arXiv subjects

Jun Yin

Publications and source records attributed to Jun Yin.

At least 127 records · Page 7Linked to original sources

arXiv2019

A Closer Look at Disentangling in $β$-VAE

In many data analysis tasks, it is beneficial to learn representations where each dimension is statistically independent and thus disentangled from the others. If data generating factors are also statistically independent, disentangled representations can be formed by Bayesian inference of latent variables. We examine a generalization of the Variational Autoencoder (VAE), $β$-VAE, for learning such representations using variational inference. $β$-VAE enforces conditional independence of its bottleneck neurons controlled by its hyperparameter $β$. This condition is in general not compatible with the statistical independence of latents. By providing analytical and numerical arguments, we show that this incompatibility leads to a non-monotonic inference performance in $β$-VAE with a finite optimal $β$.

stat.ML↗

arXiv2019

Electronic phase separation in topological surface states of rhombohedral graphite

Of the two stable forms of graphite, hexagonal (HG) and rhombohedral (RG), the former is more common and has been studied extensively. RG is less stable, which so far precluded its detailed investigation, despite many theoretical predictions about the abundance of exotic interaction-induced physics. Advances in van der Waals heterostructure technology have now allowed us to make high-quality RG films up to 50 graphene layers thick and study their transport properties. We find that the bulk electronic states in such RG are gapped and, at low temperatures, electron transport is dominated by surface states. Because of topological protection, the surface states are robust and of high quality, allowing the observation of the quantum Hall effect, where RG exhibits phase transitions between gapless semimetallic phase and gapped quantum spin Hall phase with giant Berry curvature. An energy gap can also be opened in the surface states by breaking their inversion symmetry via applying a perpendicular electric field. Moreover, in RG films thinner than 4 nm, a gap is present even without an external electric field. This spontaneous gap opening shows pronounced hysteresis and other signatures characteristic of electronic phase separation, which we attribute to emergence of strongly-correlated electronic surface states.

cond-mat.mes-hall↗

arXiv2019

Stacking Order in Graphite Films Controlled by Van der Waals Technology

In graphite crystals, layers of graphene reside in three equivalent, but distinct, stacking positions typically referred to as A, B, and C projections. The order in which the layers are stacked defines the electronic structure of the crystal, providing an exciting degree of freedom which can be exploited for designing graphitic materials with unusual properties including predicted high-temperature superconductivity and ferromagnetism. However, the lack of control of the stacking sequence limits most research to the stable ABA form of graphite. Here we demonstrate a strategy to control the stacking order using van der Waals technology. To this end, we first visualise the distribution of stacking domains in graphite films and then perform directional encapsulation of ABC-rich graphite crystallites with hexagonal boron nitride (hBN). We found that hBN-encapsulation which is introduced parallel to the graphite zigzag edges preserves ABC stacking, while encapsulation along the armchair edges transforms the stacking to ABA. The technique presented here should facilitate new research on the important properties of ABC graphite.

cond-mat.mes-hall↗

arXiv2019

Large Polaron Generation and Dynamics in 3D Metal-Halide Perovskites

In recent years, metal halide perovskites have generated tremendous interest for optoelectronic applications and their underlying fundamental properties. Due to the large electron-phonon coupling characteristic of soft lattices, self-trapping phenomena are expected to dominate hybrid perovskite photoexcitation dynamics. Yet, while the photogeneration of small polarons was proven in low dimensional perovskites, the nature of polaron excitations in technologically relevant 3D perovskites, and their influence on charge carrier transport, remain elusive. In this study, we used a combination of first principle calculations and advanced spectroscopy techniques spanning the entire optical frequency range to pin down polaron features in 3D metal halide perovskites. Mid-infrared photoinduced absorption shows the photogeneration of states associated to low energy intragap electronic transitions with lifetime up to the ms time scale, and vibrational mode renormalization in both frequency and amplitude. Density functional theory supports the assignment of the spectroscopic features to large polarons leading to new intra gap transitions, hardening of phonon mode frequency, and renormalization of the oscillator strength. Theory provides quantitative estimates of the charge carrier masses and mobilities increase upon polaron formation, confirming experimental results. Overall, this work contributes to complete the scenario of elementary photoexcitations in metal halide perovskites and highlights the importance of polaronic transport in perovskite-based optoelectronic devices.

physics.app-ph↗

arXiv2019

Energy Constraints for Climate Models from Hydrologic Partitioning

It is well known that evaporative cooling of Earth's surface water reduces the amount of radiation that goes into sensible heat, namely the portion of radiation that produces higher temperatures. However, a rigorous use of long-term hydrologic measurements and the related theories of hydrologic partitioning have not yet been fully exploited to quantify these effects on climate. Here, we show that the Budyko's curve, a well-known and efficient framework for water balance estimation, can be effectively utilized to partition the surface energy fluxes by expressing the long-term evaporative fraction as a function of the dryness index. The combination of this energy partitioning method with hydrological observations allows us to estimate the surface energy components at watershed and continental scales. Analyzing climate model outputs through this new lens reveals energy biases due to inaccurate parameterization of hydrological and atmospheric processes, offering insight into model parameterization and providing useful information for improving climate projections.

physics.geo-ph↗

arXiv2019

Exploring the Star Formation Histories of Galaxies in Different Environments from MaNGA Spectra

The star formation history (SFH) of galaxies allow us to investigate when galaxies formed their stars and assembled their mass. We can constrain the SFH with high level of precision from galaxies with resolved stellar populations, since we are able to discriminate between stars of different ages from the spectrum they emit. However, the relative importance of secular evolution (nature) over nurture is not yet clear, and separating the effects of interaction-driven evolution in the observed galaxy properties is not trivial. The aim of this study is to use MaNGA (Mapping Nearby Galaxies at APO) Integral Field Unit (IFU) data, in combination with multi-wavelength data, to constrain the SFH of nearby isolated galaxies. We present here the new techniques we are developing to constrain the SFH with high level of precision from Spectral Energy Distribution (SED) fitting. This study is part of a China-Chile collaboration program where we are applying these new techniques to investigate how galaxies formed and evolve in different environments.

astro-ph.GA↗

arXiv2019

Planar and van der Waals heterostructures for vertical tunnelling single electron transistors

Despite a rich choice of two-dimensional materials, which exists these days, heterostructures, both vertical (van der Waals) and in-plane, offer an unprecedented control over the properties and functionalities of the resulted structures. Thus, planar heterostructures allow p-n junctions between different two-dimensional semiconductors and graphene nanoribbons with well-defined edges; and vertical heterostructures resulted in the observation of superconductivity in purely carbon-based systems and realisation of vertical tunnelling transistors. Here we demonstrate simultaneous use of in-plane and van der Waals heterostructures to build vertical single electron tunnelling transistors. We grow graphene quantum dots inside the matrix of hexagonal boron nitride, which allows a dramatic reduction of the number of localised states along the perimeter of the quantum dots. The use of hexagonal boron nitride tunnel barriers as contacts to the graphene quantum dots make our transistors reproducible and not dependent on the localised states, opening even larger flexibility when designing future devices.

cond-mat.mes-hall↗

arXiv2018

Dimensional reduction, quantum Hall effect and layer parity in graphite films

The quantum Hall effect (QHE) originates from discrete Landau levels forming in a two-dimensional (2D) electron system in a magnetic field. In three dimensions (3D), the QHE is forbidden because the third dimension spreads Landau levels into multiple overlapping bands, destroying the quantisation. Here we report the QHE in graphite crystals that are up to hundreds of atomic layers thick - thickness at which graphite was believed to behave as a 3D bulk semimetal. We attribute the observation to a dimensional reduction of electron dynamics in high magnetic fields, such that the electron spectrum remains continuous only in the direction of the magnetic field, and only the last two quasi-one-dimensional (1D) Landau bands cross the Fermi level. In sufficiently thin graphite films, the formation of standing waves breaks these 1D bands into a discrete spectrum, giving rise to a multitude of quantum Hall plateaux. Despite a large number of layers, we observe a profound difference between films with even and odd numbers of graphene layers. For odd numbers, the absence of inversion symmetry causes valley polarisation of the standing-wave states within 1D Landau bands. This reduces QHE gaps, as compared to films of similar thicknesses but with even layer numbers because the latter retain the inversion symmetry characteristic of bilayer graphene. High-quality graphite films present a novel QHE system with a parity-controlled valley polarisation and intricate interplay between orbital, spin and valley states, and clear signatures of electron-electron interactions including the fractional QHE below 0.5 K.

cond-mat.mes-hall↗

arXiv2018

Stellar population synthesis of galaxies with chemical evolution model

The derivation of accurate stellar populations of galaxies is a non-trivial task because of the well-known age-metallicity degeneracy. We aim to break this degeneracy by invoking a chemical evolution model(CEM) for isolated disk galaxy, where its metallicity enrichment history(MEH) is modelled to be tightly linked to its star formation history(SFH). Our CEM has been successfully tested on several local group dwarf galaxies whose SFHs and MEHs have been both independently measured from deep color-magnitude diagrams of individual stars. By introducing the CEM into the stellar population fitting algorithm as a prior, we expect that the SFH of galaxies could be better constrained.

astro-ph.GA↗

arXiv2018

Random band matrices in the delocalized phase, I: Quantum unique ergodicity and universality

Consider $N\times N$ symmetric one-dimensional random band matrices with general distribution of the entries and band width $W \geq N^{3/4+\varepsilon}$ for any $\varepsilon>0$. In the bulk of the spectrum and in the large $N$ limit, we obtain the following results. (i) The semicircle law holds up to the scale $N^{-1+\varepsilon}$ for any $\varepsilon>0$. (ii) The eigenvalues locally converge to the point process given by the Gaussian orthogonal ensemble at any fixed energy. (iii) All eigenvectors are delocalized, meaning their ${\rm L}^\infty$ norms are all simultaneously bounded by $N^{-\frac{1}{2}+\varepsilon}$ (after normalization in ${\rm L}^2$) with overwhelming probability, for any $\varepsilon>0$. (iv )Quantum unique ergodicity holds, in the sense that the local ${\rm L}^2$ mass of eigenvectors becomes equidistributed with overwhelming probability. We extend the mean-field reduction method \cite{BouErdYauYin2017}, which required $W=Ω(N)$, to the current setting $W \ge N^{3/4+\varepsilon}$. Two new ideas are: (1) A new estimate on the "generalized resolvent" of band matrices when $W \geq N^{3/4+\varepsilon}$. Its proof, along with an improved fluctuation average estimate, will be presented in parts 2 and 3 of this series \cite {BouYanYauYin2018,YanYin2018}. (2) A strong (high probability) version of the quantum unique ergodicity property of random matrices. For its proof, we construct perfect matching observables of eigenvector overlaps and show they satisfying the eigenvector moment flow equation \cite{BouYau2017} under the matrix Brownian motions.

math.PR↗

arXiv2018

Random band matrices in the delocalized phase, II: Generalized resolvent estimates

This is the second part of a three part series abut delocalization for band matrices. In this paper, we consider a general class of $N\times N$ random band matrices $H=(H_{ij})$ whose entries are centered random variables, independent up to a symmetry constraint. We assume that the variances $\mathbb E |H_{ij}|^2$ form a band matrix with typical band width $1\ll W\ll N$. We consider the generalized resolvent of $H$ defined as $G(Z):=(H - Z)^{-1}$, where $Z$ is a deterministic diagonal matrix such that $Z_{ij}=\left(z 1_{1\leq i \leq W}+\widetilde z 1_{ i > W} \right) δ_{ij}$, with two distinct spectral parameters $z\in \mathbb C_+:=\{z\in \mathbb C:{\rm Im} z>0\}$ and $\widetilde z\in \mathbb C_+\cup \mathbb R$. In this paper, we prove a sharp bound for the local law of the generalized resolvent $G$ for $W\gg N^{3/4}$. This bound is a key input for the proof of delocalization and bulk universality of random band matrices in \cite{PartI}. Our proof depends on a fluctuations averaging bound on certain averages of polynomials in the resolvent entries, which will be proved in \cite{PartIII}.

math.PR↗

arXiv2018

Magnon-assisted tunnelling in van der Waals heterostructures based on CrBr3

The growing family of two-dimensional (2D) materials that are now available can be used to assemble van der Waals heterostructures with a wide range of properties. Of particular interest are tunnelling heterostructures, which have been used to study the electronic states both in the tunnelling barrier and in the emitter and collector contacts. Recently, 2D ferromagnets have been studied theoretically and experimentally. Here we investigate electron tunnelling through a thin (2-6 layers) ferromagnetic CrBr3 barrier. For devices with non-magnetic barriers, conservation of momentum can be relaxed by phonon-assisted tunnelling or by tunnelling through localised states. In the case of our ferromagnetic barrier the dominant tunnelling mechanisms are the emission of magnons at low temperatures or scattering of electrons on localised magnetic excitations above the Curie temperature. Tunnelling with magnon emission offers the possibility of injecting spin into the collector electrode.

cond-mat.mes-hall↗

arXiv2018

Unusual suppression of the superconducting energy gap and critical temperature in atomically thin NbSe2

It is well known that superconductivity in thin films is generally suppressed with decreasing thickness. This suppression is normally governed by either disorder-induced localization of Cooper pairs, weakening of Coulomb screening, or generation and unbinding of vortex-antivortex pairs as described by the Berezinskii-Kosterlitz-Thouless (BKT) theory. Defying general expectations, few-layer NbSe2 - an archetypal example of ultrathin superconductors - has been found to remain superconducting down to monolayer thickness. Here we report measurements of both the superconducting energy gap and critical temperature in high-quality monocrystals of few-layer NbSe2, using planar-junction tunneling spectroscopy and lateral transport. We observe a fully developed gap that rapidly reduces for devices with the number of layers N < 5, as does their ctitical temperature. We show that the observed reduction cannot be explained by disorder, and the BKT mechanism is also excluded by measuring its transition temperature that for all N remains very close to Tc. We attribute the observed behavior to changes in the electronic band structure predicted for mono- and bi- layer NbSe2 combined with inevitable suppression of the Cooper pair density at the superconductor-vacuum interface. Our experimental results for N > 2 are in good agreement with the dependences of the gap and Tc expected in the latter case while the effect of band-structure reconstruction is evidenced by a stronger suppression of the gap and the disappearance of its anisotropy for N = 2. The spatial scale involved in the surface suppression of the density of states is only a few angstroms but cannot be ignored for atomically thin superconductors.

cond-mat.supr-con↗

arXiv2018

Reinforcement of Climate Hiatus by Decadal Modulation of Daily Cloud Cycle

Based on observations and climate model results, it has been suggested that the recent slowdown of global warming trends (climate hiatus), which took place in the early 2000s, might be due to enhanced ocean heat uptake. Here we suggest an alternative hypothesis which, at least in part, would relate such slowdown to unaccounted energy reflected or reemitted by clouds. We show that the daily cloud cycle is strongly linked to pacific decadal oscillation (PDO) and that its decadal variations during the climate hiatus have an overall cooling effect. Such an effect may have partially, and temporarily, counteracted the greenhouse warming trends.

physics.ao-ph↗

arXiv2018

Radiative effects of daily cloud cycle: general methodology and application to cloud fraction

The daily cloud cycle (DCC) and its response to global warming are critical to the Earth's energy budget, but their radiative effects have not been systematically quantified. Toward this goal, here we analyze the radiation at the top of the atmosphere and propose a measure of the DCC radiative effect (DCCRE) as the difference between the total radiative fluxes with the full cloud cycle and its uniformly distributed cloud counterpart. We apply it to the cloud fraction from four climate models that participated in the second phase of the Cloud Feedback Model Inter-comparison Project. The results allow us to objectively compare inter-model differences in the daily cycle of cloud fraction and their influences on the global energy balance. In particular, the spatial patterns of the DCC response to global warming obtained in our analysis suggest possible impacts on large-scale circulation. Such a framework can be used for conducting a more systematic evaluation of the DCC in climate models and observations with the goal to reduce uncertainty in climate projections.

physics.ao-ph↗

arXiv2017

Graphene hot-electron light bulb: incandescence from hBN-encapsulated graphene in air

The excellent electronic and mechanical properties of graphene allow it to sustain very large currents, enabling its incandescence through Joule heating in suspended devices. Although interesting scientifically and promising technologically, this process is unattainable in ambient environment, because graphene quickly oxidises at high temperatures. Here, we take the performance of graphene-based incandescent devices to the next level by encapsulating graphene with hexagonal boron nitride (hBN). Remarkably, we found that the hBN encapsulation provides an excellent protection for hot graphene filaments even at temperatures well above 2000 K. Unrivalled oxidation resistance of hBN combined with atomically clean graphene/hBN interface allows for a stable light emission from our devices in atmosphere for many hours of continuous operation. Furthermore, when confined in a simple photonic cavity, the thermal emission spectrum is modified by a cavity mode, shifting the emission to the visible range spectrum. We believe our results demonstrate that hBN/graphene heterostructures can be used to conveniently explore the technologically important high-temperature regime and to pave the way for future optoelectronic applications of graphene-based systems.

cond-mat.mes-hall↗

arXiv2017

Hidden Warming Effects of Cloud Cycle Errors in Climate Models

Clouds' efficiency at reflecting solar radiation and trapping the terrestrial one is strongly modulated by their diurnal cycle. Much attention has been paid to mean cloud properties due to their critical role in climate projections; however, less research has been devoted to their diurnal cycle. Here, we quantify the mean, amplitude, and phase of the cloud cycles in current climate models and compare them with satellite observations and reanalysis data. While the mean values appear to be reliable, the amplitude and phase of the diurnal cycles of clouds show marked inconsistencies, especially over land. We show that, to compensate for the increased net radiation input implied by such errors, an overestimation of the cloud liquid water path may be introduced during calibration of climate models to keep temperatures in line with observations. These discrepancies are likely to be related to cloud parametrization problems in relation to atmospheric convection.

physics.ao-ph↗

arXiv2017

Response and Feedback of Cloud Diurnal Cycle to Rising Temperatures

By reflecting solar radiation and reducing longwave emissions, clouds regulate the earth's radiation budget, impacting atmospheric circulation and cloud dynamics. Given the diurnal fluctuation of shortwave and longwave radiation, a shift in the cloud cycle phase (CCP) may lead to substantial feedbacks to the climate system. While most efforts have focused on the overall cloud feedback, the response of CCP to climate change has received much less attention. Here we analyze the variations of CCP using both long-term global satellite records and general circulation models (GCM) simulations to evaluate their impacts on the earth's energy budget. Satellite records show that in warm periods the CCP shifts earlier in the morning over the oceans and later in the afternoon over the land. Although less marked and with large inter-model spread, similar shifting patterns also occur in GCMs over the oceans with non-negligible CCP feedbacks. Over the land, where the GCM results are not conclusive, our findings are supported by atmospheric boundary layer models. A simplified radiative model further suggests that such shifts may in turn cause reduced reflection of solar radiation, thus inducing a positive feedback on climate. The crucial role of the cloud cycle calls for increased attention to the temporal evolution of the cloud diurnal cycle in climate models.

physics.ao-ph↗