, high-speed magnonic devices requires engineering magnetic materials with low dissipation over wide frequency ranges. While optical and microwave probes are used to infer the damping of low energy/long wavelength modes, the degree to which these $q\sim0$ properties translate into higher-energy, finite-momentum modes remains an important open question. Here, we utilize a combination of ferromagnetic resonance (FMR) and resonant inelastic x-ray scattering on spinel ferrites Li$_{0.5}$Al$_x$Fe$_{2.5-x}$O$_4$ to probe magnons in both the short- and long-wavelength limits. We observe that aluminum substitution both markedly reduces the magnon bandwidth and drastically shortens the high-$q$ magnon lifetimes, in sharp contrast to the ultralow magnon damping inferred from FMR. These findings demonstrate a disparity between how non-magnetic substituents impact magnon damping in the long- and short-wavelength limits, providing a new perspective for assessing candidate materials for magnonic devices.

cond-mat.mtrl-sci

Achieving Ultrahigh Resolution with High Efficiency: Optical Design of the 2D-RIXS Spectrometer at NanoTerasu BL02U

A state-of-the-art Resonant Inelastic X-ray Scattering (RIXS) facility, composed of a dedicated beamline and a 2D-RIXS spectrometer, has been constructed and commissioned at BL02U in NanoTerasu, Japan. This paper reports the optical design and optimization of this spectrometer, aiming for an ultrahigh energy resolution of <10 meV in the soft X-ray range. Conventional RIXS spectrometers using monochromatic incident X-rays suffer from a severe trade-off between energy resolution and measurement efficiency, which makes achieving resolutions of <10 meV practically unfeasible. To overcome this limitation, we adopted the $hν^2$ concept using dispersive incident X-rays, based on a comparative study. This approach decouples the energy resolution from the incident bandwidth. We estimate that our 2D-RIXS spectrometer improves efficiency by more than a factor of 10 compared to conventional spectrometers. The 2D-RIXS spectrometer has been successfully commissioned, demonstrating that sub-10 meV resolution measurement is achievable with practical throughput. While development continues towards the ultimate design resolution, the successful implementation validates the design strategy and offers a pathway for future high-performance RIXS instrumentation.

physics.ins-det

2D-RIXS: Resonant inelastic x-ray scattering microscopy with high energy and spatial resolutions

A two-dimensional resonant inelastic x-ray scattering (2D-RIXS) microscopy system has been developed at the beamline BL02U of NanoTerasu. The instrument combines a Wolter type-I mirror for spatial imaging with a varied-line-spacing grating spectrometer, simultaneously achieving micrometer-scale spatial resolution and ultrahigh energy resolution in the soft x-ray regime. Test chart measurements confirm a vertical spatial resolution of 1.0 um near the field-of-view center, and the horizontal resolution determined by the incident beam footprint is 0.8 um. RIXS imaging capabilities have been demonstrated by the measurements of a patterned NanoTerasu logo and exfoliated NiPS${}_3$ nanoflakes, highlighting its efficiency in locating specific microscale regions within inhomogeneous samples. These results establish 2D-RIXS microscopy as a position-sensitive probe of elementary excitations in quantum materials and functional devices.

cond-mat.mtrl-sci

Localized character of charge excitations for La$_{2-x}$Sr$_{x}$NiO$_{4+δ}$ revealed by oxygen $K$-edge resonant inelastic X-ray scattering

We performed a resonant inelastic X-ray scattering (RIXS) study of La$_{2-x}$Sr$_{x}$NiO$_{4+δ}$ (LSNO) at the oxygen $K$ edge to investigate the nature of the doped holes with regard to charge excitations. Charge excitations of the hole-doped nickelates are found to be almost independent of momentum transfer, indicating that the doped holes are strongly localized in character. Additionally, conspicuous changes in energy position are in temperature dependence. These characters are observed in stark contrast to those of the high-$T_{c}$ cuprate La$_{2-x}$Sr$_{x}$CuO$_{4}$ (LSCO), where delocalized doped holes form charge excitations with sizable momentum dependence in the CuO$_2$ plane. This distinct nature of charge excitations of doped holes is consistent with the metallicity of the materials and could be caused by strong electron-phonon coupling and weak quantum spin fluctuation in the nickelates.

cond-mat.str-el

Revisiting the phase diagram of T*-type La$_{1-x/2}$Eu$_{1-x/2}$Sr$_x$CuO$_4$ using Oxygen $K$-edge X-ray absorption spectroscopy

Oxygen $K$-edge X-ray absorption spectroscopy measurements were conducted on T*-type La$_{1-x/2}$Eu$_{1-x/2}$Sr$_x$CuO$_4$ (LESCO) to estimate the hole density ($n_{\rm h}$) and investigate the oxidation annealing effect on $n_{\rm h}$. A drastic increase in $n_{\rm h}$ due to annealing was found. The increase in $n_{\rm h}$ cannot be explained solely by the oxygen gain due to annealing, suggesting that delocalized holes are introduced into the CuO$_2$ plane. A phase diagram of LESCO was redrawn against $n_{\rm h}$.

cond-mat.supr-con

Electronic Structures of Ferromagnetic CeAgSb$_2$:Soft X-ray Absorption, Magnetic Circular Dichroism and Angle-Resolved Photoemission Spectroscopies

We report a combined study for the electronic structures of ferromagnetic CeAgSb$_2$ using soft X-ray absorption (XAS), magnetic circular dichroism (XMCD), and angle-resolved photoemission (ARPES) spectroscopies. The Ce $M_{4, 5}$ XAS spectra show very small satellite structures, reflecting a strongly localized character of the Ce $4f$ electrons. The linear dichroism effects in the Ce $M_{4, 5}$ XAS spectra demonstrate the ground state Ce $4f$ symmetry of $Γ{_6}$, the spatial distribution of which is directed along the $c$-axis. The XMCD results give support to the picture of local-moment magnetism in CeAgSb$_2$. Moreover it is also found that the theoretical band dispersions for LaAgSb$_2$ provides better description of the ARPES band structures than those for CeAgSb$_2$. Nevertheless, ARPES spectra at the Ce $3d$-$4f$ resonance show the momentum dependence for the intensity ratio between Ce $4f^{1}_{5/2}$ and $4f^{1}_{7/2}$ peaks in a part of the Brillouin zone, suggesting the non-negligible momentum dependent hybridization effect between the Ce $4f$ and the conduction electrons. This is associated with the moderate mass enhancement in CeAgSb$_2$.

cond-mat.str-el