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Junjian Mi

Publications and source records attributed to Junjian Mi.

3 recordsLinked to original sources

Dimensionality-Dependent Exciton Dispersion in a Single-Band Mott Insulator

Excitonic band structure is critical for investigating exciton dynamics. Theoretically, quantum effects from exchange scattering between electron-hole pairs significantly modulate exciton dispersion. Here, we report the direct observation of dimensionality-dependent exciton dispersion in a single-band Mott insulator Nb3Cl8 through high-resolution electron energy loss spectroscopy. In the high-temperature phase, the exciton in Nb3Cl8 hosts an exceptionally large binding energy, and exhibits clear quasi-two-dimensional massless linear dispersion. In contrast, in the low-temperature phase, the exciton splits into two bands, both displaying three-dimensional parabolic dispersion. These dramatic changes in the exciton dispersion stem from the dimensional mutation driven by a substantial enhancement of interlayer coupling across the phase transition. This Letter provides a clear and typical example of how exciton behavior evolves with dimensionality.

cond-mat.str-el

Extremely large magnetoresistance and chiral anomaly in the nodal-line semimetal ZrAs2

We performed the detailed magnetotransport measurements and first principle calculations to study the electronic properties of the transition metal dipnictides ZrAs2, which is a topological nodal-line semimetal. Extremely large unsaturated magnetoresistance (MR) which is up to 1.9 * 10^4 % at 2 K and 14 T was observed with magnetic field along the c-axis. The nonlinear magnetic field dependence of Hall resistivity indicates the multi-band features, and the electron and hole are nearly compensated according to the analysis of the two-band model, which may account for the extremely large unsaturated MR at low temperatures. The evident Shubnikov-de Haas (SdH) oscillations at low temperatures are observed and four distinct oscillation frequencies are extracted. The first principle calculations and angle-dependent SdH oscillations reveal that the Fermi surface consists of three pockets with different anisotropy. The observed twofold symmetry MR with electric field along the b-axis direction is consistent with our calculated Fermi surface structures. Furthermore, the negative magnetoresistance (NMR) with magnetic field in parallel with electric field is observed, which is an evident feature of the chiral anomaly.

cond-mat.mtrl-sci

Third order nonlinear transport properties in topological chiral antiferromagnetic semimetal CoNb3S6

The topology between Bloch states in reciprocal space has attracted tremendous attention in recent years. The quantum geometry of the band structure is composed of quantum metric as real part and berry curvature as imaginary part. While the Berry curvature, the Berry curvature dipole and Berry connection polarizability have been recently revealed by the first order anomalous hall, second order and third order nonlinear Hall effect respectively, the quantum metric induced second order nonlinear transverse and longitudinal response in topological antiferromagnetic material MnBi2Te4 was only very recently reported. Here we demonstrate the similar third order nonlinear transport properties in the topological antiferromagnetic CoNb3S6. We observed that the third order nonlinear longitudinal V3ω xx increase significantly at the antiferromagnetic transition temperature TN ~ 29 K, which was probably induced by the quantum metric without time-reversal symmetry or inversion symmetry. Besides, temperature-dependent nonlinear behaviour was observed in the first order I-V curve below the Neel temperature TN, which was not reported in MnBi2Te4 and FeSn. Such nonlinear I-V behaviour hints for the possible existence of Charge Density Wave (CDW) state, which has been discovered in its sister material FeNb3S6. Simultaneously, two plateaus in the third order nonlinear longitudinal V3ω xx~ I^ω curve are observed, which is also speculated to be related with the possible CDW state. However, the genuine mechanism for the first order nonlinear I-V and its relation with the third order nonlinear transport call for more experimental investigations and theoretical interpretation. Our work provides a way to explore third harmonic nonlinear transport and interaction with magnetic order and CDW.

cond-mat.mtrl-sci