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K. A. Chipps

Publications and source records attributed to K. A. Chipps.

At least 19 recordsLinked to original sources

Detailed Study of the $^{59}$Cu(p,$α)^{56}$Ni Reaction and Constraints on Its Astrophysical Reaction Rate

The $^{59}$Cu$(p,α)^{56}$Ni reaction plays an important role in explosive astrophysical scenarios such as Type I X-ray bursts and the $νp$-process in neutrino-driven winds following a core-collapse supernova, where it regulates the flow of nucleosynthesis through the NiCu cycle and the synthesis of heavier nuclei. We present a direct measurement of the $^{59}\mathrm{Cu}(p,α)^{56}\mathrm{Ni}$ excitation function from 2.43--5.88~MeV in the center-of-mass frame, performed in inverse kinematics with the high-efficiency MUSIC active-target detector at FRIB. The angle- and energy-integrated cross sections extend direct measurements to lower energies than previously reported and remove the angular-integration model dependence of earlier work. To extrapolate the rate to astrophysical energies, we constrain the statistical-model description through a systematic optimization of the DEM-3 $α$-optical model potential geometry, and quantify the model-selection uncertainty with a Bayesian model averaging analysis over 96 TALYS combinations. The resulting stellar rate carries a temperature-dependent uncertainty factor of 1.26--1.63 over $T_9 = 0.2$--10 and is systematically lower than the REACLIB evaluation, remaining below the competing $(p,γ)$ rate for $T_9 \lesssim 3.94$. These results substantially weaken the inferred NiCu cycle strength and establish the $^{59}$Cu$(p,γ)^{60}$Zn rate as the dominant remaining uncertainty.

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Direct Measurement of the $^{59}$Cu$(p,α)^{56}$Ni Excitation Function to Constrain the Ni--Cu Cycle Strength and Its Impact on Explosive Nucleosynthesis

A new direct measurement of the 59Cu(p,a)56Ni excitation function from 2.43-5.88 MeV in the center-of-mass was performed in inverse kinematics using the high-efficiency MUSIC active-target detector at FRIB. This reaction plays a critical role in constraining the strength of the NiCu cycle in different explosive astrophysical scenarios such as Type I X-ray bursts and the nu-p process in neutrino-driven winds after a core-collapse supernova. The newly derived stellar rate is systematically lower than previous estimates, suppressing NiCu cycle recycling in X-ray bursts to below 3% and enhancing nu-p process efficiency throughout the relevant temperature range, potentially extending its effective operation to temperatures as high as T9 = 3.94 (+0.99/-0.85).

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Study of the $in ^{34}$Ar($α,p$)$^{37}$K reaction rate via proton scattering on $^{37}$K, and its impact on properties of modeled X-Ray bursts

Background: Type I X-Ray bursts (XRBs) are energetic stellar explosions that occur on the surface of a neutron star in an accreting binary system with a low-mass H/He-rich companion. The rate of the $^{34}$Ar($α,p$)$^{37}$K reaction may influence features of the light curve that results from the underlying thermonuclear runaway, as shown in recent XRB stellar modelling studies. Purpose: In order to reduce the uncertainty of the rate of this reaction, properties of resonances in the compound nucleus $^{38}$Ca, such as resonance energies, spins, and particle widths, must be well constrained. Method: This work discusses a study of resonances in the $^{38}$Ca compound nucleus produced in the $^{34}$Ar($α,p$) reaction. The experiment was performed at the National Superconducting Cyclotron Laboratory, with the ReA3 facility by measuring proton scattering using an unstable $^{37}$K beam. The kinematics were designed specifically to identify and characterize resonances in the Gamow energy window for the temperature regime relevant to XRBs. Results: The spins and proton widths of newly identified and previously known states in $^{38}$Ca in the energy region of interest for the $^{34}$Ar($α,p$)$^{37}$K reaction have been constrained through an R-Matrix analysis of the scattering data. Conclusions: Using these constraints, a newly estimated rate is applied to an XRB model built using Modules for Experiments in Stellar Astrophysics (MESA), to examine its impact on observables, including the light curve. It is found that the newly determined reaction rate does not substantially affect the features of the light curve.

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Object Detection with Deep Learning for Rare Event Search in the GADGET II TPC

In the pursuit of identifying rare two-particle events within the GADGET II Time Projection Chamber (TPC), this paper presents a comprehensive approach for leveraging Convolutional Neural Networks (CNNs) and various data processing methods. To address the inherent complexities of 3D TPC track reconstructions, the data is expressed in 2D projections and 1D quantities. This approach capitalizes on the diverse data modalities of the TPC, allowing for the efficient representation of the distinct features of the 3D events, with no loss in topology uniqueness. Additionally, it leverages the computational efficiency of 2D CNNs and benefits from the extensive availability of pre-trained models. Given the scarcity of real training data for the rare events of interest, simulated events are used to train the models to detect real events. To account for potential distribution shifts when predominantly depending on simulations, significant perturbations are embedded within the simulations. This produces a broad parameter space that works to account for potential physics parameter and detector response variations and uncertainties. These parameter-varied simulations are used to train sensitive 2D CNN object detectors. When combined with 1D histogram peak detection algorithms, this multi-modal detection framework is highly adept at identifying rare, two-particle events in data taken during experiment 21072 at the Facility for Rare Isotope Beams (FRIB), demonstrating a 100% recall for events of interest. We present the methods and outcomes of our investigation and discuss the potential future applications of these techniques.

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Machine-Learning-Enabled Measurements of Astrophysical (p,n) Reactions with the SECAR Recoil Separator

The synthesis of heavy elements in supernovae is affected by low-energy (n,p) and (p,n) reactions on unstable nuclei, yet experimental data on such reaction rates are scarce. The SECAR (SEparator for CApture Reactions) recoil separator at FRIB (Facility for Rare Isotope Beams) was originally designed to measure astrophysical reactions that change the mass of a nucleus significantly. We used a novel approach that integrates machine learning with ion-optical simulations to find an ion-optical solution for the separator that enables the measurement of (p,n) reactions, despite the reaction leaving the mass of the nucleus nearly unchanged. A new measurement of the $^{58}$Fe(p,n)$^{58}$Co reaction in inverse kinematics with a 3.66$\pm$0.12 MeV/nucleon $^{58}$Fe beam (corresponding to 3.69$\pm$0.12 MeV proton energy in normal kinematics) yielded a cross-section of 20.3$\pm$6.3 mb and served as a benchmark for the new technique demonstrating its effectiveness in achieving the required performance criteria. This novel approach marks a significant advancement in experimental nuclear astrophysics, as it paves the way for studying astrophysically important (p,n) reactions on unstable nuclei produced at FRIB.

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Measurement of Charge State Distributions using a Scintillation Screen

Absolute cross sections measured using electromagnetic devices to separate and detect heavy recoiling ions need to be corrected for charge state fractions. Accurate prediction of charge state distributions using theoretical models is not always a possibility, especially in energy and mass regions where data is sparse. As such, it is often necessary to measure charge state fractions directly. In this paper we present a novel method of using a scintillation screen along with a CMOS camera to image the charge dispersed beam after a set of magnetic dipoles. A measurement of the charge state distribution for 88Sr passing through a natural carbon foil is performed. Using a Bayesian model to extract statistically meaningful uncertainties from these images, we find agreement between the new method and a more traditional method using Faraday cups. Future work is need to better understand systematic uncertainties. Our technique offers a viable method to measure charge state distributions.

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First direct measurement constraining the $^{34}$Ar($α$,p)$^{37}$K reaction cross section for mixed hydrogen and helium burning in accreting neutron stars

The rate of the final step in the astrophysical $α$p-process, the $^{34}$Ar($α$,\textit{p})$^{37}$K reaction, suffers from large uncertainties due to lack of experimental data, despite having a considerable impact on the observable light curves of x-ray bursts and the composition of the ashes of hydrogen and helium burning on accreting neutron stars. We present the first direct measurement constraining the $^{34}$Ar($α$,p)$^{37}$K reaction cross section, using the Jet Experiments in Nuclear Structure and Astrophysics (JENSA) gas jet target. The combined cross section for the $^{34}$Ar,Cl($α$,p)$^{37}$K,Ar reaction is found to agree well with Hauser-Feshbach predictions. The $^{34}$Ar($α$,2p)$^{36}$Ar cross section, which can be exclusively attributed to the $^{34}$Ar beam component, also agrees to within the typical uncertainties quoted for statistical models. This indicates the applicability of the statistical model for predicting astrophysical ($α$,p) reaction rates in this part of the $α$p process, in contrast to earlier findings from indirect reaction studies indicating orders-of-magnitude discrepancies. This removes a significant uncertainty in models of hydrogen and helium burning on accreting neutron stars.

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Executive Summary of the Topical Program: Nuclear Isomers in the Era of FRIB

We report on the Facility for Rare Isotope Beams (FRIB) Theory Alliance topical program "Nuclear Isomers in the Era of FRIB". We outline the many ways isomers influence and contribute to nuclear science and technology, especially in the four FRIB pillars: properties of rare isotopes, nuclear astrophysics, fundamental symmetries, and applications for the nation and society. We conclude with a resolution stating our recommendation that the nuclear physics community actively pursue isomer research. A white paper is forthcoming.

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Study of the Isomeric State in $^{16}$N Using the $^{16}$N$^{g,m}$($d$,$^3$He) Reaction

The isomeric state of $^{16}$N was studied using the $^{16}$N$^{g,m}$($d$,$^3$He)~proton-removal reactions at \mbox{11.8~MeV/$u$} in inverse kinematics. The $^{16}$N beam, of which 24% was in the isomeric state, was produced using the ATLAS in-fight facility and delivered to the HELIOS spectrometer, which was used to analyze the $^{3}$He ions from the ($d$,$^{3}$He) reactions. The simultaneous measurement of reactions on both the ground and isomeric states, reduced the systematic uncertainties from the experiment and in the analysis. A direct and reliable comparison of the relative spectroscopic factors was made based on a Distorted-Wave Born Approximation approach. The experimental results suggest that the isomeric state of $^{16}$N is an excited neutron-halo state. The results can be understood through calculations using a Woods-Saxon potential model, which captures the effects of weak-binding.

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Quenching of Single-Particle Strength in A=15 Nuclei

Absolute cross sections for the addition of $s$- and $d$-wave neutrons to $^{14}$C and $^{14}$N have been determined simultaneously via the ($d$,$p$) reaction at 10 MeV/u. The difference between the neutron and proton separation energies, $ΔS$, is around $-20$ MeV for the $^{14}$C$+$$n$ system and $+8$ MeV for $^{14}$N$+$$n$. The population of the $1s_{1/2}$ and $0d_{5/2}$ orbitals for both systems is reduced by a factor of approximately 0.5 compared to the independent single-particle model, or about 0.6 when compared to the shell model. This finding strongly contrasts with results deduced from intermediate-energy knockout reactions between similar nuclei on targets of $^{9}$Be and $^{12}$C. The simultaneous technique used removes many systematic uncertainties.

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Horizons: Nuclear Astrophysics in the 2020s and Beyond

Nuclear Astrophysics is a field at the intersection of nuclear physics and astrophysics, which seeks to understand the nuclear engines of astronomical objects and the origin of the chemical elements. This white paper summarizes progress and status of the field, the new open questions that have emerged, and the tremendous scientific opportunities that have opened up with major advances in capabilities across an ever growing number of disciplines and subfields that need to be integrated. We take a holistic view of the field discussing the unique challenges and opportunities in nuclear astrophysics in regards to science, diversity, education, and the interdisciplinarity and breadth of the field. Clearly nuclear astrophysics is a dynamic field with a bright future that is entering a new era of discovery opportunities.

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In-flight production of an isomeric beam of $^{16}$N

An in-flight beam of $^{16}$N was produced via the single-neutron adding ($d$,$p$) reaction in inverse kinematics at the recently upgraded Argonne Tandem Linear Accelerator System (ATLAS) in-flight system. The amount of the $^{16}$N beam which resided in its excited 0.120-MeV $J^π=0^-$ isomeric state (T$_{1/2}\approx5$ $μ$s) was determined to be 40(5)% at a reaction energy of 7.9(3) MeV/$u$, and 24(2)% at a reaction energy of 13.2(2) MeV/$u$. The isomer measurements took place at an experimental station $\approx30$ m downstream of the production target and utilized an Al beam-stopping foil and a HPGe Clover detector. Composite $^{16}$N beam rate determinations were made at the experimental station and the focal plane of the Argonne in-flight radioactive ion-beam separator (RAISOR) with Si $Δ$E-E telescopes. A Distorted Wave Born Approximation (DWBA) approach was coupled with the known spectroscopic information on $^{16}$N in order to estimate the relative $^{16}$N isomer yields and composite $^{16}$N beam rates. In addition to the observed reaction-energy dependence of the isomer fraction, a large sensitivity to angular acceptance of the recoils was also observed.

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Constraining the $^{30}$P($p,γ)^{31}$S reaction rate in ONe novae via the weak, low-energy, $β$-delayed proton decay of $^{31}$Cl

The $^{30}$P$(p,γ)^{31}$S reaction plays an important role in understanding nucleosynthesis of $A\geq 30$ nuclides in oxygen-neon novae. The Gaseous Detector with Germanium Tagging was used to measure $^{31}$Cl $β$-delayed proton decay through the key $J^π=3/2^{+}$, 260-keV resonance. The intensity $I^{260}_{βp} = 8.3^{+1.2}_{-0.9} \times 10^{-6}$ represents the weakest $β$-delayed, charged-particle emission ever measured below 400 keV, resulting in a proton branching ratio of $Γ_p / Γ= 2.5^{+0.4}_{-0.3} \times 10^{-4}$. By combining this measurement with shell-model calculations for $Γ_γ$ and past work on other resonances, the total $^{30}$P$(p,γ)^{31}$S rate has been determined with reduced uncertainty. The new rate has been used in hydrodynamic simulations to model the composition of nova ejecta, leading to a concrete prediction of $^{30}$Si/$^{28}$Si excesses in presolar nova grains and the calibration of nuclear thermometers.

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Online Bayesian Optimization for a Recoil Mass Separator

The SEparator for CApture Reactions (SECAR) is a next-generation recoil separator system at the Facility for Rare Isotope Beams (FRIB) designed for the direct measurement of capture reactions on unstable nuclei in inverse kinematics. To maximize the performance of this system, stringent requirements on the beam alignment to the central beam axis and on the ion-optical settings need to be achieved. These can be difficult to attain through manual tuning by human operators without potentially leaving the system in a sub-optimal and irreproducible state. In this work, we present the first development of online Bayesian optimization with a Gaussian process model to tune an ion beam through a nuclear astrophysics recoil separator. We show that this method achieves small incoming angular deviations (\textless 1 mrad) in an efficient and reproducible manner that is at least three times faster than standard hand-tuning. Additionally, we present a Bayesian method for experimental optimization of the ion optics, and show that it validates the nominal theoretical ion-optical settings of the device, and improves the mass separation by 32\% for some beams.

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Superallowed $0^+ \rightarrow 0^+$ $β$ decay of $T =2$ $^{20}$Mg: $Q_{\textrm{EC}}$ value and $βγ$ branching

\textbf{Background}: Superallowed $0^+ \rightarrow 0^+$ $β$ decays of isospin $T=2$ nuclides can be used to test theoretical isospin symmetry breaking corrections applied to extract the CKM matrix element $V_{ud}$ from $T = 0,1$ decays by measuring precise $ft$ values and also to search for scalar currents using the $β-ν$ angular correlation. Key ingredients include the $Q_{\textrm{EC}}$ value and branching of the superallowed transition and the half life of the parent. \textbf{Purpose}: To determine a precise experimental $Q_{\textrm{EC}}$ value for the superallowed $0^+ \rightarrow 0^+$ $β$ decay of $T=2$ $^{20}$Mg and the intensity of $^{20}$Mg $β$-delayed $γ$ rays through the isobaric analog state in $^{20}$Na. \textbf{Method}: A beam of $^{20}$Mg was produced using the in-flight method and implanted into a plastic scintillator surrounded by an array of high-purity germanium detectors used to detect $β$-delayed $γ$ rays. The high-resolution $γ$-ray spectrum was analyzed to measure the $γ$-ray energies and intensities. \textbf{Results}: The intensity of $^{20}$Mg $β$-delayed $γ$ rays through the isobaric analog state in $^{20}$Na was measured to be $(1.60 \pm 0.04_{\textrm{stat}} \pm 0.15_{\textrm{syst}} \pm 0.15_{\textrm{theo}}) \times 10^{-4}$, where the uncertainties are statistical, systematic, and theoretical, respectively. The $Q_{\textrm{EC}}$ value for the superallowed transition was determined to be $4128.7 \pm 2.2$ keV based on the measured excitation energy of $6498.4 \pm 0.2_{\textrm{stat}} \pm 0.4_{\textrm{syst}}$ keV and literature values for the ground-state masses of $^{20}$Na and $^{20}$Mg. \textbf{Conclusions}: The $β$-delayed $γ$-decay branch and $Q_{\textrm{EC}}$ value are now sufficiently precise to match or exceed the sensitivity required for current low-energy tests of the standard model.

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A direct measurement of the 17O(a,g)21Ne reaction in inverse kinematics and its impact on heavy element production

During the slow neutron capture process in massive stars, reactions on light elements can both produce and absorb neutrons thereby influencing the final heavy element abundances. At low metallicities, the high neutron capture rate of 16-O can inhibit s-process nucleosynthesis unless the neutrons are recycled via the 17O(a,n)20Ne reaction. The efficiency of this neutron recycling is determined by competition between the 17O(a,n)20Ne and 17O(a,g)21Ne reactions. While some experimental data are available on the former reaction, no data exist for the radiative capture channel at the relevant astrophysical energies. The 17O(a,g)21Ne reaction has been studied directly using the DRAGON recoil separator at the TRIUMF Laboratory. The reaction cross section has been determined at energies between 0.6 and 1.6 MeV Ecm, reaching into the Gamow window for core helium burning for the first time. Resonance strengths for resonances at 0.63, 0.721, 0.81 and 1.122 MeV Ecm have been extracted. The experimentally based reaction rate calculated represents a lower limit, but suggests that significant s-process nucleosynthesis occurs in low metallicity massive stars.

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$s$-wave scattering lengths for the $^7$Be+p system from an $\textit{R}$-matrix analysis

The astrophysical $S$-factor for the radiative proton capture reaction on $^7$Be ($S_{17}$) at low energies is affected by the $s$-wave scattering lengths. We report the measurement of elastic and inelastic scattering cross sections for the $^7$Be+p system in the center-of-mass energy range 0.474 - 2.740 MeV and center-of-mass angular range of 70$^\circ$- 150$^\circ$. A radioactive $^7$Be beam produced at Oak Ridge National Laboratory's (ORNL) Holifield Radioactive Ion Beam Facility was accelerated and bombarded a thin polypropylene (CH$_{2}$)$_\text n$ target. Scattered ions were detected in the segmented Silicon Detector Array. Using an $\textit{R}$-matrix analysis of ORNL and Louvain-la-Neuve cross section data, the $s$-wave scattering lengths for channel spins 1 and 2 were determined to be 17.34$^{+1.11}_{-1.33}$ and -3.18$^{+0.55}_{-0.50}$ fm, respectively. The uncertainty in the $s$-wave scattering lengths reported in this work is smaller by a factor of 5-8 compared to the previous measurement, which may reduce the overall uncertainty in $S_{17}$ at zero energy. The level structure of $^8$B is discussed based upon the results from this work. Evidence for the existence of 0$^+$ and 2$^+$ levels in $^8$B at 1.9 and 2.21 MeV, respectively, is observed.

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New $γ$-ray Transitions Observed in $^{19}$Ne with Implications for the $^{15}$O($α$,$γ$)$^{19}$Ne Reaction Rate

The $^{15}$O($α$,$γ$)$^{19}$Ne reaction is responsible for breakout from the hot CNO cycle in Type I x-ray bursts. Understanding the properties of resonances between $E_x = 4$ and 5 MeV in $^{19}$Ne is crucial in the calculation of this reaction rate. The spins and parities of these states are well known, with the exception of the 4.14- and 4.20-MeV states, which have adopted spin-parities of 9/2$^-$ and 7/2$^-$, respectively. Gamma-ray transitions from these states were studied using triton-$γ$-$γ$ coincidences from the $^{19}$F($^{3}$He,$tγ$)$^{19}$Ne reaction measured with GODDESS (Gammasphere ORRUBA Dual Detectors for Experimental Structure Studies) at Argonne National Laboratory. The observed transitions from the 4.14- and 4.20-MeV states provide strong evidence that the $J^π$ values are actually 7/2$^-$ and 9/2$^-$, respectively. These assignments are consistent with the values in the $^{19}$F mirror nucleus and in contrast to previously accepted assignments.

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