arXiv subjects

Justin C. W. Song

Publications and source records attributed to Justin C. W. Song.

At least 55 records · Page 3Linked to original sources

arXiv2019

Symmetry, spin-texture, and tunable quantum geometry in a WTe$_2$ monolayer

The spin orientation of electronic wavefunctions in crystals is an internal degree of freedom, typically insensitive to electrical knobs. We argue from a general symmetry analysis and a $\vec k \cdot \vec p$ perspective, that monolayer 1T'-WTe$_2$ possesses a gate-activated canted spin texture that produces an electrically tunable bulk band quantum geometry. In particular, we find that due to its out-of-plane asymmetry, an applied out-of-plane electric field breaks inversion symmetry to induce both in-plane and out-of-plane electric dipoles. These in-turn generate spin-orbit coupling to lift the spin degeneracy and enable a bulk band Berry curvature and magnetic moment distribution to develop. Further, due to its low symmetry, Berry curvature and magnetic moment in 1T'-WTe$_2$ possess a dipolar distribution in momentum space, and can lead to unconventional effects such as a current induced magnetization and quantum non-linear anomalous Hall effect. These render 1T'-WTe$_2$ a rich two-dimensional platform for all-electrical control over quantum geometric effects.

cond-mat.mes-hall↗

arXiv2018

Fermi arc induced vortex structure in Weyl beam shifts

In periodic media, despite the close relationship between geometrical effects in the bulk and topological surface states, the two are typically probed separately. We show that when beams in a Weyl medium reflect off an interface with a gapped medium, the trajectory is influenced by both bulk geometrical effects and the Fermi arc surface states. The reflected beam experiences a displacement, analogous to the Goos-Hänchen or Imbert-Fedorov shifts, that forms a half-vortex in the two-dimensional surface momentum space. The half-vortex is centered where the Fermi arc of the reflecting surface touches the Weyl cone, with the magnitude of the shift scaling as an inverse square root away from the touching-point, and diverging at the touching-point. This striking feature provides a way to use bulk transport to probe the topological characteristics of a Weyl medium.

cond-mat.mes-hall↗

arXiv2018

Giant intrinsic photoresponse in pristine graphene

When the Fermi level matches the Dirac point in graphene, the reduced charge screening can dramatically enhance electron-electron (e-e) scattering to produce a strongly interacting Dirac liquid. While the dominance of e-e scattering already leads to novel behaviors, such as electron hydrodynamic flow, further exotic phenomena have been predicted to arise specifically from the unique kinematics of e-e scattering in massless Dirac systems. Here, we use optoelectronic probes, which are highly sensitive to the kinematics of electron scattering, to uncover a giant intrinsic photocurrent response in pristine graphene. This photocurrent emerges exclusively at the charge neutrality point and vanishes abruptly at non-zero charge densities. Moreover, it is observed at places with broken reflection symmetry, and it is selectively enhanced at free graphene edges with sharp bends. Our findings reveal that the photocurrent relaxation is strongly suppressed by a drastic change of fast photocarrier kinematics in graphene when its Fermi level matches the Dirac point. The emergence of robust photocurrents in neutral Dirac materials promises new energy-harvesting functionalities and highlights intriguing electron dynamics in the optoelectronic response of Dirac fluids.

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arXiv2018

Electron quantum metamaterials in van der Waals heterostructures

In recent decades, scientists have developed the means to engineer synthetic periodic arrays with feature sizes below the wavelength of light. When such features are appropriately structured, electromagnetic radiation can be manipulated in unusual ways, resulting in optical metamaterials whose function is directly controlled through nanoscale structure. Nature, too, has adopted such techniques -- for example in the unique coloring of butterfly wings -- to manipulate photons as they propagate through nanoscale periodic assemblies. In this Perspective, we highlight the intriguing potential of designer sub-electron wavelength (as well as wavelength-scale) structuring of electronic matter, which affords a new range of synthetic quantum metamaterials with unconventional responses. Driven by experimental developments in stacking atomically layered heterostructures -- e.g., mechanical pick-up/transfer assembly -- atomic scale registrations and structures can be readily tuned over distances smaller than characteristic electronic length-scales (such as electron wavelength, screening length, and electron mean free path). Yet electronic metamaterials promise far richer categories of behavior than those found in conventional optical metamaterial technologies. This is because unlike photons that scarcely interact with each other, electrons in subwavelength structured metamaterials are charged, and strongly interact. As a result, an enormous variety of emergent phenomena can be expected, and radically new classes of interacting quantum metamaterials designed.

cond-mat.mes-hall↗

arXiv2018

Ultrafast Spin-To-Charge Conversion at the Surface of Topological Insulator Thin Films

Strong spin-orbit coupling, resulting in the formation of spin-momentum-locked surface states, endows topological insulators with superior spin-to-charge conversion characteristics, though the dynamics that govern it have remained elusive. Here, we present an all-optical method that enables unprecedented tracking of the ultrafast dynamics of spin-to-charge conversion in a prototypical topological insulator Bi$_2$Se$_3$/ferromagnetic Co heterostructure, down to the sub-picosecond timescale. Compared to pure Bi$_2$Se$_3$ or Co, we observe a giant terahertz emission in the heterostructure than originates from spin-to-charge conversion, in which the topological surface states play a crucial role. We identify a 0.12-picosecond timescale that sets a technological speed limit of spin-to-charge conversion processes in topological insulators. In addition, we show that the spin-to-charge conversion efficiency is temperature independent in Bi$_2$Se$_3$ as expected from the nature of the surface states, paving the way for designing next-generation high-speed opto-spintronic devices based on topological insulators at room temperature.

cond-mat.mtrl-sci↗

arXiv2018

Non-saturating large magnetoresistance in semimetals

The rapidly expanding class of quantum materials known as {\emph{topological semimetals}} (TSM) display unique transport properties, including a striking dependence of resistivity on applied magnetic field, that are of great interest for both scientific and technological reasons. However, experimental signatures that can identify or discern the dominant mechanism and connect to available theories are scarce. Here we present the magnetic susceptibility ($χ$), the tangent of the Hall angle ($\tanθ_H$) along with magnetoresistance in four different non-magnetic semimetals with high mobilities, NbP, TaP, NbSb$_2$ and TaSb$_2$, all of which exhibit non-saturating large MR. We find that the distinctly different temperature dependences, $χ(T)$ and the values of $\tanθ_H$ in phosphides and antimonates serve as empirical criteria to sort the MR from different origins: NbP and TaP being uncompensated semimetals with linear dispersion, in which the non-saturating magnetoresistance arises due to guiding center motion, while NbSb$_2$ and TaSb$_2$ being {\it compensated} semimetals, with a magnetoresistance emerging from nearly perfect charge compensation of two quadratic bands. Our results illustrate how a combination of magnetotransport and susceptibility measurements may be used to categorize the increasingly ubiquitous non-saturating large magnetoresistance in TSMs.

cond-mat.str-el↗

arXiv2018

Berryogenesis: self-induced Berry flux and spontaneous non-equilibrium magnetism

Spontaneous symmetry breaking is central to the description of interacting phases of matter. Here we reveal a new mechanism through which a driven interacting system subject to a time-reversal symmetric driving field can spontaneously magnetize. We show that the strong internal ac fields of a metal driven close to its plasmon resonance may enable Berryogenesis: the spontaneous generation of a self-induced Bloch band Berry flux. The self-induced Berry flux supports and is sustained by a circulating plasmonic motion, which may arise even for a linearly polarized driving field. This non-equilibrium phase transition occurs above a critical driving amplitude, and may be of either continuous or discontinuous type. Berryogenesis relies on feedback due to interband coherences induced by internal fields, and may readily occur in a wide variety of multiband systems. We anticipate that graphene devices, in particular, provide a natural platform to achieve Berryogenesis and plasmon-mediated spontaneous non-equilibrium magnetization in present-day devices.

cond-mat.mes-hall↗

arXiv2018

Intra-cell dynamics and cyclotron motion without magnetic field

Intra-cell motion endows rich non-trivial phenomena to a wide variety of quantum materials. The most prominent example is a transverse current in the absence of a magnetic field (i.e. the anomalous Hall effect). Here we show that, in addition to a dc Hall effect, anomalous Hall materials possess circulating currents and cyclotron motion without magnetic field. These are generated from the intricate wavefunction dynamics within the unit cell, and correspond to interband transitions (coherences) in much the same way that cyclotron resonances arise from inter-Landau level transitions in magneto-optics. Curiously, anomalous cyclotron motion exhibits an intrinsic decay in time (even in pristine materials) displaying a characteristic power law decay. This reveals an intrinsic dephasing similar to that of inhomogeneous broadening of spinors. Circulating currents can manifest as the emission of circularly polarized light pulses in response to incident linearly polarized (pulsed) electric field, and provide a direct means of interrogating the intra-unit-cell dynamics of quantum materials.

cond-mat.mes-hall↗

arXiv2018

Low-dissipation edge currents without edge states

We show that bulk free carriers in topologically trivial multi-valley insulators with non-vanishing Berry curvature give rise to low-dissipation edge currents, which are squeezed within a distance of the order of the valley diffusion length from the edge. This happens even in the absence of edge states [topological (gapless) or otherwise], and when the bulk equilibrium carrier concentration is thermally activated across the gap. Physically, the squeezed edge current arises from the spatially inhomogeneous orbital magnetization that develops from valley-density accumulation near the edge. While this current possesses neither topology nor symmetry protection and, as a result, is not immune to dissipation, in clean enough devices it can mimic low-loss ballistic transport.

cond-mat.mes-hall↗

arXiv2017

Plasmon geometric phase and plasmon Hall shift

The collective plasmonic modes of a metal comprise a pattern of charge density and tightly-bound electric fields that oscillate in lock-step to yield enhanced light-matter interaction. Here we show that metals with non-zero Hall conductivity host plasmons with a fine internal structure: they are characterized by a current density configuration that sharply departs from that of ordinary zero Hall conductivity metals. This non-trivial internal structure dramatically enriches the dynamics of plasmon propagation, enabling plasmon wavepackets to acquire geometric phases as they scatter. Strikingly, at boundaries these phases accumulate allowing plasmon waves that reflect off to experience a non-reciprocal parallel shift along the boundary displacing the incident and reflected plasmon trajectories. This plasmon Hall shift, tunable by Hall conductivity as well as plasmon wavelength, displays the chirality of the plasmon's current distribution and can be probed by near-field photonics techniques. Anomalous plasmon dynamics provide a real-space window into the inner structure of plasmon bands, as well as new means for directing plasmonic beams.

cond-mat.mes-hall↗

arXiv2017

Long-lived domain wall plasmons in gapped bilayer graphene

Topological domain walls in dual-gated gapped bilayer graphene host edge states that are gate- tunable and valley polarized. Here we predict that plasmonic collective modes can propagate along these topological domain walls even at zero bulk density, and possess a markedly different character from that of bulk plasmons. Strikingly, domain wall plasmons are extremely long-lived, with plasmon lifetimes that can be orders of magnitude larger than the transport scattering time in the bulk. While most pronounced at low temperatures, long domain wall plasmon lifetimes persist even at room temperature with values up to a few picoseconds. Domain wall plasmons possess a rich phenomenology including a wide range of frequencies (up to the mid-infrared), tunable sub-wavelength electro-magnetic confinement lengths, as well as a valley polarization for forward/backward propagating modes. Its unusual features render them a new tool for realizing low-dissipation plasmonics that transcend the restrictions of the bulk.

cond-mat.mes-hall↗

arXiv2017

Large optical conductivity of Dirac semimetal Fermi arc surfaces states

Fermi arc surface states, a hallmark of topological Dirac semimetals, can host carriers that exhibit unusual dynamics distinct from that of their parent bulk. Here we find that Fermi arc carriers in intrinsic Dirac semimetals possess a strong and anisotropic light matter interaction. This is characterized by a large Fermi arc optical conductivity when light is polarized transverse to the Fermi arc; when light is polarized along the Fermi arc, Fermi arc optical conductivity is significantly muted. The large surface spectral weight is locked to the wide separation between Dirac nodes and persists as a large Drude weight of Fermi arc carriers when the system is doped. As a result, large and anisotropic Fermi arc conductivity provides a novel means of optically interrogating the topological surfaces states of Dirac semimetals.

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arXiv2017

Fermi arc plasmons in Weyl semimetals

In the recently discovered Weyl semimetals, the Fermi surface may feature disjoint, open segments -- the so-called Fermi arcs -- associated with topological states bound to exposed crystal surfaces. Here we show that the collective dynamics of electrons near such surfaces sharply departs from that of a conventional three-dimensional metal. In magnetic systems with broken time reversal symmetry, the resulting Fermi arc plasmons (FAPs) are chiral, with dispersion relations featuring open, hyperbolic constant frequency contours. As a result, a large range of surface plasmon wave vectors can be supported at a given frequency, with corresponding group velocity vectors directed along a few specific collimated directions. Fermi arc plasmons can be probed using near field photonics techniques, which may be used to launch highly directional, focused surface plasmon beams. The unusual characteristics of FAPs arise from the interplay of bulk and surface Fermi arc carrier dynamics, and give a window into the unusual Fermiology of Weyl semimetals.

cond-mat.mes-hall↗

arXiv2016

Giant Hall photoconductivity in narrow-gapped Dirac materials

Carrier dynamics acquire a new character in the presence of Bloch-band Berry curvature, which naturally arises in gapped Dirac materials (GDMs). Here we argue that photoresponse in GDMs with small band gaps is dramatically enhanced by Berry curvature. This manifests in a giant and saturable Hall photoconductivity when illuminated by circularly polarized light. Unlike Hall motion arising from a Lorentz force in a magnetic field, which impedes longitudinal carrier motion, Hall photoconductivity arising from Berry curvature can boost longitudinal carrier transport. In GDMs, this results in a helicity-dependent photoresponse in the Hall regime, where photoconductivity is dominated by its Hall component. We find that the induced Hall conductivity per incident irradiance is enhanced by up to six orders of magnitude when moving from the visible regime (with corresponding band gaps) to the far infrared. These results suggest that narrow-gap GDMs are an ideal test-bed for the unique physics that arise in the presence of Berry curvature, and open a new avenue for infrared and terahertz optoelectronics.

cond-mat.mes-hall↗

arXiv2016

Enhanced thermionic-dominated photoresponse in graphene Schottky junctions

Vertical heterostructures of van der Waals materials enable new pathways to tune charge and energy transport characteristics in nanoscale systems. We propose that graphene Schottky junctions can host a special kind of photoresponse which is characterized by strongly coupled heat and charge flows that run vertically out of the graphene plane. This regime can be accessed when vertical energy transport mediated by thermionic emission of hot carriers overwhelms electron-lattice cooling as well as lateral diffusive energy transport. As such, the power pumped into the system is efficiently extracted across the entire graphene active area via thermionic emission of hot carriers into a semiconductor material. Experimental signatures of this regime include a large and tunable internal responsivity ${\cal R}$ with a non-monotonic temperature dependence. In particular, ${\cal R}$ peaks at electronic temperatures on the order of the Schottky potential $ϕ$ and has a large upper limit ${\cal R} \le e/ϕ$ ($e/ϕ=10\,{\rm A/W}$ when $ϕ= 100\,{\rm meV}$). Our proposal opens up new approaches for engineering the photoresponse in optically-active graphene heterostructures.

cond-mat.mes-hall↗

arXiv2016

Chiral plasmons without magnetic field

Plasmons, the collective oscillations of interacting electrons, possess emergent properties that dramatically alter the optical response of metals. We predict the existence of a new class of plasmons -- chiral Berry plasmons (CBPs) -- for a wide range of two-dimensional metallic systems including gapped Dirac materials. As we show, in these materials the interplay between Berry curvature and electron-electron interactions yields chiral plasmonic modes at zero magnetic field. The CBP modes are confined to system boundaries, even in the absence of topological edge states, with chirality manifested in split energy dispersions for oppositely directed plasmon waves. We unveil a rich CBP phenomenology and propose setups for realizing them, including in anomalous Hall metals and optically-pumped 2D Dirac materials. Realization of CBPs will offer a new paradigm for magnetic field-free, sub-wavelength optical non-reciprocity, in the mid IR-THz range, with tunable splittings as large as tens of THz, as well as sensitive all-optical diagnostics of topological bands.

cond-mat.mes-hall↗

arXiv2016

Persistent Hall response in a quantum quench

Out-of-equilibrium systems can host phenomena that transcend the usual restrictions of equilibrium systems. Here we unveil how out-of-equilibrium states, prepared via a quantum quench, can exhibit a non-zero Hall-type response that persists at long times, and even when the instantaneous Hamiltonian is time reversal symmetric; both these features starkly contrast with equilibrium Hall currents. Interestingly, the persistent Hall effect arises from processes beyond those captured by linear response, and is a signature of the novel dynamics in out-of-equilibrium systems. We propose quenches in two-band Dirac systems as natural venues to realize persistent Hall currents, which exist when either mirror or time-reversal symmetry are broken (before or after the quench). Its long time persistence, as well as sensitivity to symmetry breaking, allow it to be used as a sensitive diagnostic of the complex out-equilibrium dynamics readily controlled and probed in cold-atomic optical lattice experiments.

cond-mat.quant-gas↗

arXiv2015

Linear magnetoresistance in metals: guiding center diffusion in a smooth random potential

We predict that guiding center (GC) diffusion yields a linear and non-saturating (transverse) magnetoresistance in 3D metals. Our theory is semi-classical and applies in the regime where the transport time is much greater than the cyclotron period, and for weak disorder potentials which are slowly varying on a length scale much greater than the cyclotron radius. Under these conditions, orbits with small momenta along magnetic field $B$ are squeezed and dominate the transverse conductivity. When disorder potentials are stronger than the Debye frequency, linear magnetoresistance is predicted to survive up to room temperature and beyond. We argue that magnetoresistance from GC diffusion explains the recently observed giant linear magnetoresistance in 3D Dirac materials.

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