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Jyotirmay Dwivedi

Publications and source records attributed to Jyotirmay Dwivedi.

6 recordsLinked to original sources

Nanoscale imaging of ferromagnetic vortex dynamics with scanning NV magnetometry

The generation and manipulation of spin waves at the nanoscale via magnetic vortices are of considerable importance because of their broad applications across magnonic and quantum technologies. Previously, fixed nitrogen-vacancy (NV) centers in diamond have been used to locally characterize vortex dynamics, and scanning NV magnetometry (SNVM) has been used to image vortices' static stray fields. Here, we demonstrate SNVM imaging of both the static and microwave fields generated by vortices in mesoscopic permalloy structures with $\sim$50 nm spatial resolution, achieving excellent agreement with micromagnetic simulations, while revealing the effects of disorder. We further demonstrate a 40$\times$ microwave field enhancement near a vortex core and image the disorder-dependent, spatially varying, evanescent decay of these microwaves. Our ambient, tabletop technique surpasses diffraction-limited techniques' resolutions by at least 5$\times$, with far greater accessibility and throughput than synchrotron radiation-based techniques, offering new opportunities in the study and development of magnonic devices.

cond-mat.mes-hall↗

Emergent anisotropic three-phase order in critically doped superconducting diamond films

Two decades since its discovery, superconducting heavily boron-doped diamond (HBDD) still presents unresolved fundamental questions whose resolution is relevant to the development of this material for quantum technologies. We use electrical magnetotransport measurements of critically-doped homoepitaxial single crystal HBDD films to reveal signatures of intrinsic (electronic) granular superconductivity. By studying the dependence of electrical resistivity on temperature and magnetic field vector, we infer that this granularity arises from electron correlations. This is revealed by a striking three-phase anisotropy in the magnetoresistance, accompanied by a spontaneous transverse voltage (Hall anomaly). Our findings indicate an emergent magnetically tunable intrinsic order in an otherwise isotropic three dimensional single crystal HBDD film, offering new insights into the mechanism of superconductivity in this quantum material.

cond-mat.supr-con↗

Flux channeling induced nano-confinement and enhancement of microwaves imaged by Rabi oscillation mapping

With rapid advances in qubit technologies, techniques for localizing, modulating, and measuring RF fields and their impact on qubit performance are of the utmost importance. Here, we demonstrate that flux-channeling from a permalloy nanowire can be used to achieve localized spatial modulation of an RF field and that the modulated field can be mapped with high resolution using the Rabi oscillations of an NV center. Rabi maps reveal ~100 mm wavelength microwaves concentrated in sub-300 nm-scale regions with up to ~16$\times$ power enhancement. This modulation is robust over a 20 dBm power range and has no adverse impact on NV $T_2$ coherence time. Micromagnetic simulations confirm that the modulated field results from the nanowire's stray field through its constructive/destructive interference with the incident RF field. Our findings provide a new pathway for controlling qubits, amplifying RF signals, and mapping local fields in various on-chip RF technologies.

cond-mat.mes-hall↗

Off-Resonant Detection of Domain Wall Oscillations Using Deterministically Placed Nanodiamonds

Nitrogen-vacancy (NV) centers in diamond offer a sensitive method of measuring the spatially localized dynamics of magnetization and associated spin textures in ferromagnetic materials. We use NV centers in a deterministically positioned nanodiamond to demonstrate off-resonant detection of GHz-scale microwave field driven oscillations of a single domain wall (DW). The technique exploits the enhanced relaxation of NV center spins due to the broadband stray fields generated by an oscillating DW pinned at an engineered defect in a lithographically patterned ferromagnetic nanowire. Discrepancies between the observed DW oscillation frequency and predictions from micromagnetic simulations suggest extreme sensitivity of DW dynamics to patterning imperfections such as edge roughness. These experiments and simulations identify potential pathways toward quantum spintronic devices that exploit current driven DWs as nanoscale microwave generators for qubit control, greatly increasing the driving field at an NV center and thus drastically reducing the π pulse time.

cond-mat.mes-hall↗

Giant spin torque efficiency in naturally oxidized polycrystalline TaAs thin films

We report the measurement of efficient charge-to-spin conversion at room temperature in Weyl semimetal/ferromagnet heterostructures with both oxidized and pristine interfaces. Polycrystalline films of the Weyl semimetal, TaAs, are grown by molecular beam epitaxy on (001) GaAs and interfaced with a metallic ferromagnet (Ni$_{0.8}$Fe$_{0.2}$). Spin torque ferromagnetic resonance (ST-FMR) measurements in samples with an oxidized interface yield a spin torque efficiency as large as $ξ_{\mathrm{FMR}}=0.45\pm 0.25$ for a 8 nm Ni$_{0.8}$Fe$_{0.2}$ layer thickness. By studying ST-FMR in these samples with varying Ni$_{0.8}$Fe$_{0.2}$ layer thickness, we extract a damping-like torque efficiency as high as $ξ_{\mathrm{DL}}=1.36\pm 0.66$. In samples with a pristine (unoxidized) interface, the spin torque efficiency has opposite sign to that observed in oxidized samples ($ξ_{\mathrm{FMR}}=-0.27\pm 0.14$ for a 5 nm Ni$_{0.8}$Fe$_{0.2}$ layer thickness). We also find a lower bound on the spin Hall conductivity ($424 \pm 110 \frac{\hbar}{e}$ S/cm) which is surprisingly consistent with theoretical predictions for the single crystal Weyl semimetal state of TaAs.

cond-mat.mtrl-sci↗

Local ferromagnetic resonance measurements of mesoscopically patterned ferromagnets using deterministically placed nanodiamonds

Nitrogen-vacancy centers in diamond have recently been established as effective sensors of the magnetization dynamics in vicinal ferromagnetic materials. We demonstrate sub-100 nm placement accuracy of nitrogen-vacancy-containing nanodiamonds and use these as local sensors that probe optically detected ferromagnetic resonance in mesoscopically patterned Permalloy islands. These measurements reveal variations in the ferromagnetic resonance signal at different sites on these structures with distinct behavior in the edge and the bulk of patterned features. These test measurements establish an easily implemented approach for spatially targeted measurements of spin dynamics in mesoscale ferromagnets. In principle, the methodology can also be extended to local studies of nanoscale ferromagnets such as single magnetic nanowires and nanoparticles.

cond-mat.mes-hall↗