arXiv subjects
Publications and source records attributed to Jyotipratim Ray Chaudhuri.
We consider the motion of an overdamped particle in a force field in presence of an external, adiabatic noise, without the restriction that the noise process is Gaussian or the stochastic process is Markovian. We examine the condition for attainment of steady state for this nonequilibrium open system and calculate the adiabatic noise-induced rate of escape of the particle over a barrier.
We extend the quantum theory of dissipation in the context of system-reservoir model, where the reservoir in question is kept in a nonequilibrium condition. Based on a systematic separation of time scales involved in the dynamics, appropriate generalizations of the fluctuation-dissipation and Einstein's relations have been pointed out. We show that the Wigner-Weisskopf decay of the system mode results in a rate constant which depending on the relaxation of nonequilibrium bath is dynamically modified. We also calculate the time-dependent spectra of a cavity mode with a suitable gain when the cavity is kept in contact with a nonequilibrium bath.
Based on the system-reservoir description we propose a simple solvable microscopic model for a nonequilibrium bath. This captures the essential features of a nonstationary quantum Markov process. We establish an appropriate generalization of the fluctuation-dissipation relation pertaining to this process and explore the essential modifications of the Bloch equations to reveal the nonexponential decay of the Bloch vector components and transient spectral broadening in resonance fluorescence. We discuss a simple experimental scheme to verify the theoretical results.
We have explored a simple microscopic model to simulate a thermally activated rate process where the associated bath which comprises a set of relaxing modes is not in an equilibrium state. The model captures some of the essential features of non-Markovian Langevin dynamics with a fluctuating barrier. Making use of the Fokker-Planck description we calculate the barrier dynamics in the steady state and non-stationary regimes. The Kramers-Grote-Hynes reactive frequency has been computed in closed form in the steady state to illustrate the strong dependence of the dynamic coupling of the system with the relaxing modes. The influence of nonequilibrium excitation of the bath modes and its relaxation on the kinetics of activation of the system mode is demonstrated. We derive the dressed time-dependent Kramers rate in the nonstationary regime in closed analytical form which exhibits strong non-exponential relaxation kinetics of the reaction co-ordinate. The feature can be identified as a typical non-Markovian dynamical effect.