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Junqiu Liu

Publications and source records attributed to Junqiu Liu.

At least 19 recordsLinked to original sources

Platicon purification in self-injection locking regime via gain switching

Integrated photonic devices leveraging optical frequency microcombs have emerged as essential instruments for modern photonic systems, prized for their chip-scale footprint, high energy efficiency, and inherent stability. This work introduces a novel approach to microwave photonic oscillator based on generation of a Kerr platicon microcomb by a gain-switched self-injection-locked distributed feedback (DFB) laser diode. The system leverages direct modulation of the current of the laser diode, generating optical sidebands around the pump line. The beatnote between the Kerr comb lines and sidebands of the modulated pump at a high-speed photodetector allows to obtain tunable, low-noise microwave signals at frequencies close to the platicon repetition rate, which is many times higher than used for gain switching. We experimentally demonstrate continuous microwave signal frequency tuning from 100 MHz to 3.6 GHz by sweeping the modulation frequency, thereby shifting the generated sidebands relative to a platicon beatnote. We match third harmonics of the modulation frequency of the gain-switch signal with the free spectral range of the microresonator simultaneously generating the platicon microcomb. That leads to significant spectral purification of the platicon beatnote decreasing its phase noise by more than 30 dB. The novel architecture proposed offers a robust and versatile method for microwave synthesis, presenting significant potential for the advancement of integrated microwave photonic systems and their applications in communications, sensing, and metrology.

physics.optics

An ultralow-loss integrated photonic platform for discrete-variable quantum information processing

Photonic integrated circuits offer a scalable and robust route toward quantum information technologies by consolidating photon sources and linear optical networks onto compact, wafer-manufacturable chips. Although silicon photonics has enabled diverse discrete-variable quantum breakthroughs -- spanning multiphoton entanglement, quantum networking, and photonic qubit fusion for quantum computing -- scaling these platforms beyond proof-of-principle demonstrations remains severely constrained by a critical system-level bottleneck. Optical loss compounds rapidly across photon generation, routing, and state analysis, causing multiphoton generation probabilities to plummet exponentially as circuit depth and complexity grow. Here we overcome this rate-loss barrier by demonstrating a monolithic, ultralow-loss silicon nitride (Si$_3$N$_4$) integrated photonic platform engineered for high-performance discrete-variable quantum information processing. Our architecture seamlessly integrates narrowband photon-pair sources with low-loss qubit-fusion circuits and reconfigurable state-analysis interferometers. The on-chip sources prepare Einstein-Podolsky-Rosen (EPR) states with a fidelity of 0.9875(3) and exhibit near-unity photon indistinguishability, yielding a heralded Hong-Ou-Mandel interference visibility of 0.990(6). By executing on-chip fusion of two EPR states, we synthesize and characterize four-photon Greenberger-Horne-Zeilinger states with a record fidelity of 0.943(8) and a fourfold count rate of 27 Hz -- more than two orders of magnitude higher than previous silicon-photonic implementations. Combined with standard CMOS-compatible fabrication on 150-mm-diameter wafers, these results establish ultralow-loss Si$_3$N$_4$ integrated photonics as a definitive, manufacturable platform for deployable, large-scale quantum information processors.

quant-ph

Material-Anisotropy-Driven Topological Optical Lattices on Thin-Film Lithium Niobate

Integrated structured-light sources usually obtain high-dimensional orbital angular momentum (OAM) states by encoding each channel into separate gratings, waveguides or metasurfaces, which ties modal capacity to structural complexity. Here we show that intrinsic material anisotropy can instead act as a built-in angular-momentum coupler. In an X-cut thin-film lithium niobate (TFLN) microring vortex emitter, the in-plane optical axis causes a circulating whispering-gallery mode to sample a periodically varying effective index, producing continuous azimuthal phase modulation. This modulation converts each resonance from a nominal single-charge emitter into a coherent topological sideband lattice with charges l=l_p+2n and Bessel-weighted amplitudes. Broadband measurements resolve a representative principal-charge series from l_p=-13 to +13, while additional devices with 100 and 200 GHz free spectral ranges (FSRs) show scalable resonance addressability. The emitted lattices are reproduced by a forward-calculated Fourier--Bessel model, supported by OAM projection measurements, and exhibit focusing into annular perfect-vortex fields and self-healing after obstruction. Waveguide-induced circular polarization further adds a vectorial spin--orbit channel. These results turn TFLN anisotropy from a material constraint into a compact mechanism for resonance-addressed high-dimensional structured-light generation.

physics.optics

1-Mbps Twin-Field Quantum Key Distribution over 200 km Using Independent Dissipative Kerr Solitons

Twin-field quantum key distribution (TF-QKD) dramatically enhances the secure key rate (SKR) over inter-city distances through its square-root scaling. Further improvements in aggregate SKR can be achieved by wavelength-division multiplexing (WDM) of parallel QKD channels. However, direct implementation in TF-QKD poses significant challenges, as each wavelength channel requires an independent ultra-stable seed laser, narrow-linewidth transmitters, and optical phase-locked loops (OPLLs), which are not easily scalable. Here, we circumvent these limitations by employing two independent, integrated dissipative Kerr soliton (DKS) microcombs at Alice and Bob as multi-wavelength sources. High-visibility single-photon interference across all wavelength channels is achieved by stabilizing the frequencies of every comb line - requiring only the stabilization of the pump wavelength and repetition rates of the two microcombs. Based on this architecture, we perform a full TF-QKD experiment using the sending-or-not-sending protocol, achieving a total SKR of 1.57 Mbps over 201.1 km of fiber using 16 DWDM channels. This result represents more than an order-of-magnitude enhancement compared with single-wavelength TF-QKD at the same distance. Given that a single DKS comb can support over 100 coherent lines across the C-band, this approach offers a scalable pathway toward high-rate quantum key distribution over inter-city distances.

quant-ph

Kramers-Kronig causality in integrated photonics: The spectral tension between ultraviolet transition and mid-infrared absorption

Dispersion engineering via geometric confinement is essential to integrated photonics, enabling phenomena such as soliton microcombs, supercontinua, parametric oscillators, and entangled photons. However, prevailing methodologies rely on semi-empirical Sellmeier models that assume idealized material purity, neglecting the pronounced dispersion shifts induced by residual impurities like hydrogen-related bonds. Here, we demonstrate that these residual bonds fundamentally alter the dispersion landscape spanning from the ultraviolet (UV) to the mid-infrared (MIR) spectra. Specifically, they introduce MIR vibrational absorption while simultaneously modifying UV electronic transition, shifting the bandgap and UV pole. We show that the spectral tension between these UV and MIR modifications dictates the group velocity dispersion from the visible to the near-infrared (NIR) via the Kramers-Kronig causality. We experimentally validate this phenomenon through systematic characterization of broadband loss and dispersion in ultralow-loss silicon nitride photonic integrated circuits. By rigorously incorporating these effects, we bridge the gap between empirical fitting and predictive physical modelling. Our study resolves long-standing discrepancies in dispersion engineering, providing precision control essential for next-generation integrated photonics.

physics.optics

Enhancement of vacuum-ultraviolet dispersive-wave emission using gas-filled tapered hollow-core fibers

The recent breakthroughs in laser-driving 229Th nuclear transition have created an urgent demand for coherent vacuum-ultraviolet (VUV) sources delivering high spectral brightness at the critical 148.38 nm isomer energy. However, generating sufficient photon flux to overcome the low nuclear excitation probability remains a challenge for compact setups. While resonant dispersive wave emission in gas-filled hollow-core fibers offers a promising route, standard capillaries face a fundamental trade-off: maximizing input coupling requires large core diameters, whereas efficient nonlinear VUV conversion demands the high intensities using small cores. Here, we resolve this conflict using a gas-filled tapered capillary fiber. This architecture utilizes a longitudinally decreasing core diameter to combine a large input aperture with adiabatic field concentration, thereby continuously enhancing the nonlinear interaction. Experimentally, we demonstrate a widely tunable source (135-240 nm) that achieves a twofold efficiency enhancement specifically at the 148.38 nm wavelength compared to uniform geometries. By providing a scalable route to high-flux VUV generation, this work establishes a critical tabletop tool for advancing solid-state nuclear clocks and time-resolved spectroscopy.

physics.optics

Reconfigurable Resonant Multimode Nonlinear Coupling for UV-to-infrared Frequency Generation

On-chip coherent visible and near-infrared (NIR) light generation has broad applications in metrology, bio-sensing, and quantum information. High-Q microresonators are ideal candidates for generating light across such broad wavelength ranges via efficient second- ($\chi^{(2)}$) and third-order ($\chi^{(3)}$) nonlinear optical processes. However, harnessing these diverse nonlinearities simultaneously in a single microresonator remains elusive yet highly attractive both fundamentally and technologically. Here, we demonstrate coherent light generation from the ultraviolet to NIR in a silicon nitride microresonator pumped by a single continuous-wave telecom laser. This broad frequency generation arises from the interplay of $\chi^{(2)}$ and $\chi^{(3)}$ nonlinear processes. A cascade of nonlinear processes, including harmonic generation and optical parametric oscillation (OPO), is initiated by the photoinduced second harmonic generation enabled by all-optical poling. The dynamic reconfigurability of this $\chi^{(2)}$ nonlinearity enables access to different transverse spatial modes at the second harmonic, enabling highly tunable OPO processes triggered by hybrid modal phase matching conditions and yielding milliwatt-level NIR light. This work sheds new insights into the fundamental physics of cooperative nonlinear multimode interactions in resonant systems and provides a versatile approach for reconfigurable OPOs, highlighting their potential to generate light at wavelengths beyond the reach of photonic integrated lasers.

physics.optics

Photonic timing-engineered solitons for dual-microcomb metrology

Dissipative microcavity solitons offer a route to integrate comb-based metrology systems on photonic chips. However, integrated solitons generally lack agile control of comb parameters, particularly pulse timing control, hindering their application in quantum-limited metrology. Here we introduce dynamical soliton trapping to enable optically timing-engineered microcombs (OTEM). By injecting an auxiliary laser to anchor one of the microcomb lines, we create a potential well to trap and steer the soliton. Thus, soliton timing can be engineered by phase modulating the injected laser. Theory and measurement reveal the fast response bandwidth of the OTEM, which enabled a soliton slew rate of 31.3 ps/$\mu$s, surpassing existing time-programmable fiber laser combs by more than two orders of magnitude. Leveraging the timing scan, we used a single OTEM for single-pixel and parallel ranging by retrieving the phase of the multi-heterodyne beat spectrum. Picometer-scale ranging precision was achieved, establishing new record for optical absolute ranging. Our work can transform timing-engineering of microcavity solitons and endow integrated dual-microcomb metrology systems with enhanced precision.

physics.optics

Deep Learning-based Method for Expressing Knowledge Boundary of Black-Box LLM

Large Language Models (LLMs) have achieved remarkable success, however, the emergence of content generation distortion (hallucination) limits their practical applications. The core cause of hallucination lies in LLMs' lack of awareness regarding their stored internal knowledge, preventing them from expressing their knowledge state on questions beyond their internal knowledge boundaries, as humans do. However, existing research on knowledge boundary expression primarily focuses on white-box LLMs, leaving methods suitable for black-box LLMs which offer only API access without revealing internal parameters-largely unexplored. Against this backdrop, this paper proposes LSCL (LLM-Supervised Confidence Learning), a deep learning-based method for expressing the knowledge boundaries of black-box LLMs. Based on the knowledge distillation framework, this method designs a deep learning model. Taking the input question, output answer, and token probability from a black-box LLM as inputs, it constructs a mapping between the inputs and the model' internal knowledge state, enabling the quantification and expression of the black-box LLM' knowledge boundaries. Experiments conducted on diverse public datasets and with multiple prominent black-box LLMs demonstrate that LSCL effectively assists black-box LLMs in accurately expressing their knowledge boundaries. It significantly outperforms existing baseline models on metrics such as accuracy and recall rate. Furthermore, considering scenarios where some black-box LLMs do not support access to token probability, an adaptive alternative method is proposed. The performance of this alternative approach is close to that of LSCL and surpasses baseline models.

cs.CL

Metrology-grade mid-infrared spectroscopy for multi-dimensional perception

The mid-infrared spectral window is essential for molecular fingerprinting and atmospheric sensing, yet unlocking its full potential is currently constrained by a fundamental instrumental trade-off: existing systems cannot simultaneously deliver broad bandwidth, high photon flux, and metrological frequency fidelity. Here, we resolve this bottleneck by demonstrating a metrology-grade spectroscopic system based on difference frequency generation, driven by widely tunable, near-infrared diode lasers traceable to atomic standards. Our system achieves continuous tunability across the 3-3.7 $\mu$m atmospheric window and delivers output power exceeding 45 mW with an absolute frequency accuracy of 7.2 MHz. We harness this convergence to overcome a critical barrier in integrated photonics, unambiguously identifying and eliminating hydrogen-induced absorption in silicon nitride microresonators to achieve an 88-fold reduction in optical loss. We further reveal multi-phonon absorption in the silica cladding as the fundamental limit to mid-infrared integrated photonics. Finally, we demonstrate the system's versatility through scattering-resilient LiDAR capable of penetrating optically dense fog, and dual-modality sensing that simultaneously retrieves target distance and chemical composition. By unifying the rigor of frequency metrology with the versatility of broadband sensing, this architecture establishes a new paradigm for multi-dimensional perception in complex environments.

physics.optics

A scalable near-visible integrated photon-pair source for satellite quantum science

Quantum state distribution over vast distances is essential for global-scale quantum networks and fundamental test of quantum physics at space scale. While satellite platforms have demonstrated thousand-kilometer entanglement distribution, quantum key distribution and quantum teleportation with ground, future constellations and deep-space missions demand photon sources that are robust, compact, and power-efficient. Integrated photonics offers a scalable solution, yet a critical spectral gap persists. Although telecom-band integrated photon-pair sources are well established, near-visible photons offer distinct advantages for satellite-to-ground links by mitigating diffraction loss and maximizing the collection efficiency of optical telescopes. Scalable integrated sources in this regime have remained elusive due to the fundamental challenge of achieving anomalous dispersion in materials transparent at visible wavelengths. Here we bridge this gap by demonstrating an integrated near-visible photon-pair source based on a wide-bandgap, ultralow-loss, silicon nitride (Si$_3$N$_4$) microresonator. By engineering the dispersion of higher-order waveguide modes, we overcome the intrinsic normal dispersion limit to achieve efficient phase matching. The device exhibits a spectral brightness of 4.87$\times$10$^7$ pairs/s/mW$^2$/GHz and a narrow photon linewidth of 357 MHz. We report high-purity heralded single-photon generation with a heralding rate up to 2.3 MHz and a second-order correlation function as low as 0.0041. Furthermore, we observe energy-time entanglement with 98.4% interference visibility, violating the CHSH limit even at flux exceeding 40.6 million pairs/s. Combined with the proven radiation hardness of Si$_3$N$_4$, this source constitutes a flight-ready hardware foundation for daylight quantum communications and protocols requiring on-orbit multiphoton interference.

quant-ph

Intraresonance frequency combs in Kerr microresonators

For more than 20 years, optical microresonators have served as the backbone of integrated nonlinear photonics, exploiting Kerr nonlinearity to generate octave-spanning frequency combs, enable quantum effects, and drive optical parametric oscillators. Since the inception of microresonator-based nonlinear optics, related studies have focused primarily on regimes in which photons with distinct resonant modes can interact. Although multiple comb lines can occupy a single resonance during the Kerr comb formation process, their mutual interactions have remained largely unexplored. Here we demonstrate a Kerr comb formation that is confined to a single resonance of a microresonator via dual-pumping. MHz-scale comb-line spacing reveals previously unobserved Kerr-comb dynamics, featuring parametrically driven phase multistability that can be observed directly in the temporal domain. Two laser pumps serve as phase-coupled references for heterodyne read-out, simplifying the measurements.

physics.optics

Coherent Tunneling by Adiabatic Passage in Silicon Nitride based Integrated Waveguide Structures

Nowadays silicon nitride photonic integrated circuits serve as a mature platform for numerous applications. Planar waveguides and directional couplers made by CMOS-compatible technology are its basic elements. Here we demonstrate the possibilities of efficient light routing and transfer provided by the integrated planar Si3N4 waveguides structure based on the coherent tunneling by adiabatic passage (CTAP) at the 1.55um telecom band. We addressed both high- and low-confinement silicon nitride CTAP structures and proved high efficiency of light routing in them. The mechanisms that limit the light control efficiency have been revealed. The accessible parameters of such structures have been determined. Besides that, there was proposed the original hybrid Si3N4 Si - Si3N4 waveguides structure providing the enhanced efficiency and flexibility of the CTAP in comparison with the single-material Si3N4 waveguide structures.

physics.optics

Light coupling to photonic integrated circuits using optimized lensed fibers

Efficient and reliable light coupling between optical fibers and photonic integrated circuits has arguably been the most essential issue in integrated photonics for optical interconnects, nonlinear signal conversion, neuromorphic computing, and quantum information processing. A commonly used approach is to use inverse tapers interfacing with lensed fibers, particularly for waveguides of relatively low refractive index, such as silicon nitride (Si3N4), silicon oxynitride, and lithium niobate. This approach simultaneously enables broad operation bandwidth, high coupling efficiency, and simplified fabrication. Although diverse taper designs have been invented and characterized to date, lensed fibers play equally important roles here, yet their optimization has long been underexplored. Here, we fill this gap and introduce a comprehensive co-optimization strategy that synergistically refines the geometries of the taper and the lensed fiber. By incorporating the genuine lensed fiber's shape into the simulation, we accurately capture its non-Gaussian emission profile, thereby nullifying the widely accepted approximation based on a paraxial Gaussian mode. We further characterize many lensed fibers and Si3N4 tapers of varying shapes using different fabrication processes. Our experimental and simulation results show remarkable agreement, both achieving maximum coupling efficiencies exceeding 80% per facet. Finally, we summarize the optimal choices of lensed fibers and Si3N4 tapers that can be directly deployed in modern CMOS foundries for scalable manufacturing of Si3N4 photonic integrated circuits. Our study not only contributes to light-coupling solutions but is also critical for photonic packaging and optoelectronic assemblies that are currently revolutionizing data centers and AI.

physics.optics

Photonic chip-based high-efficiency soliton microcombs via electroopitc-Kerr synergy

Temporal soliton mode-locking in coherently pumped microcavities provides a promising platform for miniaturized frequency comb systems. While significant progress has been made, achieving high conversion efficiency in such microcombs remains a critical challenge. Soliton generation through pulse pumping has emerged as an effective strategy to improve conversion efficiency. However, the on-chip integration of pulse generation with dissipative Kerr soliton (DKS) formation within the photonic chip has not yet been realized. In this work, we demonstrate a photonic chip-based soliton microcomb with high conversion efficiency, achieved by integrating on-chip pulse generation and DKS generation. The pulsed laser, fabricated on a lithium niobate-on-insulator (LNOI) platform, delivers a 35.5GHz repetition rate with broadly tunable center frequencies. By coupling these on-chip pulses to a silicon nitride microresonator, we achieve stable DKS generation with a pump-to-soliton conversion efficiency of 43.9% under steady-state conditions. This integrated architecture establishes a viable pathway toward chip-scale soliton microcombs with unprecedented efficiency, opening up new possibilities for optical communications, precision spectroscopy, and photonic sensing.

physics.optics

Laser transfer and retrieval via nanophotonic supercontinuum process

The nature of optical metrology is to perform efficient transfer and precise retrieval for lasers and optical signals, which is beneficial for a variety of applications ranging from optical clocking, spectroscopy, to telecommunications and quantum optics. While efforts have been made to promote the detection accuracy of optical frequencies, retrieval on optical waveforms remains on the autocorrelation scheme with limited performances. Here, we demonstrate a novel scheme for optical metrology, particularly on direct retrieval of optical waveform in terms of the field amplitude profile. The scheme is based on massive four-wave-mixings underlying a nanophotonic supercontinuum process, which enables arbitrary transfer of an additive laser to modulational sidebands of the broadened continuum. Detection of the transferred signals is then flexible to be within the whole span of the supercontinuum from visible to the mid-infrared range. We demonstrate such a transfer scheme for both CW lasers and pulsed lasers. For the latter, the temporal amplitude profile of the optical wave can be retrieved, which reveals high-order dynamics of solitary pulses including the self-steepening, self-compression, and the soliton splitting, and shows a remarkable square-fold increase of signal-to-noise ratio in the power spectrum. Our results may contribute to advance optical metrology particularly towards chip scale optical waveform detection, and more fundamentally, they reveal insights of massive ultrafast nonlinear interactions underlying the soliton-based supercontinuum process.

physics.optics

Hybrid-integrated dark-pulse microcombs towards visible light spectrum

Leveraging hybrid integration, we demonstrate dark-pulse formation at 780-nm wavelength band in integrated Si$_3$N$_4$ microresonators driven by high-power AlGaAs-based chip-scale lasers. The device outputs coherent frequency combs with electronically detectable repetition rates down to 20 GHz, paving a route to efficient and compact atom-chip interfaces for spectroscopy, metrology and sensing.

physics.optics

Space compatibility of emerging, wide-bandgap, ultralow-loss integrated photonics

Integrated photonics has revolutionized optical communication, sensing, and computation, offering miniaturized and lightweight solutions for spacecraft with limited size and payload. Novel chip-scale instruments based on ultralow-loss integrated photonic platforms, including lasers, frequency combs and atomic traps, have been developed for space applications. Therefore, quantifying the space compatibility of ultralow-loss photonic integrated circuits (PICs), particularly their radiation resistance, is critical. This study experimentally evaluates the radiation resistance of ultralow-loss Si$_3$N$_4$, 4H-SiC, and LiNbO$_3$ PICs under intense $\gamma$-ray and high-energy proton irradiation. Results show that proton irradiation with $1.1 \times 10^{10}$ $\mathrm{p/cm^2}$ total flux does not significantly increase optical loss or alter the refractive index of these PICs, while $\gamma$-ray irradiation with 1.2 Mrad accumulated dose only marginally increases their optical loss. These findings provide preliminary evidence of the excellent space compatibility of ultralow-loss Si$_3$N$_4$, 4H-SiC, and LiNbO$_3$ PICs, highlighting their potential for compact and lightweight space systems.

physics.optics