Searcharxiv⌕ Search

arXiv subjects

K. -L. Kratz

Publications and source records attributed to K. -L. Kratz.

At least 19 recordsLinked to original sources

On the Origin of the Early Solar System Radioactivities. Problems with the AGB and Massive Star Scenarios

Recent improvements in stellar models for intermediate-mass and massive stars are recalled, together with their expectations for the synthesis of radioactive nuclei of lifetime $τ\lesssim 25$ Myr, in order to re-examine the origins of now extinct radioactivities, which were alive in the solar nebula. The Galactic inheritance broadly explains most of them, especially if $r$-process nuclei are produced by neutron star merging according to recent models. Instead, $^{26}$Al, $^{41}$Ca, $^{135}$Cs and possibly $^{60}$Fe require nucleosynthesis events close to the solar formation. We outline the persisting difficulties to account for these nuclei by Intermediate Mass Stars (2 $\lesssim $ M/M$_\odot \lesssim 7 - 8$). Models of their final stages now predict the ubiquitous formation of a $^{13}$C reservoir as a neutron capture source; hence, even in presence of $^{26}$Al production from Deep Mixing or Hot Bottom Burning, the ratio $^{26}$Al/$^{107}$Pd remains incompatible with measured data, with a large excess in $^{107}$Pd. This is shown for two recent approaches to Deep Mixing. Even a late contamination by a Massive Star meets problems. In fact, inhomogeneous addition of Supernova debris predicts non-measured excesses on stable isotopes. Revisions invoking specific low-mass supernovae and/or the sequential contamination of the pre-solar molecular cloud might be affected by similar problems, although our conclusions here are weakened by our schematic approach to the addition of SN ejecta. The limited parameter space remaining to be explored for solving this puzzle is discussed.

astro-ph.SR↗

The Hamburg/ESO R-process Enhanced Star survey (HERES) XI. The highly $r$-process-enhanced star CS 29497-004

We report an abundance analysis for the highly r-process-enhanced (r-II) star CS 29497-004, a very metal-poor giant with Teff = 5013K and [Fe/H]=-2.85, whose nature was initially discovered in the course of the HERES project. Our analysis is based on high signal-to-noise, high-resolution (R~75000) VLT/UVES spectra and MARCS model atmospheres under the assumption of local thermodynamic equilibrium, and obtains abundance measurements for a total of 46 elements, 31 of which are neutron-capture elements. As is the case for the other 25 r-II stars currently known, the heavy-element abundance pattern of CS 29497-004 well-matches a scaled Solar System second peak r-process-element abundance pattern. We confirm our previous detection of Th, and demonstrate that this star does not exhibit an "actinide boost". Uranium is also detected (log e(U) =-2.20+/-0.30), albeit with a large measurement error that hampers its use as a precision cosmo-chronometer. Combining the various elemental chronometer pairs that are available for this star, we derive a mean age of 12.2+/-3.7 Gyr using the theoretical production ratios from waiting-point approximation models (Kratz et al. 2007). We further explore the high-entropy wind model (Farouqi et al. 2010) production ratios arising from different neutron richness of the ejecta (Y_e), and derive an age of 13.7+/-4.4 Gyr for a best-fitting Y_e=0.447. The U/Th nuclei-chronometer is confirmed to be the most resilient to theoretical production ratios and yields an age of 16.5+:-6.6 Gyr. Lead (Pb) is also tentatively detected in CS 29497-004, at a level compatible with a scaled Solar r-process, or with the theoretical expectations for a pure r-process in this star.

astro-ph.GA↗

Theoretical neutron-capture cross sections for r-process nucleosynthesis in the $^{48}$Ca region

We calculate neutron capture cross sections for r-process nucleosynthesis in the $^{48}$Ca region, namely for the isotopes $^{40-44}$S, $^{46-50}$Ar, $^{56-66}$Ti, $^{62-68}$Cr, and $^{72-76}$Fe. While previously only cross sections resulting from the compound nucleus reaction mechanism (Hauser-Feshbach) have been considered, we recalculate not only that contribution to the cross section but also include direct capture on even-even nuclei. The level schemes, which are of utmost importance in the direct capture calculations, are taken from quasi-particle states obtained with a folded-Yukawa potential and Lipkin-Nogami pairing. Most recent deformation values derived from experimental data on $β$-decay half lives are used where available. Due to the consideration of direct capture, the capture rates are enhanced and the "turning points" in the r-process path are shifted to slightly higher mass numbers. We also discuss the sensitivity of the direct capture cross sections on the assumed deformation.

nucl-th↗

Origin of Anomalous Xe-H in Nanodiamond Stardust

Still today, the nucleosynthesis origin of Xe-H in presolar nanodiamonds is far from understood. Historically, possible explanations were proposed by a secondary "neutron-burst" process occurring in the He- or C/O-shells of a type-II supernova (SN-II), which are, however, not fully convincing in terms of modern nucleosynthesis conditions. Therefore, we have investigated Xe isotopic abundance features that may be diagnostic for different versions of a classical, primary r-process in high-entropy-wind (HEW) ejecta of core-collapse SN-II. We report here on parameter tests for non-standard r-process variants, by varying electron abundances (Y$_e$), ranges of entropies (S) and expansion velocities (V$_{exp}$) with their correlated neutron-freezeout times ($τ$(freeze)) and temperatures (T$_9$(freeze)). From this study, we conclude that a best fit to the measured Xe-H abundance ratios $^i$Xe/$^{136}$Xe can be obtained with the high-S "main" component of a "cold" r-process variant.

astro-ph.EP↗

Measurement of the reaction O-17(α,n)Ne-20 and its impact on the s process in massive stars

The ratio between the rates of the reactions O-17(α,n)Ne-20 and O-17(α,γ)Ne-21 determines whether O-16 is an efficient neutron poison for the s process in massive stars, or if most of the neutrons captured by O-16(n,γ) are recycled into the stellar environment. This ratio is of particular relevance to constrain the s process yields of fast rotating massive stars at low metallicity. Recent results on the (α,γ) channel have made it necessary to measure the (α,n) reaction more precisely and investigate the effect of the new data on s process nucleosynthesis in massive stars. We present a new measurement of the O-17(α, n) reaction using a moderating neutron detector. In addition, the (α, n_1) channel has been measured independently by observation of the characteristic 1633 keV γ-transition in Ne-20. The reaction cross section was determined with a simultaneous R-matrix fit to both channels. (α,n) and (α, γ) resonance strengths of states lying below the covered energy range were estimated using their known properties from the literature. A new O-17(α,n) reaction rate was deduced for the temperature range 0.1 GK to 10 GK. It was found that in He burning conditions the (α,γ) channel is strong enough to compete with the neutron channel. This leads to a less efficient neutron recycling compared to a previous suggestion of a very weak (α,γ) channel. S process calculations using our rates confirm that massive rotating stars do play a significant role in the production of elements up to Sr, but they strongly reduce the s process contribution to heavier elements.

nucl-ex↗

Beta-decay of nuclei around Se-90. Search for signatures of a N=56 sub-shell closure relevant the r-process

Nuclear structure plays a significant role on the rapid neutron capture process (r-process) since shapes evolve with the emergence of shells and sub-shells. There was some indication in neighboring nuclei that we might find examples of a new N=56 sub-shell, which may give rise to a doubly magic Se-90 nucleus. Beta-decay half lives of nuclei around Se-90 have been measured to determine if this nucleus has in fact a doubly-magic character. The fragmentation of Xe-136 beam at the National Superconducting Cyclotron Laboratory at Michigan State University was used to create a cocktail of nuclei in the A=90 region. We have measured the half lives of twenty-two nuclei near the r-process path in the A=90 region. The half lives of As-88 and Se-90 have been measured for the first time. The values were compared with theoretical predictions in the search for nuclear-deformation signatures of a N=56 sub-shell, and its possible role in the emergence of a potential doubly-magic Se-90. The impact of such hypothesis on the synthesis of heavy nuclei, particularly in the production of Sr, Y and Zr elements was investigated with a weak r-process network. The new half lives agree with results obtained from a standard global QRPA model used in r-process calculations, indicating that Se-90 has a quadrupole shape incompatible with a closed N=56 sub-shell in this region. The impact of the measured Se-90 half-life in comparison with a former theoretical predication associated with a spherical half-life on the weak-r-process is shown to be strong.

nucl-ex↗

Half-lives and branchings for β-delayed neutron emission for neutron-rich Co-Cu isotopes in the r-process

The β decays of very neutron-rich nuclides in the Co-Zn region were studied experimentally at the National Superconducting Cyclotron Laboratory using the NSCL β-counting station in conjunction with the neutron detector NERO. We measured the branchings for β-delayed neutron emission (Pn values) for 74Co (18 +/- 15%) and 75-77Ni (10 +/- 2.8%, 14 +/- 3.6%, and 30 +/- 24%, respectively) for the first time, and remeasured the Pn values of 77-79Cu, 79,81Zn, and 82Ga. For 77-79Cu and for 81Zn we obtain significantly larger Pn values compared to previous work. While the new half-lives for the Ni isotopes from this experiment had been reported before, we present here in addition the first half-life measurements of 75Co (30 +/- 11 ms) and 80Cu (170+110 -50 ms). Our results are compared with theoretical predictions, and their impact on various types of models for the astrophysical rapid neutron-capture process (r-process) is explored. We find that with our new data, the classical r-process model is better able to reproduce the A = 78-80 abundance pattern inferred from the solar abundances. The new data also influence r-process models based on the neutrino-driven high-entropy winds in core collapse supernovae.

nucl-ex↗

The Ubiquity of the Rapid Neutron-Capture Process

To better characterize the abundance patterns produced by the r-process, we have derived new abundances or upper limits for the heavy elements zinc (Zn), yttrium (Y), lanthanum (La), europium (Eu), and lead (Pb). Our sample of 161 metal-poor stars includes new measurements from 88 high resolution and high signal-to-noise spectra obtained with the Tull Spectrograph on the 2.7m Smith Telescope at McDonald Observatory, and other abundances are adopted from the literature. We use models of the s-process in AGB stars to characterize the high Pb/Eu ratios produced in the s-process at low metallicity, and our new observations then allow us to identify a sample of stars with no detectable s-process material. In these stars, we find no significant increase in the Pb/Eu ratios with increasing metallicity. This suggests that s-process material was not widely dispersed until the overall Galactic metallicity grew considerably, perhaps even as high as [Fe/H]=-1.4. We identify a dispersion of at least 0.5 dex in [La/Eu] in metal-poor stars with [Eu/Fe]<+0.6 attributable to the r-process, suggesting that there is no unique "pure" r-process elemental ratio among pairs of rare earth elements. We confirm earlier detections of an anti-correlation between Y/Eu and Eu/Fe bookended by stars strongly enriched in the r-process (e.g., CS 22892-052) and those with deficiencies of the heavy elements (e.g., HD 122563). We can reproduce the range of Y/Eu ratios using simulations of high-entropy neutrino winds of core-collapse supernovae that include charged-particle and neutron-capture components of r-process nucleosynthesis. The heavy element abundance patterns in most metal-poor stars do not resemble that of CS 22892-052, but the presence of heavy elements such as Ba in nearly all metal-poor stars without s-process enrichment suggests that the r-process is a common phenomenon.

astro-ph.SR↗

The neutron long counter NERO for studies of beta-delayed neutron emission in the r-process

The neutron long counter NERO was built at the National Superconducting Cyclotron Laboratory (NSCL), Michigan State University, for measuring beta-delayed neutron-emission probabilities. The detector was designed to work in conjunction with a beta-decay implantation station, so that beta decays and beta-delayed neutrons emitted from implanted nuclei can be measured simultaneously. The high efficiency of about 40%, for the range of energies of interest, along with the small background, are crucial for measuring beta-delayed neutron emission branchings for neutron-rich r-process nuclei produced as low intensity fragmentation beams in in-flight separator facilities.

nucl-ex↗

Charged-Particle and Neutron-Capture Processes in the High-Entropy Wind of Core-Collapse Supernovae

The astrophysical site of the r-process is still uncertain, and a full exploration of the systematics of this process in terms of its dependence on nuclear properties from stability to the neutron drip-line within realistic stellar environments has still to be undertaken. Sufficiently high neutron to seed ratios can only be obtained either in very neutron-rich low-entropy environments or moderately neutron-rich high-entropy environments, related to neutron star mergers (or jets of neutron star matter) and the high-entropy wind of core-collapse supernova explosions. As chemical evolution models seem to disfavor neutron star mergers, we focus here on high-entropy environments characterized by entropy $S$, electron abundance $Y_e$ and expansion velocity $V_{exp}$. We investigate the termination point of charged-particle reactions, and we define a maximum entropy $S_{final}$ for a given $V_{exp}$ and $Y_e$, beyond which the seed production of heavy elements fails due to the very small matter density. We then investigate whether an r-process subsequent to the charged-particle freeze-out can in principle be understood on the basis of the classical approach, which assumes a chemical equilibrium between neutron captures and photodisintegrations, possibly followed by a $β$-flow equilibrium. In particular, we illustrate how long such a chemical equilibrium approximation holds, how the freeze-out from such conditions affects the abundance pattern, and which role the late capture of neutrons originating from $β$-delayed neutron emission can play.

astro-ph.SR↗

The Hamburg/ESO R-process Enhanced Star survey (HERES) IV. Detailed abundance analysis and age dating of the strongly r-process enhanced stars CS 29491-069 and HE 1219-0312

We report on a detailed abundance analysis of two strongly r-process enhanced, very metal-poor stars newly discovered in the HERES project, CS 29491-069 ([Fe/H]=-2.51, [r/Fe]=+1.1) and HE 1219-0312 ([Fe/H]=-2.96, [r/Fe]=+1.5). The analysis is based on high-quality VLT/UVES spectra and MARCS model atmospheres. We detect lines of 15 heavy elements in the spectrum of CS 29491-069, and 18 in HE 1219-0312; in both cases including the Th II 4019 Å line. The heavy-element abundance patterns of these two stars are mostly well-matched to scaled solar residual abundances not formed by the s-process. We also compare the observed pattern with recent high-entropy wind (HEW) calculations, which assume core-collapse supernovae of massive stars as the astrophysical environment for the r-process, and find good agreement for most lanthanides. The abundance ratios of the lighter elements strontium, yttrium, and zirconium, which are presumably not formed by the main r-process, are reproduced well by the model. Radioactive dating for CS 29491-069 with the observed thorium and rare-earth element abundance pairs results in an average age of 9.5 Gyr, when based on solar r-process residuals, and 17.6 Gyr, when using HEW model predictions. Chronometry seems to fail in the case of HE 1219-0312, resulting in a negative age due to its high thorium abundance. HE 1219-0312 could therefore exhibit an overabundance of the heaviest elements, which is sometimes called an "actinide boost".

astro-ph.SR↗

Co-production of light p-, s- and r-process isotopes in the high-entropy wind of type II supernovae

We have performed large-scale nucleosynthesis calculations within the high-entropy-wind (HEW) scenario of type II supernovae. The primary aim was to constrain the conditions for the production of the classical "p-only" isotopes of the light trans-Fe elements. We find, however, that for electron fractions in the range 0.458 $\le$ Y$_e$ $\le$ 0.478, sizeable abundances of p-, s- and r-process nuclei between $^{64}$Zn and $^{98}$Ru are coproduced in the HEW at low entropies (S $\le$ 100) by a primary charged-particle process after an $α$-rich freezeout. With the above Y$_e$ -- S correlation, most of the predicted isotopic abundance ratios within a given element (e.g. $^{64}$Zn(p)/$^{70}$Zn(r) or $^{92}$Mo(p)/$^{94}$Mo(p)), as well as of neighboring elements (e.g. $^{70}$Ge(s+p)/$^{74}$Se(p) or $^{74}$Se(p)/$^{78}$Kr(p)) agree with the observed Solar-System ratios. Taking the Mo isotopic chain as a particularly challenging example, we show that our HEW model can account for the production of all 7 stable isotopes, from "p-only" $^{92}$Mo, via "s-only" $^{96}$Mo up to "r-only" $^{100}$Mo. Furthermore, our model is able to reproduce the isotopic composition of Mo in presolar SiC X-grains.}

astro-ph.SR↗

Beta-decay half-lives and beta-delayed neutron emission probabilities of nuclei in the region below A=110, relevant for the r-process

Measurements of the beta-decay properties of r-process nuclei below A=110 have been completed at the National Superconducting Cyclotron Laboratory, at Michigan State University. Beta-decay half-lives for Y-105, Zr-106,107 and Mo-111, along with beta-delayed neutron emission probabilities of Y-104, Mo-109,110 and upper limits for Y-105, Zr-103,104,105,106,107 and Mo-108,111 have been measured for the first time. Studies on the basis of the quasi-random phase approximation are used to analyze the ground-state deformation of these nuclei.

nucl-ex↗

Nucleosynthesis Modes in the High-Entropy-Wind of Type II Supernovae: Comparison of Calculations with Halo-Star Observations

While the high-entropy wind (HEW) of Type II supernovae remains one of the more promising sites for the rapid neutron-capture (r-) process, hydrodynamic simulations have yet to reproduce the astrophysical conditions under which the latter occurs. We have performed large-scale network calculations within an extended parameter range of the HEW, seeking to identify or to constrain the necessary conditions for a full reproduction of all r-process residuals N_{r,\odot}=N_{\odot}-N_{s,\odot} by comparing the results with recent astronomical observations. A superposition of weighted entropy trajectories results in an excellent reproduction of the overall N_{r,\odot}-pattern beyond Sn. For the lighter elements, from the Fe-group via Sr-Y-Zr to Ag, our HEW calculations indicate a transition from the need for clearly different sources (conditions/sites) to a possible co-production with r-process elements, provided that a range of entropies are contributing. This explains recent halo-star observations of a clear non-correlation of Zn and Ge and a weak correlation of Sr - Zr with heavier r-process elements. Moreover, new observational data on Ru and Pd seem to confirm also a partial correlation with Sr as well as the main r-process elements (e.g. Eu).

astro-ph.SR↗

Beta decay studies of r-process nuclei at the National Superconducting Cyclotron Laboratory

The impact of nuclear physics on astrophysical r-process models is discussed, emphasizing the importance of beta-decay properties of neutron-rich nuclei. Several r-process motivated beta-decay experiments performed at the National Superconducting Cyclotron Laboratory are presented. The experiments include the measurement of beta-decay half-lives and neutron emission probabilities of nuclei in regions around Ni-78; Se-90; Zr-106 and Rh-120, as well as spectroscopic studies of Pd-120. A summary on the different experimental techniques employed, data analysis, results and impact on model calculations is presented.

nucl-ex↗

R-process Experimental Campaign at the National Superconducting Cyclotron Laboratory

A JINA/VISTARS r-process campaign was completed at the A1900 Fragment Separator of the National Superconducting Cyclotron Laboratory in the fall of 2005. The purpose of the campaign was the measurement of the beta-decay half-lives and beta-delayed neutron-emission probabilities of different unknown neutron-rich nuclei participating in the r-process. Details of this campaign will be presented.

astro-ph↗

Nucleosynthesis in the Early Galaxy

Recent observations of r-process-enriched metal-poor star abundances reveal a non-uniform abundance pattern for elements $Z\leq47$. Based on non-correlation trends between elemental abundances as a function of Eu-richness in a large sample of metal-poor stars, it is shown that the mixing of a consistent and robust light element primary process (LEPP) and the r-process pattern found in r-II metal-poor stars explains such apparent non-uniformity. Furthermore, we derive the abundance pattern of the LEPP from observation and show that it is consistent with a missing component in the solar abundances when using a recent s-process model. As the astrophysical site of the LEPP is not known, we explore the possibility of a neutron capture process within a site-independent approach. It is suggested that scenarios with neutron densities $n_{n}\leq10^{13}$ $cm^{-3}$ or in the range $n_{n}\geq10^{24}$ $cm^{-3}$ best explain the observations.

astro-ph↗

Half Life of the Doubly-magic r-Process Nucleus 78Ni

Nuclei with magic numbers serve as important benchmarks in nuclear theory. In addition, neutron-rich nuclei play an important role in the astrophysical rapid neutron-capture process (r-process). 78Ni is the only doubly-magic nucleus that is also an important waiting point in the r-process, and serves as a major bottleneck in the synthesis of heavier elements. The half-life of 78Ni has been experimentally deduced for the first time at the Coupled Cyclotron Facility of the National Superconducting Cyclotron Laboratory at Michigan State University, and was found to be 110 (+100 -60) ms. In the same experiment, a first half-life was deduced for 77Ni of 128 (+27 -33) ms, and more precise half-lives were deduced for 75Ni and 76Ni of 344 (+20 -24) ms and 238 (+15 -18) ms respectively.

nucl-ex↗