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Jun-Ming Liu

Publications and source records attributed to Jun-Ming Liu.

44 records · Page 3Linked to original sources

Spin-glass ground state in a triangular-lattice compound YbZnGaO$_4$

We report on comprehensive results identifying the ground state of a triangular-lattice structured YbZnGaO$_4$ to be spin glass, including no long-range magnetic order, prominent broad excitation continua, and absence of magnetic thermal conductivity. More crucially, from the ultralow-temperature a.c. susceptibility measurements, we unambiguously observe frequency-dependent peaks around 0.1 K, indicating the spin-glass ground state. We suggest this conclusion to hold also for its sister compound YbMgGaO$_4$, which is confirmed by the observation of spin freezing at low temperatures. We consider disorder and frustration to be the main driving force for the spin-glass phase.

cond-mat.str-el↗

Cycloidal magnetism driven ferroelectricity in double tungstate LiFe(WO$_4$)$_2$

Tungstates $A$WO$_4$ with the wolframite structure characterized by the $A$O$_6$ octahedral zigzag chains along the $c$-axis, can be magnetic if $A$=Mn, Fe, Co, Cu, Ni. Among them, MnWO$_4$ is a unique member with a cycloid Mn$^{2+}$ spin order developed at low temperature, leading to an interesting type-II multiferroic behavior. However, so far no other multiferroic material in the tungstate family has been found. In this work, we present the synthesis and the systematic study of the double tungstate LiFe(WO$_4$)$_2$. Experimental characterizations including structural, thermodynamic, magnetic, neutron powder diffraction, and pyroelectric measurements, unambiguously confirm that LiFe(WO$_4$)$_2$ is the secondly found multiferroic system in the tungstate family. The cycloidal magnetism driven ferroelectricity is also verified by density functional theory calculations. Although here the magnetic couplings between Fe ions are indirect, namely via the so-called super-super-exchanges, the temperatures of magnetic and ferroelectric transitions are surprisingly much higher than those of MnWO$_4$.

cond-mat.mtrl-sci↗

High density array of epitaxial BiFeO3 nanodots with robust and reversibly switchable topological domain states

The exotic topological domains in ferroelectrics and multiferroics have attracted extensive interest in recent years due to their novel functionalities and potential applications in nanoelectronic devices. One of the key challenges for such applications is a realization of robust yet reversibly switchable nanoscale topological domain states with high density, wherein spontaneous topological structures can be individually addressed and controlled. This has been accomplished in our work using high density arrays of epitaxial BiFeO3 (BFO) nanodots with lateral size as small as ~60 nm. We demonstrate various types of spontaneous topological domain structures, including center-convergent domains, center-divergent domains, and double-center domains, which are stable over sufficiently long time yet can be manipulated and reversibly switched by electric field. The formation mechanisms of these topological domain states, assisted by the accumulation of compensating charges on the surface, have also been revealed. These result demonstrated that these reversibly switchable topological domain arrays are promising for applications in high density nanoferroelectric devices such as nonvolatile memories

cond-mat.mtrl-sci↗

Weyl Ferroelectric Semimetal

The recent discoveries of ferroelectric metal and Weyl semimetal (WSM) have stimulated a natural question: whether these two exotic states of matter can coexist in a single material or not. These two discoveries ensure us that physically it is possible since both of them share the same necessary condition, the broken inversion symmetry. Here, by using first-principles calculations, we demonstrate that the experimentally synthesized nonmagnetic HgPbO$_3$ represents a unique example of such hybrid "\emph{Weyl ferroelectric semimetal}". Its centrosymmetric $R\bar{3}c$ phase will undergo a ferroelectric phase transition to the ferroelectric $R3c$ structure. Both phases are metallic and the ferroelectric phase owns a spontaneous polarization of 33 $μ$C/cm$^2$. Most importantly, it also harbors six pairs of chiral Weyl nodes around the Fermi level to be an oxide WSM. The structural symmetry broken phase transition induces a topological phase transition. The coexistence of ferroelectricity and Weyl nodes in HgPbO$_3$ is an ideal platform for exploring multiphase interaction and mutual control. The Weyl nodes can be tuned by external pulse electric field, which is promising for potential applications of integrated topotronic and ferroelectric devices.

cond-mat.mtrl-sci↗

An extensive survey of dayside diffuse aurora based on optical observations at Yellow River Station

By using 7 years optical auroral observations obtained at Yellow River Station (magnetic latitude $76.24\,^{\circ}{\rm C}$N) at Ny-Alesund, Svalbard, we performed the first extensive survey for the dayside diffuse auroras (DDAs) and acquired observational results as follows. (1) The DDAs can be classified into two broad categories, i.e., unstructured and structured DDAs. The unstructured DDAs are mainly distributed in the morning and afternoon, but the structured DDAs predominantly occurred around the magnetic local noon (MLN). (2) The unstructured DDAs observed in morning and afternoon present obviously different properties. The afternoon ones are much stable and seldom show pulsating property. (3) The DDAs are more easily observed under geomagnetically quiet times. (4) The structured DDAsmainly show patchy, stripy, and irregular forms and are often pulsating and drifting. The drifting directions are mostly westward (with speed $\sim$5km/s), but there are cases showing eastward or poleward drifting. (5) The stripy DDAs are exclusively observed near theMLN and,most importantly, their alignments are confirmed to be consistent with the direction of ionospheric convection near the MLN. (6) A new auroral form, called throat aurora, is found to be developed from the stripy DDAs. Based on the observational results and previous studies, we proposed our explanations to the DDAs. We suggest that the unstructured DDAs observed in the morning are extensions of the nightside diffuse aurora to the dayside, but that observed in the afternoon are predominantly caused by proton precipitations. $\textit{(Abstract continues in PDF).}$

physics.space-ph↗

Multiferroic materials and magnetoelectric physics: symmetry, entanglement, excitation, and topology

Multiferroics are those materials with more than one ferroic order, and magnetoelectricity refers to the mutual coupling between magnetism and electricity. The discipline of multiferroicity has never been so highly active as that in the first decade of the twenty-first century, and it has become one of the hottest disciplines of condensed matter physics and materials science. A series of milestones and steady progress in the past decade have enabled our understanding of multiferroic physics substantially comprehensive and profound, which is further pushing forward the research frontier of this exciting area. The availability of more multiferroic materials and improved magnetoelectric performance are approaching to make the applications within reach. While seminal review articles covering the major progress before 2010 are available, an updated review addressing the new achievements since that time becomes imperative. In this review, following a concise outline of the basic knowledge of multiferroicity and magnetoelectricity, we summarize the important research activities on multiferroics, especially magnetoelectricity and related physics in the last six years. We consider not only single-phase multiferroics but also multiferroic heterostructures. We address the physical mechanisms regarding magnetoelectric coupling so that the backbone of this divergent discipline can be highlighted. A series of issues on lattice symmetry, magnetic ordering, ferroelectricity generation, electromagnon excitations, multiferroic domain structure and domain wall dynamics, and interfacial coupling in multiferroic heterostructures, will be revisited in an updated framework of physics. In addition, several emergent phenomena and related physics, including magnetic skyrmions and generic topological structures associated with magnetoelectricity will be discussed.

cond-mat.mtrl-sci↗

Multiferroicity and Magnetoelectric Coupling in TbMnO3 Thin Films

In this work, we report the growth and functional characterizations of multiferroic TbMnO3 thin films grown on Nb-doped SrTiO3 (001) substrates using pulsed laser deposition. By performing detailed magnetic and ferroelectric properties measurements, we demonstrate that the multiferroicity of spin origin known in the bulk crystals can be successfully transferred to TbMnO3 thin films. Meanwhile, anomalous magnetic transition and unusual magnetoelectric coupling related to Tb moments are observed, suggesting a modified magnetic configuration of Tb in the films as compared to the bulk counterpart. In addition, it is found that the magnetoelectric coupling enabled by Tb moments can even be seen far above the Tb spin ordering temperature, which provides a larger temperature range for the magnetoelectric control involving Tb moments.

cond-mat.mtrl-sci↗

Recent Progress of Multiferroic Perovskite Manganites

Many multiferroic materials, with various chemical compositions and crystal structures, have been discovered in the past years. Among these multiferroics, some perovskite manganites with ferroelectricity driven by magnetic orders are of particular interest. In these multiferroic perovskite manganites, not only their multiferroic properties are quite prominent, but also the involved physical mechanisms are very plenty and representative. In this Brief Review, we will introduce some recent theoretical and experimental progress on multiferroic manganites.

cond-mat.mtrl-sci↗