arXiv subjects

Junghyun Lee

Publications and source records attributed to Junghyun Lee.

40 records · Page 3Linked to original sources

arXiv2019

Decoherence of dipolar spin ensembles in diamond

We present a combined theoretical and experimental study of solid-state spin decoherence in an electronic spin bath, focusing specifically on ensembles of nitrogen vacancy (NV) color centers in diamond and the associated substitutional nitrogen spin bath. We perform measurements of NV spin free induction decay times $T_2^*$ and spin-echo coherence times $T_2$ in 25 diamond samples with nitrogen concentrations [N] ranging from 0.01 to 300\,ppm. We introduce a microscopic model and perform numerical simulations to quantitatively explain the degradation of both $T_2^*$ and $T_2$ over four orders of magnitude in [N]. Our results resolve a long-standing discrepancy observed in NV $T_2$ experiments, enabling us to describe NV ensemble spin coherence decay shapes as emerging consistently from the contribution of many individual NV.

quant-ph↗

arXiv2018

Geometric phase magnetometry using a solid-state spin

Magnetometry is a powerful technique for the non-invasive study of biological and physical systems. A key challenge lies in the simultaneous optimization of magnetic field sensitivity and maximum field range. In interferometry-based magnetometry, a quantum two-level system acquires a dynamic phase in response to an applied magnetic field. However, due to the 2π periodicity of the phase, increasing the coherent interrogation time to improve sensitivity results in reduced field range. Here we introduce a route towards both large magnetic field range and high sensitivity via measurements of the geometric phase acquired by a quantum two-level system. We experimentally demonstrate geometric-phase magnetometry using the optically addressable electronic spin associated with the nitrogen vacancy (NV) color center in diamond. Our approach enables unwrapping of the 2π phase ambiguity, decoupling of magnetic field range from sensitivity, and enhancement of the field range by about 400 times. We also find additional improvement in sensitivity in the nonadiabatic regime, and study how geometric-phase decoherence depends on adiabaticity. Our results show that the geometric phase can be a versatile tool for quantum sensing applications.

quant-ph↗

arXiv2017

High Resolution Magnetic Resonance Spectroscopy Using Solid-State Spins

We demonstrate a synchronized readout (SR) technique for spectrally selective detection of oscillating magnetic fields with sub-millihertz resolution, using coherent manipulation of solid state spins. The SR technique is implemented in a sensitive magnetometer (~50 picotesla/Hz^(1/2)) based on nitrogen vacancy (NV) centers in diamond, and used to detect nuclear magnetic resonance (NMR) signals from liquid-state samples. We obtain NMR spectral resolution ~3 Hz, which is nearly two orders of magnitude narrower than previously demonstrated with NV based techniques, using a sample volume of ~1 picoliter. This is the first application of NV-detected NMR to sense Boltzmann-polarized nuclear spin magnetization, and the first to observe chemical shifts and J-couplings.

quant-ph↗

arXiv2015

NMR Technique for Determining the Depth of Shallow Nitrogen-Vacancy Centers in Diamond

We demonstrate a robust experimental method for determining the depth of individual shallow Nitrogen-Vacancy (NV) centers in diamond with $\sim1$ nm uncertainty. We use a confocal microscope to observe single NV centers and detect the proton nuclear magnetic resonance (NMR) signal produced by objective immersion oil, which has well understood nuclear spin properties, on the diamond surface. We determine the NV center depth by analyzing the NV NMR data using a model that describes the interaction of a single NV center with the statistically-polarized proton spin bath. We repeat this procedure for a large number of individual, shallow NV centers and compare the resulting NV depths to the mean value expected from simulations of the ion implantation process used to create the NV centers, with reasonable agreement.

quant-ph↗